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Oxygen vacancy promoting artificial atom(RuPd)by d-orbital coupling for efficient water dissociation

Nano Research 2024年第8期17卷 7045-7052页

作者： Ruofan Shen Yanyan Liu Shuling Liu Shuyan Guan Huanhuan Zhang Sehrish Mehdi Saima Ashraf ting-hui xiao Erjun Liang Jianchun Jiang Yongfeng Wang Baojun Li Laboratory of Zhongyuan Light School of PhysicsZhengzhou UniversityZhengzhou 450001China Key Laboratory of Materials Physics Ministry of EducationSchool of PhysicsZhengzhou UniversityZhengzhou 450001China College of Chemistry Zhengzhou UniversityZhengzhou 450001China College of Science Henan Agricultural UniversityZhengzhou 450002China Department of Chemistry Tsinghua UniversityBeijing 100084China National Engineering Lab.for Biomass Chemical Utilization Institute of Chemical Industry of Forest ProductsCAFNanjing 210042China Center for Carbon-based Electronics and Key Laboratory for the Physics and Chemistry of Nanodevices Department of ElectronicsPeking UniversityBeijing 100871China

Rational design of highly active catalysts for breaking hydrogen-oxygen bonds is of great significance in energy chemical reactions involving ***,an efficient strategy for the artificial atom(RuPd)established by d-orbital coupling and adjusted by oxygen vacancy(V_(O))is verified for water *** an experimental verification,the turnover frequency of RuPd-TiO_(2)-VO(RuPdTVO)catalyst in ammonia borane hydrolysis reaches up to 2750 min^(−1)(26,190 min−1 based on metal dispersion)in the absence of alkali,exceeding the highest active catalysts(Rh-based catalysts).The d-orbital coupling effect between Ru and Pd simulates the outer electronic structure of *** transfer from V_(O) to(RuPd)constructs an electron-rich state of active sites that further enhances the ability of the artificial atom to dissociate *** work provides an effective electronic regulation strategy from V_(O) and artificial atom constructed by d-orbital coupling effect for efficient water dissociation.

关键词： ammonia borane hydrolysis d-orbital coupling oxygen vacancy artificial atom water dissociation

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Analytical solution for the time-fractional heat conduction equation in spherical coordinate system by the method of variable separation

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Acta Mechanica Sinica 2011年第6期27卷 994-1000页

作者： ting-hui Ning xiao-Yun Jiang School of Mathematics Shandong University 250100 Jinan China

In this paper,using the fractional Fourier law,we obtain the fractional heat conduction equation with a time-fractional derivative in the spherical coordinate *** method of variable separation is used to solve the timefractional heat conduction *** Caputo fractional derivative of the order 0 〈 α≤ 1 is *** solution is presented in terms of the Mittag-Leffler *** results are illustrated graphically for various values of fractional derivative.

关键词： Fractional Fourier law Fractional heat conduction equation - Spherical coordinate system - The separation of variables Mittag-Leffler function

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Unlocking the secrets of the invisible world:incredible deep optical imaging through in-silico clearing

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光:科学与应用(英文版) 2023年第8期12卷 1439-1440页

作者： ting-hui xiao Yuqi Zhou Keisuke Goda Henan Key Laboratory of Diamond Optoelectronic Materials and Devices School of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052China Institute of Quantum Materials and Physics Henan Academy of SciencesZhengzhou 450046China Department of Chemistry School of ScienceThe University of TokyoTokyo 113-0033Japan institute of Technological Sciences Wuhan UniversityWuhan 430072China Department of Bioengineering University of CaliforniaLos AngelesCA 90095USA

In-silico clearing enables deep optical imaging of biological samples by correcting image blur caused by scattering and *** breakthrough method offers researchers unprecedented insights into three-dimensional biological systems,with enormous potential for advancing biology and medicine to better understand living organisms and human health.

关键词： clearing visible breakthrough

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Graphene surface plasmon polaritons transport on curved substrates

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Photonics Research 2015年第6期3卷 300-307页

作者： ting-hui xiao Lin Gan Zhi-Yuan Li Laboratory of Optical Physics Institute of Physics Chinese Academy of Sciences

We theoretically investigate the transport property of graphene surface plasmon polaritons(GSPPs) on curved graphene substrates. The dispersion relationship, propagation length, and field confinement are calculated by an analytical method and compared with those on planar substrates. Based on our theory, the bend of graphene nearly does not affect the property of GSPPs except for an extremely small shift to the lower frequency for the same effective mode index. The field distributions and the eigenfrequencies of GSPPs on planar and cylindrical substrates are calculated by the finite element method, which validates our theoretical analysis. Moreover, three types of graphene-guided optical interconnections of GSPPs, namely, planar to curved graphene film, curved to planar graphene film, and curved to curved graphene film, are proposed and examined in detail. The theoretical results show that the GSPPs propagation on curved graphene substrates and interconnections will not induce any additional losses if the phase-matching condition is satisfied. Additionally, the extreme tiny size of curved graphene for interconnection at a certain spectra range is predicted by our theory and validated by the simulation of 90° turning of GSPPs. The bending effect on the property of GSPPs is systematically analyzed and identified. Our studies would be helpful to instruct design of plasmonic devices involving curved GSPPs, such as nanophotoniccircuits, flexible plasmonic, and biocompatible devices.

关键词： Graphene surface plasmon polaritons transport on curved substrates

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Burning Numbers of Barbells

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 526-538页

作者： hui-qing LIU Rui-ting ZHANG xiao-lan HU Hubei Key Laboratory of Applied Mathematics&Faculty of Mathematics and Statistic Hubei UniversityWuhan 430062China Hubei Key Laboratory of Mathematical Sciences&School of Mathematics and Statistics Central China Normal UniversityWuhan 430079China

Motivated by a discrete-time process intended to measure the speed of the spread of contagion in a graph,the burning number b(G)of a graph G,is defined as the smallest integer k for which there are vertices x1,…xk su... 详细信息

关键词： burning number short/long barbell isometric subtree cycle

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High-Q germanium optical nanocavity

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Photonics Research 2018年第9期6卷 925-928页

作者： ting-hui xiao ZIQIANG ZHAO WEN ZHOU MITSURU TAKENAKA HON Ki TSANG ZHENZHOU CHENG KEISUKE GODA Department of Chemistry The University of TokyoTokyo 113-0033Japan Department of Electrical Engineering and Information Systems The University of TokyoTokyo 113-0033Japan Department of Electronic Engineering The Chinese University of Hong KongShatinHong Kong SARChina Department of Electrical Engineering University of CaliforniaLos AngelesCalifornia 90095USA

Mid-infrared(MIR) integrated photonics has attracted broad interest due to its promising applications in biochemical sensing, environmental monitoring, disease diagnosis, and optical communication. Among MIR integration platforms, germanium-based platforms hold many excellent properties, such as wide transparency windows, high refractive indices, and high nonlinear coefficients; however, the development of MIR germanium photonic devices is still in its infancy. Specifically, MIR high-Q germanium resonators with comparable performance to their silicon counterparts remain unprecedented. Here we experimentally demonstrate an MIR germanium nanocavity with a Q factor of ~18,000, the highest-to-date of reported nanocavities across MIR germanium-based integration platforms. This is achieved through a combination of a feasible theoretical design,Smart-Cut methods for wafer development, and optimized device fabrication processes. Our nanocavity, with its high Q factor and ultrasmall mode volume, opens new avenues for on-chip applications in the MIR spectral range.

关键词：薄膜热光性能通讯技术发展现状

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USP19 Stabilizes TAK1 to Regulate High Glucose/Free Fatty Acid-induced Dysfunction in HK-2 Cells

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Current Medical Science 2024年第4期44卷 707-717页

作者： xiao-hui YAN Yin-na ZHU Yan-ting ZHU Kidney Disease and Dialysis Center Shaanxi Provincial People's HospitalXi'an 710068China Department of Nephrology The Third Affiliated Hospital of Xi'an Medical UniversityXi'an 710000China Nephrology and Hemodialysis Center Shaanxi Provincial People's HospitalXi'an 710068China

Objective Obesity-induced kidney injury contributes to the development of diabetic nephropathy(DN).Here,we identified the functions of ubiquitin-specific peptidase 19(USP19)in HK-2 cells exposed to a combination of high glucose(HG)and free fatty acid(FFA)and determined its association with TGF-beta-activated kinase 1(TAK1).Methods HK-2 cells were exposed to a combination of HG and ***19 mRNA expression was detected by quantitative RT-PCR(qRT-PCR),and protein analysis was performed by immunoblotting(IB).Cell growth was assessed by Cell Counting Kit-8(CCK-8)viability and 5-ethynyl-2′-deoxyuridine(EdU)proliferation *** cycle distribution and apoptosis were detected by flow *** USP19/TAK1 interaction and ubiquitinated TAK1 levels were assayed by coimmunoprecipitation(Co-IP)assays and *** In HG+FFA-challenged HK-2 cells,USP19 was highly ***19 knockdown attenuated HG+FFA-triggered growth inhibition and apoptosis promotion in HK-2 ***,USP19 knockdown alleviated HG+FFA-mediated PTEN-induced putative kinase 1(PINK1)/Parkin pathway inactivation and increased mitochondrial reactive oxygen species(ROS)generation in HK-2 ***,USP19 stabilized the TAK1 protein through ***,increased TAK1 expression reversed the USP19 knockdown-mediated phenotypic changes and PINK1/Parkin pathway activation in HG+FFA-challenged HK-2 *** The findings revealed that USP19 plays a crucial role in promoting HK-2 cell dysfunction induced by combined stimulation with HG and FFAs by stabilizing TAK1,providing a potential therapeutic strategy for combating DN.

关键词： HK-2 cells high glucose free fatty acid dysfunction USP19 deubiquitination

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Solution processable transition metal dichalcogenides-based hybrids for photodetection

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Nano Materials Science 2019年第4期1卷 288-298页

作者： Yingdong Han Jie Wang Haoran Wan Shuang Wang Haofeng Hu ting-hui xiao Zhenzhou Cheng Tiegen Liu School of Precision Instruments and Optoelectronics Engineering Tianjin UniversityTianjin300072China Key Laboratory of Optoelectronics Information Technology Ministry of EducationTianjin300072China Department of Chemistry University of TokyoTokyo113-0033Japan

Transition metal dichalcogenides(TMDs), as one of the most promising two-dimensional(2D) materials, have attracted considerable attention for use in photodetection applications over the past few years due to their distinct properties, such as atomic-scale thickness, tunable direct bandgaps, and decent carrier mobilities at room temperature. Compared with pure 2D TMDs, the construction of hybrids consisting of TMDs and other low-dimensional materials can further improve the performance of photodetectors including their spectral range, responsivity and detectivity, which significantly boosts interest in the development of TMDs-based photodetectors. On the other hand, solution-phase synthesis methods provide a facile strategy for the scalable production of TMD hybrids, opening an exciting avenue to develop low-cost devices. In this review, we summarize the material synthesis, characterizations, and photodetection applications of the solution processable TMDs-based hybrids, as well as provide insights into their prospects.

关键词： temperature. synthesis process

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Adhesion Performances Between Two Orthotropic Solids Influenced by Temperature Increment

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Acta Mechanica Solida Sinica 2024年第3期37卷 430-443页

作者： Qing-hui Luo Yue-ting Zhou School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghai200092China

The classical adhesive contact models belong to isothermal adhesion theories,where the effect of temperature on adhesion was ***,a number of experimental results indicated that the adhesion behaviors can be significantly affected by *** this paper,the two-dimensional non-slipping anisothermal adhesion behaviors between two orthotropic elastic cylinders are investigated within the framework of the Johnson-Kendall-Roberts *** stated problem is reduced to the coupled singular integral equations by virtue of the Fourier integral transform,which are solved analytically with the analytical function *** closed-form solutions for the stress fields in the presence of thermoelastic effect are *** stable equilibrium state of contact system is determined by virtue of the Griffith energy *** effect of temperature difference on adhesion behaviors between orthotropic solids is *** is found that the difference between the oscillatory and non-oscillatory solutions increases with increasing the degree of anisotropy of orthotropic *** oscillatory solution cannot be well approximated by the non-oscillatory solution for the orthotropic materials with relatively high anisotropy.

关键词： Adhesive contact Non-slipping JKR model Temperature Griffith energy balance

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Ultrafast imaging for uncovering laser–material interaction dynamics

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International Journal of Mechanical System Dynamics 2022年第1期2卷 65-81页

作者： Du Wang Shubin Wei Xiandan Yuan Zhiyuan Liu Yueyun Weng Yuqi Zhou ting‐hui xiao Keisuke Goda Sheng Liu Cheng Lei The Institute of Technological Sciences Wuhan UniversityWuhanChina The Key Laboratory of Transients in Hydraulic Machinery of Ministry of Education School of Power and Mechanical EngineeringWuhan UniversityWuhanChina Department of Chemistry University of TokyoTokyoJapan Department of Bioengineering University of CaliforniaLos AngelesCaliforniaUSA

The physical mechanism of the dynamics in laser–material interaction has been an important research *** addition to theoretical analysis,direct imaging‐based observation of ultrafast dynamic processes is an important approach to understand many fundamental issues in laser–material interaction such as inertial confinement fusion(ICF),laser accelerator construction,and advanced laser *** this review,the principles and applications of three types of commonly used ultrafast imaging methods are introduced,including the pump–probe,X‐ray diagnosis,and single‐shot optical burst *** focus on the technical features such as the spatial and temporal resolution for each technique,and present several conventional applications.

关键词： high‐energy‐density physics laser–material interaction laser processing ultrafast dynamics ultrafast imaging

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