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Facile synthesis of intra-nanogap enhanced Raman tags with different shapes

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Nano Research 2024年第9期17卷 8415-8423页

作者： Sanjun Fan Brian t.Scarpitti Zhewen Luo Abigail E.Smith Jian Ye Zachary D.Schultz Department of Chemistry and Biochemistry The Ohio State UniversityColumbusOhio 43210USA School of Biomedical Engineering Shanghai Jiao Tong UniversityShanghai 200030China

Hot spot engineering in plasmonic nanostructures plays a significant role in surface-enhanced Raman scattering(SERS)for bioanalysis and cell ***,creating stable,reproducible,and strong SERS signals remains challenging due to the potential interference from surrounding chemicals and locating SERS-active analytes into hot-spot ***,we developed a straightforward approach to synthesize intra-gap nanoparticles encapsulating 4-nitrobenzenethiol(4-NBt)as a reporter molecule within these gaps to avoid outside *** made three kinds of intra-gap nanoparticles using nanorods,bipyramids,and nanospheres as cores,in which the nanorods based intra-gap nanoparticles exhibit the highest SERS *** advantage of our method is the ease of preparation of high-yield and stable intra-gap nanoparticles characterized by a short incubation time(10 min)with 4-NBt and quick synthesis without requiring an additional step to centrifuge for the purification of core *** intense localized field in the synthesized hot spots of these plasmonic gap nanostructures holds great promise as a SERS substrate for a broad range of quantitative optical applications.

关键词： hot spot engineering surface enhanced Raman scattering intra-gap nanoparticles 4-nitrobenzenethiol

Spatiotemporal mapping of(ultra‐)mafic magmatic mine areas:Implications of economic and political realities in China

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Deep Underground Science and Engineering 2024年第1期3卷 91-102页

作者： Heling Li Liang tang tim t.Werner Zhengmeng Hou Fan Meng Jingjing Li College of Earth Sciences Chengdu University of TechnologyChengduChina Institute of Subsurface Energy Systems Clausthal University of TechnologyClausthal ZellerfeldGermany School of Geography Earth and Atmospheric SciencesFaculty of ScienceThe University of MelbourneMelbourneVictoriaAustralia

the spatiotemporal extension/expansion of mine areas is affected by multiple *** far,very little has been done to examine the interaction between mine areas and political or economic ***(ultra‐)mafic magmatic mines in China played a specific role in supporting national development and providing an ideal research subject for monitoring their *** this study,remote sensing and mining‐related GIS data were used to identify and analyze 1233(ultra‐)mafic magmatic mine area polygons in China,which covered approximately 322.96 km2 of land and included a V–ti–Fe mine,a copper–nickel mine,a chromite mine,an asbestos mine,and a diamond *** was found that(1)the areal expansion of mines is significantly related to the mine types,perimeter,topography,and population density.(2)the mine area variation also reflects market and policy *** temporal expansion of the mine area from 2010 to 2020 followed an S‐shaped pattern(with the turning point occurring in 2014),closely related to iron overcapacity and tightened mining policies.(3)the complexity(D)of the mine area may reflect mine design and excavation *** be specific,lower D indicates early‐stage or artisanal/small‐scale mining,whereas higher D represents large‐scale *** study demonstrates that the detailed mapping of mine land can serve as an indicator to implement miningrelated market and policy ***(ultra‐)mafic mines area data set can be accessed at https://***/record/7636616#.Y-p0uXaZOa0.

关键词： complexity mine area mining and socioeconomic interaction spatiotemporal distribution (ultra‐)mafic magmatic mine

Hydrothermal treatment of pearl millet grains:Effects on nutritional composition,antinutrients and flour properties

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Grain & Oil Science and technology 2024年第2期7卷 87-95页

作者： P.Prashanth t.Jayasree Joshi Shagolshem Mukta Singh P.Srinivasa Rao Agricultural and Food Engineering Department Indian Institute of Technology KharagpurKharagpurWest Bengal 721302India

Pearl millet(Pennisetum glaucum)is one of the major millets with high nutritional *** crop exhibits exceptional resilience to drought and high ***,the processing of pearl millet poses a significant challenge due to its high lipid content,enzyme activity,and presence of ***,it becomes imperative to enhance the quality and prolong the shelf life of pearl millet flour by employing suitable *** treatment in the food industry has long been seen as promising due to its potential to reduce microbial load,inactivate enzymes,and improve nutrient *** study aims to investigate the effects of hydrothermal treatment on the quality characteristics of pearl *** independent variables of the study were soaking temperature(35,45,55℃),soaking time(2,3,4 h),and steaming time(5,10,15 min).treatment conditions had a statistically significant effect on nutrient *** antinutrients like tannins and phytates were reduced by 0.99% to 5.94% and 0.36% to 6.00%,respectively,after the *** activity decreased significantly up to 10% with the treatment *** findings of this study could potentially encourage the use of pearl millet flour in the production of various food items and promote the application of hydrothermal treatment in the field of food processing.

关键词： Pearl millet Hydrothermal treatment Nutritional properties Antinutrients

Life under tension: the relevance of force on biological polymers

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Biophysics Reports 2024年第1期10卷 48-56页

作者： Matthew t.J.Halma Longfu Xu Department of Physics and Astronomy and Laser Lab Vrije Universiteit Amsterdam LUMICKS B.V.

Optical tweezers have elucidated numerous biological processes, particularly by enabling the precise manipulation and measurement of tension. One question concerns the biological relevance of these experiments and the generalizability of these experiments to wider biological systems. Here, we categorize the applicability of the information garnered from optical tweezers in two distinct categories: the direct relevance of tension in biological systems, and what experiments under tension can tell us about biological systems, while these systems do not reach the same tension as the experiment, still, these artificial experimental systems reveal insights into the operations of biological machines and life processes.

关键词： tension Optical tweezers Molecular force

Instance Segmentation of Characters Recognized in Palmyrene Aramaic Inscriptions

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Computer Modeling in Engineering & Sciences 2024年第9期140卷 2869-2889页

作者： Adéla Hamplová Alexey Lyavdansky tomášNovák Ondrej Svojše David Franc Arnošt Veselý Czech University of Life Sciences in Prague(CULS) Faculty of Economics and ManagementDepartment of Information EngineeringPrague16500Czech Republic National Research University Higher School of Economics(HSE) Faculty of HumanitiesInstitute for Oriental and Classical StudiesMoscow101000The Russian Federation

this study presents a single-class and multi-class instance segmentation approach applied to ancient Palmyrene inscriptions,employing two state-of-the-art deep learning algorithms,namely YOLOv8 and Roboflow *** goal is to contribute to the preservation and understanding of historical texts,showcasing the potential of modern deep learning methods in archaeological *** research culminates in several key findings and scientific *** comprehensively compare the performance of YOLOv8 and Roboflow 3.0 in the context of Palmyrene character segmentation—this comparative analysis mainly focuses on the strengths and weaknesses of each algorithm in this *** also created and annotated an extensive dataset of Palmyrene inscriptions,a crucial resource for further research in the *** dataset serves for training and evaluating the segmentation *** employ comparative evaluation metrics to quantitatively assess the segmentation results,ensuring the reliability and reproducibility of our findings and we present custom visualization tools for predicted segmentation *** study advances the state of the art in semi-automatic reading of Palmyrene inscriptions and establishes a benchmark for future *** availability of the Palmyrene dataset and the insights into algorithm performance contribute to the broader understanding of historical text analysis.

关键词： Optical character recognition instance segmentation Palmyrene ancient languages computer vision

Radiative decays D*(s)→ D(s)γ in covariant confined quark model

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Chinese Physics C 2024年第2期48卷 45-56页

作者： C.t.tran M.A.Ivanov P.Santorelli Q.C.Vo Department of Physics HCMC University of Technology and EducationVo Van Ngan 1700000 Ho Chi Minh CityVietnam Bogoliubov Laboratory of theoretical Physics Joint Institute for Nuclear Research141980 DubnaRussia Dipartimento di Fisica"E.Pancini" Universitàdi Napoli Federico ⅡComplesso Universitario di Monte S.AngeloVia CintiaEdificio 680126 NapoliItaly Istituto Nazionale di Fisica Nucleare Sezione di Napoli80126 NapoliItaly University of Science 700000 Ho Chi Minh CityVietnam

Radiative decays D((s))*→D((s))γare revisited in light of new experimental data from the BaBar and BESⅢ*** radiative couplings gD*Dγencoding nonperturbative QCD effects are calculated in the framework of the covariant confined quark model developed by *** compare our results with other theoretical studies and experimental *** couplings(in GeV-1)|g(D*+D+γ)|=0.45(9)and|g(D*0D0γ)|=1.72(34)calculated in our model agree with the corresponding experimental data|g(D*+D+γ)|=0.47(7)and|g(D*0D0γ)|=1.77(16).the most interesting case is the decay Ds*→Dsγ,for which a recent prediction based on light-cone sum rules at next-to-leading order|gDs*Dsγ|=0.60(19)deviates from the first(and only to date)lattice QCD result|gDs*Dsγ|=0.11(2)at nearly3σ.Our calculation yields|gDs*Dsγ|=0.29(6),which falls somehow between the two mentioned results,although it is larger than those predicted in other studies using quark models or QCD sum rules.

关键词： covariant quark model radiative decay charmed meson

theoretical and experimental investigations on an X-shaped vibration isolator with active controlled variable stiffness

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Applied Mathematics and Mechanics(English Edition) 2024年第8期45卷 1371-1386页

作者： Zeyu CHAI J.t.HAN Xuyuan SONG Jian ZANG Yewei ZHANG Zhen ZHANG College of Aerospace Engineering Shenyang Aerospace University Jacobs School of Engineering University of California San Diego Key Laboratory of Vibration and Control of Aero-Propulsion System Ministry of EducationNortheastern University

A novel X-shaped variable stiffness vibration isolator(X-VSVI) is *** Runge-Kutta method, harmonic balance method, and wavelet transform spectra are introduced to evaluate the performance of the X-VSVI under various excitations. the layer number, the installation angle of the X-shaped structure, the stiffness, and the active control parameters are systematically analyzed. In addition, a prototype of the X-VSVI is manufactured, and vibration tests are carried out. the results show that the proposed X-VSVI has a superior adaptability to that of a traditional X-shaped mechanism, and shows excellent vibration isolation performance in response to different amplitudes and forms of excitations. Moreover, the vibration isolation efficiency of the device can be improved by appropriate adjustment of parameters.

关键词： 70J35 70K30 70K50 bionic vibration isolation nonlinear dynamics O322 prototype experiment variable stiffness structure X-shaped structure

Protein ubiquitination in plant peroxisomes

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Journal of Integrative Plant Biology 2023年第2期65卷 371-380页

作者： Delara akhter Yuchan Zhang Jianping Hu Ronghui Pan State Key Laboratory of Rice Biology Zhejiang Provincial Key Laboratory of Crop Genetic ResourcesCollege of Agriculture and Biotechnology&ZJU-Hangzhou Global Scientific and Technological Innovation CenterZhejiang UniversityHangzhou 310058/311200China Zhejiang Laboratory Hangzhou 311121China Department of Genetics and Plant Breeding Sylhet Agricultural UniversitySylhet 3100Bangladesh Department of Energy Plant Research Laboratory and Plant Biology Department Michigan State UniversityEast LansingMichiganUSA Department of Plant Biology Michigan State UniversityEast LansingMichiganUSA

Protein ubiquitination regulates diverse cellular processes in eukaryotic organisms,from growth and development to stress *** subjected to ubiquitination can be found in virtually all subcellular locations and organelles,including peroxisomes,singlemembrane and highly dynamic organelles ubiquitous in *** contain metabolic functions essential to plants and animals such as lipid catabolism,detoxification of reactive oxygen species(ROS),biosynthesis of vital hormones and cofactors,and *** peroxisomes possess a complex proteome with functions varying among different tissue types and developmental stages,and during plant response to distinct environmental ***,how these diverse functions are regulated at the post-translational level is poorly understood,especially in *** this review,we summarized current knowledge of the involvement of protein ubiquitination in peroxisome protein import,remodeling,pexophagy,and metabolism,focusing on plants,and referencing discoveries from other eukaryotic systems when *** on previous ubiquitinomics studies,we compiled a list of 56 ubiquitinated Arabidopsis peroxisomal proteins whose functions are associated with all the major plant peroxisomal metabolic *** discovery suggests a broad impact of protein ubiquitination on plant peroxisome functions,therefore substantiating the need to investigate this significant regulatory mechanism in peroxisomes at more depths.

关键词： peroxins peroxisome peroxisome biogenesis peroxisome metabolism pexophagy ubiquitination

Al-Ca-Cu三元合金体系中与铝平衡的金属间化合物

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transactions of Nonferrous Metals Society of China 2024年第5期34卷 1380-1392页

作者： t.K.AKOPYAN t.A.SVIRIDOVA N.A.BELOV N.V.LEtYAGIN A.V.KOROtItSKIY National University of Science and technology MISiS 4 Leninsky pr.Moscow 119049Russia

对三元Al-Ca-Cu合金体系中与铝固溶体平衡的(Al,Cu)_(4)Ca、Al_(27)Ca_(3)Cu_(7)和Al_(8)CaCu_(4)金属间化合物的结构和性能进行全面分析。基于Al4Ca相中部分Al原子被Cu取代,将(Al,Cu)_(4)Ca金属间化合物视为线性化合物。化合物中铜的... 详细信息

对三元Al-Ca-Cu合金体系中与铝固溶体平衡的(Al,Cu)_(4)Ca、Al_(27)Ca_(3)Cu_(7)和Al_(8)CaCu_(4)金属间化合物的结构和性能进行全面分析。基于Al4Ca相中部分Al原子被Cu取代,将(Al,Cu)_(4)Ca金属间化合物视为线性化合物。化合物中铜的溶解度达到10 at.%(19 wt.%),导致化合物的晶格结构、物理和力学性能发生显著变化。例如,化合物的密度从2.22 g/cm^(3)增加到2.79 g/cm^(3),显微硬度从HV 180增加到HV 250。将Al_(27)Ca_(3)Cu_(7)相视为具有严格化学计量比和BaHg11型初始晶体结构的三元化合物,其空间群为Pm3m,晶格参数为8.514Å,密度为3.45 g/cm^(3)。Al_(8)CaCu_(4)相也是严格化学计量比的三元化合物,具有Mn_(12)th型晶格结构,最高的显微硬度(HV 505)和密度(4.57 g/cm^(3))。属于二元(Al)+(Al,Cu)_(4)Ca相场和准二元(Al)+Al_(27)Ca_(3)Cu_(7)截面的合金,有前景作为新型天然铝基复合材料的基材。

关键词：金属间化合物 Al-Ca合金显微组织晶体结构物理性能力学性能