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Geochemical Characteristics and Development Significances of Constant and Trace Elements from Coalbed Methane Co-Produced Water:A Case Study of the Shizhuangnan Block,the Southern Qinshui Basin

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Journal of Earth Science 2024年第1期35卷 51-61页

作者： Yang Li shuheng tang Jian Chen Songhang Zhang Zhaodong Xi Key Laboratory of Universities in Anhui Province for Prevention of Mine Geological Disasters Anhui University of Science and TechnologyHuainan 232001China School of Earth and Environment Anhui University of Science and TechnologyHuainan 232001China National Key Laboratory of Petroleum Resources and Engineering China University of PetroleumBeijing 102249China School of Energy Resource China University of GeosciencesBeijing 100083China Key Laboratory of Marine Reservoir Evolution and Hydrocarbon Enrichment Mechanism Ministry of EducationBeijing 100083China Key Laboratory of Strategy Evaluation for Shale Gas Ministry of Land and ResourcesBeijing 100083China

As an unconventional natural gas resource,coalbed methane(CBM)development releases a large amount of CBM wells co-produced *** characteristics of the co-produced water provide an essential foundation for the production dynamics of CBM reservoirs if the impacts of fracturing fluids and other aquifers can be *** the Shizhuangnan Block of the southern Qinshui Basin,constant and trace elements in CBM co-produced water from the wellheads were collected and determined,which is applied to assess water source,fracturing fluid effect,and CBM *** on principle component analysis and hierarchical clustering analysis,the water samples are divided into four *** suggests that different characteristics affected by water-rock interaction,reservoir environment,aquifer recharge,and hydraulic fracturing result in the various ratios of Na^(+)/Cl^(-),alkalinity(HCO_(3)^(-)+CO_(3)^(2-))/Cl^(-)and other specific ***,Cl^(-)is selected as a dividing line for complete fracturing fluid flow back,associated with organic-bound chlorine complexes in the original coal seam *** to constant elements,there is a significant correlation between Li and Sr concentrations and CBM productivity,so templates regarding trace elements can be used to distinguish various sources of the co-produced water.

关键词： coalbad methane CBM co-produced water hydraulic fracturing Qinshui Basin

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原位储层生物地球化学评价及其对煤层气开采的指示意义——以沁水盆地南部柿庄南区块为例

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煤炭学报 2024年第1期49卷 555-562页

作者：唐书恒李洋吕建伟中国地质大学(北京)能源学院北京100083 安徽理工大学地球与环境学院安徽淮南232001 油气资源与工程全国重点实验室中国石油大学(北京)北京102249

煤储层是微生物生存代谢的良好场所,其中与碳循环相关的微生物群落普遍存在,但微生物的地理分布与代谢表达尚未与储层建立有效联系。通过微生物代谢难以在自然条件形成有效气藏,但微生物群落受有机物供给、环境条件等影响,对储层原位环... 详细信息

煤储层是微生物生存代谢的良好场所,其中与碳循环相关的微生物群落普遍存在,但微生物的地理分布与代谢表达尚未与储层建立有效联系。通过微生物代谢难以在自然条件形成有效气藏,但微生物群落受有机物供给、环境条件等影响,对储层原位环境与煤层气保存条件形成良好响应。沁水盆地南部煤层气资源丰富,是我国最早实现煤层气商业开发的区域之一。以沁水盆地南部柿庄南区块为例,通过研究区储层水的生物地球化学特征与生物基因测序,分析离子质量浓度、溶解无机碳同位素、硫酸盐同位素和微生物丰度与多样性,以产甲烷菌、硫酸盐还原菌等微生物为依据评价储层环境条件。研究表明,储层地球化学受水岩作用、离子交换和微生物代谢等因素影响。较高的钠离子和碳酸氢根离子质量浓度说明储层为相对还原环境或滞留条件。硫酸盐还原菌和产甲烷菌在降解煤过程中发挥协同作用,但硫酸盐还原菌在硫酸盐满足代谢需求时与产甲烷菌竞争可用底物占优而抑制产甲烷菌代谢。硫酸盐同位素、溶解无机碳同位素以及微生物丰度和多样性等可表征上述微生物间的共生关系与储层环境条件。硫酸盐还原作用活跃而产甲烷作用不明显的区域不具备有效保存煤层气的条件。相对还原或滞留的储层环境适宜产甲烷菌代谢,也是煤层气保存的有利区。研究认识丰富了储层生物地球化学评价方法,指导了煤层气勘探开发有利区优选,为我国煤层气生物工程的现场实施提供理论基础与方案指导。

关键词：煤层气开采氧化还原环境生物地理分布产甲烷菌硫酸盐还原

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宁武盆地深部煤储层地温场特征及其对含气性的影响

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煤田地质与勘探 2024年第2期52卷 92-101页

作者：郗兆栋唐书恒刘忠屈晓荣张鹏豹苏育飞张迁中国地质大学(北京)能源学院北京100083 中国石油华北油田勘探开发研究院河北任丘062550 山西省煤炭地质勘查研究院山西太原030000

温度是影响深部煤储层含气性的重要因素,继而影响深部煤层气的开发效果。因此,明确煤储层地温条件及其对深部煤储层含气性的影响是系统认识深部煤层气富集特征及生产规律的关键。宁武盆地太原组9号煤层埋深大于1000 m的面积占比超过90%... 详细信息

温度是影响深部煤储层含气性的重要因素,继而影响深部煤层气的开发效果。因此,明确煤储层地温条件及其对深部煤储层含气性的影响是系统认识深部煤层气富集特征及生产规律的关键。宁武盆地太原组9号煤层埋深大于1000 m的面积占比超过90%,盆地腹部煤层埋深基本大于1500 m,最大埋深超过2500 m,属于典型的深部煤层气。以宁武南区块为例,基于井温测井数据、实验测试数据、录井资料及试井资料,确定宁武南煤储层地温场特征及其对含气性的影响效应。结果显示,宁武南区块9号煤储层温度为15.5~40.1℃,与煤层埋深具有显著的正相关性,地温梯度为1.27~1.95℃/hm,平均为1.52℃/hm,显示出低地温场特征。研究区煤储层含气饱和度为40.1%~93.7%,平均为71.7%,显示出深部煤储层低含气饱和度的特征。随着埋藏深度的增加,较低的地温梯度使得研究区煤储层温度增加缓慢,导致在相似埋深下,温度对研究区深部煤储层吸附能力的负效应显著低于大宁-吉县、临兴等深部煤层气区块,使得研究区煤储层吸附气向游离气的转换深度加深且转换比例降低。低地温条件是影响研究区深部煤层含气性的重要因素之一,继而影响其可开采程度。在深部煤层气的勘探开发中应重视煤储层地温条件的研究。

关键词：宁武盆地深部煤层气地温梯度地温场含气性

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宁武盆地南部深部煤层气临界深度与成藏特征

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天然气工业 2024年第1期44卷 108-118页

作者：郗兆栋唐书恒刘忠张迁张鹏豹杨雄雄张珂中国地质大学(北京)能源学院中国石油华北油田公司勘探开发研究院

近年来,随着深部煤层气勘探开发技术的不断突破,深部煤层气已逐渐成为中国油气资源重要的勘探开发新领域。但是,关于煤层气深度界线的科学内涵、深部煤层气藏的地质特征、煤层气富集模式等基础科学问题仍处于初期探索阶段。为此,以宁武... 详细信息

近年来,随着深部煤层气勘探开发技术的不断突破,深部煤层气已逐渐成为中国油气资源重要的勘探开发新领域。但是,关于煤层气深度界线的科学内涵、深部煤层气藏的地质特征、煤层气富集模式等基础科学问题仍处于初期探索阶段。为此,以宁武盆地宁武南区块上石炭统太原组9号煤层为研究对象,基于区块20余口煤层气井的钻井、测井及试井资料等,联合等温吸附、气体同位素等实验测试手段,探讨了宁武南区块深部煤层气临界深度与成藏特征。研究结果表明:①研究区深部煤层气临界深度为1200 m,临界深度以深,深部煤层气藏具有煤层厚度大、热演化程度高、含气量及含气饱和度高、煤体结构好和孔隙度低的地质特征。②地温梯度和热演化程度是影响研究区深部煤层气临界深度及煤层气成藏条件的重要因素。结论认为,该盆地的宁武南区块深部煤层气地质特征与鄂尔多斯盆地大宁—吉县、临兴、延川南等深部煤层气区块具有可比性,展现出宁武盆地深部煤层气良好的勘探开发前景。

关键词：宁武盆地上石炭统太原组深层煤层气临界深度成藏特征

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Resources Conditions of Coalbed Methane Districts in China

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Acta Geologica Sinica(English Edition) 2000年第3期74卷 701-705页

作者： tang shuheng LIN Dayang China University of Mining and Technology Beijing 100083 China National Administration of Coal Geology Zhuozhou 072752

The China National Administration of Coal Geology accomplished an assessment of coalbed methane resources of China in 1988. The total amount of coalbed methane resources in China is 14336.944 billion m3, occurring in recoverable coal seams and beneath weathering zones, with coalbed methane content equal to or higher than 4 m3 per ton and buried depths smaller than 2000 m, among which there are 967.51 billion m3 of predicted reserves and 13369.434 billion m3 of future reserves. The resources in coal reservoirs with methane content of more than 8 m3 per ton are 12444.087 billion m3, and those with methane content between 4 to 8 m3 per ton are 1892.856 billion m3. There are 35 districts in which the resources abundance is higher than 150 million m3/km2, 49 districts with the abundance between 50 million and 150 million m3/km2, and 31 districts with the abundance less than 50 million m3/km2. There is 9256.078 billion m3 of methane occurring in coal seams with buried depths less than 1500 m, and 5080.866 billion m3 in coal seams with buried depths between 1500 and 2000 m. There are 28 large-scale districts in which coalbed methane resources are more than 100 billions m3, 28 medium-scale districts with coalbed methane resources between 20 billion and 100 billion m3 and 59 small-scale districts with resources amount less than 20 billion m3. The Jincheng area is one of the most favourable districts for coalbed methane resources in China.

关键词： coalbed methane resources assessment resources amount target district China

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Microbial Geochemical Characteristics of the Coalbed Methane in the Shizhuangnan Block of Qinshui Basin, North China and their Geological Implications

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Acta Geologica Sinica(English Edition) 2019年第3期93卷 660-674页

作者： LI Yang SHI Wei tang shuheng School of Energy Resource China University of GeosciencesBeijing 100083China Key Laboratory of Marine Reservoir Evolution and Hydrocarbon Enrichment Mechanism Ministry of EducationBeijing 100083China Key Laboratory of Strategy Evaluation for Shale Gas Ministry of Land and ResourcesBeijing 100083China

Methanogens and sulfate reducing bacteria were detected by the 16SrRNA sequencing of coalbed methane(CBM)co-produced water in the south of the Qinshui Basin,which is indicative of the presence of secondary biological gas in the south of this basin,in contradiction to the previous understanding of thermogenic *** work systematically collected water samples from the CBM wells in the Shizhuangnan Block and analyzed the microbial geochemical characteristics from the aspects of water ions,hydrogen and oxygen isotopes,dissolved inorganic carbon and microbial *** is shown that the Shizhuangnan Block has a nearly SN-trending monoclinic structure,and the elevation of coal seam decreases gradually from the east to *** of the water blocking effect of Sitou fault in the west,the precipitation flowed from the east to west,and gradually transited to stagnant flow *** concentration variation of some ions such as Na^+,K^+,Ca2^+,Mg2^+,Cl^-,HCO3^-and total dissolved solids(TDS)suggest the variation of redox condition in the coal reservoir *** 16SrDNA sequencing analysis of the collected water samples detected the presence of methanogens and sulfate reduction *** presence of methane production zone and sulfate methane transition zone(SMTZ)was *** effect of methanogens in the methane production zone leads to an increase in the methane concentration,resulting in a high gas content in the study *** the SMTZ,most methane is consumed by anaerobic oxidation due to high sulfate concentrations.

关键词： CBM co-produced water microbial geochemistry sulfate methane transition zone Shizhuangnan Block

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A review on microbial metabolism to increase coalbed methane generation and coal pretreatment to improve its bioavailability

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Frontiers of Earth Science 2023年第1期17卷 218-229页

作者： Yang LI shuheng tang Jian CHEN Songhang ZHANG School of Earth and Environment Anhui University of Science and TechnologyHuainan 232001China State Key Laboratory of Mining Response and Disaster Prevention and Control in Deep Coal Mines Anhui University of Science and TechnologyHuainan 232001China School of Energy Resource China University of GeosciencesBeijing 100083China Key Laboratory of Marine Reservoir Evolution and Hydrocarbon Enrichment Mechanism(Ministry of Education) Beijing 100083China Key Laboratory of Strategy Evaluation for Shale Gas(Ministry of Land and Resources) Beijing 100083China

Abundant unminable coal in deep strata and abandoned mines are also precious sources of clean gas energy,under which biotransformation is a potential *** recent years,substantial progress has been made in laboratory research on coal degradation to produce methane by microbial *** paper systematically reviews the research progress of microbial enhancement and microbial stimulation of coal,physicochemical pretreatments of coal,and environmental factors affecting coal *** research idea of coal biotransformation should aim at field production increase and gradually clarify the microbial mechanism of coal degradation and the regional distribution and functional composition of microbial communities on the block *** research on coal biotransformation helps improve the development level of coalbed methane and the sustainable development of unconventional natural gas resources.

关键词： coal biotransformation methanogens microbial mechanism in situ environment carbon cycle

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Quartz types,genesis and their geological significance within the Wufeng-Longmaxi Formation in north-western Hunan,China

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Frontiers of Earth Science 2023年第2期17卷 455-469页

作者： Ke ZHANG shuheng tang Zhaodong XI Yapei YE School of Energy Resource China University of Geosciences(Beijing)Beijing 100083China Key Laboratory of Marine Reservoir Evolution and Hydrocarbon Enrichment Mechanism Ministry of EducationBeijing 100083China Key Laboratory of Strategy Evaluation for Shale Gas Ministry of Land and ResourcesBeijing 100083China

Quartz is an important mineral component in the Late Ordovician–Early Silurian Wufeng-Longmaxi Formation with various forms and sources and has a significant impact on the properties of shale gas *** this study,geochemical analysis,scanning electron microscopy(SEM)observation,and rock mechanics testing were performed on shale samples from the Wufeng-Longmaxi Formation in north-western Hunan,South *** is classified into four types based on morphological features and cathodoluminescence(CL)images under SEM–terrigenous detrital quartz,quartz overgrowths,biogenic skeletal quartz and *** quartz in Upper Longmaxi Formation is predominantly of terrigenous origin and contains a small amount of quartz formed by clay *** quartz in the Wufeng-Lower Longmaxi Formation is predominantly *** biogenic quartz has a direct effect on organic matter(OM)abundance,pore structure and *** is indicated by the positive correlation with TOC content and biogenic Ba content that biogenic quartz-rich strata have high *** rigid frameworks formed by biogenic quartz during the early diagenesis stage facilitated the preservation of the primary *** interparticle pores of biogenic quartz are the space for OM preservation and migration,creating conditions for the development of OM ***,the calculated brittleness index(BI)shows a positive correlation with biogenic quartz content,indicating that layers rich in biogenic quartz are more conducive to ***,the Wufeng-Lower Longmaxi Formation has higher OM content,porosity and represents a more favorable exploration and development target.

关键词： quartz silica source porosity organic matter rock mechanics

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沁水盆地榆社—武乡区块二叠系煤系页岩储层地质建模及“甜点”预测

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岩性油气藏 2024年第4期36卷 98-108页

作者：申有义王凯峰唐书恒张松航郗兆栋杨晓东自然资源部矿业城市自然资源调查监测与保护重点实验室山西晋中030600 山西省煤炭地质物探测绘院有限公司山西晋中030600 中国地质大学(北京)能源学院北京100083 非常规天然气能源地质评价与开发工程北京市重点实验室北京100083

沁水盆地煤系页岩气资源丰富,但勘探开发处于初期阶段。基于钻井、测井和地震解释资料,结合有机地球化学与储层物性实验测试数据,通过三维地质建模技术,建立了沁水盆地榆社—武乡区块二叠系山西组底部—太原组上部煤系页岩地质模型,并... 详细信息

沁水盆地煤系页岩气资源丰富,但勘探开发处于初期阶段。基于钻井、测井和地震解释资料,结合有机地球化学与储层物性实验测试数据,通过三维地质建模技术,建立了沁水盆地榆社—武乡区块二叠系山西组底部—太原组上部煤系页岩地质模型,并预测了煤系页岩气“甜点”区。研究结果表明:(1)沁水盆地榆社—武乡区块石炭系—二叠系煤系地层模型反映了煤系页岩储层的发育主要受控于构造活动,呈“东浅西深、整体连续”的分布格局。(2)基于序贯指示法建立沉积相模型,指示研究区在太原期—山西期由海陆过渡相转变为近海陆相沉积环境,为稳定优质页岩储层的形成提供了有利的沉积环境。(3)通过相控属性建模实现了储层参数空间分布模拟和精细表征,泥地比、孔隙度、含气量、总有机碳含量和镜质体反射率的平均值分别为0.57,10.02%,1.21 m^(3)/t,2.18%,2.45%,揭示了研究区煤系页岩较好的储集能力、含气性、有机质丰度和资源潜力,脆性指数模型指示出页岩压裂后的有利区带。(4)在精细三维地质建模的基础上,将三维网格单元赋值积分,计算研究区二叠系煤系页岩气地质资源量为1 344.98×10^(8)m^(3),运用层次分析法和模糊评价法预测页岩气“甜点”区,Ⅰ类“甜点”区为地质与工程双重甜点,分布于研究区东北部、中部和西北部局部区域。

关键词：煤系地层页岩气地质建模储层特征 “甜点”预测地质资源量二叠系榆社—武乡区块沁水盆地

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A Comprehensive Model for Evaluating Coalbed Methane Reservoirs in China

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Acta Geologica Sinica(English Edition) 2008年第6期82卷 1253-1270页

作者： YAO Yanbin LIU Dameng tang Dazhen HUANG Wenhui tang shuheng CHE Yao School of Energy Resources China University of Geosciences Beijing 100083 China

Coalbed methane reservoir （CBMR） evaluation is important for choosing the prospective target area for coalbed methane exploration and production. This study aims at identifying the characteristic parameters and methods to evaluate CBMR. Based on the geological surveys, laboratory measurements and field works, a four-level analytic hierarchy process （AHP） model for CBMR evaluation is proposed. In this model, different weights are prioritized and assigned on the basis of three main criteria （including reservoir physical property, storage capacity and geological characteristics）, 15 sub-criteria, and 18 technical alternatives; the later of which are discussed in detail. The model was applied to evaluate the CBMR of the Permo-Carboniferous coals in the Qinshui Basin, North China. This GIS-based fuzzy AHP comprehensive model can be used for the evaluation of CBMR of medium-high rank （mean maximum vitrinite reflectance 〉0.5 %） coal districts in China.

关键词： coalbed methane reservoir reservoir evaluation reservoir characterization comprehensive model Fuzzy Hierarchy Process Approach (FAHP)

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建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

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