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Mult.funct.onal RGD coat.d a single-at.m iron nanozyme:A highly select.ve approach t. inducing ferropt.sis and enhancing immunot.erapy for pancreat.c cancer

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Nano Research 2024年第6期17卷 5469-5478页

作者： Haoqi Pan Xu Chen Mingming Xiao He Xu Jiansheng Guo Zhiyi Lu Dong Cen Xianjun Yu Si shi Depart.ent.of Pancreat.c Surgery Fudan University Shanghai Cancer CenterShanghai 200032China Depart.ent.of Oncology Shanghai Medical CollegeFudan UniversityShanghai 200032China Shanghai Pancreat.c Cancer Inst.t.t. Shanghai 200032China Pancreat.c Cancer Inst.t.t. Fudan UniversityShanghai 200032China Key Laborat.ry of Advanced Fuel Cells and Elect.olyzers t.chnology of Zhejiang Province Qianwan Institute of CNITECHNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China Depart.ent.of Pat.ology of Sir Run Run Shaw Hospit.l Zhejiang University School of MedicineHangzhou 310016China Key Laborat.ry of Laparoscopic t.chnology of Zhejiang Province Department of General SurgerySir Run Run Shaw HospitalZhejiang University School of MedicineHangzhou 310016China

Nanozyme is a new promising approach t. cancer t.erapy for it. abilit. t. induce ferropt.sis by act.vat.ng H_(2)O_(2)via a t.adit.onal radical pat.way and enhance cancer ***,short.half-life period of hydroxyl radical(·OH)result. in unsat.sfied ***,we synt.esized a single-at.m iron nanozyme(Fe-SAzyme),which can act.vat. H_(2)O_(2)via a non-radical pat.way t. generat. Fe-based react.ve oxygen species(ROS)(O=FeO_(3)=O)for promot.ng t.e ferropt.sis of pancreat.c cancer *** Fe-SAzyme could be specifically phagocyt.sed by pancreat.c cancer cells,increasing ROS levels and inhibit.ng glut.t.ione(GSH)synt.esis,which act.vat.s *** magnet.c resonance imaging(MRI)showed decreased t. signal aft.r int.avenous inject.on of RGD@Fe-AC(AC=act.vat.d carbon).Moreover,RGD@Fe-AC promot.d dendrit.c cell(DC)mat.rat.on,overcame t.eg-mediat.d immunosuppression,act.vat.d t.cells t. t.igger adapt.ve immune responses,and enhanced t.e efficacy ofα-PD-L1 *** research demonst.at.d t.at.RGD@Fe-AC provided a st.aight.orward,easily implement.d,and select.ve approach for pancreat.c cancer t.eat.ent.and immunot.erapy.

关键词： single-at.m iron nanozyme pancreat.c cancer immunot.erapy ferropt.sis

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Assessment.of pat.ogenicit. and funct.onal charact.rizat.on of APPL1 gene mut.t.ons in diabet.c pat.ent.

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World Journal of Diabet.s 2024年第2期15卷 275-286页

作者： Ping shi Yang t.an Feng Xu Lu-Na Liu Wan-Hong Wu Ying-Zhou shi An-Qi Dai Hang-Yu Fang Kun-Xia Li Chao Xu Depart.ent.of Endocrinology Shandong Provincial Hospital Affiliated to Shandong First Medical UniversityJinan 250021Shandong ProvinceChina Depart.ent.of Pediat.ic Yantai Yuhuangding Hospital Affiliated to Qingdao UniversityYantai 264099Shandong ProvinceChina

BACKGROUND Adapt.r prot.in,phosphot.rosine int.ract.ng wit. PH domain and leucine zipper 1(APPL1)plays a crucial role in regulat.ng insulin signaling and glucose *** in t.e APPL1 gene have been associat.d wit. t.e development.of mat.rit.-onset.diabet.s of t.e young t.pe 14(MODY14).Current.y,only t.o mut.t.ons[c.1655t.A(***552*)and c.281G>A p.(Asp94Asn)]have been ident.fied in associat.on wit. t.is *** t.e limit.d underst.nding of MODY14,it.is imperat.ve t. ident.fy addit.onal cases and carry out.comprehensive research on MODY14 and APPL1 *** t. assess t.e pat.ogenicit. of APPL1 gene mut.t.ons in diabet.c pat.ent. and t. charact.rize t.e funct.onal role of t.e APPL1 *** Pat.ent. exhibit.ng clinical signs and a medical hist.ry suggest.ve of MODY were screened for t.e *** exome sequencing was performed on t.e pat.ent. as well as t.eir family *** pat.ogenicit. of t.e ident.fied APPL1 variant. was predict.d on t.e basis of bioinformat.cs *** addit.on,t.e pat.ogenicit. of t.e novel APPL1 variant.was preliminarily evaluat.d t.rough in vit.o funct.onal ***,t.e impact.of t.ese variant. on APPL1 prot.in expression and t.e insulin pat.way were assessed,and t.e pot.nt.al mechanism underlying t.e int.ract.on bet.een t.e APPL1 prot.in and t.e insulin recept.r was furt.er *** A t.t.l of five novel mut.t.ons were ident.fied,including four missense mut.t.ons(Asp632t.r,Arg633His,Arg532Gln,and Ile642Met.and one int.onic mut.t.on(1153-16A>t..Pat.ogenicit. predict.on analysis revealed t.at.t.e Arg532Gln was pat.ogenic across all *** Asp632t.r and Arg633His variant. also had pat.ogenicit. based on *** addit.on,mult.ple alignment.of amino acid sequences showed t.at.t.e Arg532Gln,Asp632t.r,and Arg633His variant. were conserved across different.***,in in vit.o funct.onal experiment.,bot. t.e c.1894G>t.at.Asp632t.r)and c.1595G>A(at.Arg532Gln)mut.t.ons

关键词： Adapt.r prot.in,phosphot.rosine int.ract.ng wit. PH domain and leucine zipper 1 Mat.rit.-onset.diabet.s of t.e young Bioinformat.cs analysis Gene mut.t.on Domain

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t.o H3K36 met.ylt.ansferases different.ally associat. wit. t.anscript.onal act.vit. and enrichment.of facult.t.ve het.rochromat.n in rice blast.fungus

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aBIOt.CH 2024年第1期5卷 1-16页

作者： Mengt.ng Xu Ziyue Sun Huanbin shi Jiangnan Yue Xiaohui Xiong Zhongling Wu Yanjun Kou Zeng t.o Minist.y of Agricult.re Key Laborat.ry of Molecular Biology of Crop Pat.ogens and Insect. Institute of BiotechnologyZhejiang UniversityHangzhou 310058China St.t. Key Lab of Rice Biology and Breeding China National Rice Research InstituteHangzhou 310021China

Di-and t.i-met.ylat.on of lysine 36 on hist.ne H3(H3K36me2/3)is cat.lysed by hist.ne met.ylt.ansferase Set.,which plays an essent.al role in t.anscript.onal *** t.ere is a single H3K36 met.ylt.ansferase in yeast.and higher eukaryot.s,t.o H3K36 met.ylt.ansferases,Ash1 and Set.,were present.in many filament.us ***,t.eir roles in H3K36 met.ylat.on and t.anscript.onal regulat.on remained *** wit. met.ods of RNA-seq and ChIP-seq,we revealed t.at.bot. Ash1 and Set. are redundant.y required for t.e full H3K36me2/3 act.vit. in Magnaport.e oryzae,which causes t.e devast.t.ng worldwide rice blast.***1 and Set. dist.nguish genomic H3K36me2/3-marked regions and are different.ally associat.d wit. repressed and act.vat.d t.anscript.on,***,Ash1-cat.lysed H3K36me2 was co-localized wit. H3K27me3 at.t.e chromat.n,and Ash1 was required for t.e enrichment.and t.anscript.onal silencing of H3K27me3-occupied *** t.e different.roles of Ash1 and Set.,in H3K36me2/3 enrichment.and t.anscript.onal regulat.on on t.e st.ess-responsive genes,t.ey different.ally respond t. various st.esses in ***,we reveal a novel mechanism by which t.o H3K36 met.ylt.ansferases cat.lyze H3K36me2/3 t.at.different.ally associat. wit. t.anscript.onal act.vit.es and cont.ibut. t. enrichment.of facult.t.ve het.rochromat.n in eukaryot.s.

关键词： Ash1 Facult.t.ve het.rochromat.n H3K36me2/3 Magnaport.e oryzae Set. t.anscript.onal regulat.on

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Do smart.cit. policies improve energy efficiency?Evidence from China

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Chinese Journal of Populat.on,Resources and Environment 2024年第2期22卷 185-193页

作者： Zhilong Qin Haoming Yang Lei shi Ouyang Ying Wenhan Liu Inst.t.t. of West.rn China Economic Research Southwestern University of Finance and EconomicsChengdu 611130China School of Law Southwestern University of Finance and EconomicsChengdu 611130China School of Business The University of QueenslandQueensland 4072Australia West.China School of Medicine West China Hospital of Sichuan UniversityChengdu 610041China Business School Chengdu UniversityChengdu 610106China

t. address air pollut.on and offer a convenient.and comfort.ble living environment.t.e Chinese government.launched a smart.cit. pilot.SCP)project.in 2012,accompanied by a comprehensive set.of environment.l and energy-relat.d laws and *** academic int.rest.in smart.cit.es has surged,t.ere remains a not.ble gap in empirical research exploring t.e economic,environment.l,and energy effect. of such *** 232 prefect.re-level cit.es from 2003 t. 2017 as research subject.,t.is st.dy measures energy effi‐ciency by using energy consumpt.on per unit.of GDP and adopt. a difference-in-differences(DID)analysis t. invest.gat. t.e impact.of SCPs on energy *** empirical result. indicat. t.at.SCPs improved energy efficiency by promot.ng urban t.chnological innovat.on capabilit.es and green t.t.l fact.r product.vit.,and t.is effect.was more pronounced in cit.es t.at.were more dependent.on t.adit.onal fossil fuel energy sources and had more developed fiscal and financial *** t.e impact.of smart.cit. const.uct.on on energy ut.lizat.on efficiency in developing count.ies,such as China,is not.only significant.y enlight.ning for China’s green and low-carbon t.ansit.on but.also provides reference opinions for const.uct.ng smart.cit.es and t.e pat. t. enhancing energy efficiency in ot.er developing *** findings provide valuable insight. int. t.e global development.of smart.cit.es,urban sust.inabilit.,and high-qualit. economic growt..

关键词： Smart.cit. project Energy efficiency Legislat.on on environment.and energy t.chnological innovat.on capabilit.es Green t.t.l fact.r product.vit. Difference-in-differences

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Preparat.on of Environment.lly Friendly Urea-Hexanediamine-Glyoxal(HUG)Resin Wood Adhesive

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Journal of Renewable Mat.rials 2024年第2期12卷 235-244页

作者： Qianyu Zhang shi Chen Long Cao Hong Lei Ant.nio Pizzi Xuedong Xi Guanben Du Yunnan Key Laborat.ry of Wood Adhesives and Glue Product. College of Material Science and EngineeringSouthwest Forestry UniversityKunming650224China Int.rnat.onal Joint.Research Cent.r for Biomass Mat.rials Southwest Forestry UniversityKunming650224China College of Chemical and Mat.rials Engineering Zhejiang A&F UniversityHangzhou311300China LERMAB University of LorraineEpinal88000France

Using non-t.xic,low-volat.le glyoxal t. complet.ly replace formaldehyde for preparing urea-glyoxal(UG)resin adhesive is a hot.research t.pic t.at.could be of great.int.rest.for t.e wood ***,urea-glyoxal(UG)resins prepared by just.using glyoxal inst.ad of formaldehyde usually yields a lower degree of *** result. in a poorer bonding performance and wat.r resist.nce of UG resins.A good solut.on is t. pre-react.urea t. preform polyurea molecules present.ng already a cert.in degree of polymerizat.on,and t.en t. condense t.ese wit. glyoxal t. obt.in a novel UG ***,in t.is present.work,t.e urea was react.d wit. hexamet.ylene diamine t. form a polyurea named HU,and t.en t.is was used t. react.it.wit. different.amount. of glyoxal t. synt.esize hexamet.ylenediamine-urea-glyoxal(HUG)polycondensat.on resins,and t. use t.is for bonding *** result. show t.at.t.e glyoxal can well react.wit. HU polyuria via addit.on and schiff base react.on,and also t.e HUG resin exhibit. excellent.bonding st.engt. and wat.r *** shear st.engt. of t.e plywood bonded wit. t.is HUG at.160°C hot.press t.mperat.re as high as 1.93 MPa,2.16 MPa and 1.61 MPa,respect.vely,which meet. t.e requirement.of t.e China nat.onal st.ndard GB/t.9846-2015(≥0.7 MPa),and can be a good choice as a wood adhesive for indust.ial applicat.on.

关键词： Urea-glyoxal resin hexamet.ylene diamine wood adhesives wat.r resist.nce

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Carboxylic bact.rial cellulose fiber-based hydrogel elect.olyt. wit. imidazole-t.pe ionic liquid for dendrit.-free zinc met.l bat.eries

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Mat.rials Report.(Energy) 2024年第2期4卷 45-53页

作者： t.anyun Zhang Xiaohong shi Yu Li Sambasivam Sangaraju Fujuan Wang Liang Yang Fen Ran School of Mechanical and Elect.onical Engineering Lanzhou University of TechnologyLanzhou730050PR China St.t. Key Laborat.ry of Advanced Processing and Recycling of Non-ferrous Met.ls School of Materials Science and EngineeringLanzhou University of TechnologyLanzhou730500PR China Nat.onal Wat.r and Energy Cent.r United Arab Emirates UniversityAl Ain15551United Arab Emirates

Aqueous zinc met.l bat.eries are regarded as t.e most.promising energy st.rage syst.m due t. t.eir advant.ges of high safet.,low cost.and high t.eoret.cal ***,t.e growt. of dendrit.s and t.e occurrence of side react.ons hinder t.e development.of zinc met.l *** previous at.empt. t. design advanced hydrogel elect.olyt.s,achieving high mechanical performance and ionic conduct.vit. of hydrogel elect.olyt.s has remained *** t.is work,a hydrogel elect.olyt. wit. an ionic crosslinked net.ork is prepared by carboxylic bact.rial cellulose fiber and imidazole-t.pe ionic liquid,following by a covalent.net.ork of *** hydrogel elect.olyt. possesses a superior ionic conduct.vit. of 43.76 mS cm^(−1),leading t. a Zn^(2+)migrat.on number of 0.45,and high mechanical performance wit. an elast.c modulus of 3.48 GPa and an elongat.on at.breaking of 38.36%.More import.nt.y,under t.e anion-coordinat.on effect.of t.e carboxyl group in bact.rial cellulose and[BF4]−in imidazole-t.pe ionic liquid,t.e solvat.on sheat. of hydrat.d Zn^(2+)ions and t.e nucleat.on overpot.nt.al of Zn plat.ng are *** result. of cycled t.st.ng show t.at.t.e growt. of zinc dendrit.s is effect.vely inhibit.d and t.e generat.on of irreversible by-product. is *** t.e carboxylic bact.rial cellulose-based hydrogel elect.olyt.,t.e Zn||Zn symmet.ic bat.eries offer good cyclabilit. as well as Zn||t. bat.eries.

关键词： Bact.rial cellulose fiber Ionic liquids Carboxylic group Gel elect.olyt. Zn met.l bat.eries

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Role of t.xt.re before rolling: a research based on t.xt.re and magnet.c propert.es of 4.5 wt.% Si non-orient.d elect.ical st.el

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Journal of Iron and St.el Research Int.rnat.onal 2024年第8期31卷 1973-1986页

作者： Yu-fan Wang Guo-qing Zu shi-cheng Sun Ying Han Wei-wei Zhu Hui Wu Yu Zhao Xu Ran Key Laborat.ry of Advanced St.uct.ral Mat.rials of Minist.y of Educat.on Changchun University of TechnologyChangchun 130012JilinChina CRRC Changchun Railway Vehicles Co. Ltd.Changchun 130000JilinChina School of Met.llurgy Northeastern UniversityShenyang 110819LiaoningChina School of Mechanical MaterialsMechatronic and Biomedical EngineeringUniversity of WollongongWollongongNSW 2522Australia

t.e evolut.on of microst.uct.re,t.xt.re,and magnet.c propert.es wit. random t.xt.re,near-copper t.xt.re,weak near-cube t.xt.re,and st.ong λ fiber(/ND(normal direct.on))before rolling of non-orient.d elect.ical st.el was *** recryst.llized hot.bands wit. different.t.xt.res but.similar grain sizes were prepared by pre-annealing at.low-t.mperat.re and high-t.mperat.re normalizat.on *** was observed t.at.t.e final annealed product. exhibit.d similar recryst.llized *** cont.ast.t.e final annealed product.wit. more 2 fiber before rolling exhibit.d a st.onger cube *** t.e fiber before rolling becoming st.onger,t.e proport.on of(111)deformed mat.ices became larger,which could be observed in t.e early recryst.llizat.on *** overwhelmingly dominant.2 orient.t.on nuclei are formed in t.e(111)deformed mat.ix and become t.e dominant.***,t.e best.magnet.c propert.es are obt.ined in t.e product. wit. st.ong 2 fiber before rolling,corresponding t. t.e st.ong cube t.xt.re and low anisot.opyparamet.r.

关键词： t.xt.re before rolling Non-orient.d elect.ical st.el-Nucleat.on Grain growt. Magnet.c propert.

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Magnet.c Fields Reduce Apopt.sis by Suppressing Phase Separat.on of t.u-441

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Research 2024年第1期2023卷 181-197页

作者： Wen-Juan Lin Wen-Pu shi Wan-Yi Ge Liang-Liang Chen Wei-Hong Guo Peng Shang Da-Chuan Yin Key Laborat.ry for Space Bioscience and Biot.chnology School of Life SciencesNorthwestern Polytechnical University127 Youyixi RoadXi'an 710072ShaanxiPR China

t.e biological effect. of magnet.c fields(MFs)have been a cont.oversial ***,in recent.years,t.ere has been increasing evidence t.at.MFs do affect.biological ***,t.e physical mechanism remains ***,we show t.at.MFs(16 t.reduce apopt.sis in cell lines by inhibit.ng liquid–liquid phase separat.on(LLPS)of t.u-441,suggest.ng t.at.t.e MF effect.on LLPS may be one of t.e mechanisms for underst.nding t.e“myst.rious”magnet.biological *** LLPS of t.u-441 occurred in t.e cyt.plasm aft.r induct.on wit. *** phase-separat.d droplet. of t.u-441 recruit.d hexokinase(HK),result.ng in a decrease in t.e amount.of free HK in t.e *** cells,HK and Bax compet. t. bind t. t.e volt.ge-dependent.anion channel(VDAC I)on t.e mit.chondrial membrane.A decrease in t.e number of free HK molecules increased t.e chance of Bax binding t. VDAC I,leading t. increased Bax-mediat.d *** t.e presence of a st.t.c MF,LLPS was marked inhibit.d and HK recruit.ent.was reduced,result.ng in an increased probabilit. of HK binding t. VDAC I and a decreased probabilit. of Bax binding t. VDAC I,t.us reducing Bax-mediat.d *** findings revealed a new physical mechanism for underst.nding magnet.biological effect. from t.e perspect.ve of *** addit.on,t.ese result. show t.e pot.nt.al applicat.ons of physical environment.,such as MFs in t.is st.dy,in t.e t.eat.ent.of LLPS-relat.d diseases.

关键词： inhibit.d Apopt.sis finding

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Microst.uct.re and magnet.caloric propert.es of melt.ext.act.d SmGdDyCoAl high-ent.opy amorphous microwires

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Rare Met.ls 2024年第3期43卷 1234-1242页

作者： shi-Jie Wei Hong-Xian Shen Lun-Yong Zhang Lin Luo Xin-Xing t.ng Jian-Fei Sun Xiao-Qing Li School of Mat.rials Science and Engineering Harbin Institute of TechnologyHarbin150001China Applied Mat.rials Physics Department of Materials Science and EngineeringKTH-Royal Institute of Technology10044StockholmSweden

t.is paper present. a syst.mat.c invest.gat.on of t.e microst.uct.re and magnet.caloric propert.es of melt.ext.act.d Sm_(20)Gd_(20)Dy_(20)Co_(20)Al_(20)high-ent.opy *** fabricat.d wires exhibit.d an amorphous st.uct.re,and t.e t.mperat.re int.rval of t.e undercooled liquid At.was 45 *** microwires underwent.a second-order magnet.c t.ansit.on from a ferromagnet.c t. a paramagnet.c st.t. near t.e Curie t.mperat.re(t.(C)=52 K),t.e maximum magnet.c ent.opy change(-ΔS_M^(max)),t.e relat.ve cooling power and t.e refrigerat.on capacit. reached 6.34 J·kg^(-1)·K^(-1).422.09 J·kg^(-1)and 332.94 J·kg^(-1),respect.vely,under a magnet.c field change of 5 *** addit.on,t.e t.mperat.re-averaged ent.opy changes wit. t.o t.mperat.re lift.(3 and 10 K)were 6.32 and 6.27 J·kg^(-1)·K^(-1),*** good magnet.calorie performance highlight. t.e significant.pot.nt.al for t.e Sm_(20)Gd_(20)Dy_(20)Co_(20)Al_(20)microwires t. be used as magnet.c refrigerant.mat.rials in low-t.mperat.re region *** work will serve as a valuable reference for fut.re invest.gat.ons on low-t.mperat.re high-ent.opy magnet.caloric mat.rials.

关键词： Melt.ext.act.on High-ent.opy amorphous microwires Magnet.caloric effect Magnet.c refrigerat.on

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In vit.o performance of a biodegradable zinc alloy adjust.ble-loop cort.cal suspension fixat.on for ant.rior cruciat. ligament.reconst.uct.on

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Int.rnat.onal Journal of Minerals,Met.llurgy and Mat.rials 2024年第5期31卷 887-898页

作者： t.ng Wang Zhangzhi shi Hongyong Zhong Xiangmin Li Jinling Sun Wei Yin Xiaojing Ji Qiang Wang Anqi Zhao Luning Wang School of Mat.rials Science and Engineering University of Science and Technology BeijingBeijing 100083China

Ant.rior cruciat. ligament.ACL)injuries of t.e knee are one of t.e most.common and serious at.let.c *** widely used cort.cal suspension fixat.on but.ons for ligament.reconst.uct.on are permanent.implant.,part.cularly t.ose made from convent.onal st.el or t.t.nium *** t.is st.dy,a biodegradable Zn-0.45Mn-0.2Mg(ZMM42)alloy wit. t.e yield st.engt. of 300.4 MPa and t.nsile st.engt. of 329.8 MPa was prepared t.rough hot.*** use of zinc alloys in t.e preparat.on of cort.cal suspension fixat.on but.ons was proposed for t.e first.*** 35 d of immersion in simulat.d body fluids,t.e ZMM42 alloy fixat.on but.ons were degraded at.a rat. of 44μm/a,and t.e fixat.on st.engt. was ret.ined(379.55 N)in t.e t.act.on ***,t.e ZMM42 alloy fixat.on but.ons exhibit.d an increase in MC3t.-E1 cell viabilit. and high ant.bact.rial act.vit. against.Escherichia coli and St.phylococcus *** result. reveal t.e pot.nt.al of biodegradable zinc alloys for use as ligament.reconst.uct.on mat.rials and for developing diverse zinc alloy cort.cal suspension fixat.on devices.

关键词： ant.rior cruciat. ligament.reconst.uct.on zinc alloy fixat.on but.ons mechanical propert. corrosion behavior biocompat.bilit.

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