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A Generic strategy to Create Mechanically Interlocked Nanocomposite/Hydrogel Hybrid Electrodes for Epidermal Electronics

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Nano-Micro Letters 2024年第5期16卷 120-133页

作者： Qian Wang Yanyan Li Yong Lin Yuping sun Chong Bai Haorun Guo ting Fang Gaohua Hu Yanqing Lu Desheng kong College of Engineering and Applied sciences National Laboratory of Solid State Microstructureand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210023People’s Republic of China state key Laboratory of Analytical Chemistry for Life science and Jiangsu Key Laboratory of Artificial Functional MaterialsNanjing UniversityNanjing 210023People’s Republic of China College of Chemical Engineering and Technology Engineering Research Center of Seawater Utilization Technology of Ministry of EducationState Key Laboratory of Reliability and Intelligence of Electrical EquipmentHebei University of TechnologyTianjin 300130People’s Republic of China key Laboratory of Intelligent Optical sensing and Manipulation Nanjing UniversityNanjing 210093People’s Republic of China

stretchable electronics are crucial enablers for next-generation wearables intimately integrated into the human *** the primary compliant conductors used in these devices,metallic nanostructure/elastomer composites often struggle to form conformal contact with the textured *** electrodes have been consequently developed based on conductive nanocomposite and soft hydrogels to establish seamless skin-device ***,chemical modifications are typically needed for reliable bonding,which can alter their original *** overcome this limitation,this study presents a facile fabrication approach for mechanically interlocked nanocomposite/hydrogel hybrid *** this physical process,soft microfoams are thermally laminated on silver nanowire nanocomposites as a porous interface,which forms an interpenetrating network with the *** microfoam-enabled bonding strategy is generally compatible with various *** resulting interlocked hybrids have a 28-fold improved interfacial toughness compared to directly stacked *** electrodes achieve firm attachment to the skin and low contact impedance using tissue-adhesive *** have been successfully integrated into an epidermal sleeve to distinguish hand gestures by sensing mus-cle *** nanocomposite/hydrogel hybrids reported here offer a promising platform to combine the benefits of both materials for epidermal devices and systems.

关键词： stretchable electronics Epidermal electronics silver nanowire Conductive nanocomposites Hydrogel

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surface-induced Microstructure and Performance Changes in P3HT Ultrathin Films

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Chinese Journal of Polymer science 2024年第6期42卷 805-814页

作者： Hong-Tao shan Jia-Xin He Bing-Yan Zhu Xue-ting Cao Ying-Ying Yan Jian-Jun Zhou Hong Huo Beijing key Laboratory of Energy Conversion and storage Materials College of ChemistryBeijing Normal UniversityBeijing100875China

In this work,poly(3-hexylthiophene)(P3HT)ultrathin films(P3HT-T)were prepared by spin-coating a dilute P3HT solution(in a toluene:o-dichlorobenzene(Tol:ODCB)blend with a volume ratio of 80:20)with ultrasonication and the addition of the nucleating agent bicycle[2.2.1]heptane-2,3-dicarboxylic acid disodium salt(HPN-68L)on glass,si wafers and indium tin oxide(ITO)*** electrical and mechanical properties of the P3HT-T ultrathin films were investigated,and it was found that the conductivity and crack onset strain(COs)were simultaneously improved in comparison with those of the corresponding pristine P3HT film(P3HT-0,without ultrasonication and nucleating agent)on the same substrate,regardless of what substrate was ***,the conductivity of P3HT-T ultrathin films on different substrates was similar(varying from 3.7 s·cm^(-1)to 4.4 s·cm^(-1)),yet the COs increased from 97%to 138%by varying the substrate from a si wafer to *** grazing-incidence wide-angle X-ray diffraction(GIXRD),UV-visible(UV-Vis)spectroscopy and atomic force microscopy(AFM),we found that the solid order and crystallinity of the P3HT-T ultrathin film on the si wafer are highest,followed by those on glass,and much lower on ***,the surface energy and roughness of three substrates were investigated,and it was found that the polar component of the surface energyγp plays a critical role in determining the crystalline microstructures of P3HT ultrathin films on different *** work indicates that the P3HT ultrathin film can obviously improve the stretchability and simultaneously retain similar electrical performance when a suitable substrate is *** findings offer a new direction for research on stretchable CP ultrathin films to facilitate future practical applications.

关键词： P3HT ultrathin film substrate Crystalline microstructures Polar component of the surface energy Electrical and stretchable performances

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Celastrol inhibits inflammatory factors expression in glioblastoma

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Traditional Medicine Research 2024年第6期9卷 1-11页

作者： Na Qin shu-Xian Yang shi-Man Gao ting Zhu Institute of Neuroregeneration&Neurorehabilitation Department of PathophysiologySchool of Basic MedicineQingdao UniversityQingdao 266071China Department of Pharmacy Beijing Tiantan HospitalCapital Medical UniversityBeijing 100070China Women and Children’s Hospital Qingdao UniversityQingdao 266034China

Background:Glioblastoma is one of the most common primary intracranial tumors of the central nervous system in *** chemotherapy is an important component of glioblastoma treatment,its effectiveness remains *** to multiple immunosuppressive mechanisms,glioblastoma immunotherapy has not been effective in treating many patients as a result of the clinical breakthroughs in the ***,the development of cancer immunotherapy relies on the understanding of how tumors interact with the immune system and the analysis of their molecular *** study identified the key interactions between immune cells in the glioma microenvironment using RNA microarrays and single-cell ***:First,we screened differentially expressed genes in tumor and control samples from GsE29796 and GsE50161 datasets using *** differentially expressed genes were used to perform enrichment analysis and construct protein-protein interaction topological analysis to analyze the interaction between *** single-cell RNA sequencing data from the GsE162631 database,we identified immune cell types within the glioblastoma microenvironment,and validated the hub gene expression in these *** addition,based on the GEPIA and TIMER databases,hub genes were investigated and compared with immune infiltration to determine differential ***,CellChat was used to visualize the gene expression distribution and cell-to-cell communication analysis of the proteins between different types of ***:We found that monocytes/macrophages may communicate with each other in the tumor microenvironment through MIF-(CD74+CXCR4)and MIF-(CD74+CD44).In addition,our study indicated that celastrol has the ability to inhibit inflammatory factors expression by MIF/CD74 signaling pathway in U87 ***:This study improved the effectiveness of cancer immunotherapy strategies and developed new ideas for immunotherapy that can be applied to gl

关键词： glioblastoma monocytes/macrophages single-cell RNA sequencing MIF/CD74 signaling pathway celastrol

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The chance of sodium titanate anode for the practical sodium-ion batteries

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Chinese Journal of Chemical Engineering 2024年第8期72卷 226-244页

作者： Feng Chen Haoyu Li Xianyan Qiao Ruoyang Wang Changyan Hu ting Chen Yifan Niu Benhe Zhong Zhenguo Wu Xiaodong Guo school of Chemical Engineering Sichuan UniversityChengdu 610065China Institute for Advanced study Chengdu UniversityChengdu 610106China Chengdu No.7 High school Chengdu 6100412China

supporting sustainable green energy systems,there is a big demand gap for grid energy *** storage,especially sodium-ion batteries(sIBs),have advanced significantly and are now emerging as a feasible alternative to the lithium-ion batteries equivalent in large-scale energy storage due to their natural abundance and prospective inexpensive *** various anode materials of sIBs,beneficial properties,such as outstanding stability,great abundance,and environmental friendliness,make sodium titanates(NTOs),one of the most promising anode materials for the rechargeable ***,there are still enormous challenges in application of NTO,owing to its low intrinsic electronic conductivity and collapse of *** research on NTOs is still in its infancy;there are few conclusive reviews about the specific function of various modification ***,we summarize the typical strategies of optimization and analysis the fine structures and fabrication methods of NTO anodes combined with the application of in situ characterization *** work provides effective guidance for promoting the continuous development,equipping NTOs in safety-critical systems,and lays a foundation for the development of NTO-anode materials in sIBs.

关键词： sodium titanates sodium-ion batteries Modification methods Electronic materials Electrochemistry synthesis

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Working condition recognition of sucker rod pumping system based on 4-segment time-frequency signature matrix and deep learning

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Petroleum science 2024年第1期21卷 641-653页

作者： Yun-Peng He Hai-Bo Cheng Peng Zeng Chuan-Zhi Zang Qing-Wei Dong Guang-Xi Wan Xiao-ting Dong state key Laboratory of Robotics Shenyang Institute of AutomationChinese Academy of SciencesShenyang 110016LiaoningChina key Laboratory of Networked Control systems Chinese Academy of SciencesShenyang 110016LiaoningChina Institutes for Robotics and Intelligent Manufacturing Chinese Academy of SciencesShenyang 110169LiaoningChina University of Chinese Academy of sciences Beijing100049China school of Artifcial Intelligence Shenyang University of TechnologyShenyang 110870LiaoningChina

High-precision and real-time diagnosis of sucker rod pumping system(sRPs)is important for quickly mastering oil well *** learning-based method for classifying the dynamometer card(DC)of oil wells is an efficient diagnosis ***,the input of the DC as a two-dimensional image into the deep learning framework suffers from low feature utilization and high computational ***,different sRPss in an oil field have various system parameters,and the same sRPs generates different DCs at different ***,there is heterogeneity in field data,which can dramatically impair the diagnostic *** solve the above problems,a working condition recognition method based on 4-segment time-frequency signature matrix(4s-TFsM)and deep learning is presented in this ***,the 4-segment time-frequency signature(4s-TFs)method that can reduce the computing power requirements is proposed for feature extraction of DC ***,the 4s-TFsM is constructed by relative normalization and matrix calculation to synthesize the features of multiple data and solve the problem of data ***,a convolutional neural network(CNN),one of the deep learning frameworks,is used to determine the functioning conditions based on the *** on field data verify that the proposed diagnostic method based on 4s-TFsM and CNN(4s-TFsM-CNN)can significantly improve the accuracy of working condition recognition with lower computational *** the best of our knowledge,this is the first work to discuss the effect of data heterogeneity on the working condition recognition performance of sRPs.

关键词： sucker-rod pumping system Dynamometer card Working condition recognition Deep learning Time-frequency signature Time-frequency signature matrix

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Towards Lessening Learners’Aversive Emotions and Promoting Their Mental Health:Developing and Validating a Measurement of English speaking Demotivation in the Chinese EFL Context

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International Journal of Mental Health Promotion 2024年第2期26卷 161-175页

作者： Chili Li Xinxin Zhao Ziwen Pan ting Yi Long Qian school of Foreign Languages Hubei University of TechnologyWuhan430068China Faculty of Education The University of Hong KongHong Kong999077China school of Foreign Languages Henan UniversityKaifeng450046China Research Institute of International Chinese Language Education Beijing Language and Culture UniversityBeijing100083China Faculty of Humanities The Hong Kong Polytechnic UniversityHong Kong100872China school of Humanities Wuhan University of Engineering ScienceWuhan430200China

While a plethora of studies has been conducted to explore demotivation and its impact on mental health in second language(L2)education,scanty research focuses on demotivation in L2 speaking ***,little research explores the measures to quantify L2 speaking *** present two-phase study attempts to develop and validate an English speaking Demotivation scale(EsDs).To this end,an independent sample of 207 Chinese tertiary learners of English as a Foreign Language(EFL)participated in the development phase,and another group of 188 Chinese EFL learners was recruited for the validation of the *** Factor Analysis(EFA)and Confirmatory Factor Analysis(CFA)were employed to determine the factor structure of the *** EFA results revealed a six-factor solution with Teacher-related Factors in Learning spoken English(TFLsE),Interest and Valence in Learning spoken English(IVLsE),self-efficacy in Learning spoken English(sELsE),Negative Peer Influence in Learning spoken English(NPILsE),Undesirable Environment for Learning spoken English(UELsE),and Negative Influence of Assessment and Learning Materials in speaking class(NIALM).In the validation phase,Confirmatory Factor Analysis(CFA)was performed to validate the internal structure of the *** CFA results showed that the model fits the data ***,the EsDs is a robust and trustworthy psychometric tool that could be utilized to examine L2 speaking *** for diminishing EFL learners’demotivation,lessening their aversive emotions and promoting their mental health are also discussed.

关键词： Demotivation for learning English speaking EsDs scale development and validation Chinese EFL learners mental health

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Turning Cold Resources into Hot Economic Gains

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China Today 2024年第3期73卷 50-52页

作者： LIU ting 不详

Ice and snow tourism injects new momentum into rural revitalization and high-quality development in northwest China’s *** temperatures reached minus 20 degrees Celsius in December 2023 in Altay,Xinjiang Uygur Autonomous Region,but such harsh weather did not hinder well-equipped enthusiasts from skiing in the local Jiangjun Mountain ski *** its opening in November,the resort has received an average of more than 4,000 visitors per day,far exceeding that of the same period in previous years.

关键词： northwest weather Xinjiang

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Geochemical identification of a source rock affected by migrated hydrocarbons and its geological significance:Fengcheng Formation,southern Mahu sag,Junggar Basin,NW China

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Petroleum science 2024年第1期21卷 100-114页

作者： Wen-Long Dang Gang Gao Xin-Cai You ke-ting Fan Jun Wu De-Wen Lei Wen-Jun He Yong Tang state key Laboratory of Petroleum Resource and Prospecting China University of Petroleum(Beijing)Beijing102249China school of Geosciences China University of Petroleum(Beijing)Beijing102249China Exploration&Development Institute Xinjiang Oil Field CompanyKaramay834000XinjiangChina

The Fengcheng Formation is a crucial source rock and the primary reservoir for oil accumulation in the Mahu *** oils are distributed throughout the Fengcheng Formation,ranging from the edge to the interior of the sag in the southern Mahu *** crude oils originate from in-situ source rocks in shallowly buried areas and the inner deep *** migration,the crude oil from the inner deep sag affects the source rocks close to carrier beds,leading to changes in the organic geochemical characteristics of the source *** changes might alter source rock evaluations and oil-source *** on data such as total organic carbon(TOC),Rock-Eval pyrolysis of source rocks,and gas chromatography-mass spectrometry(GC-Ms)of the saturated fraction,and considering the geological characteristics of the study area,we define the identification characteristics of source rock affected by migrated hydrocarbons and establish the various patterns of influence that migrated hydrocarbons have on the source rock of the Fengcheng Formation in the southern Mahu *** source rocks of the Fengcheng Formation are mostly fair to good,containing mainly Type II organic matter and being thermally mature enough to generate *** rocks affected by migrated hydrocarbons exhibit relatively high hydrocarbon contents(s1/TOC>110 mg HC/g TOC,Extract/TOC>30%,HC:hydrocarbon),relatively low Rock-Eval Tmax values,and relatively high tricyclic terpane contents with a descending and mountain-shaped ***,biomarker composition parameters indicate a higher thermal maturity than in-situ source *** a comparison of the extract biomarker fingerprints of adjacent reservoirs and mudstones in different boreholes,three types of influence patterns of migrated hydrocarbons are identified:the edge-influence of thin sandstone-thick mudstone,the mixed-influence of sandstone-mudstone interbedded,and the full-influence of thick sandstone-thin *** finding reminds

关键词： Organic geochemistry source rock Influence of migrated hydrocarbons Fengcheng Formation southern Mahu sag

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Deformable Catalytic Material Derived from Mechanical Flexibility for Hydrogen Evolution Reaction

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Nano-Micro Letters 2024年第2期16卷 287-311页

作者： Fengshun Wang Lingbin Xie Ning sun ting Zhi Mengyang Zhang Yang Liu Zhongzhong Luo Lanhua Yi Qiang Zhao Longlu Wang College of Electronic and Optical Engineering&College of Flexible Electronics(Future Technology) Nanjing University of Posts&Telecommunications(NJUPT)9 WenyuanNanjing 210023People’s Republic of China key Laboratory of Environmentally Friendly Chemistry and Applications of Ministry of Education School of ChemistryXiangtan UniversityXiangtan 411105People’s Republic of China state key Laboratory of Organic Electronics and Information Displays&Jiangsu key Laboratory for Biosensors Institute of Advanced Materials(IAM)&Institute of Flexible Electronics(Future Technology)Nanjing University of Posts&Telecommunications9 WenyuanNanjing 210023People’s Republic of China

Deformable catalytic material with excellent flexible structure is a new type of catalyst that has been applied in various chemical reactions,especially electrocatalytic hydrogen evolution reaction(HER).In recent years,deformable catalysts for HER have made great progress and would become a research *** catalytic activities of deformable catalysts could be adjustable by the strain engineering and surface *** surface curvature of flexible catalytic materials is closely related to the electrocatalytic HER ***,firstly,we systematically summarized self-adaptive catalytic performance of deformable catalysts and various micro–nanostructures evolution in catalytic HER ***,a series of strategies to design highly active catalysts based on the mechanical flexibility of lowdimensional nanomaterials were *** but not least,we presented the challenges and prospects of the study of flexible and deformable micro–nanostructures of electrocatalysts,which would further deepen the understanding of catalytic mechanisms of deformable HER catalyst.

关键词： Deformable catalytic material Micro-nanostructures evolution Mechanical flexibility Hydrogen evolution reaction

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Circularly polarized luminescence switch based on a photochromic europium(Ⅲ) helicate derived coordination polymer

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Chinese Chemical Letters 2024年第2期35卷 272-277页

作者： Mei Li Yanyan Zhou Jingya Li Wenru Huang Zhiwei Yao Yuying Li ting Gao Pengfei Yan Hongfeng Li key Laboratory of Functional Inorganic Material Chemistry Ministry of EducationSchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080China state key Laboratory of Baiyunobo Rare Earth Resource Researches and Comprehensive Utilization Institution Baotou 014030China

Chiroptical switches based on circularly polarized luminescence(CPL)have shown the promising applications in advanced information ***,a pair of lanthanide coordination polymer enantiomers[Eu_(2)(L^(R))_(3)(BTFPO)_(2)]_(n) and[Eu_(2)(L^(s))_(3)(BTFPO)_(2)]_(n) with light-regulated CPL property are designed,which are assembled by a chiral binuclear triple-stranded Eu^(3+) helicates[Eu_(2)(L^(R/s))_(3)]coordinated with two photochromic triphenylphosphine oxides(BTFPO).Upon the alternative UV and 526 nm light irradiation,the complexes show the reversible photochromism,PL and CPL ***,the luminescence dissymmetry factor,g lum of ^(5)D_(0)→^(7)F_(1)(591 nm)transition shows an obvious increase from 0.19 to 0.29 before and after 275 nm light ***,the emission from Eu^(3+) center is not completely quenched in closed-ring state due to the low photocyclization(Ф_(o-c))quantum yield of the *** partial maintenance of emissive intensity is of essential importance for the monitor of CPL *** importantly,the CPL photo-switching property of the complexes in solid hybrid film is maintained,and still displays the enhanced CPL emission in photostationary ***,the potential applications of the doping film in logic gate and anti-counterfeiting were investigated.

关键词： Chiroptical switches Coordination polymer CPL Anti-counterfeiting Logic gate

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