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Photocatalytic reduction of CO_(2) with H_(2)O into C_(2)H_(6) mediated by dual metalation strategy

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Science China Chemistry 2024年第5期67卷 1381-1383页

作者： mei Wang tong-Bu Lu School of Materials Science and Engineering Institute for New Energy Materials&Low Carbon TechnologiesTianjin University of TechnologyTianjin 300384China

Artificial solar-energy-driven CO_(2) reduction into value-added fuels under mild conditions provides a promising strategy to mitigate energy crisis and alleviate environmental issues around the world. Among diverse products of CO_(2) reduction reaction, C_(2+) compounds are more desirable in terms of their high energy density and commercial value [1].Thus far, various photocatalysts have been constructed for CO_(2) reduction.

关键词： reduction desirable value

Self-organized TiO_(2)Nanotube Arrays with Controllable Geometric Parameters for Highly Efficient PEC Water Splitting

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Chinese Journal of Structural Chemistry 2022年第2期41卷 159-167,I0012页

作者： WANG Tian-Ming CHEN Yan-Xin tong mei-hong LIN Shi-Wei ZHOU Jing-Wen JIANG Xia LU Can-Zhong CAS Key Laboratory of Design and Assembly of Functional Nanostructures and Fujian Provincial Key Laboratory of NanomaterialsFujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China College of Chemistry and Materials Science Fujian Normal UniversityFuzhou 350007China Xiamen Institute of Rare-earth Materials Haixi InstitutesChinese Academy of SciencesXiamen 361021China

In this report,a series of self-organized TiO_(2)nanotube arrays were prepared by anodization of titanium foil in mixed electrolytes composed of water,ethylene glycol,and NH_(4)*** photoelectrochemical(PEC)performance as a photoanode was characterized by the PEC water-splitting hydrogen(H_(2))generation *** internal relationship between the TiO_(2)nanotube arrays(TNTAs)morphology and their PECperformance was thoroughly *** results show that when the etching time is 10 hours,the length of the as-prepared TNTAs is about 20.78μm and the measured photocurrent density is around 1.25 m A·cm^(-2)with applied bias voltage 0.6 V(***/Ag Cl)under simulated sunlight irradiation,which is 976 times higher than that of the TiO_(2)substrate without nanotubes architecture(0.00128 m A×cm^(-2)).More interestingly,the results of the IPCEmeasurement show that the band-gap of the as-prepared TNTAs is reduced from 3.20 to 2.83 *** corresponding optical response limit is also extended from 400 nm to TiO_(2)nanotube arrays is 510 nm,which indicates that the increasement of the TNTAs PEC performance benefits from the great improvement of its utilization of both the UVand visible light irradiation.

关键词： photoelectrochemistry water-splitting TiO_(2)nanotube arrays H_(2)

The Non-inclusion Diagnosability of Hypercubes Under the PMC Model

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Journal of the Operations Research Society of China 2024年第2期12卷 478-484页

作者： mei-Jie Ma Min Xu tong-tong Ding Xiang-Jun Li Qiang Zhu School of Mathematics and Statistics Qilu University of Technology(Shandong Academy of Sciences)Jinan 250353ShandongChina School of Mathematical Sciences Beijing Normal UniversityLaboratory of Mathematics and Complex SystemsMinistry of EducationBeijing 100875China School of Information and Mathematics Yangtze UniversityJingzhou 434023HubeiChina School of Mathematics and Statistics XiDian UniversityXi'an 710071ShaanXiChina

Diagnosability of a multiprocessor system is an important measure of the reliability of interconnection ***-level diagnosis is a primary strategy to identify the faulty processors in a multiprocessor *** on a sound assumption proposed by Zhu et ***,we proposed a new diagnosability named non-inclusion diagnosability and showed that the non-inclusion diagnosability t_(N)(Q_(n))of the hypercube under the PMC model is *** is,assume that if two vertex sets F_(1) and F_(2) are both consistent with a syndrome and F_(1)C F_(2),then F_(2) is not the faulty set which we are looking for;the faulty set F is 1-step diagnosable if|F|≤2n-2 in Q_(n) under the PMC model.

关键词： Interconnection network Diagnosability Hypercube PMC model

Video caching and scheduling with edge cooperation

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Digital Communications and Networks 2024年第2期10卷 450-460页

作者： Zhidu Li Fuxiang Li tong Tang hong Zhang Jin Yang School of Communication and Information Engineering Chongqing University of Posts and TelecommunicationsChongqing400065China Advanced Network and Intelligent Connection Technology Key Laboratory of Chongqing Education Commission of China Chongqing400065China Key Laboratory of Ubiquitous Sensing and Networking in Chongqing Chongqing400065China

In this paper,we explore a distributed collaborative caching and computing model to support the distribution of adaptive bit rate video *** aim is to reduce the average initial buffer delay and improve the quality of user *** the difference between global and local video popularities and the time-varying characteristics of video popularity,a two-stage caching scheme is proposed to push popular videos closer to users and minimize the average initial buffer *** on both long-term content popularity and short-term content popularity,the proposed caching solution is decouple into the proactive cache stage and the cache update *** the proactive cache stage,we develop a proactive cache placement algorithm that can be executed in an off-peak *** the cache update stage,we propose a reactive cache update algorithm to update the existing cache policy to minimize the buffer *** results verify that the proposed caching algorithms can reduce the initial buffer delay efficiently.

关键词： Video service Distributed and collaborative caching Long-term popularity Short-term popularity

Overcoming the Limits of Cross-Sensitivity:Pattern Recognition Methods for Chemiresistive Gas Sensor Array

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Nano-Micro Letters 2024年第12期16卷 285-341页

作者： Haixia mei Jingyi Peng Tao Wang Tingting Zhou hongran Zhao tong Zhang Zhi Yang Key Lab Intelligent Rehabil&Barrier Free Disable(Ministry of Education) Changchun UniversityChangchun 130022People’s Republic of China Shanghai Key Laboratory of Intelligent Sensing and Detection Technology School of Mechanical and Power EngineeringEast China University of Science and TechnologyShanghai 200237People’s Republic of China National Key Laboratory of Advanced Micro and Nano Manufacture Technology Department of Micro/Nano ElectronicsSchool of Electronic Information and Electrical EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012People’s Republic of China

As information acquisition terminals for artificial olfaction,chemiresistive gas sensors are often troubled by their cross-sensitivity,and reducing their cross-response to ambient gases has always been a difficult and important point in the gas sensing *** recognition based on sensor array is the most conspicuous way to overcome the cross-sensitivity of gas *** is crucial to choose an appropriate pattern recognition method for enhancing data analysis,reducing errors and improving system reliability,obtaining better classification or gas concentration prediction *** this review,we analyze the sensing mechanism of crosssensitivity for chemiresistive gas *** further examine the types,working principles,characteristics,and applicable gas detection range of pattern recognition algorithms utilized in gas-sensing ***,we report,summarize,and evaluate the outstanding and novel advancements in pattern recognition methods for gas *** the same time,this work showcases the recent advancements in utilizing these methods for gas identification,particularly within three crucial domains:ensuring food safety,monitoring the environment,and aiding in medical *** conclusion,this study anticipates future research prospects by considering the existing landscape and *** is hoped that this work will make a positive contribution towards mitigating cross-sensitivity in gas-sensitive devices and offer valuable insights for algorithm selection in gas recognition applications.

关键词： Pattern recognition Sensor array Chemiresistive gas sensor Cross-sensitivity Artificial olfactory

Effect of Hyperconjugation on Photovoltaic Performance in Pseduo-2D Perylene Diimide Derivatives

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Chinese Journal of Chemistry 2024年第7期42卷 725-730页

作者： Zhilong He Yuwen hong Guangyu Li tong Shan Yi Zhang hongliang Zhong Schoolof Chemistry and Chemical Engineering Shanghai Key Lab of Electrical Insulation and Thermal AgingShanghai Jiao Tong UniversityShanghai200230China Shanghai Institute of Organic Chemistry Chinese Academy of SciencesShanghai 200032China Shenzhen Research Institute Shanghai Jiao Tong UniversityShenzhenGuangdong 518057China

Theπ-πinteraction is acknowledged as the predominant factor to determine the molecular packing in organic photovoltaic materials,while other non-covalent intermolecular interactions especially theσ-πhyperconjugation are often ***,a perylene diimide(PDI)derivative named FIDT-PDI is designed and synthesized to shed light into the effect of hyperconjugation on the molecular packing and further the photovoltaic *** NMR and 2D NOE NMR demonstrate the formation of intermolecularσ-πhyperconjugation between the C—H bond of the PDI moiety in one molecule and the phenyl sidechain in another molecule of *** from theσ-πhyperconjugation,FIDT-PDI with twisted backbone reversely exhibits more ordered packing and stronger crystallinity compared with another PDI derivative FIDTT-PDI which has better planarity,consequently achieving superior PCE and higher carrier *** contribution is the first paradigm to unravel the structure-property relationship betweenσ-πhyper-conjugation of conjugated materials and corresponding photovoltaic performance.

关键词： Hyperconjugation Weak intermolecular interactions Conformation Organic solar cells Nonfullerene acceptor Perylene diimide

R2R3-type Lo MYB21 affects jasmonate-regulated development and dehiscence of anthers in lily(Lilium oriental hybrids)

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Horticultural Plant Journal 2024年第1期10卷 239-251页

作者： Zheng tong Tingting Dong Qiuhua Li Rui Wang Junna He Bo hong Institute of Tropical Bioscience and Biotechnology Chinese Academy of Tropical Agricultural Sciences&Hainan Institute for Tropical Agricultural ResourcesHaikouHainan 571101China Beijing Key Laboratory of Development and Quality Control of Ornamental Crops Department of Ornamental HorticultureChina Agricultural UniversityBeijing 100193China Beijing Garden Expo Management Center Beijing 100072China

Lilies are widely cultivated for cut flowers,but their large anthers carry a considerable amount of colored pollen that is dispersed *** the molecular mechanism of anther development and dehiscence could help solve this ***21,encoding a putative R2R3v-myb avian myeloblastosis viral oncogene homolog(MYB)transcription factor,was identified from oriental lilies(Lilium‘Siberia’).Real-time quantitative PCR analysis showed that LoMYB21 was mainly expressed in the anther,filament and stigma and had high expression during the late stages of lily anther ***21 had transactivation activity and was located in the nucleus through yeast one-hybrid assays and transient expression in Nicotiana *** of LoMYB21 by virus-induced gene silencing(VIGS)in Lilium‘Siberia’led to anther indehiscence and reduced the expression of genes related to Jasmonate acid(JA)biosynthesis and signal *** of LoMYB21 in DEX::LoMYB21 transgenic Arabidopsis caused procumbent inflorescences that became infertile,accompanied by higher expression of JA biosynthetic and signaling *** results demonstrated that JA content and signaling were abnormal in silenced lily and transgenic LoMYB21 Arabidopsis,which affected anther *** study indicated that LoMYB21 could regulate lily anther dehiscence through JA biosynthesis and signaling during the late stages of anther development.

关键词： Lilium LoMYB21 Anther dehiscence Jasmonate acid

A low-profile dual-broadband dual-circularly-polarized reflectarray for K-/Ka-band space applications

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Frontiers of Information Technology & Electronic Engineering 2024年第8期25卷 1145-1161页

作者： Xuanfeng tong Zhi Hao JIANG Yuan LI Fan WU Lin PENG Taiwei YUE Wei hong State Key Laboratory of Milimeter Waves School of Information Science and EngineeringSoutheast UniversityNanjing 210096China Purple Mountain Laboratories Nanjing 21lllChina State Key Laboratory of Mobile Network and Mobile Multimedia Technology ZTE CorporationShenzhen 518057China Apple Inc. One Apple Park WayCupertinoCA 95014USA

A low-profile dual-broadband dual-circularly-polarized(dual-CP)reflectarray(RA)is proposed and demonstrated,supporting independent beamforming for right-/left-handed CP waves at both K-band and *** functionality is achieved by incorporating multi-layered phase shifting elements individually operating in the K-and Ka-band,which are then interleaved in a shared aperture,resulting in a cell thickness of only about *** rotating the designed K-and Ka-band elements around their own geometrical centers,the dual-CP waves in each band can be modulated *** reduce the overall profile,planar K-/Ka-band dual-CP feeds with a broad band are designed based on the magnetoelectric dipoles and multi-branch hybrid *** planar feeds achieve bandwidths of about 32%and 26%at K-and Ka-band respectively with reflection magnitudes below-13 dB,an axial ratio smaller than 2 dB,and a gain variation of less than 1 dB.A proof-of-concept dual-band dual-CP RA integrated with the planar feeds is fabricated and characterized which is capable of generating asymmetrically distributed dual-band dual-CP *** measured peak gain values of the beams are around 24.3 and 27.3 dBic,with joint gain variation<1 dB and axial ratio<2 dB bandwidths wider than 20.6%and 14.6%at the lower and higher bands,*** demonstrated dual-broadband dual-CP RA with four degrees of freedom of beamforming could be a promising candidate for space and satellite communications.

关键词： Broadband Dual-band Dual-circularly-polarized Reflectarray Shared-aperture

崆峒山自然保护区百合科药用植物资源多样性研究及评价

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西北林学院学报 2013年第5期28卷 82-85页

作者：童红梅甘肃省平凉医学高等专科学校甘肃平凉744000

为了摸清崆峒山自然保护区百合科药用植物资源状况,为其开发利用提供科学依据。通过资料、路线、样地和补查相结合方法进行系统的调查研究。结果表明:以崆峒山后山百合科药用植物的丰富度(2.74)与多样性指数(0.41)最高,共有18属37种,分... 详细信息

为了摸清崆峒山自然保护区百合科药用植物资源状况,为其开发利用提供科学依据。通过资料、路线、样地和补查相结合方法进行系统的调查研究。结果表明:以崆峒山后山百合科药用植物的丰富度(2.74)与多样性指数(0.41)最高,共有18属37种,分别占本区百合科植物资源总属数的78.26%和82.22%,主要以多年生草本为主;地理分布以温带分布为主,占本区总属数的33.33%;中国特有种占到总种数的54.05%;药用部位以根状茎类入药的最多;药用功效主要有解表药、清热药、补益药、化痰止咳等;并参照国家药典药用价值综合评价标准对37种百合科药用植物进行了评价。崆峒山自然保护区百合科药用植物具有生物多样性特点,总体药用价值较高,极具开发与利用价值。

关键词：崆峒山百合科药用植物多样性药用价值评价