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Photocatalytic activity of porous TiO_2 films prepared by anodic oxidation

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Rare Metals 2007年第2期26卷 136-141页

作者： WANG Wei tao Jie WANG tao WANG ling College of Material Science ＆ Technology Nanjing University of Aeronautics and Astronautics Nanjing 210016 China

Anatase titanium dioxide is an active photocatalyst, however, it is difficult to be immobilized on the substrate. The crystalline TiO2 porous film was prepared directly on the surface of pure titanium by anodic oxidation. The film was then used for photocatalysis via the methyl orange degradation method. The effects of anodization voltage, pH value, TiO2 film area and degradation time on the photocatalyst were investigated respectively by UV-visible spectrum. It was indicated that the TiO2 film prepared by anodic oxidation at 140 V had the best photocatalysis capability and the degradation of methyl orange was accelerated with acid addition.

关键词： titanium porous films anodic oxidation photocatalysis methyl orange

Experimental study of wind loads on gable roofs of low-rise buildings with overhangs

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Frontiers of Structural and Civil Engineering 2018年第3期12卷 300-317页

作者： Peng HUANG ling tao Ming GU Yong QUAN i University Shanghai 200092China

Gable roofs with overhangs （eaves） are the common constructions of low-rise buildings on the southeastern coast of China, and they were vulnerable to typhoons from experience. The wind pressure distributions on gable roofs of low-rise buildings are investigated by a series of wind tunnel tests which consist of 99 test cases with various roof pitches, height-depth ratios and width-depth ratios. The block pressure coefficients and worst negative （block） pressure coefficients on different roof regions of low-rise buildings are proposed for the main structure and building envelope, respectively. The effects of roof pitch, height-depth ratio, and width-depth ratio on the pressure coefficients of each region are analyzed in detail. In addition, the pressure coefficients on the roofs for the main structure and building envelope are fitted according to roof pitch, height-depth ratio and width-depth ratio of the low-rise building. Meanwhile, the rationality of the fitting formulas is verified by comparing the fitting results with the codes of different countries. Lastly, the block pressure coefficients and worst negative pressure coefficients are recommended to guide the design of low-rise buildings in typhoon area and act as references for the future＇s modification of wind load codes.

关键词： low-rise building gable roof wind loads wind tunnel test block pressure coefficient load code

In situ construction of Cu(Ⅰ)-Cu(Ⅱ) pairs for efficient electrocatalytic nitrate reduction reaction to ammonia

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Journal of Energy Chemistry 2025年第1期 106-113页

作者： Muyun Zheng Yuchi Wan Leping Yang Shen Ao Wangyang Fu Zhengjun Zhang Zheng-Hong Huang tao ling Feiyu Kang Ruitao Lv State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua University Institute of New Energy Materials and Engineering School of Materials Science and Engineering Fuzhou University Key Laboratory of Advanced Materials (MOE) School of Materials Science and Engineering Tsinghua University Key Laboratory for Advanced Ceramics and Machining Technology of Ministry of Education Tianjin Key Laboratory of Composite and Functional Materials School of Materials Science and Engineering Tianjin University

Electrocatalytic nitrate reduction reaction （NO3-RR） to ammonia under ambient conditions is expected to be a green process for ammonia synthesis and alleviate water pollution *** report a CuO nanoparticles incorporated on nitrogen-doped porous carbon （CuO@NC） catalyst for *** of Cu（Ⅱ） is reduced to Cu（Ⅰ） during the NO3-RR process to construct Cu（Ⅰ）-Cu（Ⅱ） pairs,confirmed by in situ X-ray photoelectron spectroscopy （XPS） and Raman *** functional theory （DFT） calculations indicated that the formation of Cu（Ⅰ） could provide a reaction path with smaller energy barrier for NO3-RR,while Cu（Ⅱ） effectively suppressed the competition of hydrogen evolution reaction （HER）.As a result,CuO@NC catalyst achieved a Faradaic efficiency of 84.2% at -0.49 V versus reversible hydrogen electrode （RHE）,and a NH3yield rate of 17.2 mg *** -0.79 V ***,higher than the HaberBosch process (<3.4 g h-1g-1cat.).This work may open a new avenue for effective NO3-RR by modulating oxidation states.

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Desulfurization Characteristics of CaO-SiO_2-BaO-CaF_2-Al_2O_3-MgO Refining Slag

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Journal of Iron and Steel Research International 2005年第5期12卷 1-2,20页

作者： GAO Yan-hong BIAN ling-tao Chongqing University of Science and Technology Chongqing 400005 China lingyuan Iron and Steel Group Co Lingyuan 122504 China

The desulfurization characteristics of CaO-SiO2-BaO-CaF2-Al2O3-MgO refining slag were studied in laboratory with the methodology of orthogonal design. The influence of basicity, Al2O3, MgO, BaO and CaF2 contents in sl... 详细信息

关键词： refining slag desulfurization orthogonal design

Evaluating the Stability of Active Manganese Sites During Electrochemical Reactions by Cyclic Voltammetry

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Transactions of Tianjin University 2022年第3期28卷 193-198页

作者： Ziang Ma Jisi Li tao ling Key Laboratory for Advanced Ceramics and Machining Technology of Ministry of Education TianjinChina Key Laboratory of Composite and Functional Materials School of Materials Science and EngineeringTianjin UniversityTianjin 300072China

Manganese oxides are a promising class of electrocatalysts for renewable energy devices,such as fuel ***(Ⅲ) ions with e_(g) electron filling of-1 are the active sites for manganese-based ***,Mn(Ⅲ) sites may be disproportionated during electrochemical reactions,thus reducing the number of Mn(Ⅲ) active sites and decreasing the catalytic activity of manganese *** this work,we developed a facile cyclic voltammetry method to monitor the evolution of Mn(Ⅲ) sites on a series of manganese oxides under "working" *** proposed a descriptor S_(Mn(Ⅲ)) to describe the stability of Mn(Ⅲ).Our simulated and experimental results show that the higher is S_(Mn(Ⅲ)),the higher the active Mn(Ⅲ)density,and the higher the electrocatalytic activity of the manganese oxide electrocatalyst.

关键词： Manganese oxides Mn(III)sites Cyclic voltammetry

Nonsmooth dynamic analysis of rigid-flexible interaction collision

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Applied Mathematics and Mechanics(English Edition) 2022年第11期43卷 1731-1746页

作者： ling tao Zhongpan LI Yan LI Huijian CHEN Zhiqiang FENG School of Mechanics and Aerospace Engineering Southwest Jiaotong UniversityChengdu 610031China Laboratoire de Mécanique et d'Energétique d'Evry Univ-Evry Université Paris-SaclayEvry 91020France

This paper aims to explore the deformation of the collided bodies in multibody systems and to effectively simulate the motion path of colliding ***,we describe the geometrically nonlinear problems of materials by the total Lagrangian ***,a first-order integration scheme is used to solve the dynamics *** algorithm combining the bi-potential method with the node-to-point contact identification is proposed to solve the interface problems of rigid-flexible interaction *** observe the collision process more intuitively,the internal software FER/VIEW is introduced to visualize the *** accuracy is proved by comparing the proposed method with the analytical solution or another numerical ***,the proposed method has more numerical robustness,such as occupying less computer storage,saving the computational cost,and broadening the application range of the bi-potential method.

关键词： collision bi-potential method node-to-point rigid-flexible FER/VIEW

Editable semiconductor photo-electrodes for sustainable ammonia synthesis

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Nano Research 2024年第4期17卷 3107-3112页

作者： Ning Lan Kun Du Erling Zhao Wei Zhao tao ling Key Laboratory for Advanced Ceramics and Machining Technology of Ministry of Education Institute of New-EnergySchool of Materials Science and EngineeringTianjin UniversityTianjin 300072China School of Materials Science and Engineering Tianjin Chengjian UniversityTianjin 300384China

Powered by an inexhaustible supply of solar energy,photoelectrochemical(PEC)nitrogen reduction reaction(NRR)provides an ideal solution for the synthesis of green ammonia(NH_(3)).Although great efforts have been made in the past decades,there are still significant challenges in increasing the NH_(3) yields of the PEC-NRR *** addition to the issues of low activity and selectivity similar to electrochemical NRR,the progress of PEC-NRR is also impeded by the limited increase in NH_(3) yields as the electrode is ***,we propose an editable electrode design strategy that parallels unit photo-electrodes to achieve a linear increase in NH_(3) yields with electrode active *** demonstrate that the editable electrode design strategy minimizes the electrode charge transfer resistance,allowing more photo-generated carriers to reach the electrode surface and promote the catalytic *** believe that this editable electrode design strategy provides an avenue to achieve sustainable PEC NH_(3) production.

关键词： editable electrode photoelectrochemical nitrogen reduction reaction parallel electrode ZnSe

Thermodynamic analysis and simulation for gas baffle entrance collimator of EAST-NBI system based on thermo-fluid coupled method

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Nuclear Science and Techniques 2018年第1期29卷 90-95页

作者： ling tao Chun-Dong Hu Yuan-Lai Xie Institute of Plasma Physics Chinese Academy of Sciences

The world's first full Experimental Advanced Superconducting Tokamak(EAST) is designed with the auxiliary heating method of neutral beam injection(NBI)system. Beam collimators are arranged on both sides of the beam channel for absorbing the divergence beam during the beam transmission process in the EAST-NBI *** gas baffle entrance collimator(GBEC) is a typical high-heat-flux component located at the entrance of gas baffle. An efficient and accurate analysis of its thermodynamic performance is of great significance to explore the working limit and to ensure safe operation of the system under a high-parameter steady-state condition. Based on the thermo-fluid coupled method, thermodynamic analysis and simulation of GBEC is performed to get the working states and corresponding operating limits at different beam extraction conditions. This study provides a theoretical guidance for the next step to achieve long pulse with highpower experimental operation and has an important reference to ensure the safe operation of the system.

关键词： Neutral beam injection High-heat-flux component Beam collimator Thermo-fluid coupled method Thermodynamic analysis

Numerical simulation of fluid flow and alloy melting in RH process for electrical steels

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Journal of Iron and Steel Research International 2022年第9期29卷 1423-1433页

作者： Haijun Wang Rui Xu Hai-tao ling Wei Zhong Li-zhong Chang Sheng-tao Qiu Anhui Province Key Laboratory of Metallurgical Engineering and Resources Reeyeling Anhui University of TechnologyMa'anshan 243002AnhuiChina School of Metalurgical Engineering Anhui University of Technology.Ma'anshan 243002AnhuiChina State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Xinyu Iron and Steel Co. Ltd.Xinyu 338001JiangxiChina National Engineering and Research Centerfor Continuous Casting Technology Central Iron and Steel Research InstituteBeijing 100081China

Based on the Eulerian-Lagrangian approach,a mathematical model was established to describe the gas-liquid flow behavior in the Ruhrstahl-Heraeus(RH)*** momentum source and the turbulent kinetic energy source due to the motion of gas bubbles were considered for the liquid *** effect of the expansion of gas bubbles on the liquid velocity,recirculation rate,and mixing time was quantitatively *** the fluid flow reached the steady state,the melting and mixing processes of aluminum alloys in the RH degasser were also *** results indicate that the expansion of gas bubbles has a significant infuence on the recirculation rate and the mixing time in the RH *** the superheat of liquid steel and decreasing the initial diameter of alloy particles are beneficial to promote the melting and mixing of alloy *** to the existence of solidified steel shells,the maximum diameter of the alloy particle is about 1.5 times its initial diameter.

关键词： Discrete particle model Multiphase flow Gas expansion-Mixing time Alloy melting Numerical simulation