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Broadband,Polarization-Sensitive,and Self-Powered High-Performance Photodetection of Hetero-Integrated MoS_(2)on Lithium Niobate

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Research 2024年第2期2023卷 203-212页

作者： Zhigang He Heyuan Guan Xijie Liang Junteng Chen manyan Xie Kaiwen Luo Ran An Liang ma Fengkai ma Tiefeng Yang Huihui Lu Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications Jinan UniversityGuangzhou 510632China Key Laboratory of Optoelectronic Information and Sensing Technologies of Guangdong Higher Education Institutes Jinan UniversityGuangzhou 510632China institute of Fluid Physics China Academy of Engineering PhysicsMianyang 621900China College of Physics and Electronic Engineering Hengyang Normal UniversityHengyang 421008China

High-performance photodetectors hold promising potential in optical communication and imaging ***,conventional counterparts are suffering narrow detection range,high power consumption,and poor polarization *** originating from switchable polarization in ferroelectrics can be used to optimize the photo-to-electric procedure and improve the photodetection *** this regard,we constructed a configuration by integrating 2-dimensional molybdenum disulfide(MoS_(2))with ferroelectric lithium niobate(LiNbO_(3)),resulting in the MoS_(2)/LiNbO_(3)heterostructured *** from the pyroelectric effect of LiNbO_(3),the limitation of bandgap on the detection range can be broken,thus broadening the response band of the detector to 365 to 1,064 nm,as well as enabling the self-powered ***,high carrier mobility and decent light absorbance of MoS_(2)introduce robust light-matter interactions with the underlying LiNbO_(3),leading to ultrafast rise/fall times of≈150μs/250μs and switching ratios of up to≈***,the highest responsivity,specific detectivity,and external quantum efficiency achieved were 17.3 A·W^(-1),4.3×10^(11)Jones,and 4,645.78%,***,because of the anisotropy of the spontaneous-polarized LiNbO_(3)substrate,the photocurrent of the device achieved a dichroic ratio of 7.42,comparing favorably to most MoS_(2)-based *** work demonstrates the integration potential between ferroelectric LiNbO_(3)and 2-dimensional materials for high-performance photodetection.

关键词： polarization ferroelectric Polarization

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maP4K inhibition as a potential therapy for amyotrophic lateral sclerosis

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Neural Regeneration Research 2024年第8期19卷 1639-1640页

作者： Shuaipeng ma Chun-Li Zhang Department of Molecular Biology University of Texas Southwestern Medical CenterDallasTXUSA Hamon Center for Regenerative Science and Medicine University of Texas Southwestern Medical CenterDallasTXUSA

Amyotrophic lateral sclerosis(ALS)is a rare neurological disease,featuring gradual loss of muscle controls due to degeneration of motor ***,there is currently no cure for *** available therapies only offer a limited e... 详细信息

关键词： degeneration sclerosis maP4

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Photothermal catalysts for efficient and clean fuel production at atmospheric pressure

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Science China Chemistry 2024年第6期67卷 1762-1764页

作者： Xinwei Guan Yang Chen Tianyi ma School of Science RMIT UniversityMelbourneVIC3000Australia Institute of Clean Energy Chemistry Key Laboratory for Green Synthesis and Preparative Chemistry of Advanced Materials of Liaoning ProvinceCollege of ChemistryLiaoning UniversityShenyang110036China

The use of waste carbon resources to produce valuable chemicals and hydrocarbon fuels has attracted great interest in recent *** a transformation not only maximises the utilisation of carbon resources but also plays a... 详细信息

关键词： thermal transformation clean

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Armoring lithium metal anode with soft±rigid gradient interphase toward high-capacity and long-life all-solid-state battery

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Green Energy & Environment 2024年第8期9卷 1279-1289页

作者： Rui Zhang Biao Chen Yuhan ma Yue Li Junwei Sha Liying ma Chunsheng Shi Naiqin Zhao School of materials Science and Engineering and Tianjin Key Laboratory of Composite and Functional materials Tianjin University Joint School of National University of Singapore and Tianjin University International Campus of Tianjin University Department of Chemical and Biomolecular Engineering National University of Singapore Collaborative Innovation Centre of Chemical Science and Engineering

Solid polymer electrolytes （SPEs） are highly promising for realizing high-capacity,low-cost,and safe Li metal ***,the Li dendritic growth and side reactions between Li and SPEs also plague these ***,a fluorinated lithium salt coating （FC） with organicinorganic gradient and soft-rigid feature is introduced on Li surface as an artificial protective layer by the in-situ reaction between Li metal and fluorinated carboxylic *** FC layer can improve the interface stability and wettability between Li and SPEs,assist the transport of Li ions,and guide Li nucleation,contributing to a dendrite-free Li deposition and long-lifespan Li metal *** symmetric cell with FC-Li anodes exhibits a high areal capacity of 1 mah cm-2at 0.5 ma cm-2,and an ultra-long lifespan of 2000 h at a current density of 0.1 m A ***,the full cell paired with the LiFePO4cathode exhibits improved cycling stability,remaining 83.7%capacity after 500 cycles at 1 *** matching with the S cathode,the FC layer can prevent the shuttle effect,contributing to stable and high-capacity Li-S *** work provided a promising way for the construction of stable all-solid-state lithium metal batteries with prolonged lifespan.

关键词： All-solid-state battery Solid polymer electrolyte Li metal anode Li nucleation Interface stability

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Alloy/layer double hydroxide interphasic synergy via nano-heterointerfacing for highly reversible CO_(2)redox reaction in Li-CO_(2)batteries

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Nano Research 2024年第6期17卷 5206-5215页

作者： Tianzhen Jian Wenqing ma Jiagang Hou Jianping ma Xianhong Li Haiyang Gao Caixia Xu Hong Liu Institute for Advanced Interdisciplinary Research(iAIR) Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of ShandongSchool of Chemistry and Chemical EngineeringUniversity of JinanJinan 250022China Kyiv College at Qilu University of Technology Qilu University of Technology(Shandong Academy of Sciences)Jinan 250353China State Key Laboratory of Crystal materials Shandong UniversityJinan 250100China Shandong Sacred Sun Power Sources Co. Ltd.Qufu 273100China

Li-CO_(2)batteries are among the most intriguing techniques for balancing the carbon cycle,but are challenged by the annoyed thermodynamic barrier of the Li_(2)CO_(3)decomposition ***,we demonstrate the electrocatalytic performances of two-dimensional(2D)CoAl-layer double hydroxide(LDH)nanosheets can be significantly improved by trans-dimensional crosslinking with three-dimensional(3D)multilevel nanoporous(MP)-RuCoAl alloy(MP-RuCoAl alloy⊥CoAl-LDH).The MP-RuCoAl alloy⊥CoAl-LDH with multiscale pore channels and abundant nano-heterointerface is directly prepared by controllable etching Al from a Ru-Co-Al master alloy along with simultaneous partial oxidization of Al and Co *** MP-RuCoAl is composed of various intermetallic compounds and Ru with abundant grain boundaries,and forms numerous heterointerface with 2D CoAl-LDH *** multiscale porous metallic network benefits mass and electron transportation as well as discharge product storage and enables a rich multiphase reaction *** situ differential electrochemical mass spectrometry shows that the mass-to-charge ratio in the charging process is~0.733 which is consistent with the theoretical value of 3/4,stating that the reversible co-decomposition of Li_(2)CO_(3)and C can be achieved with the MP-RuCoAl alloy⊥*** Ketjen black(KB)/MP-RuCoAl⊥CoAl-LDH battery demonstrates a high cyclability for over 2270 h(227 cycles)with a lower voltage gap stabilized at~1.3 V at 200 ma·g^(−1).Our findings here provide useful guidelines for developing high efficiency transition metal based electrocatalysts by coupling with conductive porous substrate for impelling the development of practical Li-CO_(2)battery systems.

关键词： heterojunction interface nanoporous Li-CO_(2)battery dealloying

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Americium/lanthanide separation enabled by a distinct polyoxometalate cluster

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Science China Chemistry 2024年第1期67卷 312-313页

作者： Hui Yang Xiangke Wang Shengqian ma College of Environmental Science and Engineering North China Electric Power UniversityBeijing 102206P.R.China Department of Chemistry University of North TexasDentonTexas 76201United States

Nuclear energy is viewed as a low carbon-emission electricity-generating technology with high-energy density,which has attracted extensive attention and shown broad development prospects[1].However,to ensure sustainability and cleanability in the development of nuclear energy,one crucial challenge is to exploit efficient and economical technologies to simultaneously recover fissionable nuclides from nuclear waste and separate long-lived toxic fission products[2].

关键词： lanthanide separation cluster

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Lifetime-tunable circularly polarized luminescent system based on triplet-to-singlet F?rster resonance energy transfer

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Science China Chemistry 2024年第9期67卷 2918-2922页

作者： Zhenyi He Zizhao Huang Xiang ma Key Laboratory for Advanced materials and Feringa Nobel Prize Scientist Joint Research Center Institute of Fine Chemicals School of Chemistry and Molecular Engineering East China University of Science and Technology

Circularly polarized luminescence(CPL) materials have received widespread attention due to their remarkable performance and broad applications. However, current CPL material research primarily focuses on tunable color, intensity, and *** CPL with adjustable lifetime remains a significant challenge. Herein, a series of CPL polymeric materials with tunable lifetime were obtained by employing phosphorescent terephthalic acid and chiral organic small molecule R/S-BNAF(a luminescent binaphthol derivative) to copolymerize with acrylamide in different ratios. It was verified that this performance results from the different energy transfer efficiency between luminophores with varying ratios of the monomers for copolymerization. This strategy to realize CPL with tunable lifetime by modulating the energy transfer efficiency will provide a new perspective to broaden the applications of CPL materials.

关键词： circularly polarized luminescence tunable lifetime Förster resonance energy transfer room temperature phosphorescence

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Gyroid Triply Periodic Minimal Surface Lattice Structure Enables Improved Superelasticity of CuAlMn Shape Memory Alloy

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Acta Metallurgica Sinica(English Letters) 2024年第6期37卷 1047-1065页

作者： Mengwei Wu Chunmei ma Ruiping Liu Huadong Fu Department of materials Science and Engineering China University of Mining and Technology(Beijing)Beijing100083China Institute for Advanced materials and Technology University of Science and Technology BeijingBeijing100083China

Improving the shape memory effect and superelasticity of Cu-based shape memory alloys(Smas)has always been a research hotspot in many *** work systematically investigates the effects of Gyroid triply periodic minimal surface(TPMS)lattice structures with different unit sizes and volume fractions on the manufacturing viability,compressive mechanical response,superelasticity and heating recovery properties of CuAlMn *** results show that the increased specific surface area of the lattice structure leads to increased powder adhesion,making the manufacturability proportional to the unit size and volume *** compressive response of the CuAlMn Smas Gyroid TPMS lattice structure is negatively correlated with the unit size and positively correlated with the volume *** superelastic recovery of all CuAlMn Smas with Gyroid TPMS lattice structures is within 5%when the cyclic cumulative strain is set to be 10%.The lattice structure shows the maximum superelasticity when the unit size is 3.00 mm and the volume fraction is 12%,and after heating recovery,the total recovery strain increases as the volume fraction *** study introduces a new strategy to enhance the superelastic properties and expand the applications of CuAlMn Smas in soft robotics,medical equipment,aerospace and other fields.

关键词： Shape memory alloys Superelasticity Gyroid triply periodic minimal surface(TPMS)lattice structure Selective laser melting(SLM)

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Future Changes in Various Cold Surges over China in CMIP6 Projections

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Advances in Atmospheric Sciences 2024年第9期41卷 1751-1768页

作者： Li ma Zhigang WEI Xianru LI Shuting WU Key Laboratory of Environmental Change and Natural Disasters of Chinese Ministry of Education Beijing Normal UniversityBeijing 100875China State Key Laboratory of Earth Surface Processes and Resource Ecology(ESPRE) Beijing Normal UniversityBeijing 100875China Academy of Disaster Reduction and Emergency management Ministry of Emergency Management and Ministry of EducationBeijing 100875China Faculty of Geographical Science Beijing Normal UniversityBeijing 100875China

Cold surges(CSs)often occur in the mid-latitude regions of the Northern Hemisphere and have enormous effects on socioeconomic *** report that the occurrences of CSs and persistent CSs(PCSs)have rebounded since the 1990s,but the trends related to the frequencies of strong CSs(SCSs)and extreme CSs(ECSs)changed from increasing to decreasing after *** highest-ranked model ensemble approach was used to project the occurrences of various CSs under the SSP1-2.6,SSP2-4.5,and SSP5-8.5 *** frequencies of the total CSs show overall decreasing ***,under the SSP1-2.6 scenario,slight increasing trends are noted for SCSs and ECSs in *** circulations that are characterized by an anomalous anticyclonic circulation with a significantly positive 500-hPa geopotential height(Z500)anomaly at high latitudes along with significant negative anomalies in China were favorable for cold air intrusions into *** addition,the frequencies of all CS types under the SPP5-8.5 scenario greatly decreased in the long term(2071-2100),a finding which is thought to be related to negative SST anomalies in the central and western North Pacific,differences in sea level pressure(SLP)between high-and mid-latitude regions,and a weaker East Asian *** terms of ECSs,the decreasing trends observed during the historical period were maintained until 2024 under the SSP1-2.6 *** to the SSP1-2.6 scenario,the Z500 pattern showed a trend of strengthened ridges over the Ural region and northern East Asia and weakened troughs over Siberia(60°-90°E)under the SSP2-4.5 and SSP5-8.5 scenarios,contributing to the shift to increasing trends of ECSs after 2014.

关键词： cold surge “highest-ranked”model ensemble anticyclonic circulation geopotential height China

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Contrasts of bimodal tropical instability waves(TIWs)-induced wind stress perturbations in the Pacific Ocean among observations,ocean models,and coupled climate models

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Journal of Oceanology and Limnology 2024年第1期42卷 1-23页

作者： Kai ma Chuanyu LIU Junli XU Fan WANG School of mathematics and Physics Research Institute for Mathematics and Interdisciplinary SciencesQingdao University of Science and TechnologyQingdao 266100China Key Laboratory of Ocean Circulation and Waves Institute of OceanologyChinese Academy of SciencesQingdao 266071China Pilot National Laboratory for marine Science and Technology(Qingdao) Qingdao 266237China

The coupling between wind stress perturbations and sea surface temperature(SST)perturbations induced by tropical instability waves(TIWs)in the Pacific Ocean has been revealed previously and proven crucial to both the atmosphere and ***,an overlooked fact by previous studies is that the loosely defined“TIWs”actually consist of two modes,including the Yanai wave-based TIW on the equator(hereafter eTIW)and the Rossby wave-based TIW off the equator(hereafter vTIW).Hence,the individual feedbacks of the wind stress to the bimodal TIWs remain *** this study,individual coupling relationships are established for both eTIW and v TIW,including the relationship between the TIW-induced SST perturbations and two components of wind stress perturbations,and the relationship between the TIW-induced wind stress perturbation divergence(curl)and the downwind(crosswind)TIW-induced SST *** show that,due to different distributions of eTIW and vTIW,the coupling strength induced by the eTIW is stronger on the equator,and that by the vTIW is stronger off the *** results of any of eTIW and vTIW are higher than those of the loosely defined *** further investigated how well the coupling relationships remained in several widely recognized oceanic general circulation models and fully coupled climate ***,the coupling relationships cannot be well represented in most numerical ***,we confirmed that higher resolution usually corresponds to more accurate ***,the coupling models established in this study are complementary to previous research and can be used to refine the oceanic and coupled climate models.

关键词： bimodal tropical instability waves mesoscale air-sea interaction coupled models Yanai wave

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