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Cesium removal from radioactive wastewater by adsorption and membrane technology

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Frontiers of Environmental Science & Engineering 2024年第3期18卷 161-175页

作者： Shuting zhuang Jianlong Wang School of Environment&Natural Resources Renmin University of ChinaBeijing 100872China Laboratory of Environmental Technology INETTsinghua UniversityBeijing 100084China Beijing Key Laboratory of Radioactive Waste Treatment INETTsinghua UniversityBeijing 100084China

Radiocesium is frequently present in radioactive wastewater,while its removal is still a challenge due to its small hydrated radius,high diffusion coefficient,and similar chemical behavior to other alkali metal elements with high background *** review summarized and analyzed the recent advances in the removal of Cs+from aqueous solutions,with a particular focus on adsorption and membrane separation *** inorganic,organic,and biological adsorbents have undergone assessments to determine their efficacy in the removal of cesium ***,membrane-based separation techniques,including reverse osmosis,forward osmosis,and membrane distillation,have also shown promise in effectively separating cesium ions from radioactive ***,this review summarized the main approaches,including Kurion/SARRY system+desalination system and advanced liquid processing system,implemented after the Fukushima Daiichi nuclear power plant accident in Japan to remove radionuclides from contaminated *** technology and membrane separation technology play a vital role in treatment of contaminated water.

关键词： Cesium Adsorption Membrane separation Advanced liquid processing system Fukushima nuclear accident

Diverse atomic structure configurations of metal-doped transition metal dichalcogenides for enhancing hydrogen evolution

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Nano Research 2024年第5期17卷 3586-3602页

作者： Longlu Wang Yuxin Zhang Chen Gu Haoxuan Yu Yanling zhuang Zechao zhuang College of Electronic and Optical Engineering and College of Flexible Electronics(Future Technology) Jiangsu Province Engineering Research Center for Fabrication and Application of Special Optical Fiber Materials and DevicesNanjing University of Posts and TelecommunicationsNanjing 210023China Department of Chemical Engineering Columbia UniversityNew YorkNY 10027USA

Doping foreign metal atoms into the substrate of transition metal dichalcogenides(TMDs)enables the formation of diverse atomic structure configurations,including isolated atoms,chains,and ***,it is very important to reasonably control the atomic structure and determine the structure-activity relationship between the atomic configurations and the hydrogen evolution reaction(HER)*** numerous studies have indicated that doping can yield diverse atomic structure configurations,there remains an incomplete understanding of the relationship between atomic configurations within the lattice of TMDs and their ***,diverse atomic structure configurations of adsorptive doping,substitutional doping,and TMDs alloys are *** structure-activity relationship between different atomic configurations and HER performance can be determined by micro-nanostructure devices and density functional theory(DFT)*** diverse atomic structure configurations are of great significance for activating the inert basal plane of TMDs and improving the catalytic activity of ***,we have summarized the current challenges and future opportunities,offering new perspectives for the design of highly active and stable metal-doped TMDs catalysts.

关键词： transition metal dichalcogenides(TMDs) dopant effect diverse atomic structure configurations hydrogen evolution reaction(HER)

Preparation of Chemically Recyclable Poly(ether-alt-ester) by the Ring Opening Polymerization of Cyclic Monomers Synthesized by Coupling Glycolide and Epoxides

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Chinese Journal of Polymer Science 2024年第2期42卷 168-175,I0006页

作者： Feng Ren zhuang-zhuang Liang Ming-Xin Niu Chen-Yang Hu Xuan Pang Key Laboratory of Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei230026China

Polyester and polyether are two key oxygenated polymers, and completely alternative sequence of poly(ester-alt-ether) could efficiently combine the advantages(including flexibility, degradability, etc.) of both segments. Currently, despite their copolymers could be synthesized from one-pot mixture of cyclic esters and epoxides, perfectly alternative microstructure is very challenging to realize and typically restricted to certain monomer pairs. Moving forward, synthesizing poly(ester-alt-ether) from commercially available and largescale monomers would be a significant advance. For example, successfully commercialized poly(glycolic acid)(PGA), which is not easily soluble in polymers due to its high crystallinity and is brittle and difficult to control the degradation cycle, would encounter a new paradigm if engineered into poly(ester-altether). In this work, starting from the design of monomer with hybrid structures, we successfully synthesized a series of 1,4-dioxan-2-one containing different substituents based on glycolide(GA) and epoxides using commercially available Salen-Cr(III) and PPNCl catalytic *** new monomers underwent ring-opening polymerization(ROP) to form a series of poly(ester-alt-ether) with perfectly alternating glycolic acid and propylene glycol repeat units under catalytic system of thiourea/base. The poly(ester-alt-ether) have significantly lower glass-transition temperature than PGA. Additionally, the poly(ester-alt-ether) can be chemically recovered to monomer using Sn(Oct)2 or 1,8-diazabicyclo[5.4.0]undecane-7-ene(DBU) as a catalyst in solution, thus establishing a closed-loop life cycle. From monomers derived from GA and epoxides, this work furnishes a novel strategy for the synthesis of poly(ester-alt-ether) with chemical recyclability.

关键词： Polyester Polyether Alternative copolymer Ring-opening polymerization

A whole-net cooperative positioning method based on CDGNSS and inter-vehicle ranging

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Chinese Journal of Aeronautics 2024年第2期37卷 401-416页

作者： Shan HU Hongbo ZHAO Chen zhuang School of Electronics and Information Engineering Beihang UniversityBeijing 100191China

Relative positioning is recognized as an important issue for vehicles in urban ***-vehicle Cooperative Positioning(CP)techniques which fuse the Global Navigation Satellite System(GNSS)and inter-vehicle ranging have attracted attention in improving the performance of baseline estimation between ***,current CP methods estimate the baselines separately and ignore the interactions among the positioning information of different *** interactions are called’information coupling’.In this work,we propose a new multivehicle precise CP framework using the coupled information in the network based on the Carrier Differential GNSS(CDGNSS)and inter-vehicle *** demonstrate the benefit of the coupled information by deriving the Cramer-Rao Lower Bound(CRLB)of the float estimation in *** fully use this coupled information,we propose a Whole-Net CP(WN-CP)method which consists of the Whole-Net Extended Kalman Filter(WN-EKF)as the float estimation filter,and the Partial Baseline Fixing(PBF)as the ambiguity resolution *** WN-EKF fuses the measurements of all baselines simultaneously to improve the performance of float estimation,and the PBF strategy fixes the ambiguities of the one baseline to be estimated,instead of full ambiguity resolution,to reduce the computation load of ambiguity *** tests involving four vehicles were conducted in urban *** results show that the proposed WN-CP method can achieve better performance and meanwhile maintain a low computation load compared to the existing methods.

关键词： GNSS Cooperative positioning Baseline Ambiguity resolution Information coupling

Ordering silver nanowires for chiroptical activity

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Science China Materials 2022年第5期65卷 1362-1368页

作者： Xueru Guo Dan Wu Yi Li Zhen He Jin-Long Wang Chong Zhang Zhao Pan Yuanjie Pang taotao zhuang Shu-Hong Yu Division of Nanomaterials&Chemistry Hefei National Laboratory for Physical Sciences at the MicroscaleInstitute of EnergyHefei Comprehensive National Science CenterCAS Center for Excellence in NanoscienceDepartment of ChemistryInstitute of Biomimetic Materials&ChemistryAnhui Engineering Laboratory of Biomimetic MaterialsUniversity of Science and Technology of ChinaHefei 230026China School of Optical and Electronic Information Wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhan 430076China

With the development of chiral materials, remarkable progress has been made in the application fields of biology, chemistry, and physics in the past decades. Here we develop a solo-Ag-nanowire(NW)-based, bottom-up chiral construction strategy to fabricate a chiral plasmonic film with strong chiroptical activity in the purple-blue band. Finitedifference time-domain simulations predict that helical structures made by Ag NWs with certain interlayer angles possess strong chiroptical intensity. We then apply a Langmuir-Blodgett technique to construct the layered NW assemblies with both handedness via regulating interlayer angle direction. The Ag NW assemblies show the interlayer-angleand film-thickness-dependent circular dichroism, reaching the highest anisotropic factor of 0.03. These new chiral structures will serve as ideal candidates for chiral sensors thanks to their specific plasmonic properties.

关键词： chiral assembly finite-difference time-domain simulations Ag nanowires chiroptical activity

Digital Twin Modeling Enabled Machine Tool Intelligence:A Review

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Chinese Journal of Mechanical Engineering 2024年第2期37卷 29-54页

作者： Lei Zhang Jianhua Liu Cunbo zhuang School of Mechanical Engineering Tianjin University of CommerceTianjin 300134China Laboratory of Digital Manufacturing School of Mechanical EngineeringBeijing Institute of TechnologyBeijing 10081China

Machine tools,often referred to as the“mother machines”of the manufacturing industry,are crucial in developing smart manufacturing and are increasingly becoming more *** twin technology can promote machine tool intelligence and has attracted considerable research ***,there is a lack of clear and systematic analyses on how the digital twin technology enables machine tool ***,digital twin modeling was identified as an enabling technology for machine tool intelligence based on a comparative study of the characteristics of machine tool intelligence and digital *** review then delves into state-of-the-art digital twin modelingenabled machine tool intelligence,examining it from the aspects of data-based modeling and mechanism-data dual-driven ***,it highlights three bottleneck issues facing the *** these problems,the architecture of a digital twin machine tool(DTMT)is proposed,and three key technologies are expounded in detail:Data perception and fusion technology,mechanism-data-knowledge hybrid-driven digital twin modeling and virtual-real synchronization technology,and dynamic optimization and collaborative control technology for multilevel ***,future research directions for the DTMT are *** work can provide a foundation basis for the research and implementation of digital-twin modeling-enabled machine tool intelligence,making it significant for developing intelligent machine tools.

关键词： Machine tool Digital twin Smart manufacturing Synchronization

An oscillation-free Hermite WENO scheme for hyperbolic conservation laws

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Science China Mathematics 2024年第2期67卷 431-454页

作者： zhuang Zhao Jianxian Qiu School of Mathematical Sciences and Institute of Natural Sciences Shanghai Jiao Tong UniversityShanghai 200240China School of Mathematical Sciences and Fujian Provincial Key Laboratory of Mathematical Modeling and High-Performance Scientific Computing Xiamen UniversityXiamen 361005China

In this paper, the sixth-order oscillation-free Hermite weighted essentially non-oscillatory (OFHWENO) scheme is proposed for hyperbolic conservation laws on structured meshes, where the zeroth- andfirst-order moments are the variables for the governing equations. The main difference from other HWENOschemes existing in the literature is that we add high-order numerical damping terms in the first-order momentequations to control spurious oscillations for the OF-HWENO scheme. The OF-HWENO scheme not only canachieve the designed optimal numerical order, but also can be easily implemented as we use only one set ofstencils in the reconstruction procedure and the same reconstructed polynomials are applied for the zeroth- andfirst-order moment equations. In order to obtain the adaptive order resolution when facing discontinuities, atransition polynomial is added in the reconstruction, where the associated linear weights can also be any positivenumbers as long as their summation equals one. In addition, the OF-HWENO scheme still keeps compactnessas only immediate neighbor values are needed in the space discretization. Some benchmark numerical tests areperformed to illustrate the high-order accuracy, high resolution and robustness of the proposed scheme.

关键词： Hermite WENO scheme hyperbolic conservation laws oscillation-free adaptive order discontinuous Galerkin method

Aerial target threat assessment based on gated recurrent unit and self-attention mechanism

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Journal of Systems Engineering and Electronics 2024年第2期35卷 361-373页

作者： CHEN Chen QUAN Wei SHAO zhuang School of Automation Beijing Institute of TechnologyBeijing 100081China State Key Laboratory of Intelligent Control and Decision of Complex Systems Beijing 100081China

Aerial threat assessment is a crucial link in modern air combat, whose result counts a great deal for commanders to make decisions. With the consideration that the existing threat assessment methods have difficulties in dealing with high dimensional time series target data, a threat assessment method based on self-attention mechanism and gated recurrent unit(SAGRU) is proposed. Firstly, a threat feature system including air combat situations and capability features is established. Moreover, a data augmentation process based on fractional Fourier transform(FRFT) is applied to extract more valuable information from time series situation features. Furthermore, aiming to capture key characteristics of battlefield evolution, a bidirectional GRU and SA mechanisms are designed for enhanced ***, after the concatenation of the processed air combat situation and capability features, the target threat level will be predicted by fully connected neural layers and the softmax classifier. Finally, in order to validate this model, an air combat dataset generated by a combat simulation system is introduced for model training and testing. The comparison experiments show the proposed model has structural rationality and can perform threat assessment faster and more accurately than the other existing models based on deep learning.

关键词： target threat assessment gated recurrent unit(GRU) self-attention(SA) fractional Fourier transform(FRFT)

Enhancement of low-temperature toughness of Fe-Mn-C-Al alloy by rare earth Ce-modified inclusions

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Journal of Iron and Steel Research International 2024年第1期31卷 157-173页

作者： Guang-kai Yang Chang-ling zhuang Yi-zhuang Li Chen Hu Shao-bo Li College of Materials and Metallurgy Guizhou UniversityGuiyang550025GuizhouChina Department of Mechanical Engineering University of Hong KongHong Kong999077China The State Key Laboratory of Rolling and Automation Northeastern UniversityShenyang110819LiaoningChina State Key Laboratory of Public Big Data Guizhou UniversityGuiyang550025GuizhouChina

Fe-Mn-C-Al alloys have been recognized as promising materials for certain low-temperature applications due to their exceptional mechanical properties and ***,their limited low-temperature toughness restricts their large-scale applications in specific *** influence of trace amounts of rare earth cerium(Ce)on the low-temperature toughness of Fe-18Mn-0.6C-1.8Al alloys was *** addition of Ce effectively alters the inclu-sions in the alloy,transforming large-sized irregular inclusions into fine ellipsoidal rare earth *** leads to a significant reduction in both the proportion and average size of the inclusions,resulting in their effective dispersion throughout the matrix and improved cryogenic *** presence of Ce-containing inclusions within the matrix reduces stress concentration,thereby inhibiting microcrack formation and improving impact absorption ***-cally,the addition of rare earth Ce alters the fracture behavior of the material at room temperature and low temperature,changing from brittle cleavage fracture to a more ductile failure *** impact toughness of the Fe-Mn-C-Al alloy is significantly improved by the addition of 0.0048 wt.%Ce,particularly at-196℃where the impact toughness reaches 103.6 J/cm^(2),representing an impressive improvement of 87.3%.

关键词： Fe-Mn-C-Al alloy Rare earth Low-temperature toughness Inclusion Fracture