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Enhanced photothermal dehydration of methanol over W_(18)O_(49)/Au/SAPO-34 catalysts with broadened light absorption

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Rare Metals 2024年第3期43卷 1139-1152页

作者： Ya-Qin Tang Meng-Xia yan chang-Qian Lu Shao-Yuan Li Kui-Xian wei tao Qu Wen-huiMa Yong-Nian Dai Kong-zhai Li Da-Jun Luo Xue-Liang Zhang Yi-Ke Liu Faculty of Metallurgical and Energy Engineering Kunming University of Science and TechnologyKunming650093China School of Materials and Energy Engineering Guizhou Institute of TechnologyGuiyang550003China

Methanol-to-olefins(MTO)process is one of the most critical pathways to produce low carbon ***,the reaction is driven by thermal catalysis,which inevitably needs to consume large amounts of fossil *** a new technique to substitute for the fuel burning is urgent for MTO process to improve the industry prospects and ***,we report a novel W_(18)O_(49)/Au/SAPO-34(W/Au/S),a multifunctional photothermal catalyst for the MTO reaction.A high methanol conversion was achieved under xenonum(Xe)lamp irradiation,yielding methyl ether(ME)and ethylene as the main *** optimized W/Au/S catalysts showed ethylene yield as high as 250μmol in 60 min,which was 2.5 times higher than that of Au/*** physiochemical characterization revealed that the SAPO-34 molecular sieves were surrounded by Au and W_(18)O_(49)nanoparticles,which exhibited a strong localized surface plasmon resonance excitation around 540 nm and light absorption beyond 500 *** multifunctional catalysts showed a strong photothermal effect,arising from the broadened light absorption of Au and W_(18)O_(49)nanoparticles,leading to a temperature as high as 250℃on the surface of the *** study showed that the superior ethylene selectivity of W/Au/S catalysts was attributed to the moderating acidic sites of W_(18)O_(49)for methanol dehydration to *** research may provide new insight for designing heterostructures to improve photo-to-chemical conversion performance and is expected to accelerate progress toward the excellent multifunctional photothermal catalysts with broad light absorption for methanol activation and C-C bond formation.

关键词： Methanol conversion Ethylene Photothermal catalysis W_(18)O_(49) BrΦnsted-acid

Differential expression profile of circular RNAs in mouse peritoneum with peritoneal fibrosis and the potential regulatory role of novel_circ_0007527

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Genes & Diseases 2024年第3期11卷 59-62页

作者： Yingfeng Shi yan Hu hui Chen Jinqing Li Min tao Xun Zhou Qin zhong Andong Qiu Shougang Zhuang Na Liu Department of Nephrology Shanghai East HospitalTongji University School of MedicineShanghai 200120China School of Life Science and Technology Advanced Institute of Translational MedicineTongji UniversityShanghai 200092China Department of Medicine Rhode Island Hospital and Alpert Medical SchoolBrown UniversityProvidenceRI 02912USA

CircRNAs,a novel type of endogenous non-coding RNAs(ncRNAs),are typically produced by back-splicing from exons of protein-coding genes,which are characterized by a covalently closed structure with neither 5'to 3'polarity nor a poly(A)tail.'On the one hand,circRNAs are involved in the regulation of a variety of important biological processes,such as apoptosis,proliferation,migration,and inflammatory responses.'On the other hand,the relationship between circRNAs and several fibrotic diseases has been reported.2 However.

关键词： endogenous peritoneal diseases

Searching for^(76)Ge neutrinoless double beta decay with the CDEX-1B experiment

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Chinese Physics C 2024年第10期48卷 11-22页

作者： Bing-tao Zhang Jun-Zheng Wang Li-tao yang Qian Yue Ke-Jun Kang Yuan-Jing Li Hai-Peng An C.Greeshma Jian-Ping chang Yun-Huan Chen Jian-Ping Cheng Wen-Han Dai Zhi Deng chang-hao Fang Xin-Ping Geng hui Gong Qiu-Ju Guo Xu-Yuan Guo Li he Sheng-Ming he Jin-wei Hu Han-Xiong Huang Tu-Chen Huang Hai-tao Jia Xi Jiang S.Karmakar hao-Bin Li Jian-Min Li Jin Li Qian-Yun Li Ren-Ming-Jie Li Xue-Qian Li Yu-Lan Li Yi-Fan Liang Bin Liao Fong-Kay Lin Shin-Ted Lin Jia-Xuan Liu Shu-Kui Liu yan-Dong Liu Yu Liu Yuan-Yuan Liu zhong-Zhi Liu hao Ma Yu-cai Mao Qi-Yuan Nie Jin-Hua Ning hui Pan Ning-Chun Qi Jie Ren Xi-Chao Ruan Ze She Manoj Kumar Singh Tian-Xi Sun chang-Jian Tang wei-You Tang yang Tian Guang-Fu Wang Li Wang Qing Wang Yu-Feng Wang Yun-Xiang Wang henry-Tsz-King Wong Shi-Yong Wu Yu-Cheng Wu hao-yang Xing Rui Xu Yin Xu tao Xue Yu-Lu yan Nan Yi Chun-Xu Yu Hai-Jun Yu Jian-Feng Yue Ming Zeng Zhi Zeng Feng-Shou Zhang Lei Zhang Zhen-Hua Zhang Zhen-Yu Zhang Kang-Kang Zhao Ming-Gang Zhao Ji-Fang Zhou Zu-Ying Zhou Jing-Jun Zhou Key Laboratory of Particle and Radiation Imaging(Ministry of Education)and Department of Engineering Physics Tsinghua UniversityBeijing 100084 Department of Physics Tsinghua UniversityBeijing 100084 Institute of Physics Academia SinicaTaipei 11529 NUCTECH Company Beijing 100084 YaLong River Hydropower Development Company Chengdu 610051 College of Nuclear Science and Technology Beijing Normal UniversityBeijing 100875 College of Physics Sichuan UniversityChengdu 610065 School of Physics Peking UniversityBeijing 100871 Department of Nuclear Physics China Institute of Atomic EnergyBeijing 102413 Sino-French Institute of Nuclear and Technology Sun Yat-sen UniversityZhuhai 519082 School of Physics Nankai UniversityTianjin 300071 Department of Physics Banaras Hindu UniversityVaranasi 221005 Department of Physics Beijing Normal UniversityBeijing 100875

We operated a p-type point contact high purity germanium(PPCGe)detector(CDEX-1B,1.008 kg)in the China Jinping Underground Laboratory(CJPL)for 500.3 days to search for neutrinoless double beta(0νββ)decay of^(76)Ge.A total of 504.3 kg⋅day effective exposure data was *** anti-coincidence and the multi/single-site event(MSE/SSE)discrimination methods were used to suppress the background in the energy region of interest(ROI,1989–2089 keV for this work)with a factor of 23.A background level of 0.33 counts/(keV⋅kg⋅yr)was *** lower limit on the half life of^(76)Ge 0νββdecay was constrained as T_(1/2)^(0ν)>1.0×10^(23)yr(90%C.L.),corresponding to the upper limits on the effective Majorana neutrino mass:<3.2–7.5 eV.

关键词： neutrinoless double beta decay CDEX point-contact germanium detector ^(76)Ge

Incidence and warning signs for complications of human brucellosis: a multi-center observational study from China

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Infectious Diseases of Poverty 2024年第1期13卷 53-62页

作者： Qing-Nan Shi hui-Jie Qin Qiao-Shan Lu hu Li zhong-Fa tao Meng-Guang Fan Mu-heta Aishan Zeng-Qiang Kou Qiu-Lan Chen Wen-Wu Yin yan-Ping Zhang National Key Laboratory of Intelligent Tracking and Forecasting for Infectious Diseases Chinese Center for Disease Control and PreventionChangbai RoadChangping DistrictBejing 102206China School of Public health Guangxi Medical UniversityNanningChina Nanning Center for Disease Control and Prevention NanningChina Guizhou Center for Disease Control and Prevention GuiyangChina Inner Mongolia Center for Disease Control and Prevention HohhotChina Xinjiang Uighur Autonomous Region Center for Disease Control and Prevention UrumqiChina Shandong Center for Disease Control and Prevention JinanChina

Background Brucellosis is a severe zoonotic disease that is often overlooked, particularly in impoverished countries. Timely identification of focal complications in brucellosis is crucial for improving treatment outcomes. However, there is currently a lack of established indicators or biomarkers for diagnosing these complications. Therefore, this study aimed to investigate potential warning signs of focal complications in human brucellosis, with the goal of providing practical parameters for clinicians to aid in the diagnosis and management of *** A multi-center cross-sectional study was conducted in China from December 2019 to August 2021. The study aimed to investigate the clinical characteristics and complications of patients with brucellosis using a questionnaire survey and medical record system. The presence of warning signs for complications was assessed using univariate and multivariate logistic regression models. Receiver operating characteristic (ROC) curves and the area under the curve (AUC) were used for variable screening and model *** A total of 880 participants diagnosed with human brucellosis were enrolled. The median age of the patients was 50 years [interquartile range (IQR): 41.5-58.0], and 54.8% had complications. The most common organ system affected by complications was the osteoarticular system (43.1%), with peripheral arthritis (30.0%), spondylitis (16.6%), paravertebral abscess (5.0%), and sacroiliitis (2.7%) being the most prevalent. Complications in other organ systems included the genitourinary system (4.7%), respiratory system (4.7%), and hematologic system (4.6%). Several factors were found to be associated with focal brucellosis. These factors included a long delay in diagnosis [odds ratio (OR) = 3.963, 95% confidence interval(CI): 1.906-8.238 for > 90 days], the presence of underlying disease (OR = 1.675, 95%CI: 1.176-2.384), arthralgia (OR = 3.197, 95%CI: 1.986-5.148), eye bulging pain (OR = 3.482, 95%CI:

关键词： Brucellosis Complications Clinical spectrum Warning signs

Efficient hydrolysis of hemicellulose to furfural by novel superacid SO_4H-functionalized ionic liquids

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Green Energy & Environment 2019年第1期4卷 49-55页

作者： wei hui yan Zhou yan Dong Zhi-Jun Cao Fei-Qiang he Min-zhong cai Duan-Jian tao College of Chemistry and Chemical Engineering Institute of Advanced Materials Jiangxi Normal University

Novel superacid SO_4H-functionalized ionic liquids(SFILs) were designed and prepared in this work. The catalytic activities of SFILs were evaluated in xylan hydrolysis and xylose dehydration to produce furfural. Combined with the results of acid strength of SFILs characterized by solid-state ^(31)P MAS NMR, it was found that the catalytic performance of SFILs was positively correlated to their acid strength. The superacid SFIL [Ch-SO_4H][CF_3SO_3] displayed the best catalytic performance with more than 80% yield of furfural, and it was also obviously superior to usual SO_3H-functionalized acidic ILs, mineral liquid acids, and acidic resin Amberlyst-15 catalysts in catalytic activity under optimized conditions. In addition, the superacid SFIL [Ch-SO_4H][CF_3SO_3] could be easily separated from reaction system and reused at least five times without obvious decrease.

关键词： Superacid Ionic liquids hemicellulose Hydrolysis Furfural

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考虑水盐运移的分散性盐渍土冻融破坏机制

长安大学学报（自然科学版） 2024年第2期44卷 1-11页

作者：孔元元梁晨涛王智慧谢柏涵成忠焱长安大学公路学院陕西西安710064

为探究冻融循环过程中土体冻-盐胀破坏机理,结合冻结温度试验和扫描电子显微镜进行研究,分析了不同循环次数、不同盐的种类和不同含水率条件下的冻融循环对土体结构和性质的影响,得到了不同循环次数下的冻结温度变化曲线和不同含水率条... 详细信息

为探究冻融循环过程中土体冻-盐胀破坏机理,结合冻结温度试验和扫描电子显微镜进行研究,分析了不同循环次数、不同盐的种类和不同含水率条件下的冻融循环对土体结构和性质的影响,得到了不同循环次数下的冻结温度变化曲线和不同含水率条件下冻土的SEM电镜扫描图片,并基于经典传热理论和水盐运移方程,建立数值模型,再现了冻融过程中的水盐运移过程,在此基础上结合试验对水盐运移过程中土体的破坏机制进行分析研究。研究结果表明:由于研究区土体的分散性,其冻结过程只存在恒定阶段和递降阶段,且随着冻融循环次数的增大,土体的冻结温度会先升高然后在某一温度保持稳定,这与冻融循环过程中土体粒度大小和颗粒排布的方式改变相关,内部的微裂隙逐渐贯通;土体在冻融循环过程所发生的水盐迁移是土体强度和结构发生变化的重要原因,且随着冻融循环过程的进行,土中的水盐成分会在温度梯度和溶质梯度的影响下产生迁移和积累;相较于碳酸氢钠,硫酸钠在冻融过程中对于土体结构的改变更为显著,具体表现在冻结过程中硫酸钠结晶析出体积变为原来的3.18倍,导致冻融循环后土体膨胀。本研究有助于揭示季节性冻土区含盐冻土工程的冻融破坏机制。

关键词：道路工程水盐运移数值模拟盐渍土冻融循环

松辽盆地西缘构造带构造格架、演化及油气资源潜力

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地质通报 2024年第7期43卷 1073-1089页

作者：汪岩钱程钟辉李成立秦涛杨晓平赵维俊中国地质调查局沈阳地质调查中心辽宁沈阳110034 东北地质科技创新中心辽宁沈阳110034 中国地质调查局军民融合地质调查中心四川成都610036

松辽盆地西缘构造带是研究松辽盆地形成演化的关键地带,但目前关于该构造带的构造格架、活动历史、控盆特征等仍不清晰,构造带深部物质架构及中—新生代构造演化的精细厘定为解决这一科学问题提供了新的证据。松辽盆地西缘地区布格重力... 详细信息

松辽盆地西缘构造带是研究松辽盆地形成演化的关键地带,但目前关于该构造带的构造格架、活动历史、控盆特征等仍不清晰,构造带深部物质架构及中—新生代构造演化的精细厘定为解决这一科学问题提供了新的证据。松辽盆地西缘地区布格重力异常与综合地球物理剖面特征指示,松辽盆地西缘构造带为区域上带状展布的超壳深大构造带。通过对综合构造变形带的产状、性质、运动学等资料分析,提出松辽盆地西缘构造带东西分带、倾向相背的“两带八字形”构造格架。依据构造带发育的基底背景、构造样式、地球物理特征等差异,建立了南北分段的“四段式”展布构架。在此基础上,结合区域构造演化、变形带构造解析与40Ar/39Ar构造年代学等资料,恢复了晚三叠世、中晚侏罗世、早白垩世中期、晚白垩世中期、古新世—渐新世和新近纪—更新世6期中—新生代构造活动年代格架。结合构造带的控盆作用指出,外盆带控制的中侏罗世和早白垩世中期沉积盆地是油气资源勘查的重要选区,为中国东北地区新层系油气资源勘查提供了新依据。

关键词：松辽盆地构造格架年代格架控盆作用油气资源潜力油气勘查工程

Longitudinal surface cracks of thin slabs

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International Journal of Minerals,Metallurgy and Materials 2010年第2期17卷 159-166页

作者： yan-hui Sun You-jin Ni Hai-tao Wang zhong-bo Xu Kai-ke cai School of Metallurgical and Ecological Engineering University of Science and Technology Beijing Beijing 100083 China

Based on the production practice of medium carbon thin slabs in the CSP plant,the reasons and influencing factors for the formation of longitudinal cracks were investigated,and some industrial measures were taken to eliminate the *** results show that the efficient solutions to reduce longitudinal cracks are improving the performance of the mold powder,stabilizing the mold heat flux,and maintaining a proper taper of the mold during *** pouring temperature and secondary cooling also play important roles in preventing longitudinal surface cracks.

关键词： CSP thin slab medium carbon steel surface cracks

Numerical simulation of low-Reynolds number flows past two tandem cylinders of different diameters

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Water Science and Engineering 2013年第4期6卷 433-445页

作者： Yong-tao WANG zhong-min yan hui-min WANG College of Environmental Science and Engineering Suzhou University of Science and Technology College of Water Conservancy and Hydropower Engineering Hohai University College of Environment Hohai University

The flow past two tandem circular cylinders of different diameters was simulated using the finite volume method. The diameter of the downstream main cylinder （D） was kept constant, and the diameter of the upstream control cylinder （d） varied from 0.1D to D. The studied Reynolds numbers based on the diameter of the downstream main cylinder were 100 and 150. The gap between the control cylinder and the main cylinder （G） ranged from 0.1D to 4D. It is concluded that the gap-to-diameter ratio （G/D） and the diameter ratio between the two cylinders （d/D） have important effects on the drag and lift coefficients, pressure distributions around the cylinders, vortex shedding frequencies from the two cylinders, and flow characteristics.

关键词： two tandem cylinders vortex shedding drag force lift force numerical simulation