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Advancement and new perspectives of using formulated reactive amine blends for post-combustion carbon dioxide (CO_(2)) capture technologies

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Petroleum 2017年第1期3卷 10-36页

作者： Chikezie Nwaoha teeradet supap Raphael Idem Chintana Saiwan Paitoon Tontiwachwuthikul Mohammed JAL-Marri Abdelbaki Benamor Clean Energy Technologies Research Institute(CETRI) Faculty of Engineering and Applied ScienceUniversity of ReginaSKS4S 0A2Canada The Petroleum and Petrochemical College Chulalongkorn UniversityBangkok10330Thailand Gas Processing Center Qatar UniversityDohaQatar

Chemical absorption using amine-based solvents have proven to be the most studied,as well as the most reliable and efficient technology for capturing carbon dioxide(CO_(2))from exhaust gas streams and synthesis gas in all combustion and industrial *** application of single amine-based solvents especially the very reactive monoethanolamine(MEA)is associated with a parasitic energy demand for solvent *** regeneration energy accounts for up to threeequarters of the plant operating cost,efforts in its reduction have prompted the idea of using blended amine *** review paper highlights the success achieved in blending amine solvents and the recent and future technologies aimed at increasing the overall volumetric mass transfer coefficient,absorption rate,cyclic capacity and greatly minimizing both degradation and the energy for solvent *** importance of amine biodegradability(BOD)and low ecotoxicity as well as low amine volatility is also *** and energy penalty indices that influences the capital and operating costs of CO_(2) capture process was also highlighted.A new experimental method for simultaneously estimating amine cost,degradation rate,regeneration energy and reclaiming energy is also proposed in this review paper.

关键词： Post-combustion Pre-combustion Oxy-fuel combustion CO_(2)capture Blended amines Regeneration energy Degradation Amine volatility Biodegradability Ecotoxicity Amine cost Reclaiming energy

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