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Super-elastic and mechanically durable MXene-based nanocomposite aerogels enabled by interfacial engineering with dual crosslinking strategy

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Nano Research 2023年第5期16卷 8025-8035页

作者： Yan Sun Xin Yang Ruonan Ding sung yong hong Jinwoo Lee Zongfu An Mei Wang Yifei Ma Jae-Do Nam Jonghwan Suhr China Copper Institute of Engineering and Technology Chinalco Research Institute of Science and Technology Co.Ltd.Beijing 102200China Center for Composite Materials and Concurrent Design Sungkyunkwan UniversitySuwon 16419Republic of Korea Key Laboratory for Light-weight Materials Nanjing Tech UniversityNanjing 210009China Department of Energy Science Sungkyunkwan UniversitySuwon 16419Republic of Korea MPP PJT.PO R&D Center Polyolefin Business Petrochemicals DivisionLG ChemDaejeon 34122Republic of Korea Department of Polymer Science and Engineering Sungkyunkwan UniversitySuwon 16419Republic of Korea School of Chemical Engineering Sungkyunkwan UniversitySuwon 16419Republic of Korea State Key Laboratory of Quantum Optics and Quantum Optics Devices Institute of Laser SpectroscopyCollaborative Innovation Center of Extreme OpticsShanxi UniversityTaiyuan 030006China School of Mechanical Engineering Sungkyunkwan UniversitySuwon 16419Republic of Korea

Recently,MXenes have attracted considerable attention owing to their unique physical and chemical *** of MXenes to three-dimensional(3D)porous aerogel structures can play a critical role in realizing the profound implications of MXenes,especially for environmental ***,developing mechanically robust MXene-based aerogels with reversible compressibility under harsh conditions,such as liquid environments,remains challenging due to the insufficient interfacial strength between MXene ***,3D porous MXene-based nanocomposite aerogels are developed by dual physical and chemical crosslinking strategy with poly(vinyl alcohol)and formaldehyde in this *** developed MXenebased nanocomposite aerogels with designed interfacial engineering exhibit outstanding structural stability and extremely high reversible compressibility up to 98%strain as well as unprecedented mechanical durability(2000 cycles at 50%strain)in water ***,the aerogels show adaptable compressibility when exposed to different solvents,which is explained with the Hansen solubility *** to their high compressibility in water,the robust MXene-based aerogels exhibit excellent methylene blue adsorption performance(adsorption capacity of 117.87 mg·g^(−1))and superior recycling efficiency(89.48%at the 3rd cycle).The porous MXene-based nanocomposite aerogels are also demonstrated with outstanding thermal insulation ***,by synergistically taking their porous structure and super elasticity in liquid environment,the MXene-based aerogels show great promise in diverse applications including adsorption and separation,wastewater purification desalination,and thermal management.

关键词： MXenes-based nanocomposite aerogels dual crosslinking strategy reversible compressibility methylene blue adsorption thermal insulation

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High-damping and conducting epoxy nanocomposite using both zinc oxide particles and carbon nanofibers

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Journal of Materiomics 2018年第3期4卷 187-193页

作者： Jae-Soon Jang Gyo Woo Lee Hyung-ick Kim sung yong hong Lijie Ci Jae-Do Nam Jonghwan Suhr Simulation Group Battery R&D CenterSAMSUNG SDI CO.LTDSamsung-RoYeongtong-GuSuwon-SiGyeonggi-DoSouth Korea Division of Mechanical Design Engineering Chonbuk National UniversityJeonju561-756South Korea Dongnam Regional Division Korea Institute of Industrial TechnologyJinju 52845South Korea Department of Polymer Science and Engineering Sungkyunkwan University2066SeoburoJangan-guGyeonggi-doSouth Korea School of Materials Science&Engineering Shandong UniversityChina School of Mechanical Engineering Sungkyunkwan University2066SeoburoJangan-guGyeonggi-doSouth Korea Department of Energy Science Sungkyunkwan University2066SeoburoJangan-guGyeonggi-doSouth Korea

In this study,high-damping and conducting epoxy nanocomposites were developed with carbon nanofibers as conducting materials,and zinc oxide particles as piezoelectric *** mechanical and electrical properties,electrical impedance,and loss factors were investigated by uniaxial tensile tests,voltage measurement,impedance measurement,and 3-point bending *** percolation thresholds were found:the percolation threshold of resistivity due to the carbon nanofibers forming conductive networks in the matrix;and the impedance threshold due to the zinc oxide particles acting like electric barriers.A poling treatment of the high-damping and conducting epoxy nanocomposite was considered,and we found that poling treatment helped to make the networks more conductive and to generate voltage from ZnO particles.A high-damping and conducting epoxy nanocomposite with 3 wt%CNF and 10 wt%ZnO exhibited higher loss factor than those of others tested.

关键词： Damping Piezoelectric materials Impedance Poling treatment Loss factor

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Comprehensive molecular characterization to predict immunotherapy response in advanced biliary tract cancer:a phase II trial of pembrolizumab

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Oncology Research 2025年第1期33卷 57-65页

作者： RYUL KIM JOO KYUNG PARK MINSUK KWON MINAE AN JUNG yong hong JOON OH PARK sung HEE LIM SEUNG TAE KIM Division of Hematology-Oncology Department of MedicineSamsung Medical CenterSungkyunkwan University School of MedicineSeoulKorea Division of Gastroenterology Department of MedicineSamsung Medical CenterSungkyunkwan University School of MedicineSeoulKorea Department of Hematology-Oncology Ajou University School of MedicineSuwon-siGyeonggi-doKorea Samsung Advanced Institute of Health Science and Technology Sungkyunkwan University School of MedicineSeoulKorea

Background:Immune checkpoint inhibitors(ICIs)are effective in a subset of patients with metastatic solid ***,the patients who would benefit most from ICIs in biliary tract cancer(BTC)are still *** and methods:We molecularly characterized tissues and blood from 32 patients with metastatic BTC treated with the ICI pembrolizumab as second-line ***:All patients had microsatellite stable(MSS)type *** of the 32 patients achieved partial response(PR),with an objective response rate(ORR)of 9.4%(95%confidence interval[CI],2.0–25.2)and nine showed stable disease(SD),exhibiting a disease control rate(DCR)of 37.5%(95%CI,21.1–56.3).For the 31 patients who had access to PD-1 ligand 1(PD-L1)combined positive score(CPS)testing(cut-off value≥1%),the ORR was not different between those who had PD-L1-positive(PD-L1+;1/11,9.1%)and PDL1-(2/20,10.0%)tumors(p=1.000).The tumor mutational burden(TMB)of PD-L1+BTC was comparable to that of PD-L1-BTC(p=0.630).TMB and any exonic somatic mutations were also not predictive of pembrolizumab *** analysis of blood and tumor samples demonstrated a relatively high natural killer(NK)cell proportion in the peripheral blood before pembrolizumab treatment in patients who achieved tumor ***,the tumors of these patients presented high enrichment scores for NK cells,antitumor cytokines,and Th1 signatures,and a low enrichment score for cancer-associated ***:This study shows the molecular characteristics associated with the efficacy of pembrolizumab in BTC of the MSS type.

关键词： Pembrolizumab Whole-exome sequencing Whole-transcriptome sequencing Biliary tract cancer

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Atomic-scale insights into microscopic mechanisms of grain boundary segregation in Al−Cu alloys

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Transactions of Nonferrous Metals Society of China 2025年第1期35卷 1-12页

作者： Xiong SHUAI hong MAO Sai TANG Yi KONG yong DU State Key Laboratory of Powder Metallurgy Central South UniversityChangsha 410083China College of Mechanical Engineering Hunan Institute of Science and TechnologyYueyang 414006China National Key Laboratory of Science and Technology on High-strength Structural Materials Central South UniversityChangsha 410083China

This study aims to clarify the mechanisms for the grain boundary(GB)segregation through investigating the absorption of excess solute atoms at GBs in Al−Cu alloys by using the hybrid molecular dynamics/Monte Carlo *** segregation mechanisms,substitutional and interstitial mechanisms,are *** intergranular defects,including dislocations,steps and vacancies,and the intervals in structural units are conductive to the prevalence of interstitial *** substitutional mechanism is favored by the highly ordered twin ***,the two mechanisms affect the GB structure *** is quantified that interstitial mechanism is less destructive to GB structure than substitutional one,and often leads to a segregation level being up to about 6 times higher than the *** findings contribute to atomic scale insights into the microscopic mechanisms about how solute atoms are absorbed by GB structures,and clarify the correlation among intergranular structures,segregation mechanisms and kinetics.

关键词： grain boundaries segregation Al−Cu alloy intergranular structure molecular dynamics simulation Monte Carlo simulation

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Regulation of sleep by astrocytes in the hypothalamic ventrolateral preoptic nucleus

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Neural Regeneration Research 2025年第4期20卷 1098-1100页

作者： Jae-hong Kim Ruqayya Afridi Il-sung Jang Maan Gee Lee Kyoungho Suk Brain Korea 21 four KNU Convergence Educational Program of Biomedical Sciences for Creative Future Talents School of MedicineKyungpook National UniversityDaeguRepublic of Korea Department of Pharmacology School of MedicineKyungpook National UniversityDaeguRepublic of Korea Department of Pharmacology School of DentistryKyungpook National UniversityDaeguRepublic of Korea Brain Science&Engineering Institute Kyungpook National UniversityDaeguRepublic of Korea

Astrocytes are functionally dynamic cells that support neurons in multiple ways throughout an organism’s *** astrocytic regulation of neuronal activity has been increasingly recognized in recent *** are now recognized as playing a more complex role than mere bystanders in the central nervous ***,their role in regulating the sleep neurocircuitry is not well *** this perspective,we highlight the role of astrocytes in sleep modulation,with a particular focus on regulatory mechanisms related to the ventrolateral preoptic nucleus(VLPO)of the *** briefly discuss recent literature reporting the role of VLPO astrocytes in regulating sleep-associated behaviors.

关键词： sleep ventrolateral astrocytes

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Spatiotemporal Variation and Influencing Factors of Atmospheric CO_(2) Concentration in China

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Chinese Geographical Science 2025年第1期35卷 149-160页

作者： ZHU Weixin ZHANG hong ZHANG Xiaoyu GUO Haohao LIU yong Institute of Loess Plateau Shanxi UniversityTaiyuan 030006China Research Center for Scientific Development in Fenhe River Valley Taiyuan Normal UniversityJinzhong 030619China College of Environmental&Resource Sciences Shanxi UniversityTaiyuan 030006China

Rapid increases in Carbon dioxide(CO_(2))levels could trigger unpredictable climate *** assessment of spatiotempor-al variation and influencing factors of CO_(2) concentration are helpful in understanding the source/sink balance and supporting the formu-lation of climate *** this study,Greenhouse Gases Observing Satellite(GOSAT)data were used to explore the variability of CO_(2) concentrations in China from 2009 to *** parameters,vegetation cover,and anthropogenic activities were combined to explain the increase in CO_(2) concentration,using pixel-based correlations and Covariance Based Structural Equation Modeling(CB-SEM)*** results showed that the influence of vertical CO_(2) transport diminished with altitude,with a distinct inter-annual in-crease in CO_(2) concentrations at 17 vertical ***,the highest values were observed in East China,whereas the lowest were observed in Northwest *** were significant seasonal variations in CO_(2) concentration,with maximum and minimum values in spring(April)and summer(August),*** to the pixel-based correlation analysis,the near-surface CO_(2) concentration was positively correlated with population(r=0.99,P0.05),soil water(r=0.29,P>0.05),nightlight(r=0.28,P>0.05);and negatively correlated with wind speed(r=−0.58,P<0.05).CB-SEM analysis revealed that LAI was the most important con-trolling factor explaining CO_(2) concentration variation(total effect of 0.66),followed by emissions(0.58),temperature(0.45),precipita-tion(0.30),wind speed(−0.28),and soil water(−0.07).The model explained 93% of the increase in CO_(2) *** results provide crucial information on the patterns of CO_(2) concentrations and their driving mechanisms,which are particularly significant in the context of climate change.

关键词： Greenhouse Gases Observing Satellite(GOSAT) CO_(2) concentration influencing factors pixel-based correlation Covari-ance Based Structural Equation Modeling(CB-SEM) China

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Dynamic partition of urban network considering congestion evolution based on random walk

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Chinese Physics B 2025年第1期34卷 530-534页

作者： Zhen-Tong Feng Lele Zhang yong-hong Wu Mao-Bin Hu School of Engineering Science University of Science and Technology of ChinaHefei 230026China Department of Mathematics and Statistics University of MelbourneParkville VIC 3010Australia Department of Mathematics and Statistics Curtin UniversityPerth WA 6845Australia

The successful application of perimeter control of urban traffic system strongly depends on the macroscopic fundamental diagram of the targeted *** intensive studies on the partitioning of urban road networks,the dynamic partitioning of urban regions reflecting the propagation of congestion remains an open *** paper proposes to partition the network into homogeneous sub-regions based on random walk *** from selected random walkers,the road network is partitioned from the early morning when congestion emerges.A modified Akaike information criterion is defined to find the optimal number of *** boundary adjustment algorithms are adopted to optimize the partitioning results to further ensure the correlation of *** traffic data of Melbourne city are used to verify the effectiveness of the proposed partitioning method.

关键词： urban road networks dynamic partitioning random walk Akaike information criterion perimeter control

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Impacts of near-M_(s)austempering treatment on microstructure evolution and bainitic transformation kinetics of a medium Mn steel

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Journal of Iron and Steel Research International 2025年第1期32卷 249-259页

作者： yong-gang Yang Xin-yue Liu Rui-zhi Li Yu-lai Chen hong-xiang Wu Guo-min Sun Zhen-li Mi National Engineering Research Center for Advanced Rolling and Intelligent Manufacturing University of Science and Technology BeijingBeijing 100083China Technology Center Ningbo Iron&Steel Co.Ltd.Ningbo 315800ZhejiangChina

The microstructure evolution and bainitic transformation of an Fe-0.19C-4.03Mn-1.48Si steel subjected to near-M_(s)austempering treatment were systematically investigated by combining dilatometer,X-ray diffraction,and electron *** additional austempering treatments with isothermal temperatures above M_(s)were used as *** show that the incubation period for the bainitic transformation occurs when the medium Mn steel is treated with the austempering temperature above M_(s).However,when subjected to near-M_(s)isothermal treatment,the medium Mn steel does not show an incubation period and has the fastest bainitic transformation ***,the largest volume fraction of bainite with a value of 74.7%is obtained on the condition of near-M_(s)austempering treatment after cooling to room *** and microstructure evolution analysis indicates that the elimination of the incubation period and the fastest rate of bainitic transformation are related to the preformed *** advent of preformed martensite allows the specimen to generate more bainite in a limited *** bainitic ferrite nucleation at austenite grain boundaries and through autocatalysis at ferrite/austenite interfaces,a model is established to understand the kinetics of bainite formation and it can describe the nucleation rate of bainitic transformation well when compared to the experimental results.

关键词： Medium manganese steel Bainitic transformation Microstructure Near-M_(s)austempering Transformation modeling

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Nd@C3N4-photoredox/chlorine dual catalyzed synthesis and evaluation of antitumor activities of 4-alkylated sulfonyl ketimines

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Chinese Chemical Letters 2025年第2期36卷 412-416页

作者： hong-Tao Ji Yu-Han Lu Yan-Ting Liu Yu-Lin Huang Jiang-Feng Tian Feng Liu Yan-Yan Zeng Hai-Yan Yang yong-hong Zhang Wei-Min He Department of Ophthalmology The Affiliated Nanhua Hospital Hengyang Medical School University of South China School of Chemistry and Chemical Engineering University of South China Department of Lung Cancer and Gastroenterology Hunan Cancer Hospital The Affiliated Cancer Hospital of Xiangya School of Medicine Central South University

The first example of Nd@C3N4-photoredox/chlorine dual catalyzed alkylation with unactivated alkanes as the alkyl sources has been developed,which allows for the synthesis of various 4-alkylated cyclic sulfonyl *** this process,chlorine functions as both a redox and hydrogen atom transfer *** synergism of the reversible Nd2+/Nd3+and Clˉ/Cl˙redox pairs significantly enhances overall photocatalytic *** in vitro anticancer activity of 4-alkylated products was evaluated by using the CCK8assay against both human choroidal melanoma （MUM-2B） and lung cancer （A549） *** 3da showed approximately triple the potency of 5-fluorouracil.

关键词： Chlorine Dual catalysis Hydrogen atom transfer Redox catalyst Semiconductor

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In situ measurement of environmental γ radiation dose rates of key nuclides for large radioactive surface sources

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Nuclear Science and Techniques 2025年第1期36卷 69-79页

作者： Ze-Qian Wu Jian Sun Wei-Qi Huang Bai-Rong Wang Jin-Xing Cheng Jiang-Feng Wu yong-hong Wang Biao Yuan Sheng Qi Kun Shan Institute of NBC Defence Beijing 102205China Beijing New-High Technology Academy Beijing 100094China

To monitor nuclear and radiation emergencies,it is crucial to obtain accurate in situ measurements of the environmentalγ radiation dose rate from key radionuclides,particularly for large radioactive surface *** methods currently used for measuring dose rates are inadequate for obtaining the dose rates of key radionuclides and have large angular response errors when monitoring surface *** address this practical problem,this study proposes three methods for measuring the dose rate:the weighted peak total ratio,mean value regression,and numerical integration *** methods are based on energy-spectrum measurement data,and they were theoretically derived and numerically ***,a 1-m-long hexagonal radioactive surface source was integrated into a larger surface *** situ measurement experiments were conducted on a large radioactive surface source using a dose-rate meter and a portable HPGespectrometer to analyze the errors of the three aforementioned methods and verify their validity.

关键词： Environmentalγradiation dose rate HPGespectrometer Key radionuclides Radioactive surface source

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