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Man-made plutonium radioisotopes in the salt lakes of the Crimean peninsula

Journal of Oceanology and Limnology 2018年第6期36卷 1917-1929页

作者： tereshchenko nataliya n PROSKURnIn Vladislav Yu PARASKIV Artem A. CHUZHIKOVA-PROSKURnInA Olga D. The A.O.Kovalevsky Institute of Marine Biological Research of the Russian Academy of Sciences Sevastopol 299011Russian Federation

Investigations of ^(239+240)Pu and ^(238)Pu in the surface layer(0–5 cm) of bottom sediment in the Crimean 10 salt lakes from 4 geographical groups were carried out for the first time. The ^(239+240)Pu varied widely between regional geographical groups of lakes as well as within groups too and ranged from 11±4 to 451±43 mBq^(239+240)Pu/kg. The highest levels of ^(239+240)Pu—419±27, 443±24 and 451±43 mBq/kg were observed in the Yevpatoriya(Lake Kyzyl-Yar), the Tarkhankut(Dzharylhach) and the Kerch group(Tobechik), respectively. The lowest values of ^(239+240)Pu were identified in three lakes of the Perekop group and were 20±12, 24±6 and 48±6 mBq/kg. In all lakes ^(238)Pu was an order of magnitude lower than 239+240 Pu and varied from 4.8±2.6 to 30.7±5.5 mBq/kg. The ^(238)Pu activity was decay-corrected to 1986. The characteristic ratio of the ^(238)Pu/239+240 Pu activities in the sediment and percentage of the Chernobyl-derived Pu was calculated. The largest percentages of the Chernobyl-derived Pu were observed in the Evpatoriya group(Lake SasykSivash)—16.2%±8.26%, the Tarkhankut group(Dzharylhach)—8.4%±2.10% and the Kerch group(Aktash)—10.5%±5.56%. The study of the depth distribution of plutonium in the Lake Kyzyl-Yar bottom sediment core(0–25 cm) was fulfilled. It was shown that 239+240 Pu was high enough in all studied layers of bottom sediment, but the highest activity ratio ^(238)Pu/239+240 Pu(0.062±0.020) was found in the deepest layer of 15–20.5 cm and the percentage of Chernobyl-derived Pu was estimated at 6.8%±2.85% in this layer.

关键词： plutonium radioisotopes 238,239+240 Pu bottom sediments global fallout Chernobyl accident Crimean salt lakes

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Porous Shish-Kebab Structure Prepared from Oriented UHMWPE Films by Processing in Supercritical CO_(2)

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Chinese Journal of Polymer Science 2024年第1期42卷 97-104,I0009页

作者： Sergey A.Lermontov Aleksey V.Maksimkin nataliya A.Sipyagina Tarek Dayyoub Alena n.Malkova Evgeniy A.Kolesnikov Elena A.Straumal Inna O.Gozhikova Saidkhodzha G.nematulloev Dmitry V.Telyshev Institute of Physiologically Active Compounds of the Russian Academy of Sciences Chernogolovka 142432Russia Institute for Bionic Technologies and Engineering I.M.Sechenov First Moscow State Medical University(Sechenov University)Moscow 19991Russia national University of Science and Technology"MISIS"Moscow 119049 Russia Institute of Biomedical Systems National Research University of Electronic TechnologyZelenogradMoscow 124498Russia

For the first time, a highly crystalline porous shish-kebab structure with a high degree of crystallinity was obtained by using a combination of two methods for the formation of porous polymeric materials. A treatment procedure using supercritical carbon dioxide(sc CO_(2))was carried out for oriented ultrahigh molecular weight polyethylene(UHMWPE) films, which provided special conditions for the crystallization of dissolved UHMWPE macromolecules on the surface of oriented UHMWPE crystals. The prepared porous materials were investigated by scanning electron microscopy(SEM) and differential scanning calorimetry(DSC). The particularity of the obtained porous shish-kebab is the absence of the amorphous phase between lamellar crystals(kebabs). The obtained pores had an oval shape, and they were oriented in the orientation direction of the UHMWPE macromolecules. The pore size ranged from 0.05 μm to 4 μm. Controlling the conditions for the crystallization of the UHMWPE macromolecules using supercritical CO_(2) gives the possibility to control the size of both lamellar disks and pores formed.

关键词： UHMWPE Supercritical CO_(2) Porous shish-kebab structure

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Additive manufacturing of high entropy alloys:A practical review

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Journal of Materials Science & Technology 2021年第18期77卷 131-162页

作者： Ahmad Ostovari Moghaddam nataliya A.Shaburova Marina n.Samodurova Amin Abdollahzadeh Evgeny A.Trofimov Department of Materials Science.Physical and Chemical Properties of Materials.South Ural State University 76 Lenin AveChelyabinsk454080Russian Federation Department of Metal Forming South Ural State University76 Lenin AveChelyabinsk.454080Russian Federation Department of Materials Science and Engineering Faculty of EngineeringShahid Chamran University ofAhvazAhvazIran

The novel idea of alloying,which is based on the utilization of multiple principal elements in high concentrations,has created a novel class of promising materials called high entropy alloys(HEAs).So far,several HEAs with outstanding properties beyond those of conventional alloys have been discovered,and new superior high-entropy alloys are still expected to be developed in the ***,the fabrication process of HEAs through conventional manufacturing techniques suffers from significant limitations due to the intrinsic requirements of *** manufacturing(AM),on the other hand,has provided new opportunities for fabricating geometrically complex HEAs with the possibility of in situ tailoring of their microstructure *** the growing interest in AM of HEAs during most recent years,this review article aims at providing the state of the art in AM of *** describes the feedstock requirements for laser based AM ***,a comprehensive picture of the current state of nearly all HEAs processed by laser metal deposition(LMD),selective laser melting(SLM)and selective electron beam melting(SEBM)is *** attention is paid to the features of AM derived microstructures along with their outstanding properties and underlying mechanisms for various material processing *** AM of interstitial solute hardening HEAs,HEA matrix composites as well as non-beam based AM of HEAs will also be *** post-AM treatments and the strategies to fabricate defect-free HEAs are ***,a conclusion of current state and future prospects of additive manufacturing of HEAs will be presented.

关键词： High entropy alloys Additive manufacturing Microstructure Mechanical properties

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The effect of two COVID-19 lockdowns on physical activity of school-age children

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Sports Medicine and Health Science 2022年第2期4卷 119-126页

作者： Olena Yelizarova Tetiana Stankevych Alla Parats nadiya Polka Oksana Lynchak nataliya Diuba Svitlana Hozak State Institution“O.M.Marzieiev Institute for Public Health” National Academy of Medical Sciences of UkraineKyivUkraine Brovary School n9 Kyiv OblastUkraine

The introduction of strict quarantine restrictions in many countries initiated a direction in science to study the behavioral characteristics of children and adolescents during the social isolation at the population *** present our observations during the two lockdowns in *** objective of this study was to determine:a)the level of light(LPA)and moderate-to-vigorous(MVPA)physical activity among school-age children,and b)the impact of the external and internal factors on their physical activity during the *** Physical Activity Questionnaire(GPAQ)as part of our questionnaire Q-RAPH was *** of 1091 children 6–18 years old(54%boys)filled Q-RAPH at two measurement points in 2020 and *** performing AnCOVA and logistic regression,we found a significant decrease in MVPA by 12.7%in 2021 compared to 2020(png both *** proportion of children who reach the recommended levels of MVPA also decreased by 13.7%in 2021(pnegatively affecting the achievement of 60 min a day of MVPA were female gender,chronic diseases,overweight/obesity,non-participation in organized sports,and a decrease in the average air *** study evidences the insufficient level of preventive measures and requires an intensification of health education among the Ukrainian *** developing preventive measures,special attention should be paid to groups vulnerable to MVPA reduction as children who have chronic diseases and/or overweight/obesity as well as non-participation in sports.

关键词： Children Adolescents School-age Physical activity Lockdown COVID-19

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Enhanced photodegradation activity of ZnO:Eu3+and ZnO:Eu3+@Au 3D hierarchical structures

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Journal of Rare Earths 2020年第1期38卷 21-28页

作者： nataliya Babayevska Igor Iatsunskyi Patryk Florczak Marcin Jarek Barbara Peplińska Stefan Jurga nanoBioMedical Centre Adam Mickiewicz University

In this work the flower-like hierarchical structures(HS) based on 3 D pristine ZnO,ZnO:Eu^3+ and ZnO:Eu^3+ @Au were successfully obtained by a template-free solvothermal and deposition-precipitation *** decolorization/photodegradation of these structures towards model organic dye(rhodamine 6 G) was *** synthesized ZnO-based HS were characterized by X-ray diffraction(XRD),scanning electron microscopy(SEM),UV-vis and photoluminescence(PL) *** proposed synthesis approaches allow to obtain highly crystalline 3 D ZnO,ZnO:Eu^3+ and ZnO:Eu^3+ @Au *** of scanning microscopy show that ZnO flower-like HS are assemblies from smaller components,forming larger ones,the whole ZnO structure was approximately 3 μ*** nanoparticles(size^10 nm)are successfully deposited on ZnO HS *** studies show that ZnO is an ideal matrix for incorporation of Eu^3+ ions in broad concentration range(Eu^3+=1.0 at%-5.0 at%) with an efficient red *** strong UV emission in ZnO,as well as ZnO;Eu^3+HS is observed under 325 nm *** of ZnO HS matrix by Eu^3+ions leads to the red shift of deep level emission peak(DLE).The PL intensity reaches the maximum up to 5 at% Eu^3+.The photocatalytic properties of ZnO and ZnO:Eu^3+ @Au HS were investigated under UV-Vis light irradiation towards rhodamine 6 *** obtained results demonstrate the synergetic effect of the deposited gold nanoparticles and Eu3^+ doping on photocatalytic activity of ZnO:Eu^3+@Au HS in comparison to pristine ZnO and ZnO:Eu^3+ HS.

关键词： Zinc oxide Hierarchical structures Europium Gold Photocatalysis Rhodamine 6G

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Pulsed laser reshaping and fragmentation of upconversion nanoparticles-from hexagonal prisms to ID nanorods through“Medusa”-like structures

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nano Research 2021年第4期14卷 1141-1148页

作者： Laszlo Sajti Denis n.Karimov Vasilina V.Rocheva nataliya A.Arkharova Kirill V.Khaydukov Oleg I.Lebedev Alexey E.Voloshin Alla n.Generalova Boris n.Chichkov Evgeny V.Khaydukov AIT Austrian Institute of Technology GmbH Wiener Neustadt2700Austria Federal Scientific Research Centre“Crystallography and Photonics”Russian Academy of Sciences Moscow119333Russia Laboratoire CRISMAT UMR6508CNRS-ENSIACENUniversite CaenCaen14050France Shemyakin-Ovchinnikov Institute of Bioorganic Chemistry of the Russian Academy of Sciences Moscow 117997Russia Institutfiir Quantenoptik Leibniz Universitat HannoverHannover30167Germany Center of Biomedical Engineering Institute of Molecular Medicine Sechenov First Moscow State Medical UniversityMoscow119991Russia

One dimensional(1D)nanostructures attract considerable attention,enabling a broad application owing to their unique ***,the precise mechanism of 1D morphology attainment remains a matter of *** this study,ultrafast picosecond(ps)laser-induced treatment on upconversion nanoparticles(UCnPs)is offered as a tool for 1 D-nanostructures ***,reshaping through recrystallization process and bioadaptation of initially hydrophobic(β-na_(1.5)Y_(1.5_)F_(6):Yb^(3+),Tm^(3+)/β-na_(1.5)Y_(1.5_)F_(6))core/shell nanoparticles by means of one-step laser treatment in water are demonstrated.“True”1D nanostructures through"Medusa^-like structures can be obtained,maintaining anti-Stokes luminescence functionalities.A matter of the one-dimensional UCnPs based on direction of energy migration processes is *** proposed laser treatment approach is suitable for fast UCnP surface modification and nano-to-nano transformation,that open unique opportunities to expand UCnP applications in industry and biomedicine.

关键词： upconversion nanoparticles fluoride crystals upconversion nanorods one-dimensional(1D)structures laser-induced reshaping

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neonatal Exposure to the Dipeptidyl Peptidase-IV Inhibitors Diprotin A and Sitagliptin Induces Depression-Like Behavior, Anxiety, and Latent Aggression in Adolescent and Adult Rats

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Journal of Behavioral and Brain Science 2016年第4期6卷 167-183页

作者： nataliya A. Krupina nadezhda n. Khlebnikova Laboratory of the General Pathology of nervous System Federal State Budgetary Scientific Institution “Institute of General Pathology and Pathophysiology” Moscow Russia

Emotional and motivational disorders in adults are often considered to be the result of altered neurodevelopment. Clinical and experimental data provide evidence that serine protease dipeptidyl peptidase-IV (DPP-IV, EC 3.***.14.5) is involved in the pathophysiology of psycho-emotional disorders. Recently, we have shown that adolescent and adult rats exhibit an increase in anxiety and depression-related behaviors after neonatal administration of a synthetic non-competitive inhibitor of DPP-IV, methionyl-2(S)-cyano-pyrrolidine. In the present study, we tested the effects of two competitive, selective DPP-IV inhibitors, sitagliptin (4 mg/kg) and diprotin A (2 mg/kg), administered at postnatal days 5 - 18 on the emotional and motivational behavior of adolescent and adult rats. We observed increased anxiety in one-month-old diprotin A- or sitagliptin-treated rats in the elevated plus maze;diprotin A also enhanced the animals’ anxiety score using a ranked scale for evaluating anxiety and phobias. In the sucrose consumption and preference test, depressive-like behavior was pronounced in both the diprotin A- and sitagliptin-treated one-month-old animals, while only the diprotin A-treated rats exhibited a decrease in sucrose consumption at the age of 2 months. The diprotin A-treated rats also demonstrated behavioral despair and decreased activity in the forced swimming test within 1 - 3 months of age. Increased aggression was observed in 1 - 3-month-old diprotin A-treated rats and in two-month-old sitagliptin-treated rats. These findings support the hypothesis that DPP-IV is involved in the genesis of emotional and motivational disorders. Additionally, the results show that diprotin А impairs the adolescent and adult rats’ behavior more significantly than sitagliptin when the animals were treated with the DPP-IV inhibitors in the early postnatal period.

关键词： Dipeptidyl Peptidase IV Inhibitors Rat Depression Anxiety Aggression

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Global methylation status of sperm DnA in carriers of chromosome structural aberrations

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Asian Journal of Andrology 2017年第1期19卷 117-124页

作者： Marta Olszewska Miroslawa Z Barciszewska Monika Fraczek nataliya Huleyuk Vyacheslav B chernykh Danuta Zastavna Jan Barciszewski Maciej Kurpisz Department of Reproductive Biology and Stem Cells Institute of Human Genetics Polish Academy of Sciences Strzeszynska 32 60-479 Poznan Poland Department of RnA Biology Institute of Bioorganic Chemistry Polish Academy of Sciences Noskowskiego 12/14 61-704 Poznan Poland Institute of Hereditary Pathology Ukrainian Academy of Medical Sciences Lysenko Street 31a 79000 Lviv Ukraine Research Centre for Medical Genetics Russian Academy of Medical Sciences Moskvorechie Street 1115478 Moscow Russian Federation.

Male infertility might be clearly associated with aberrant DnA methylation patterns in human spermatozoa. An association between oxidative stress and the global methylation status of the sperm genome has also been suggested. The aim of the present study was to determine whether the global sperm DnA methylation status was affected in the spermatozoa of carriers of chromosome structural aberrations. The relationships between the 5-methylcytosine （msC） levels in spermatozoa and chromatin integrity status were evaluated. The study patients comprised male carriers of chromosome structural aberrations with reproductive failure （n = 24）, and the controls comprised normozoospermic sperm volunteers （n = 23）. The global msC level was measured using thin-layer chromatography （TLC） and immunofluorescence （IF） techniques. The sperm chromatin integrity was assessed using aniline blue （AB） staining and TUnEL assay. The mean msC levels were similar between the investigated chromosome structural aberrations carriers （P） and controls （K）. However, sperm chromatin integrity tests revealed significantly higher values in chromosomal rearrangement carriers than in controls （P 〈 0.05）. Although the potential relationship between sperm chromatin integrity status and sperm DnA fragmentation and the msC level juxtaposed in both analyzed groups （P vs K） was represented in a clearly opposite manner, the low chromatin integrity might be associated with the high hypomethylation status of the sperm DnA observed in carriers of chromosome structural aberrations.

关键词： 5-methylcytosine chromatin integrity chromosomal rearrangement chromosome translocation global DnA methylation male infertility

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Molecular cloning and characterization of a lipid transfer protein gene(PsLTP1) from Pinus sylvestris(L.)

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Journal of Forestry Research 2019年第3期30卷 1149-1158页

作者： nataliya Hrunyk Valentina Kovaleva Hryhoriy Krynytskyy Ivan Gout Francisco Amil-Ruiz Juan Munoz-Blanco Jose Luis Caballero Roman Gout Laboratory of Molecular-Genetic Markers in Woody Plants Ukrainian National Forestry UniversityGen. Chuprynka Str. 103Lviv 79057Ukraine Departamento de Bioquimica y Biologia Molecular Campus de Excelencia Internacional Agroalimentario ceiA3-Campus de RabanalesEdificio Severo Ochoa-C6Universidad de Cordoba14071 CordobaSpain Department of Structural and Molecular Biology University College LondonLondon WC1E 6BTUK

Plant nonspecific lipid transfer proteins (nsLTPs) are widely distributed through plant kingdom and are characterized by the presence of a central hydrophobic cavity, suitable for binding various hydrophobic molecules. Despite extensive research on nsLTP in different plant species, mostly angiosperm, and the great diversity of physiological processes in which they seem to be involved, their exact functions still remain unclear. Also, very limited experimental data are available on nsLTP in gymnosperm. In this study, we report for the first time on the molecular cloning of nsLTP, from Pinus sylvestris L.(PsLTP1, GenBank accession Jn980402.1) and the expression pattern of PsLTP1 during ontogenesis and in response to environmental stress conditions. Total RnA from roots of 7-day old pine seedlings was used to isolate the cDnA clone, corresponding to Scots pine lipid transfer protein. The open reading frame of PsLTP1 consists of 372 bp encoding a protein of 123 amino acids. Amino acid sequence alignment revealed that mature PsLTP1 shares high level of similarity with nsLTP from other conifers and with well-studied nsLTPs from angiosperms. The PsLTP1 contains a 27-amino-acid n-terminal signal sequence and presents all the features of a plant nsLTP. Amino acid comparison analysis and 3D structure prediction showed that PsLTP1 is a type 1 nsLTP. The results of the expression analysis of Scots pine PsLTP1 gene revealed that its transcripts accumulate in actively growing tissues. Furthermore, transcription of PsLTP1 was upregulated in response to cold and salt treatments, and downregulated during acidic, osmotic and water stresses.

关键词： Scots pine nonspecific lipid transfer protein (nsLTP) Molecular cloning Expression Abiotic stresses

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铈基模型催化剂的纳米结构:有序CeO_(2)(111)薄膜上的Pt-Co纳米颗粒

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Chinese Journal of Catalysis 2020年第6期41卷 985-997页

作者： Yaroslava Lykhach TomasSkala Armin neitzel nataliya Tsud Klara Beranova Kevin CPrince Vladimir Matolin Jorg Libuda 弗里德里希-亚历山大埃尔朗根-纽伦堡大学埃尔朗根催化资源中心界面研究与催化91058埃尔朗根德国查尔斯大学数学与物理学院表面与等离子体科学系 18000布拉格捷克共和国 Elettra-Sincrotrone Trieste SCpA StradaStatale 14km 163.534149巴索维扎-的里雅斯特意大利

制备并表征了原子分散的模型体系:氧化铈负载的Pt-Co核壳催化剂.采用超高真空物理气相沉积法制备了有序CeO2(111)膜上的Pt@Co和Co@Pt核壳纳米结构,并用同步辐射光电子能谱和共振光发射光谱对其进行了研究.在低Co覆盖率(0.5 ML)下Co在CeO... 详细信息

制备并表征了原子分散的模型体系:氧化铈负载的Pt-Co核壳催化剂.采用超高真空物理气相沉积法制备了有序CeO2(111)膜上的Pt@Co和Co@Pt核壳纳米结构,并用同步辐射光电子能谱和共振光发射光谱对其进行了研究.在低Co覆盖率(0.5 ML)下Co在CeO2(111)上沉积生成Co-CeO2(111)固溶体,然后在更高Co覆盖率下生长为金属Co纳米粒子.Pt@Co和Co@Pt两种模型结构在300-500 K温度范围内都能稳定地抗烧结.在500 K退火后, Pt@Co纳米结构含有接近纯的钴壳,而Co@Pt中的铂壳部分被金属钴覆盖.在550 K以上,在Pt@Co和Co@Pt纳米结构中近表面区域的重新排序中产生了次表层的Pt Co合金和富铂外壳.对于Co@Pt纳米粒子,近表面区域的化学有序性取决于沉积铂壳的初始厚度.无论初始铂壳的厚度如何,在有氧存在下对Co@Pt纳米结构进行退火,都会导致Pt-Co合金的分解以及Co的氧化.Co的逐步氧化与吸附质诱导的Co偏析共同导致在负载的Co@Pt纳米结构表面形成厚的Co O层.这一过程伴随着CeO2(111)薄膜的裂解,以及在550K以上氧气中退火后CeO2包裹氧化的Co@Pt纳米结构.很明显,于不同温度下在氧气和氢气的氧化-还原循环过程中,无论铂的初始厚度是多少,负载的Co@Pt纳米颗粒的结构和化学成分的变化主要是由氧化所致,而还原处理的影响则很小.

关键词：核壳纳米粒子模型催化剂 Pt-Co 氧化铈化学有序性同步辐射光电子能谱

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