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Work-function-induced interfacial electron redistribution of MoO_(2)/WO_(2) heterostructures for high-efficiency electrocatalytic hydrogen evolution reaction

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Rare Metals 2024年第2期43卷 489-499页

作者： Tong-Fei Li Jing Li Lu-Ping Zhang Jia-Wei Ke Meng-Xing Fan Li-Fang Zhang Cheng-Wei deng Yi Sun tao Qian Cheng-Lin Yan School of Chemistry and Chemical Engineering Nantong UniversityNantong226019China Jiangsu Key Laboratory of New Power Batteries Jiangsu Collaborative Innovation Centre of Biomedical Functional MaterialsSchool of Chemistry and Materials ScienceNanjing Normal UniversityNanjing210023China Aerospace Hydrogen Energy Technology(Shanghai)Co.Ltd. Shanghai201800China Key Laboratory of Core Technology of High Specific Energy Battery and Key Materials for Petroleum and Chemical Industry College of EnergySoochow UniversitySuzhou215006China Light Industry Institute of Electrochemical Power Sources Suzhou215006China

The engineering of the electronic configurations of active sites,together with the production of more accessible active sites through heterostructure design,has been established as a forceful methodology for boosting water electrolysis ***,a facile approach is developed to fabricate well-dispersed MoO_(2) and WO_(2) nanoparticles with abundant heterointerfaces entrapped in N,P-doped carbon nanofibers(referred to as MoO_(2)/WO_(2)@N,P-CNFs hereafter)as hydrogen evolution reaction(HER)electrocatalysts in alkaline and acidic *** spectroscopic analyses and theoretical findings manifest that the heterointerface formed by the work function modulation of MoO_(2)/WO_(2) triggers the spontaneous electron redistribution from MoO_(2)to WO_(2) and a built-in electric field,which is essential to promote water adsorption,optimize the H-intermediate adsorption energy,result in the enhanced charge transfer efficiency,and ultimately increase the intrinsic HER ***,the intimate confinement of MoO_(2)/WO_(2) heterostructures in the porous carbon substrate can restrain the active sites from unfavorable coarsening and detachment,thus ensuring facilitated HER kinetics and outstanding structural *** a result,MoO_(2)/WO_(2)@N,P-CNFs exhibit superior catalytic HER performance in acidic and basic solutions,requiring 118 and 95 mV overpotentials to achieve 10 mA·cm^(−2),respectively,surpassing a number of reported non-noble metal-based *** work provides guidelines for the rational design and construction of special metallic heterocomponents with optimized interfacial electronic structure for various electrochemical technologies.

关键词： Electrospinning MoO_(2)/WO_(2) heterostructure Work function Hydrogen evolution reaction

Heat Transfer and Friction Characteristics of Printed Circuit Heat Exchangers with Different Channel Structures for S-CO_(2) Power System

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Journal of Thermal Science 2024年第3期33卷 1132-1147页

作者： JIANG tao LI Mingjia Key Laboratory of Thermo-Fluid Science and Engineering of Ministry of Education School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an710049China School of Mechanical Engineering Beijing Institute of TechnologyBeijing100081China

Printed circuit heat exchanger(PCHE)has been widely used in supercritical carbon dioxide(S-CO_(2))power systems because of its high heat transfer efficiency and good ***,due to the large variety of PCHE configurations,channel selection in practical applications lacks a ***,this paper discussed the heat transfer and friction characteristics and the synergy of three fields in the channel under the guidance of the field synergy principle for four typical PCHE ***,the comprehensive performance of four channels was ***,the heat transfer and friction factor correlations for S-CO_(2)in four channels were *** findings demonstrate that the synergy of velocity and pressure fields of the straight channel PCHE is better(β≈180°),so its resistance loss is relatively *** zigzag and sinusoidal wavy channels and the airfoil fins can reduce the angle a between the temperature gradient and velocity,thus enhancing the heat *** sinusoidal wavy channel can reduce flow resistance compared to the zigzag channel due to the rounded *** streamlined airfoil structure can guide the flow and reduce backflow,thus reducing resistance *** the range of Re studied in this paper,the maximum error of the proposed heat transfer and friction factor correlations of PCHE is 7.0%,which shows good fitting *** research in this paper can provide a reference for the selection and design of PCHE with different channel configurations.

关键词： printed circuit heat exchanger supercritical carbon dioxide typical channel structure field synergy analysis

Gas-surface interaction features under effects of gas-gas molecules interaction in high-speed flows

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Chinese Journal of Aeronautics 2024年第5期37卷 228-242页

作者： Ruiling tao Zhihui WANG School of Engineering Science University of Chinese Academy of SciencesBeijing 100049China

Understanding interactions between gas molecules and solid surface is key to the aerodynamic design of high-speed,high-altitude aerospace vehicles,but there is a large dispersion of gas-surface interaction parameters or namely accommodation *** uncertainty results partly from different considerations of the interaction between gas molecules in various experimental and numerical *** this study,effects of gas-gas molecules interaction are systematically discussed by comparing two different approaches of molecular dynamics simulation of high-speed argon molecules scattering on a graphite *** popularly-used“single scattering”approach repeats the scattering process of a single gas molecule without considering the gas-gas molecules *** newly-developed“continual scattering”approach continually shoots gas molecules at the surface,considering collisions between gas molecules in addition to gas molecules’collisions with ***-surface interaction features in the two approaches are compared and discussed under various affecting factors including rarefaction degree,gas-surface interaction strength,surface temperature and incident *** is shown that these two approaches usually produce different accommodation coefficients,and the corresponding mechanisms are *** study could help clarify some doubts about the selection of accommodation coefficients in engineering practice,and also provide an instruction on design of an appropriate molecular dynamics simulation approach.

关键词： Gas-surface interaction Molecular dynamics Accommodation coefficient Aerospace vehicles High-speed flow

On m-ovoids of finite classical polar spaces with an irreducible transitive automorphism group

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Science China Mathematics 2024年第3期67卷 683-712页

作者： tao Feng Weicong Li Ran tao School of Mathematical Sciences Zhejiang UniversityHangzhou 310027China Department of Mathematics and National Center for Applied Mathematics Shenzhen Southern University of Science and TechnologyShenzhen 518055China Key Laboratory of Cryptologic Technology and Information Security Ministry of EducationShandong UniversityQingdao 266237China School of Cyber Science and Technology Shandong UniversityQingdao 266237China

In this paper, we classify the m-ovoids of finite classical polar spaces that admit a transitive automorphism group acting irreducibly on the ambient vector space. In particular, we obtain several new infinite familie... 详细信息

关键词： transitive m-ovoids irreducible action finite classical polar spaces primitive divisor

Atomically dispersed materials:Ideal catalysts in atomic era

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Nano Research 2024年第1期17卷 18-38页

作者： tao Gan Dingsheng Wang Department of Chemistry Tsinghua UniversityBeijing 100084China

Catalysts can accelerate the chemical reaction rate and effectively promote the molecules transformation,which is of great significance in the research of chemical industry and material *** extreme utilization of reactive sites has led to the emergence and development of atomically dispersed materials(ADMs).The highly active coordination unsaturated metal sites and fully utilized metal atoms make ADMs show great potential in catalytic *** adjustment of coordination environment and electronic structure provides more possibilities for constructing reactive centers with different *** review summarized the application and research progress of ADMs in different *** design strategy and structure–activity relationship of ADMs for specific reactions were summarized and ***,we also provided advices for the challenges and opportunities faced by ADMs in catalytic reactions.

关键词： atomically dispersed materials catalysis organic synthesis battery sensor enzyme

Neogene integrative stratigraphy,biotas,and paleogeographical evolution of the Qinghai-Tibetan Plateau and its surrounding areas

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Science China Earth Sciences 2024年第4期67卷 1326-1359页

作者： tao deng Xiaomin FANG Qiang LI Shiqi WANG Feixiang WU Sukuan HOU Jiao MA Qigao JIANGZUO Danhui SUN Yan ZHENG Qinqin SHI Boyang SUN Lu LI Key Laboratory of Vertebrate Evolution and Human Origins Institute of Vertebrate Paleontology and PaleoanthropologyChinese Academy of SciencesBeijing 100044China CAS Center for Excellence in Life and Paleoenvironment Beijing 100044China University of Chinese Academy of Sciences Beijing 100049China CAS Center for Excellence in Tibetan Plateau Earth Sciences and Key Laboratory of Continental Collision and Plateau Uplift Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China Key Laboratory of Orogenic Belts and Crustal Evolution School of Earth and Space SciencesPeking UniversityBeijing 100871China

The remarkable uplift of the Tibetan Plateau in the Neogene had great impacts on the climate and environment of East Asia and even the ***,establishment of the Neogene stratigraphic framework of the Tibetan Plateau is of great significance to research in various fields of *** on marine sediments,the international chronostratigraphic system of the Neogene is divided into six stages in the Miocene and two stages in the *** the beginning of the Cenozoic,the share of terrestrial strata on continents has increased *** the Neogene,it had far exceeded that of marine strata,and almost all deposits on the Tibetan Plateau and its surrounding areas were terrestrial *** China,the Miocene includes five stages and the Pliocene includes two *** for the Tunggurian of the Miocene,which has a lower boundary at 15 Ma,the other stages have the same paleomagnetic definitions and time intervals as the corresponding international marine *** fossils play a very important role in the division and correlation of Cenozoic terrestrial strata,and rodent,carnivore,proboscidean,perissodactyl and artiodactyl fossils are especially important in Neogene terrestrial *** are many basins with well-exposed strata and abundant mammalian fossils in the Tibetan *** lower boundary stratotype sections of the Neogene Xiejian and Bahean stages are located respectively in the Xining and Linxia basins,and there are precise paleomagnetic dates in coordination with mammalian *** lower boundary stratotypes of other stages can also be effectively determined in the Tibetan *** first appearing mammalian genera in East Asia also appeared in the Tibetan Plateau and its surrounding areas,especially in the Linxia Basin on the northeast margin and in the Siwaliks on the southwest *** them,Prodeinotherium first appeared at the bottom of the Miocene in the Siwaliks,and the earliest Hipparion of the Old

关键词： Tibetan Plateau Neogene Terrestrial stratum Mammalian fossil Paleomagnetism

Holder continuous weak solutions of the 2D Boussinesq equation with thermal diffusion

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Science China Mathematics 2024年第8期67卷 1777-1806页

作者： Tianwen Luo tao tao Liqun Zhang Yau Mathematical Sciences Center Tsinghua UniversityBeijing 100084China School of Mathematics Shandong UniversityJinan 250100China Institute of Mathematics Academy of Mathematics and Systems ScienceChinese Academy of SciencesBeijing 100190China School of Mathematical Sciences University of Chinese Academy of SciencesBeijing 100049China

We show the existence of Holder continuous periodic weak solutions of the 2D Boussinesq equation with thermal diffusion which satisfy the prescribed kinetic *** precisely,for any smooth e(t):[0,1]→R+andε∈(0,110),there exist v∈C 110−ε([0,1]×T2)andθ∈C 1,120−εt 2 C 2,1 x 10−ε([0,1]×T2),which satisfy(1.1)in the sense of distribution and e(t)=ˆT2|v(t,x)|2 dx,∀t∈[0,1].

关键词： 2D Boussinesq equation with thermal diffusion Holder continuous periodic weak solutions prescribed kinetic energy

An efficient online histogram publication method for data streams with local differential privacy

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Frontiers of Information Technology & Electronic Engineering 2024年第8期25卷 1096-1109页

作者： tao tao Funan ZHANG Xiujun WANG Xiao ZHENG Xin ZHAO School of Computer Science and Technology Anhui University of TechnologyMaanshan 243032China Anhui Engineering Research Center for Intelligent Applications and Security of Industrial Internet Maanshan 243032China Engineering Research Institute Anhui University of TechnologyMaanshan 243032China Shengli No.1 Middle School of Dongying City Dongying 257000China

Many areas are now experiencing data streams that contain privacy-sensitive *** the sharing and release of these data are of great commercial value,if these data are released directly,the private user information in the data will be ***,how to continuously generate publishable histograms(meeting privacy protection requirements)based on sliding data stream windows has become a critical issue,especially when sending data to an untrusted third *** histogram publication methods are unsatisfactory in terms of time and storage costs,because they must cache all elements in the current sliding window(sW).Our work addresses this drawback by designing an efficient online histogram publication(EOHP)method for local differential privacy data ***,in the EOHP method,the data collector first crafts a histogram of the current SW using an approximate counting ***,the data collector reduces the privacy budget by using the optimized budget absorption mechanism and adds appropriate noise to the approximate histogram,making it possible to publish the histogram while retaining satisfactory data *** experimental results on two different real datasets show that the EOHP algorithm significantly reduces the time and storage costs and improves data utility compared to other existing algorithms.

关键词： Data stream Differential privacy Sliding windows Approximate counting

RIPK1 plays a crucial role in maintaining regulatory T-Cell homeostasis by inhibiting both RIPK3-and FADD-mediated cell death

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Cellular & Molecular Immunology 2024年第1期21卷 80-90页

作者： Xiaoxue deng Lingxia Wang Yunze Zhai Qiuyue Liu Fengxue Du Yu Zhang Wenxing Zhao Tingtao Wu Yiwen tao Jie deng Yongbing Cao Pei Hao Jiazi Ren Yunli Shen Zuoren Yu Yuejuan Zheng Haibing Zhang Haikun Wang State Key Laboratory of Cardiology Shanghai East HospitalTongji University School of MedicineShanghai200120China CAS Key Laboratory of Molecular Virology and Immunology Shanghai Institute of Immunity and InfectionChinese Academy of SciencesUniversity of Chinese Academy of SciencesShanghai200031China CAS Key Laboratory of Nutrition Metabolism and Food SafetyShanghai Institute of Nutrition and HealthShanghai Institutes for Biological SciencesUniversity of Chinese Academy of SciencesChinese Academy of SciencesShanghai200031China The Research Center for Traditional Chinese Medicine Shanghai Institute of Infectious Diseases and BiosecurityShanghai University of Traditional Chinese MedicineShanghai201203China Institute of Vascular Disease Shanghai TCM-Integrated HospitalShanghai University of Traditional Chinese MedicineShanghai200433China

Regulatory T(T_(reg))cells play an essential role in maintaining immune balance across various physiological and pathological ***,the mechanisms underlying T_(reg)homeostasis remain incompletely ***,we report that RIPK1 is crucial for T_(reg) cell survival and *** generated mice with T_(reg) cell-specific ablation of Ripk1 and found that these mice developed fatal systemic autoimmunity due to a dramatic reduction in the Treg cell compartment caused by excessive cell *** conventional T cells,Treg cells with Ripk1 deficiency were only partially rescued from cell death by blocking FADD-dependent ***,simultaneous removal of both Fadd and Ripk3 completely restored the homeostasis of Ripk1-deficient Treg cells by blocking two cell death ***,our study highlights the critical role of RIPK1 in regulating Treg cell homeostasis by controlling both apoptosis and necroptosis,thereby providing novel insights into the mechanisms of Treg cell homeostasis.

关键词： Treg cell Homeostasis Apoptosis Necroptosis