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Enhanced ferroelectric and improved leakage of BFO-based thin films through increasing entropy strategy

International Journal of Minerals,Metallurgy and Materials 2024年第10期31卷 2263-2273页

作者： Dongfei Lu Guoqiang Xi Hangren li Jie tu Xiuqiao liu Xudong liu Jianjun Tian linxing Zhang Institute for Advanced Materials Technology University of Science and Technology BeijingBeijing 100083China

BiFeO_(3)(BFO)has received considerable attention as a lead-free ferroelectric film due to its large theoretical remnant ***,BFO suffers from a large leakage current,resulting in poor ferroelectric ***,the sol-gel method was used to deposit a series of BFO-based thin films on fluorine-doped tin oxide substrates,and the effects of the substitution of the elements Co,Cu,Mn(B-site)and Sm,Eu,La(A-site)on the crystal structure,ferroelectricity,and leakage current of the BFO-based thin films were *** confirmed that lattice distortion by X-ray diffraction can be attributed to the substitution of individual elements in the BFO-based *** and Eu substitutions contribute to the lattice distortion in a pseudo-cubic structure,while La is biased toward *** force microscopy confirmed that reversible switching of ferroelectric domains by nearly 180°can be realized through the prepared *** ferroelectric hysteresis loops showed that the order for the polarization contribution is as follows:Cu>Co>Mn(B-site),Sm>La>Eu(A-site).The current density voltage curves indicated that the order for leakage contribution is as follows:Mnlitates the formation of dense grains,and the grain size distribution statistics proved that La element promotes the reduction of grain size,leading to the increase of grain boundaries and the reduction of ***,a Bi_(0.985)Sm_(0.045)La_(0.03)Fe_(0.96)Co_(0.02)Cu_(0.02)O_(3)(SmLa-CoCu)thin film with a qualitative leap in the remnant polarization from 25.5(Bi_(0.985)Sm_(0.075)FeO_(3))to 98.8µC/cm^(2)(SmLa-CoCu)was prepared through the syner-gistic action of Sm,La,Co,and Cu *** leakage current is also drastically reduced from 160 to 8.4 mA/cm^(2)at a field strength of 150 kV/***,based on the increasing entropy strategy of chemical engineering,this st

关键词： increasing entropy synergistic ferroelectric film remnant polarization leakage current

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A Fault Detection Method for Electric Vehicle Battery System Based on Bayesian Optimization SVDD Considering a Few Faulty Samples

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Energy Engineering 2024年第9期121卷 2543-2568页

作者： Miao li Fanyong Cheng Jiong Yang Maxwell Mensah Duodu Hao tu School of Electronics and Electrical Engineering Anhui Polytechnic UniversityWuhu241000China

Accurate and reliable fault detection is essential for the safe operation of electric *** vector data description(SVDD)has been widely used in the field of fault ***,constructing the hypersphere boundary only describes the distribution of unlabeled samples,while the distribution of faulty samples cannot be effectively described and easilymisses detecting faulty data due to the imbalance of sample ***,selecting parameters is critical to the detection performance,and empirical parameterization is generally timeconsuming and laborious and may not result in finding the optimal ***,this paper proposes a semi-supervised data-driven method based on which the SVDD algorithm is improved and achieves excellent fault detection *** incorporating faulty samples into the underlying SVDD model,training deals better with the problem of missing detection of faulty samples caused by the imbalance in the distribution of abnormal samples,and the hypersphere boundary ismodified to classify the samplesmore *** Bayesian Optimization NSVDD(BO-NSVDD)model was constructed to quickly and accurately optimize hyperparameter *** the experiments,electric vehicle operation data with four common fault types are used to evaluate the performance with other five models,and the results show that the BO-NSVDD model presents superior detection performance for each type of fault data,especially in the imperceptible early and minor faults,which has seen very obvious ***,the strong robustness of the proposed method is verified by adding different intensities of noise in the dataset.

关键词： Fault detection vehicle battery system lithium batteries fault samples

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The synergistic regulatory effect of PTP1B and PTK inhibitors on the development of Oedaleus decorus asiaticus Bei-Bienko

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Journal of Integrative Agriculture 2024年第8期23卷 2752-2763页

作者： Shuang li Sibo liu Chaomin Xu Shiqian Feng Xiongbing tu Zehua Zhang State Key Laboratory for Biology of Plant Diseases and Insect Pests Institute of Plant ProtectionChinese Academy of Agricultural SciencesBeijing 100193China Chongqing Academy of Agricultural Sciences Chongqing 401329China Institute of Grassland Research Chinese Academy of Agricultural SciencesHohhot 010010China Inner Mongolia University Hohhot 010019China Scientific Observation and Experimental Station of Pests in Xilin Gol Rangeland Institute of Plant ProtectionChinese Academy of Agricultural SciencesXilinhot 026000China

Tyrosine phosphorylation is crucial for controlling normal cell growth,survival,intercellular communication,gene transcription,immune responses,and other *** tyrosine phosphatase(PTP)and protein tyrosine kinases(PTK)can achieve this goal by regulating multiple signaling *** decorus asiaticus is an important pest that infests the Mongolian Plateau *** aimed to evaluate the survival rate,growth rate,overall performance,and ovarian developmental morphology of the 4th instar nymphs of *** asiaticus while inhibiting the activity of protein tyrosine phosphatase-1B(PTP1B)and *** addition,the expression and protein phosphorylation levels of key genes in the MAPK signaling pathway and antioxidant enzyme activity were *** results showed no significant differences in survival rate,growth rate,or overall performance between PTP1B inhibitor treatment and ***,after PTK inhibitor treatment,these indexes were significantly lower than those in the *** ovarian size of female larvae after 15 days of treatment with PTK inhibitors showed significantly slower development,while female larvae treated with PTP1B exhibited faster ovarian growth than the control *** comparison to controls and nymphs treated with PTK inhibitors,the expression and phosphorylation levels of key genes in the MAPK signaling pathway under PTP1B inhibitor treatments were significantly higher in 4th instar ***,reactiveoxygen(ROS)species levels and the activities of NADPH oxidase and other antioxidant enzymes were considerably reduced,although they were significantly greater in the PTK inhibitor *** results suggest that PTP1B and PTK feedback inhibition in the mitogen-activated-protein kinases(MAPK)signal transfer can regulate the physiological metabolism of the insect as well as its developmental *** findings can facilitate future uses of PTP1B and PTK inhibitors in controlling insect development to help contro

关键词： PTP1B PTK inhibitor MAPK pathway Oedaleus decorus asiaticus development

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Association of prealbumin with short-term and long-term outcomes in patients with acute ST-segment elevation myocardial infarction

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Journal of Geriatric Cardiology 2024年第4期21卷 421-430页

作者： Jing TAN Jin SI Ke-ling XIAO Ying-hua ZHANG Qi hua Jing li Department of Cardiology Xuanwu Hospital Capital Medical UniversityBeijingChina Department of Geriatric Medicine Xuanwu Hospital Capital Medical UniversityNational Clinical Research Center for Geriatric DiseasesBeijingChina

BACKGROUND Prealbumin is considered to be a useful indicator of nutritional status. Furthermore, it has been found to be associated with severities and prognosis of a range of diseases. However, limited data on the association of baseline prealbumin level with outcomes of patients with acute ST-segment elevation myocardial infarction(STEMI) are *** We analyzed 2313 patients admitted for acute STEMI between October 2013 and December 2020. In-hospital outcomes and mortality during the 49 months(interquartile range: 26–73 months) follow-up period were compared between patients with the low prealbumin level(lization. After propensity score matching, patients with the low prealbumin level than those with the high prealbumin level experienced higher incidences of heart failure with Killip class Ⅲ(9.9%vs. 4.4%, P = 0.034), cardiovascular death(8.4% vs. 3.4%, P = 0.035) and the composite of major adverse cardiovascular events(19.2%vs. 10.3%, P = 0.012). Multivariate logistic regression analysis identified that the low prealbumin level(line prealbumin level(170 mg/L) was no longer independently associated with 49-month cardiovascular death. After propensity score matching, Kaplan-Meier survival curves revealed consistent *** Decreased prealbumin level closely related to unfavorable short-term outcomes. However, after multivariate adjustment and controlling for baseline differences, baseline prealbumin level was not independently assoc

关键词： patients admitted infarction

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The Q-index and Connectivity of Graphs

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Journal of the Operations Research Society of China 2024年第2期12卷 505-519页

作者： Peng-li Zhang li-hua Feng Wei-Jun liu Xiao-Dong Zhang School of Mathematical Sciences MOE-LSCSHL-MACShanghai Jiao Tong UniversityShanghai 200240China School of Mathematics and Statistics Central South UniversityChangsha 410083HunanChina

A connected graph G is said to be k-connected if it has more than k vertices and remains connected whenever fewer than k vertices are *** this paper,for a connected graph G with sufficiently large order,we present a tight sufficient condition for G with fixed minimum degree to be k-connected based on the *** result can be viewed as a spectral counterpart of the corresponding Dirac-type condition.

关键词： Q-index Minimum degree k-connected

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Advances in Polysaccharide-Based Microneedle Systems for the Treatment of Ocular Diseases

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Nano-Micro Letters 2024年第12期16卷 233-284页

作者： Qingdong Bao Xiaoting Zhang Zhankun Hao Qinghua li Fan Wu Kaiyuan Wang Yang li Wenlong li hua Gao State Key Laboratory Cultivation Base Shandong Provincial Key Laboratory of OphthalmologyEye Institute of Shandong First Medical UniversityQingdao 266071People’s Republic of China State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002People’s Republic of China Eye Hospital of Shandong First Medical University Jinan 250021People’s Republic of China College of Ophthalmology Shandong First Medical UniversityJinan 250000People’s Republic of China Departments of Diagnostic Radiology SurgeryChemical and Biomolecular Engineeringand Biomedical EngineeringYong Loo Lin School of Medicine and College of Design and EngineeringNational University of SingaporeSingapore 119074Singapore

The eye,a complex organ isolated from the systemic circulation,presents significant drug delivery challenges owing to its protective mechanisms,such as the blood-retinal barrier and corneal *** drug administration methods often fail to sustain therapeutic levels and may compromise patient safety and *** microneedles(PSMNs)have emerged as a transformative solution for ophthalmic drug ***,a comprehensive review of PSMNs in ophthalmology has not been published to *** this review,we critically examine the synergy between polysaccharide chemistry and microneedle technology for enhancing ocular drug *** provide a thorough analysis of PSMNs,summarizing the design principles,fabrication processes,and challenges addressed during fabrication,including improving patient comfort and *** also describe recent advances and the performance of various PSMNs in both research and clinical ***,we review the current regulatory frameworks and market barriers that are relevant to the clinical and commercial advancement of PSMNs and provide a final perspective on this research area.

关键词： Ocular delivery Polysaccharide Microneedles Drug administration

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Phase-Dislocation-Mediated High-Dimensional Fractional Acoustic-Vortex Communication

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Research 2024年第3期2023卷 575-584页

作者： Ruijie Cao Gepu Guo Wei Yue Yang huang Xinpeng li Chengzhi Kai Yuzhi li Juan tu Dong Zhang Peng Xi Qingyu Ma School of Computer and Electronic Information Nanjing Normal UniversityNanjing 210023China Department of Biomedical Engineering College of Future TechnologyPeking UniversityBeijing 100871China nstitute of Acoustics Nanjing UniversityNanjng 210093China National Biomedical Imaging Center Peking UniversityBeijing 100871China

With unlimited topological modes in mathematics,the fractional orbital angular momentum(FOAM)demonstrates the potential to infinitely increase the channel capacity in acoustic-vortex(AV)***,the accuracy and stability of FOAM recognition are still limited by the nonorthogonality and poor anti-interference of fractional AV *** popular machine learning,widely used in optics based on large datasets of images,does not work in acoustics because of the huge engineering of the 2-dimensional point-by-point ***,we report a strategy of phase-dislocation-mediated high-dimensional fractional AV communication based on pair-FOAM multiplexing,circular sparse sampling,and machine *** unique phase dislocation corresponding to the topological charge provides important physical guidance to recognize FOAMs and reduce sampling points from theory to practice.A straightforward convolutional neural network considering turbulence and misalignment is further constructed to achieve the stable and accurate communication without involving experimental *** experimentally present that the 32-point dual-ring sampling can realize the 10-bit information transmission in a limited topological charge scope from±0.6 to±2.4 with the FOAM resolution of 0.2,which greatly reduce the divergence in AV *** infinitely expanded channel capacity is further verified by the improved FOAM resolution of *** with other milestone works,our strategy reaches 3-fold OAM utilization,4-fold information level,and 5-fold OAM *** of the extra advantages of high dimension,high speed,and low divergence,this technology may shed light on the next-generation AV communication.

关键词： infinitely topological fractional

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Intestinal microecological transplantation for a patient with chronic radiation enteritis:A case report

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World Journal of Gastroenterology 2024年第19期30卷 2603-2611页

作者： lin Wang Yan li Yu-Jing Zhang li-hua Peng Department of Gastroenterology and Hepatology The First Medical CenterChinese PLA General HospitalBeijing 100853China Department of Gastroenterology and Hepatology Chinese PLA Medical SchoolBeijing 100853China

BACKGROUND The gut microbiota is strongly associated with radiation-induced gut *** study aimed to assess the effectiveness and safety of intestinal microecological transplantation for treating patients with chronic radiation *** SUMMARY A 64-year-old female with cervical cancer developed abdominal pain,diarrhea,and blood in the stool 1 year after *** electronic colonoscopy was performed to diagnose chronic radiation *** courses of intestinal microecological transplantation and full-length 16S rRNA microbiological analysis were *** patient experienced short-and long-term relief from symptoms without adverse *** 16S rRNA sequencing revealed significant differences in the intestinal flora’s composition between patient and healthy *** bacteria,such as Escherichia fergusonii and Romboutsia timonensis,were more in the *** bacteria such as Faecalibacterium prausnitzii,Fusicatenibacter saccharivorans,Ruminococcus bromii,and Bifidobacterium longum were more in the healthy *** microbiota transplantation resulted in a significant change in the patient's intestinal flora *** composition converged with the donor's flora,with an increase in core beneficial intestinal bacteria,such as Eubacterium rectale,and a decrease in pathogenic *** in the intestinal flora corresponded with the patients'alleviating clinical *** Intestinal microecological transplantation is an effective treatment for relieving the clinical symptoms of chronic radiation enteritis by altering the composition of the intestinal *** study provides a new approach for treating patients with chronic radiation enteritis.

关键词： Chronic radiation enteritis Gut microbial transplantation Intestinal microecology Cancer Quality of life Case report

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Shortest or locally quickest? A prediction-based approach for evacuation choice simulation between multiple staircases

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JOURNAL OF SAFETY SCIENCE AND RESIliENCE 2024年第3期5卷 281-294页

作者： hua, Ying Zhao, Jincheng li, Hai-Ting Duan, liping Shanghai Jiao Tong Univ Sch Ocean & Civil Engn Dept Civil Engn Shanghai 200240 Peoples R China Shanghai Jiao Tong Univ Shanghai Key Lab Digital Maintenance Bldg & Infras Shanghai 200240 Peoples R China

Staircase choice is one of the most critical factors leading to the difference in pedestrian flow and evacuation routes in buildings with multiple staircases. Neither the shortest path to the building exit nor the locally quickest path to the nearest staircase can represent the natural mode of evacuation path choices for an authentic evacuation simulation. Thus, a prediction-based approach is established to predict and simulate evacuation choices, which helps to address three key issues: (1) extracting evacuation data through a controlled experiment; (2) establishing a Logit model for staircase choice prediction based on experimental data; (3) developing a prediction-based cellular automaton model. The proposed approach has achieved the coupling between choice prediction and evacuation simulation. A comparison with Pathfinder software is conducted to reveal the superiority of the prediction-based CA model for simulating staircase choice.

关键词： Evacuation Staircase choice Prediction-based Logit Cellular automaton EXIT CHOICE MODEL

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Controllable synthesis of one-dimensional silicon nanostructures based on the dual effects of electro-deoxidation and the Kirkendall effect

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Nano Research 2024年第9期17卷 7814-7823页

作者： Jianxin tu Shuo Yu Kui Hao Le Sun Ruicheng Bai Fangzhou Zhang Aijun li Hong liu Institute of Materials School of Materials Science and EngineeringShanghai UniversityShanghai 200444China Department of Applied Physics The Hong Kong Polytechnic UniversityKowloon 999077Hong KongChina Shaoxing institute of technology Shanghai UniversityShanghai 200444China

In this study,we successfully synthesized silicon nanotubes(Si-NTs)and silicon nanowires(Si-NWs)in a controllable manner using a catalyst-and template-free method through the direct electrolysis of SiO_(2)in a molten CaCl_(2)-CaO system,while also proposing a novel formation mechanism for ***-NWs are formed through electro-deoxidation when the cell voltage is within the range of CaO decomposition voltage and SiO_(2)decomposition *** subsequently adjusting the voltage to a value between the decomposition potentials of CaCl_(2)and CaO,in-situ electro-deoxidation of CaO takes place on the surface of the synthesized Si-NWs,leading to the formation of a Ca *** formation of Ca-Si diffusion couple leads to the creation of vacancies within the Si-NWs,as the outward diffusion rate of Si exceeds the inward diffusion rate of *** differential diffusion rates between Si and Ca in a diffusion couple exhibit an analogy to the Kirkendall *** vacancies gradually accumulate and merge,forming large voids,which ultimately result in the formation of hollow *** a subsequent dealloying process,the removal of the embedded calcium leads to the formation of *** the application of a carbon coating,the Si-NTs@C composite showcases a high initial discharge capacity of 3211 mAh·g^(-1)at 1.5 A·g^(-1)and exhibits exceptional long-term cycling stability,maintaining a capacity of 977 mAh·g^(-1)after 2000 cycles at 3.0 A·g^(-1).

关键词： silicon nanotubes silicon nanowires lithium-ion battery Kirkendall effect

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