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Photogenerated singlet oxygen over zeolite-confined carbon dots for shape selective catalysis

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Science China Chemistry 2019年第4期62卷 434-439页

作者： Qiu-Ying Yu Guang-Yao Zhai tian-lu cui Hui Su Zhong-Hua Xue Jun-Jun Zhang Peter J.Pauzauskie Shin-ichi Hirano Xin-Hao Li Jie-Sheng Chen School of Chemistry and Chemical Engineering Shanghai Jiao Tong University Department of Materials Science & Engineering University of Washington Hirano Institute for Materials Innovation Shanghai Jiao Tong University

Singlet oxygen as an activated oxygen species played an important role in organic synthesis. Suitable catalyst for converting ubiquitous oxygen molecule to singlet oxygen under mild conditions has attracted a wide range of attention. Herein, carbon dots have been confined into mesopores of silicalite-1 nanocrystals framework and acted as active sites for generation of singlet oxygen. The high oxygen-adsorption capacity of zeolite nanocrystals facilitated the photocatalytic generation rate of singlet oxygen, outpacing the free-standing carbon dots for 14-fold. The integrated carbon dot-zeolite nanocrystal hybrid also exhibited a special size-dependent selectivity for organic synthesis by using the in situ formed and confined singlet oxygen as active oxygen species.

关键词： zeolite photocatalysis singlet oxygen carbon dots shape-selective

Research status and prospects of the fractal analysis of metal material surfaces and interfaces

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 20-38页

作者： Qinjin Dai Xuefeng Liu Xin Ma Shaojie tian Qinghe cui Beijing Advanced Innovation Center for Materials Genome Engineering University of Science and Technology BeijingBeijing 100083China Beijing Laboratory of Metallic Materials and Processing for Modern Transportation University of Science and Technology BeijingBeijing 100083China Laboratory for Advanced Materials Processing of Ministry of Education University of Science and Technology BeijingBeijing 100083China School of Mechanical and Electrical Engineering Xinjiang Institute of EngineeringUrumqi 830023China

As a mathematical analysis method,fractal analysis can be used to quantitatively describe irregular shapes with self-similar or self-affine *** analysis has been used to characterize the shapes of metal materials at various scales and *** methods make it difficult to quantitatively describe the relationship between the regular characteristics and properties of metal material surfaces and ***,fractal analysis can be used to quantitatively describe the shape characteristics of metal materials and to establish the quantitative relationships between the shape characteristics and various properties of metal *** the perspective of two-dimensional planes and three-dimensional curved surfaces,this paper reviews the current research status of the fractal analysis of metal precipitate interfaces,metal grain boundary interfaces,metal-deposited film surfaces,metal fracture surfaces,metal machined surfaces,and metal wear *** relationship between the fractal dimensions and properties of metal material surfaces and interfaces is *** from three perspectives of fractal analysis,namely,research scope,image acquisition methods,and calculation methods,this paper identifies the direction of research on fractal analysis of metal material surfaces and interfaces that need to be *** is believed that revealing the deep influence mechanism between the fractal dimensions and properties of metal material surfaces and interfaces will be the key research direction of the fractal analysis of metal materials in the future.

关键词： metal material surfaces and interfaces fractal analysis fractal dimension homogeneity

解淀粉芽孢杆菌wxy-b3产脂肽类物质对苹果斑点落叶病菌的抑菌活性研究

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陕西科技大学学报 2025年第1期43卷 46-51页

作者：崔皓玥田露胡乐梅龚国利陕西科技大学食品科学与工程学院陕西西安710021

苹果斑点落叶病菌是苹果生产过程中常见的病害,严重危害苹果农作物的产量.脂肽作为一种主要来源于微生物次生代谢产物的抗菌剂,具有广谱抑菌、低耐药性、安全低毒等优势.本研究发现,解淀粉芽孢杆菌wxy-b3产生的脂肽类物质能够抑制苹果... 详细信息

苹果斑点落叶病菌是苹果生产过程中常见的病害,严重危害苹果农作物的产量.脂肽作为一种主要来源于微生物次生代谢产物的抗菌剂,具有广谱抑菌、低耐药性、安全低毒等优势.本研究发现,解淀粉芽孢杆菌wxy-b3产生的脂肽类物质能够抑制苹果斑点落叶病菌的生长,对苹果斑点落叶病菌的最小抑菌浓度为16 mg/mL,此浓度可造成该病原菌细胞膜电位超极化、线粒体膜电位去极化、大分子蛋白质和核酸泄露,以及胞内活性氧和丙二醛含量分别累积增加0.33倍和5.44倍,并通过扫描电镜进一步观察到MIC处理组的细胞形态起皱、细胞膜破损.上述结果表明,脂肽可能通过破坏细胞膜系统,导致细胞形态发生变化,细胞膜破裂,改变细胞膜通透性来达到抑菌效果.该研究将为脂肽作为抑制苹果斑点落叶病菌的抗菌剂奠定理论基础.

关键词：解淀粉芽孢杆菌脂肽类物质苹果斑点落叶病菌抑菌活性

Pt nanoclusters modified porous g-C_(3)N_(4)nanosheets to significantly enhance hydrogen production by photocatalytic water reforming of methanol

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Chinese Journal of Chemical Engineering 2024年第2期66卷 40-50页

作者： Yi-Fei Liang Jin-Rong lu Shang-Kun tian Wen-Quan cui Li Liu Hebei Provincial Key Laboratory of Environmental Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshan 063210China

For the use of green hydrogen energy,it is crucial to have efficient photocatalytic activity for hydrogen generation by water reforming of methanol under mild *** attention has been paid to gC_(3)N_(4)as a promising photocatalyst for the generation of *** improve the separation of photogenerated charge,porous nanosheet g-C_(3)N_(4)was modified with Pt nanoclusters(Pt/g-C_(3)N_(4))through impregnation and following photo-induced *** catalyst showed excellent photocatalytic activity of water reforming of methanol fo r hydrogen production with a 17.12 mmol·g^(-1)·h^(-1)rate at room temperature,which was 311 times higher than that of the unmodified g-C_(3)N_(4).The strong interactions of Pt-N in Pt/g-C_(3)N_(4)constructed effective electron transfer channels to promote the separation of photogenerated electrons and holes *** addition,in-situ infrared spectroscopy was used to investigate the intermediates of the hydrogen production reaction,which proved that methanol and water eventually turn into H_(2)and CO_(2)via formaldehyde and *** study provides insights for understanding the photocatalytic hydrogen production in the water reforming of methanol.

关键词： Water reforming of methanol Photocatalysis g-C_(3)N_(4) Pt nanoclusters Hydrogen production

Mechanism of action of Linggui Zhugan Decoction in treating non-alcoholic fatty liver disease using untargeted metabolomics approach

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Traditional Medicine Research 2025年第2期10卷 65-76页

作者： Huan Pei Ren-Lin Li Xin-Ran Song Qian-Qian Wan Yu-Ming Wang Han-Zhou Li Wei-Quan Xu Jia-Bao Liao Wei-Bo Wen Jing Miao Huan-tian cui School of Basic Medicine Yunnan University of Chinese MedicineKunming 650599China School Clinical Medical College Yunnan University of Chinese MedicineKunming 650599China First School of Clinical Medicine Yunnan University of Chinese MedicineKunming 650599China School of Integrative Chinese and Western Medicine Tianjin University of Traditional Chinese MedicineTianjin 301617China Department of Pharmacy Tianjin Second People's HospitalTianjin 300192China

Background:Non-alcoholic fatty liver disease(NAFLD)is a liver disorder characterized by the accumulation and degeneration of fat in the liver cells,a condition that may further deteriorate and lead to cirrhosis and liver *** studies showed that metabolic dysfunction can promote NAFLD *** Zhugan Decoction(LGZGD)has therapeutic effects on *** mechanism of LGZGD still remains *** study was to examine the impact of LGZGD on the metabolic processes involved in the development of ***:A mice model of NAFLD was treated with *** therapeutic potential of LGZGD was evaluated by assessing the activity of transaminases,lipids levels of blood,and pathological changes in the liver of the mice model of ***,this study also evaluated the influence of LGZGD on liver inflammation and oxidative ***:The results of untargeted metabolomics analysis showed that LGZGD reduced the disordered lipid metabolism in NAFLD *** improved the oxidative stress and also reduced the levels of pro-inflammatory cytokines in the *** metabolomics analysis of liver samples revealed that LGZGD treatment improved metabolic disorders,including alanine,aspartate,glutamate,glycerophospholipid metabolism,and citrate *** RT-qPCR and Western blot results showed that LGZGD could regulate the expression of key enzymes in the metabolic pathway of the citrate cycle,including ATP-citrate lyase(ACLY),alanine-glyoxylate aminotransferase-2(AGXT2),phosphatidylethanolamine N-methyltransferase(PEMT),and succinate dehydrogenase(SDH).Conclusion:We found that LGZGD can treat NAFLD by reducing inflammatory responses,inhibiting oxidative stress,regulating alanine,aspartate,glutamate,and glycerophospholipid metabolism,and citrate cycle pathways.

关键词： NAFLD LGZGD untargeted metabolomics glycerophospholipid metabolism citrate cycle

Function of large-volume high-pressure apparatus at SECUF

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Chinese Physics B 2018年第7期27卷 81-85页

作者： Pinwen Zhu Qiang Tao lu Wang Zhi He tian cui State Key Laboratory of Superhard Materials College of PhysicsJilin UniversityChangchun 130012China

Pressure allows the precise tuning of a fundamental parameter, the interatomic distance, which controls the electronic structure and virtually all interatomic interactions that determine material properties. Hence, pressure tuning is an effective tool in the search for new materials with enhanced properties. To realize pressure tuning on matter, large-volume press （LVP） apparatuses have been widely used not only to synthesize novel materials but also to implement the in situ measurement of physical properties. Herein, we introduce the LVP apparatuses, including belt-type, cubic anvil, and 6-8 type multi-anvil, that will be constructed at the Synergetic Extreme Condition User Facility （SECUF） at Jilin University. Typically, cell volumes of 1000 mm3 can be obtained at 20 GPa in a belt-type apparatus that is significantly larger than that obtained in a 6-8 type multi-anvil apparatus at the same pressure. Furthermore, the in situ measurement of physical prop- erties, including thermological, electrical, and mechanical behaviors, is coupled to these LVP apparatuses. Some typical results of both synthetic experiments and in situ measurements obtained from the LVP apparatuses are also reviewed.

关键词： high pressure large-volume press multi-anvil apparatus in situ measurement synthesis

Electrons dynamics control by shaping femtosecond laser pulses in micro/nanofabrication: modeling, method, measurement and application

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Light(Science & Applications) 2017年第1期6卷 249-275页

作者： Lan Jiang An-Dong Wang Bo Li tian-Hong cui Yong-Feng lu Laser Micro/Nano-Fabrication Laboratory School of Mechanical EngineeringBeijing Institute of TechnologyBeijing 100081China Department of Mechanical Engineering University of MinnesotaMinneapolisMN 55455USA Department of Electrical Engineering University of Nebraska-LincolnLincolnNE 68588-0511USA

During femtosecond laser fabrication,photons are mainly absorbed by electrons,and the subsequent energy transfer from electrons to ions is of picosecond ***,lattice motion is negligible within the femtosecond pulse duration,whereas femtosecond photon-electron interactions dominate the entire fabrication ***,femtosecond laser fabrication must be improved by controlling localized transient electron dynamics,which poses a challenge for measuring and controlling at the electron level during fabrication ***-probe spectroscopy presents a viable solution,which can be used to observe electron dynamics during a chemical *** fact,femtosecond pulse durations are shorter than many physical/chemical characteristic times,which permits manipulating,adjusting,or interfering with electron ***,we proposed to control localized transient electron dynamics by temporally or spatially shaping femtosecond pulses,and further to modify localized transient materials properties,and then to adjust material phase change,and eventually to implement a novel fabrication *** review covers our progresses over the past decade regarding electrons dynamics control(EDC)by shaping femtosecond laser pulses in micro/nanomanufacturing:(1)Theoretical models were developed to prove EDC feasibility and reveal its mechanisms;(2)on the basis of the theoretical predictions,many experiments are conducted to validate our EDC-based femtosecond laser fabrication *** examples are reported,which proves that the proposed method can significantly improve fabrication precision,quality,throughput and repeatability and effectively control micro/nanoscale structures;(3)a multiscale measurement system was proposed and developed to study the fundamentals of EDC from the femtosecond scale to the nanosecond scale and to the millisecond scale;and(4)As an example of practical applications,our method was employed to fabricate some key structures in one of the 16 Ch

关键词： electrons dynamics control femtosecond laser micro/nano fabrication pulse shaping

Organic optoelectronics:materials,devices and applications

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光学精密工程 2005年第5期13卷 525-534页

作者： IAU Yi cui tian-hong Department of Mechanical Engineering University of Minnesota 111 Church Street SE Minneapolis MN 55455 USA

The interest in organic materials for optoelectronic devices has been growing rapidly in the last two decades. This growth has been propelled by the exciting advances in organic thin films for displays, low-cost electronic circuits, etc. An increasing number of products employing organic electronic devices have become commercialized, which has stimulated the age of organic optoelectronics. This paper reviews the recent progress in organic optoelectronic technology. First, organic light emitting electroluminescent materials are introduced. Next, the three kinds of most important organic optoelectronic devices are summarized, including light emitting diode, organic photovoltaic cell, and photodetectors. The various applications of these devices are also reviewed and discussed in detail. Finally, the market and future development of optoelectronic devices are also demonstrated.

关键词：光电子学 OLED PPV 显示器电路

High-Order Local Discontinuous Galerkin Method with Multi-Resolution WENO Limiter for Navier-Stokes Equations on Triangular Meshes

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Communications in Computational Physics 2023年第5期33卷 1217-1239页

作者： Yizhou lu Jun Zhu Shengzhu cui Zhenming Wang Linlin tian Ning Zhao State Key Laboratory of Mechanics and Control for Aerospace Structures Nanjing University of Aeronautics and AstronauticsJiangsu 210000P.R.China Key Laboratory of Mathematical Modeling and High Performance Computing of Air Vehicles Nanjing University of Aeronautics and AstronauticsJiangsu 210000P.R.China Jiangsu Key Laboratory of Hi-Tech Research for Wind Turbine Design Nanjing University of Aeronautics and AstronauticsJiangsu 210000P.R.China College of Aerospace Engineering Nanjing University of Aeronautics and AstronauticsJiangsu 210000P.R.China

In this paper,a new multi-resolution weighted essentially non-oscillatory(MR-WENO)limiter for high-order local discontinuous Galerkin(LDG)method is designed for solving Navier-Stokes equations on triangular *** MR-WENO limiter is a new extension of the finite volume MR-WENO *** new limiter uses information of the LDG solution essentially only within the troubled cell itself,to build a sequence of hierarchical L^(2)projection polynomials from zeroth degree to the highest degree of the *** an example,a third-order LDGmethod with associated same orderMR-WENO limiter has been developed in this paper,which could maintain the original order of accuracy in smooth regions and could simultaneously suppress spurious oscillations near strong shocks or contact *** linear weights of such new MR-WENO limiter can be any positive numbers on condition that their summation is *** is the first time that a series of different degree polynomials within the troubled cell are applied in a WENO-type fashion to modify the freedom of degrees of the LDG solutions in the troubled *** MR-WENO limiter is very simple to construct,and can be easily implemented to arbitrary high-order accuracy and in higher dimensions on unstructured *** spatial reconstruction methodology improves the robustness in the numerical simulation on the same compact spatial stencil of the original LDG methods on triangular *** classical viscous examples are given to show the good performance of this third-order LDG method with associated MR-WENO limiter.

关键词： Local discontinuous Galerkin method multi-resolution WENO limiter triangular meshes Navier-Stokes equations