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Multiphase Interfacial Regulation Based on Hierarchical Porous Molybdenum Selenide to Build Anticorrosive and Multiband Tailorable Absorbers

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Nano-Micro Letters 2024年第1期16卷 85-105页

作者： tianbao zhao Zirui Jia Jinkun Liu Yan Zhang Guanglei Wu Pengfei Yin College of Science Sichuan Agricultural UniversityYa’an 625014People’s Republic of China Institute of Materials for Energy and Environment State Key Laboratory of Bio‑Fibers and Eco‑TextilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071People’s Republic of China College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071People’s Republic of China

Electromagnetic wave(EMW)absorbing materials have an irreplaceable position in the field of military stealth as well as in the field of electromagnetic pollution *** in order to cope with the complex electromagnetic environment,the design of multifunctional and multiband high efficiency EMW absorbers remains a tremendous *** this work,we designed a three-dimensional porous structure via the salt melt synthesis strategy to optimize the impedance matching of the ***,through interfacial engineering,a molybdenum carbide transition layer was introduced between the molybdenum selenide nanoparticles and the three-dimensional porous carbon matrix to improve the absorption behavior of the *** analysis indicates that the number and components of the heterogeneous interfaces have a significant impact on the EMW absorption performance of the absorber due to mechanisms such as interfacial polarization and conduction loss introduced by interfacial ***,the prepared MoSe_(2)/MoC/PNC composites showed excellent EMW absorption performance in C,X,and Ku bands,especially exhibiting a reflection loss of−59.09 dB and an effective absorption bandwidth of 6.96 GHz at 1.9 *** coordination between structure and components endows the absorber with strong absorption,broad bandwidth,thin thickness,and multi-frequency absorption ***,it can effectively reinforce the marine anticorrosion property of the epoxy resin coating on Q235 steel *** study contributes to a deeper understanding of the relationship between interfacial engineering and the performance of EMW absorbers,and provides a reference for the design of multifunctional,multiband EMW absorption materials.

关键词： Interfacial engineering Anticorrosion Multiband Electromagnetic wave absorber

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Preface to the Special Issue on Causes, Impacts, and Predictability of Droughts for the Past, Present, and Future

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Advances in Atmospheric Sciences 2024年第2期41卷 191-192页

作者： tianbao zhao Aiguo DAI Jianping HUANG Lixia ZHANG Key Laboratory of Regional Climate-Environment Research for Temperate East Asia Institute of Atmospheric Physics(IAP)Chinese Academy of Sciences(CAS)Beijing 100029China Department of Atmospheric and Environmental Sciences University at AlbanySUNYAlbanyNew York 80307USA Key Laboratory for Semi-Arid Climate Change of the Ministry of Education Lanzhou UniversityLanzhou 730000China State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics(LASG) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

Drought is a recurring dry condition with below-normal precipitation and is often associated with warm temperatures or heatwaves. A drought event can develop slowly over several weeks or suddenly within days, commonly under abnormal atmospheric conditions(e.g., quasi-stationary high-pressure systems), and can persist for weeks, months, or even years.

关键词： drought within suddenly

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Self-assembly tungsten selenide hybrid ternary MOF derived magnetic alloys via multi-polarization to boost microwave absorption

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Nano Research 2024年第3期17卷 1625-1635页

作者： tianbao zhao Tingting Zheng Di Lan Yan Zhang Zhengshuo Sun Chao Wang Zirui Jia Guanglei Wu Institute of Materials for Energy and Environment State Key Laboratory of Bio-fibers and Eco-textilesCollege of Materials Science and EngineeringQingdao UniversityQingdao 266071China School of Materials Science and Engineering Hubei University of Automotive TechnologyShiyan 442002China College of Chemistry and Chemical Engineering Qingdao UniversityQingdao 266071China

Confronted with severe electromagnetic wave pollution,the development of high-performance electromagnetic wave shielding or absorbing materials is an effective way to deal with ***,double transition metal alloys and transition metal dichalcogenides have attracted extensive attention in electromagnetic wave absorption,but few reports have studied the effects of these two materials on electromagnetic wave absorption at the same *** this work,cobalt-based alloy with magnetic loss mechanism was selected for composition *** ternary metal-organic framework was prepared by the one-step method,and then CoCu/C was prepared by high temperature ***,in the hydrothermal process,ultra-thin tungsten selenide nanosheets were coated on the surface of magnetic component,and the final polyhedral WSe_(2)/CoCu/C composites with multiple heterogeneous interfaces were *** synergistic effect of dielectric and magnetic components optimizes impedance matching and allows more electromagnetic waves to enter the ***,through the conduction loss of high conductivity graphitized carbon,interfacial polarization,and dipole polarization of heterogeneous interfaces between the components,the magnetic loss provided by CoCu alloy can work together to maximize the attenuation ability of electromagnetic ***,the minimum reflection loss(RLmin)value of the composite reaches-53.43 dB when the matched thickness is 2.1 mm,while the maximum effective absorption bandwidth(EABmax)reaches 6.0 GHz at a thin thickness of 1.8 *** work provides some support and reference for the design of novel electromagnetic wave absorbing materials via the dielectric/magnetic loss synergistic mechanism.

关键词： metal-organic framework dielectric/magnetic loss transition metal dichalcogenide electromagnetic wave absorption

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我国西北地区干湿变化特征及其未来预估

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气候与环境研究 2024年第1期29卷 59-74页

作者：李学武张京朋赵天保李福原赵廷宁国家林业和草原局林草调查规划院北京100714 北京林业大学水土保持学院北京100083 河海大学海洋学院南京210098 西北农林科技大学资源环境学院陕西杨凌712100 中国科学院大气物理研究所东亚区域气候—环境重点实验室北京100029

基于降水量、土壤湿度、径流量和干旱指数等多种气象要素,系统分析研究了近60年我国西北地区的干湿特征演变规律,并利用最新的第六次国际耦合模式比较计划(CMIP6)多模式模拟结果对该区域未来干湿变化特征进行了预估。结果显示:近60年来... 详细信息

基于降水量、土壤湿度、径流量和干旱指数等多种气象要素,系统分析研究了近60年我国西北地区的干湿特征演变规律,并利用最新的第六次国际耦合模式比较计划(CMIP6)多模式模拟结果对该区域未来干湿变化特征进行了预估。结果显示:近60年来我国西北地区的降水量、土壤湿度和径流量均呈现出由东南向西北递减的空间分布格局;冷季的降水量和径流量明显低于暖季,但土壤湿度和干旱指数在冷暖季节差异不显著。西北地区年降水量、土壤湿度和干旱指数均呈现显著增加的趋势,增幅分别为5.07 mm/10 a、3.89 mm/10 a和0.26/10 a,特别是2000年后增加的趋势更显著,且变湿幅度最大主要出现在西北西部;而径流量在2000年之前呈现明显下降的趋势,而2000年后显著增加。在未来气候变化情境下,21世纪中期(2031~2060年)和后期(2071~2100年)西北地区呈现出湿润化的趋势,并且21世纪后期的湿润化程度更显著,高等排放情景(SSP5-8.5)比中等排放情景(SSP2-4.5)下湿润化更明显。本研究可为我国西北地区气候变化的影响评估提供参考依据。

关键词：西北地区干湿特征 CMIP6 模式未来预估

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CMIP6模式模拟的人类活动和自然强迫对全球地表气温多尺度变化的影响

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地球物理学报 2024年第2期67卷 477-491页

作者：徐川赵天保张京朋陶丽南京信息工程大学大气科学学院南京210044 中国科学院东亚区域气候-环境重点实验室北京100029 西北农林科技大学资源环境学院陕西杨凌712100

量化人类活动在气候变化中的定量贡献是气候变化检测归因研究的核心科学问题,也是提高气候变化预测和预估水平的重要科学基础.本文基于最新的第6次国际耦合模式比较计划(CMIP6)多模式历史归因模拟试验(DAMIP),检测了人为因素(ANT)和自... 详细信息

量化人类活动在气候变化中的定量贡献是气候变化检测归因研究的核心科学问题,也是提高气候变化预测和预估水平的重要科学基础.本文基于最新的第6次国际耦合模式比较计划(CMIP6)多模式历史归因模拟试验(DAMIP),检测了人为因素(ANT)和自然因素(NAT)对近百年(1915—2014年)全球地表气温多尺度变化的影响,归因了温室气体(GHG)、气溶胶(AA)、土地利用(LU)等不同人为因素对全球地表气温长期变化的相对贡献及南北半球差异.结果显示,近百年来人为因素引起的全球陆地实际增温约为1.1℃(0.8℃~1.3℃),对南北半球的贡献则分别约为0.7℃和1.2℃;全球大多数区域人为排放GHG和AA的显著作用在1960—1980年期间就能够被检测到,其中北半球AA的冷却作用要超前于GHG的增温效应;气候系统内部自然变率是调制大多数区域气温年代际(10~30年)及多年代际变率(30~60年)的主导因子,而人为和自然外强迫在全球地表气温年代际变率中的方差贡献约为5%~20%,但二者在北半球尤其在东亚和欧洲中高纬度地区地表气温多年代际变率中的方差贡献可达50%.人为因素强迫可使近50年(1965—2014)极端高温事件的发生风险概率增加3倍,其中北半球发生风险要高于南半球.

关键词： CMIP6模式多尺度气温变化人类活动检测归因

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Future Drought Changes in China Projected by the CMIP6 Models:Contributions from Key Factors

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气象学报:英文版 2023年第4期37卷 454-468页

作者： Qingxin CHEN tianbao zhao Lijuan HUA Jinhua YU Yafang WANG Chuan XU Key Laboratory of Meteorological Disaster Ministry of Education(KLME)/Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters(CIC-FEMD)Nanjing University of Information Science&TechnologyNanjing 210044 Key Laboratory of Regional Climate–Environment Research for Temperate East Asia Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100083 College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijing 100049 Collaborative Innovation Center for Western Ecological Safety College of Atmospheric SciencesLanzhou UniversityLanzhou 730000 College of Atmospheric Sciences Nanjing University of Information Science&TechnologyNanjing 210044

Model simulations show that drought may become more severe and widespread in the 21st century due to humaninduced global warming. However, the contributions from the key factors to the model-projected drought changes in China have not yet been examined in detail. We used the self-calibrated Palmer Drought Severity Index with Penman–Monteith potential evapotranspiration(scPDSIpm) based on 10 model simulations selected from the Coupled Model Intercomparison Project Phase 6(CMIP6). We investigated the contributions from precipitation(P), near-surface air temperature and specific humidity [Δ(T + q)], net surface longwave radiation(LW), net surface shortwave radiation(SW), and wind speed(WS) to the future changes in scPDSIpm, including the long-term mean, drying area,probability distribution function(PDF), drought frequency, and drought duration based on the scPDSIpm over *** results show that model-projected drying mainly occurs over southern China, whereas the dry areas under drought conditions increase from 20% to about 23%/30% under the two scenarios of the shared socioeconomic pathway(SSP2-4.5/SSP5-8.5) from 1985 to 2100, despite large uncertainties in individual projections partly due to internal variability. Drought frequency is projected to increases by about 10%–54%(15%–88%) under the SSP2-4.5(SSP5-8.5) scenario by the late 21st century, along with increases in drought duration. These changes are accompanied by a decrease in the mean scPDSIpm and flattening of the PDFs. The changes in drying over southern China are mainly attributed to surface warming and the increased surface vapor pressure deficit(VPD), with small contributions from changes in the surface net radiation. The changes in wetting over northern China mostly result from increased precipitation along with a small wetting effect from the changes in wind speed.

关键词： drought future projection key factors China Coupled Model Intercomparison Project Phase 6

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Simulation of historical and projected climate change in arid and semiarid areas by CMIP5 models

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Chinese Science Bulletin 2014年第12期59卷 412-429页

作者： tianbao zhao Liang Chen Zhuguo Ma Key Laboratory of Regional Climate-Environment Research for East Asia Institute of Atmospheric Physics (IAP) Chinese Academy of Sciences (CAS)

Based on Climatic Research Unit Time Series3.1 temperature and Global Precipitation Climatology Center full data reanalysis version 6 precipitation data,the abilities of climate models from the fifth phase of the Coupled Model Intercomparison Project to simulate climate changes over arid and semiarid areas were *** of future climate changes under different representative concentration pathways(RCPs)were also *** key findings were that most of the models are able to capture the dominant features of the spatiotemporal changes in temperature,especially the geographic distribution,during the past 60 years,both globally as well as over arid and semiarid *** addition,the models can reproduce the observed warming trends,but with magnitudes generally less than the observations of around0.1–0.3°C/*** to temperature,the models perform worse in simulating the annual evolution of observed precipitation,underestimating both the variability and tendency,and there is a huge spread among the models in terms of their simulated precipitation *** multimodel ensemble mean is overall superior to any individual model in reproducing the observed climate *** terms of future climate change,an ongoing warming projected by the multi-model ensemble over arid and semiarid areas can clearly be seen under different RCPs,especially under the high emissions scenario(RCP8.5),which is twice that of the moderate scenario(RCP4.5).Unlike the increasing temperature,precipitation changes vary across areas and are more significant under high-emission RCPs,with more precipitation over wet areas but less precipitation over dry *** particular,northern China is projected to be one of the typical areas experiencing significantly increased temperature and precipitation in the future.

关键词：未来气候变化半干旱地区仿真模型模拟降水量模拟观测预测历史降水资料

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Multi-process production occurs in the iron and steel industry,supporting‘dual carbon'target:An in-depth study of CO_(2)emissions from different processes

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Journal of Environmental Sciences 2024年第6期140卷 46-58页

作者： Hongming Na Yuxing Yuan Tao Du tianbao Zhang Xi zhao Jingchao Sun Ziyang Qiu Lei Zhang SEP Key Laboratory of Eco-Industry Northeastern UniversityShenyang 110819China School of Metallurgy Northeastern UniversityShenyang 110819China

Reducing CO_(2)emissions of the iron and steel industry,a typical heavy CO_(2)-emitting sector is the only way that must be passed to achieve the‘dual-carbon’goal,especially in *** previous studies,however,it is still unknown what is the difference between blast furnace basic oxygen furnace(BF-BOF),scrap-electric furnace(scrap-EF)and hydrogen metallurgy *** quantitative research on the key factors affecting CO_(2)emissions is insufficient There is also a lack of research on the prediction of CO_(2)emissions by adjusting industria *** on material flow analysis,this study establishes carbon flow diagrams o three processes,and then analyze the key factors affecting CO_(2)***_(2)emissions of the iron and steel industry in the future is predicted by adjusting industrial structure The results show that:(1)The CO_(2)emissions of BF-BOF,scrap-EF and hydrogen metallurgy process in a site are 1417.26,542.93 and 1166.52 kg,respectively.(2)By increasing pellet ratio in blast furnace,scrap ratio in electric furnace,etc.,can effectively reduce CO_(2)emissions(3)Reducing the crude steel output is the most effective CO_(2)reduction *** is still 5.15×10^(8)-6.17×10^(8) tons of CO_(2)that needs to be reduced by additional measures.

关键词： Blast furnace-basic oxygen furnace process Scrap-electric furnace process Hydrogen metallurgy process Carbon flow diagram Influencing factors CO_(2)emission prediction

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Evaluation of Daily Precipitation Product in China from the CMA Global Atmospheric Interim Reanalysis

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Journal of Meteorological Research 2020年第1期34卷 117-136,1-4页

作者： Chunxiang LI tianbao zhao Chunxiang SHI Zhiquan LIU Key Laboratory of Regional Climate-Environment Research for East Asia Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029 National Meteorological Information Center China Meteorological AdministrationBeijing 100081

The China Meteorological Administration(CMA)recently produced a CMA Global Atmospheric Interim Reanalysis(CRAI)dataset for the years 2007–2016.A comprehensive evaluation of the ability of CRAI to capture the spatiotemporal variability of observed precipitation,in terms of both mean states and extreme indicators over China,is *** are made with other current reanalysis datasets,namely,the ECMWF interim reanalysis(ERAI),Japanese 55-yr reanalysis(JRA55),NCEP Climate Forecast System Reanalysis(CFSR),and NASA Modern-Era Retrospective analysis for Research and Applications version 2(MERRA2),as well as NCEP Climate Prediction Center(CPC)*** results show that,for daily variations of rainfall during warm seasons in eastern China,CRAI and CFSR overestimate the precipitation of the main rain belt,while the overestimation is confined to the area south of 25°N in JRA55 but north of 24°N in MERRA2;whereas ERAI tends to underestimate the precipitation in most regions of eastern *** extreme metrics,the total amount of precipitation on days where daily precipitation exceeds the 95 th percentile(R95 pTOT)and the number of consecutive dry days(CDDs)in one month,are examined to assess the performance of reanalysis *** terms of extreme events,CRAI,ERAI,and JRA55 tend to underestimate the R95 pTOT in most of eastern China,whereas more frequent extreme rainfall can be found in most regions of China in both CFSR and MERRA2;and all of the reanalyses underestimate the *** the reanalysis products,CRAI and JRA55 show better agreement with the observed R95 pTOT than the other datasets,with fewer biases,higher correlation coefficients,and much more similar linear trend patterns,while ERAI stands out in better capturing the amount and temporal variations of the observed CDDs.

关键词： China Meteorological Administration(CMA) the CMA Global Atmospheric Interim Reanalysis(CRAI) precipitation daily

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Historical Changes and Future Projections of Extreme Temperature and Precipitation along the Sichuan-Tibet Railway

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Journal of Meteorological Research 2021年第3期35卷 402-415页

作者： Jingpeng ZHANG tianbao zhao Libo ZHOU Lingkun RAN College of Natural Resources and Environment Northwest A&F UniversityYanglingShaanxi 712100 Key Laboratory of Regional Climate-Environment Research for East Asia Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029 Department of Lower Atmosphere Observation Research Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029 State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029 Key Laboratory of Cloud-Precipitation Physics and Severe Storms Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029

Based on multiresource high-resolution in situ and satellite merged observations along with model simulations from the Coordinated Regional Climate Downscaling Experiment(CORDEX),this study first investigated historical changes in extreme temperature and precipitation during the period of 1979-2018 in areas along the Sichuan-Tibet Railway,and then projected the future changes in the frequency and intensity of extreme temperature and precipitation under the RCP(Representative Concentration Pathway)4.5 and 8.5 *** paper is expected to enhance our understanding of the spatiotemporal variability in the extreme temperature and precipitation along the Sichuan-Tibet Railway,and to provide scientific basis to advance the Sichuan-Tibet Railway construction and *** results show that temperatures in the Sichuan-Tibet region display a noticeable warming trend in the past 40 years,and the increase of minimum temperature is significantly higher than that of maximum temperature in the northwest of the *** increase of precipitation is found mainly over the northwest of the Tibetan *** for Lhasa and its surrounding areas,precipitation over other areas along the Sichuan-Tibet Railway shows no significant change in the past 40 years,as indicated in five datasets;however,precipitation along the railway has shown a remarkable decrease in the past 20 years in the TRMM satellite *** warm days and nights have clearly increased by 6 and 5 day decade1-for 1979-2019,while cold days and nights have markedly decreased by about 6.6 and 3.6 day decade-1,*** the past 20 years,the areas with increased precipitation from very wet days and extremely wet days are mainly distributed to the north of the Sichuan-Tibet Railway,while in the areas along the railway itself,the very wet days and extremely wet days are *** RCPs 4.5 and 8.5,the temperature in the Sichuan-Tibet region will increase significantly,and the frequency of

关键词： Sichuan-Tibet Railway extreme temperature and precipitation historical change future projection

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