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Function-reversible facets enabling SrTiO_(3)nanocrystals for improved photocatalytic hydrogen evolution

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Frontiers in Energy 2024年第1期18卷 101-109页

作者： Bin WANG Bei AN Xiaoqian LI Shaohua shen School of Physics Key Laboratory for Non-equilibrium Synthesis and Modulation of Condensed Matter(Ministry of Education)Key Laboratory of Shaanxi for Advanced Materials and Mesoscopic PhysicsXi’an Jiaotong UniversityXi’an 710049China International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China

It has been widely reported that,for faceted nanocrystals,the two adjacent facets with different band levels contribute to promoted charge separation,and provide active sites for photocatalytic reduction and oxidation reaction,*** such cases,only one family of facets can be used for photocatalytic hydrogen ***,by using SrTiO_(3)nanocrystals enclosed by{023}and{001}facets as a model photocatalyst,this paper proposed a strategy to achieve the full-facets-utilization of the nanocrystals for photocatalytic hydrogen via chemically depositing Pt nanoparticles on all *** photo-deposition experiment of CdS provided direct evidence to demonstrate that the{023}facets which were responsible for photooxidation reaction can be function-reversed for photocatalytic hydrogen evolution after depositing Pt nanoparticles,together with the{001}***,the full-facets-utilization led to a much-improved activity for photocatalytic hydrogen,in contrast to those SrTiO_(3)nanocrystals with only{001}facets deposited by Pt nanoparticles via a photo-deposition method.

关键词： SrTiO_(3)nanocrystals crystal facets photocatalysis hydrogen evolution

Investigation of Ce/BEA as a passive NO_(x)adsorber:*** occurrences of cerium and adsorption behavior

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Journal of Rare Earths 2024年第7期42卷 1265-1271,I0003页

作者： Minghui Yu Yiying Ding Xiaojie Yu Siwei Yan Meiqing shen Jianqiang Wang Jun Wang Gurong shen School of Materials Science and Engineering Tianjin UniversityTianjin300350China School of Chemical Engineering and Technology Tianjin UniversityTianjin300350China National Rare Earth Catalysis Research Institute Dongying257000China

Ce/BEA has great potential as a passive NO_(x)absorber(PNA)to reduce the NO_(x)emissions during the cold start phase especially in diesel engine for its high resistance to CO and suitable NO_(x)desorption temperature ***,as a novel material,its physical and chemical properties still remain *** this work,Ce/BEA was synthesized by ion-exchange method to identify the active species in NO_(x)adsorption,compared with aggregated Ce species in Ce/SiAlO_(x) prepared by impregnation method.X-ray diffraction(XRD),high resolution-transmission electron microscopy(HR-TEM)and aberration-corrected-scanning transmission electron microscopy(AC-STEM)were performed to confirm the isolated single atom formation of Ce species in Ce/***-vis diffraction reflection spectra(DRS)and X-ray photoelectron spectroscopy(XPS)were conducted to find the difference of chemical environment between the isolated Ce species and aggregated *** performance evaluation and temperature programmed reduction of hydrogen(H_(2)-TPR)results show the high NO_(x)storage capacity and active oxygen species quantity in Ce/*** is also found that the main NO_(x)adsorption species are Ce^(4+)-O^(∗)rather than Ce^(3+).NO_(x)-diffuse reflectance infrared Fourier transform spectroscopy(NO_(x)-DRIFTS)confirms that the bidentate nitrite species are the critical NO_(x)adsorption intermediates and the conception of NO_(x)adsorption and desorption processes is proposed.

关键词： Passive NO_(x)absorber Ce/BEA Isolated Ce species Rare earths

A Systematic Analysis of Early Life Exposure to the Chinese Famine(1959-1961)and the Health of Older Adults-China,2008-2023

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China CDC weekly 2024年第11期6卷 203-207,I0001-I0003页

作者： Chi shen Xi Chen School of Public Policy and Administration Xi’an Jiaotong UniversityXi’an CityShaanxi ProvinceChina Department of Health Policy and Management Yale School of Public HealthNew HavenCTU.S Department of Economics Yale UniversityNew HavenCTU.S

What is already known about this topic?There is mounting evidence indicating that the aging process initiates during early life stages,with in utero the individual’s environment playing a significant ***,it is crucial to comprehend the enduring effects of early life circumstances on health in old *** is added by this report?In this study,we conducted a meta-analysis to examine the effects of the Chinese Famine(1959–1961)on the health of older *** also explored potential mechanisms underlying these *** are the implications for public health practice?The complex interplay between early life circumstances,multiple health-related sectors,and healthy aging necessitates a comprehensive life-course approach and strategic interventions to enhance public health in an aging society.

关键词： life aging mount

Fabrication and Properties of a New Reactive Diluent for Cationic UV Curing

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Journal of Wuhan University of Technology(Materials Science) 2024年第4期39卷 1053-1060页

作者：吴正森黄笔武 LIU Yuansheng shen Han School of Physics and Materials Science Nanchang UniversityNanchang 330031China

The reactive diluent prepared by siloxane modified Trimethylene oxide can improve the performance of the UV curing ***,1,7-bis[(3-ethyl-3-methoxyoxacylobutane)propyl]octadecylosiloxane(BEMOPOMTS)was synthesized from diethyl carbonate,trimethylopropanes,allyl bromide,and 1,1,3,3,5,5,7,7-octadecylosiloxane as the main raw *** can be used as reactive diluents in the field of cationic UV *** has good thermal stability,and the addition of BEMOPOMTS significantly improves the tensile strength and elongation at break of epoxy *** with the pure epoxy resin,adding 20%BEMOPOMTS increased the elastic modulus by 25%to 677 MPa.

关键词： UV curing cation curing reactive diluent siloxane

Parallel Light Fields: A Perspective and A Framework

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 542-544页

作者： Fei-Yue Wang Yu shen IEEE State Key Laboratory for Management and Control of Complex Systems Institute of AutomationChinese Academy of SciencesBeijing 100190China School of Artificial Intelligence University of Chinese Academy of ScienceBeijing 100049

Dear Editor,Light fields give relatively complete description of scenes from perspective of angles and positions of rays. At present time, most of the computer vision algorithms take 2D images as input which are simplified expression of light fields with depth information discarded. In theory, computer vision tasks may achieve better performance as long as complete light fields are acquired.

关键词： computer Framework simplified

CMOS-level mega-pixel organic camera chips made of photocrosslinked photovoltaic nanocells

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Science China Materials 2024年第9期67卷 3043-3045页

作者： Yegang Liang Zhuoran Wang Guozhen shen School of Integrated Circuits and Electronics Beijing Institute of TechnologyBeijing100081China

Organic and hybrid optoelectronics have been driving the frontiers in displays,sensing,and energy in recent decades due to their superior performance,low-cost high-yield manufacturing,and new form factor of mechanical flexibility that is promising for lightweight and wearable applications[1-3].However,the inherent vulnerability makes organic semiconductors incompatible with conventional semiconductor microfabrication,posing significant challenges in high density integration to compete with the resolution of conventional image sensors[4].

关键词： frontier driving lightweight

High-performance flexible semiconductor fibres for multi-scenario communication applications

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Science China Materials 2024年第7期67卷 2363-2364页

作者： Qinghui Lin Yang Li Guozhen shen School of Information Science and Engineering University of JinanJinan 250022China School of Microelectronics Shandong UniversityJinan 250101China School of Integrated Circuits and Electronics Beijing Institute of Technology Beijing 100081China

With the advances in the field of flexible fibre technology in recent years,a variety of flexible fibres with different preparation processes have emerged[1,2].However,most of the flexible fibres in the past have structural breaks,making them unsuitable for long-term use as wearable fabrics[3,4].Glass semiconductors are widely used in thermally stretched fibres due to their advantages such as controllable fluidity,but they suffer from electronic defects compared with crystalline semi conductors in electronic semiconductors such as silicon(Si)and germanium(Ge)[5].Obviously,the semiconductor component in flexible optic fibres is a key component in regulating their mechanical and electrical properties[6].

关键词： wear fibres fibre

Tianmouc vision chip designed for open-world sensing

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Science China Materials 2024年第9期67卷 3046-3048页

作者： Haotian Li Qilin Hua Guozhen shen School of Integrated Circuits and Electronics Beijing Institute of TechnologyBeijing100081China Institute of Flexible Electronics Beijing Institute of TechnologyBeijing102488China

Driven by the forward development of highly interactive applications like autonomous robots and artificial intelligence[1,2],image sensors are continuously demanded to improve in terms of high speed,high resolution,wide dynamic range,and high precision[3].However,due to inherent limitations in power and bandwidth,significant enhancements in one aspect often necessitates compromises in others[4].

关键词： artificial interactive autonomous

Chipless textile electronics: human body-coupled fiber for wireless energy harvesting and signal transmission

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Science China Materials 2024年第7期67卷 2367-2368页

作者： Yixuan Wang Zuqing Yuan Guozhen shen School of Integrated Circuits and Electronics Beijing Institute of TechnologyBeijing 100081China

Wearable technology is rapidly advancing through the integration of electronic devices and textiles,enabling intelligent interaction between clothing and the surrounding *** electronics are specifically designed to provide functions such as sensing,computation,display,and ***,traditional wearable devices that rely on rigid von Neumann architectures and incorporate silicon chips face challenges in seamless integration,energy efficiency,and comfort[1–3].Difficulties arise when attempting to integrate complex circuits and electronic components,which are traditionally relied upon for signal modulation,into soft fibers[4,5].Recent reports have begun to explore alternative architectures for wearable devices that can incorporate electronics into a single fiber[6].However,this process presents challenges in simultaneously controlling energy capture and release within a single fiber.

关键词： fiber signal energy