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Hydrodechlorination of trifluoro-trichloroethane to chlorotrifluoroethylene:Revealing the deactivation mechanism and regeneration strategy of Pd-Cu/AC catalyst

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Chinese Journal of Chemical Engineering 2024年第6期70卷 261-268页

作者： Song tian Yicheng Chen Xiaoyu Wen Bingcheng Li jian Lu Zile Li Feng Feng Qingtao Wang Qunfeng Zhang Xiaonian Li State Key Laboratory Breeding Base of Green Chemistry Synthesis Technology Institute of Industrial Catalysis of Zhejiang University of TechnologyHangzhou 310014China State Key Laboratory of Fluorine&Nitrogen Chemicals Xi'an Modern Chemistry Research InstituteXi'an 710065China

Chlorotrifluoroethylene(CTFE)is a vital fluorinated olefinic monomer produced through the catalytic hydrodechlorination of trichlorotrifluoroethane(CFC-113),an eco-friendly ***,hydrodechlorination catalysts for olefin production often suffer from poor *** Pd/AC catalyst and Pd-Cu/AC catalyst prepared by co-impregnation method exhibited poor stability,Pd-Cu/AC catalyst with CFC-113 conversion dropping to around 37%after 50 h of hydrodechlorination ***-Emmett-Teller,transmission electron microscopy,X-ray photoelectron spectroscopy,and X-ray diffraction of fresh and deactivated Pd/AC catalysts indicate that the deactivation of Pd/AC catalysts is due to high-temperature agglomeration of *** analysis of fresh and deactivated Pd-Cu/AC catalysts using Brunauer-Emmett-Teller,transmission electron microscopy,and thermogravimetric analysis techniques revealed decreased dispersion of active sites,reduced surface area,catalyst aggregation deactivation,and a significant decrease in Cu ***,the results of NH3-TPD revealed that the acid sites of the catalyst increased significantly.X-ray diffraction spectra indicated the formation of new species,basic copper chloride(Cu_(2)(OH)_(3)Cl),during the *** the reaction progressed,these new species agglomerated,leading to a gradual loss of catalyst ***,the deactivated catalyst was successfully reactivated using a simple alkaline washing method.

关键词： CFC-113 Hydrodechlorination Chlorotrifluoroethylene Catalyst deactivation

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Effect of cooling method on TiN precipitation behavior of high-titanium high-strength steel during solidification

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Journal of Iron and Steel Research International 2024年第7期31卷 1692-1703页

作者： Xue-jian Zhang Guang-wei Yang Yong Wan Yong-hong Wen Chuan-sheng Tang Ming-qi Liu Li-jie tian Key Laboratory of Metallurgical Emission Reduction and Resources Recycling Anhui University of TechnologyMa'anshan 243002AnhuiChina School of Metallurgical Engineering Anhui University of TechnologyMa'anshan 243002AnhuiChina Baosteel Central Research Institute Baoshan Iron and Steel Co.Ltd.Shanghai 201999China

Metallographic microscopy,scanning electron microscopy and TiN growth thermodynamic and kinetic equations were used to investigate the morphology,quantity,and size of TiN in the center of high-titanium high-strength steels under different solidification cooling *** results showed that TiN in the center of the experimental steels mainly existed in three forms:single,composite(Al2O3-TiN),and multi-particle *** began precipitating at around 1497℃(solidification fraction of 0.74).From the end of melting to solidification for 180 s,the cooling rates in the center of the experimental steels for furnace cooling,air cooling,refractory mold cooling,and cast iron mold cooling tended to stabilize at 0.17,0.93,1.65,and 2.15℃/s,*** size of TiN in the center of the experimental steel cooled using furnace cooling was mainly concentrated in the 5-15 pm *** contrast,the size of TiN in the center of the experimental steels cooled using air cooling,refractory mold cooling,and cast iron mold cooling were mainly concentrated in the 1-5 pm *** addition,their density of TiN in the center of the experimental steels is signif-icantly higher than that of the furnace-cooled experimental *** and kinetic precipitation models of TiN established predicted the growth size of TiN in a high-titanium high-strength steel when the solidification cooling rates are not below 0.93℃/s.

关键词： High-titanium steel Cooling method TiN Thermodynamics Kinetics

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Change in self-image pressure level before and after autologous fat breast augmentation and its effect on social adaptability

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World Journal of Psychiatry 2024年第6期14卷 920-929页

作者： jian Li Hui-Min Wang Yang jiang zhen-Nan Liu Bai-Hui He Department of Plastic Surgery The First Affiliated Hospital of Xinxiang Medical UniversityXinxiang 453100Henan ProvinceChina Department of Otolaryngology The First Affiliated Hospital of Xinxiang Medical UniversityXinxiang 453100Henan ProvinceChina

BACKGROUND There is an increasingly strong demand for appearance and physical beauty in social life,marriage,and other aspects with the development of society and the improvement of material living *** increasing number of people have improved their appearance and physical shape through aesthetic plastic *** female breast plays a significant role in physical beauty,and droopy or atrophied breasts can frequently lead to psychological inferiority and lack of confidence in ***,in turn,can affect their mental health and quality of *** To analyze preoperative and postoperative self-image pressure-level changes of autologous fat breast augmentation patients and their impact on social *** We selected 160 patients who underwent autologous fat breast augmentation at the First Affiliated Hospital of Xinxiang Medical University from January 2020 to December 2022 using random sampling *** general information,selfimage pressure level,and social adaptability of the patients were investigated using a basic information survey,body image self-assessment scale,and social adaptability *** self-image pressure-level changes and their effects on the social adaptability of patients before and after autologous fat breast augmentation were *** We collected 142 valid *** single-factor analysis results showed no statistically significant difference in the self-image pressure level and social adaptability score of patients with different ages,marital status,and monthly ***,there were significant differences in social adaptability among patients with different education levels and employment *** correlation analysis results revealed a significant correlation between the self-image pressure level and social adaptability score before and after *** factors analysis results showed that the degree of concern caused by appearance in selfimage pressure,the degree of possible behavior

关键词： Autologous fat breast augmentation surgery Self-image stress level Social adaptability Analysis of correlation Structural equation model

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Design and implementation of code acquisition using sparse Fourier transform

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Journal of Systems Engineering and Electronics 2024年第5期35卷 1063-1072页

作者： ZHANG Chen WANG jian FAN Guangteng tian Shiwei College of Electronic Science and Technology National University of Defense TechnologyChangsha 410073China National Innovation Institute of Defense Technology Academy of Military ScienceBeijing 100071China

Code acquisition is the kernel operation for signal synchronization in the spread-spectrum *** reduce the computational complexity and latency of code acquisition,this paper proposes an efficient scheme employing sparse Fourier transform(SFT)and the relevant hardware architecture for field programmable gate array(FPGA)and application-specific integrated circuit(ASIC)*** are made at both the algorithmic level and the implementation level to enable merged searching of code phase and Doppler frequency without incurring massive hardware *** with the existing code acquisition approaches,it is shown from theoretical analysis and experimental results that the proposed design can shorten processing latency and reduce hardware complexity without degrading the acquisition probability.

关键词： code acquisition hardware structure sparse Fourier transform(SFT) code phase estimation Doppler frequency estimation

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Characteristics of long-distance mobile mRNAs from shoot to root in grafted plant species

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Horticultural Plant Journal 2024年第1期10卷 25-37页

作者： Mengmeng Fu zhen Xu Huaying Ma Yifan Hao Ji tian Yi Wang Xinzhong Zhang Xuefeng Xu zhenhai Han Ting Wu College of Horticulture China Agricultural UniversityBeijing 100193China Plant Science and Technology College Beijing University of AgricultureBeijing 102206China

Thousands of long-distance mobile mRNAs were identified from different grafting systems,based on high-throughput sequencing ***,the long-distance delivery of RNAs was proved to involve multiple ***,we analyzed the homology,motif,and tRNA-like structure(TLS)of long-distance mobile mRNAs identified by RNA-seq as well as the RNA-binding protein(RBP)in nine grafting combinations including Arabidopsis thaliana,Vitis vinifera,Cucumis sativus,Citrullus lanatus,Nicotiana benthamiana,Malus domestica,Pyrus spp.,Glycine max and Phaseolus *** several mRNAs were found to be shared in herbaceous,woody,and related species,the vast majority of long-distance mobile mRNAs were *** non-specific movement-related motifs were identified,while the TLS was not necessary for mRNA long distance *** addition,we found that RBPs were conserved among herbaceous and woody plants as well as related *** paper reports a further in-depth analysis of the endogenous mechanisms by which the species-specific transportable m RNAs were selected by bioinformatics,in order to provide insights for future research on long-distance mobile mRNAs.

关键词： Grafting combination Long-distance mobile mRNA TLS RNA binding proteins

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Calmodulin-like 5 promotes PEDV replication by regulating late-endosome synthesis and innate immune response

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Virologica Sinica 2024年第3期39卷 501-512页

作者： Wen-Jun tian Xiu-Zhong Zhang Jing Wang jian-Feng Liu Fu-Huang Li Xiao-Jia Wang National Key Laboratory of Veterinary Public Health and Safety College of Veterinary MedicineChina Agricultural UniversityBeijing 100193China College of Animal Science and Technology China Agricultural UniversityBeijing 100193China Beijing General Station of Animal Husbandry Service(South Section) Beijing102218China

The infection caused by porcine epidemic diarrhea virus(PEDV)is associated with high mortality in piglets *** factors involved in the efficient replication of PEDV,however,remain largely *** recent proteomic study in the virus-host interaction network revealed a significant increase in the accumulation of CALML5(EF-hand protein calmodulin-like 5)following PEDV infection.A further study unveiled a biphasic increase of CALML5 in 2 and 12 h after viral *** trends were observed in the intestines of piglets in the early and late stages of the PEDV ***,CALML5 depletion reduced PEDV mRNA and protein levels,leading to a one-order-of-magnitude decrease in virus *** the early stage of PEDV infection,CALML5 affected the endosomal trafficking pathway by regulating the expression of endosomal sorting complex related cellular ***5 depletion also suppressed IFN-βand IL-6 production in the PEDV-infected cells,thereby indicating its involvement in negatively regulating the innate immune *** study reveals the biological function of CALML5 in the virology field and offers new insights into the PEDV-host cell interaction.

关键词： Porcine epidemic diarrhea virus(PEDV) EF-hand protein calmodulin-like 5(CALML5) Late endosomes Innate immune response

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Wideband spectrum sensing using step-sampling based on the multipath nyquist folding receiver

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Defence Technology（防务技术） 2024年第1期31卷 523-536页

作者： Kai-lun tian Kai-li jiang Sen Cao jian Gao Ying Xiong Bin Tang Xu-ying Zhang Yan-fei Li University of Electronic Science and Technology of China Chengdu611731China China Electronics Technology Group Corporation 29th Research Institute Chengdu610036China

Wideband spectrum sensing with a high-speed analog-digital converter(ADC) presents a challenge for practical *** Nyquist folding receiver(NYFR) is a promising scheme for achieving cost-effective real-time spectrum sensing,which is subject to the complexity of processing the modulated *** this case,a multipath NYFR architecture with a step-sampling rate for the different paths is *** different numbers of digital channels for each path are designed based on the Chinese remainder theorem(CRT).Then,the detectable frequency range is divided into multiple frequency grids,and the Nyquist zone(NZ) of the input can be obtained by sensing these ***,high-precision parameter estimation is performed by utilizing the NYFR *** with the existing methods,the scheme proposed in this paper overcomes the challenge of NZ estimation,information damage,many computations,low accuracy,and high false alarm *** simulation experiments verify the effectiveness of the proposed architecture in this paper.

关键词： Wideband spectrum sensing Sub-Nyquist sampling Step-sampling Nyquist folding receiver(NYFR) Multisignal processing

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An open access dataset for strong-motion data(PGA,PGV,and Site V_(S30))of 2023 M6.2 Jishishan,Gansu,China earthquake

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Earthquake Science 2024年第6期37卷 584-587页

作者： jian Zhou Li Li Nan Xi Kun Chen Xin tian Chao Wang Jifeng tian Institute of Geophysics China Earthquake AdministrationBeijing 100081China China Earthquake Network Center Beijing 100045China

*** On December 18,2023,a M6.2 earthquake struck central China with epicenter at Jishishan,Gansu(35.70°N,102.79°E).In the USGS Latest Earthquake platform,the event was identified as M_(W)5.9,35.743°N,102.827°E,labeled 37 km WNW of Linxia Chengguanzhen,*** study presents an open-access dataset comprising PGA and PGV records of the main-shock from 202accelerometers and 539 Micro-Electro-Mechanical System(MEMS)sensors within two arcdegrees of the epicenter.

关键词： China. earthquake epicenter

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A 128×128 SPAD LiDAR sensor with column-parallel 25 ps resolution TA-ADCs

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Journal of Semiconductors 2024年第8期45卷 34-40页

作者： Na tian Zhe Wang Kai Ma Xu Yang Nan Qi jian Liu Nanjian Wu Runjiang Dou Liyuan Liu State Key Laboratory of Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijing 100049China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

This paper presents a design of single photon avalanche diode(SPAD)light detection and ranging(LiDAR)sensor with 128×128 pixels and 128 column-parallel time-to-analog-merged-analog-to-digital converts(TA-ADCs).Unlike the conventional TAC-based SPAD LiDAR sensor,in which the TAC and ADC are separately implemented,we propose to merge the TAC and ADC by sharing their capacitors,thus avoiding the analog readout noise of TAC’s output buffer,improving the conversion rate,and reducing chip *** reverse start-stop logic is employed to reduce the power of the *** in a 180 nm CMOS process,our prototype sensor exhibits a timing resolution of 25 ps,a DNL of+0.30/−0.77 LSB,an INL of+1.41/−2.20 LSB,and a total power consumption of 190 mW.A flash LiDAR system based on this sensor demonstrates the function of 2D/3D imaging with 128×128 resolution,25 kHz inter-frame rate,and sub-centimeter ranging precision.

关键词： 3D imaging CMOS imagers direct time-of-flight(dTOF) time-to-analog converter(TAC)

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Spatio-temporal Variation Characteristics of Extreme Climate Events and Their Teleconnections to Large-scale Ocean-atmospheric Circulation Patterns in Huaihe River Basin,China During 1959–2019

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Chinese Geographical Science 2024年第1期34卷 118-134页

作者： YAO tian ZHAO Qiang WU Chuanhao HU Xiaonong XIA Chuan'an WANG Xuan SANG Guoqiang LIU jian WANG Haijun School of Water Conservancy and Environment University of JinanJinan250022China Yangtze Institute for Conservation and Development Hohai UniversityNanjing210098China Zijin School of Geology and Mining Fuzhou UniversityFuzhou350108China Water Research Institute of Shandong Province Jinan250014China Shandong Provincial Bureau of Hydrology and Water Resources Jinan250100China

Huaihe River Basin(HRB) is located in China’s north-south climatic transition zone,which is very sensitive to global climate *** on the daily maximum temperature,minimum temperature,and precipitation data of 40 meteorological stations and nine monthly large-scale ocean-atmospheric circulation indices data during 1959–2019,we present an assessment of the spatial and temporal variations of extreme temperature and precipitation events in the HRB using nine extreme climate indices,and analyze the teleconnection relationship between extreme climate indices and large-scale ocean-atmospheric circulation *** results show that warm extreme indices show a significant(P < 0.05) increasing trend,while cold extreme indices(except for cold spell duration) and diurnal temperature range(DTR) show a significant decreasing ***,all extreme temperature indices show significant mutations during ***,a stronger warming trend occurs in eastern HRB than western HRB,while maximum 5-d precipitation(Rx5day) and rainstorm days(R25) show an increasing trend in the southern,central,and northwestern regions of *** oscillation(AO),Atlantic multidecadal oscillation(AMO),and East Atlantic/Western Russia(EA/WR) have a stronger correlation with extreme climate indices compared to other circulation *** and AMO(EA/WR) exhibit a significant(P < 0.05) negative(positive)correlation with frost days and diurnal temperature *** warm events are strongly correlated with the variability of AMO and EA/WR in most parts of HRB,while extreme cold events are closely related to the variability of AO and AMO in eastern *** contrast,AMO,AO,and EA/WR show limited impacts on extreme precipitation events in most parts of HRB.

关键词： extreme climate indices Sen’s slope variation mutation test atmospheric circulation indices Pearson’s correlation analysis Huaihe River Basin(HRB),China

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