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Decade Milestone Advancement of Defect-Engineered g-C_(3)N_(4) for Solar Catalytic Applications

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Nano-Micro Letters 2024年第4期16卷 153-218页

作者： Shaoqi Hou Xiaochun Gao Xingyue Lv Yilin zhao Xitao Yin Ying Liu juan Fang Xingxing Yu Xiaoguang Ma Tianyi Ma Dawei su School of Mathematical and Physical Sciences Faculty of ScienceUniversity of Technology Sydney(UTS)SydneyNSW 2007Australia Laboratory of Plasma and Energy Conversion School of Physics and Optoelectronic EngineeringLudong University186 Middle Hongqi RoadYantai 264025People’s Republic of China School of Energy and Environmental Engineering University of Science and Technology BeijingBeijing 100083People’s Republic of China Department of Chemistry The University of Tokyo7‑3‑1 HogoBunkyoTokyoJapan School of Science STEM CollegeRMIT UniversityMelbourneVIC 3000Australia

Over the past decade, graphitic carbon nitride(g-C_(3)N_(4)) has emerged as a universal photocatalyst toward various sustainable carbo-neutral technologies. Despite solar applications discrepancy, g-C_(3)N_(4) is still confronted with a general fatal issue of insufficient supply of thermodynamically active photocarriers due to its inferior solar harvesting ability and sluggish charge transfer dynamics. Fortunately, this could be significantly alleviated by the “all-in-one” defect engineering strategy, which enables a simultaneous amelioration of both textural uniqueness and intrinsic electronic band structures. To this end, we have summarized an unprecedently comprehensive discussion on defect controls including the vacancy/non-metallic dopant creation with optimized electronic band structure and electronic density, metallic doping with ultraactive coordinated environment(M–N_(x), M–C_(2)N_(2), M–O bonding), functional group grafting with optimized band structure, and promoted crystallinity with extended conjugation π system with weakened interlayered van der Waals interaction. Among them, the defect states induced by various defect types such as N vacancy, P/S/halogen dopants, and cyano group in boosting solar harvesting and accelerating photocarrier transfer have also been emphasized. More importantly, the shallow defect traps identified by femtosecond transient absorption spectra(fs-TAS) have also been highlighted. It is believed that this review would pave the way for future readers with a unique insight into a more precise defective g-C_(3)N_(4) “customization”, motivating more profound thinking and flourishing research outputs on g-C_(3)N_(4)-based photocatalysis.

关键词： Defect engineering g-C_(3)N_(4) Electronic band structures Photocarrier transfer kinetics Defect states

Numerical simulation of microwave-induced cracking and melting of granite based on mineral microscopic models

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1512-1524页

作者： Xiaoli su Diyuan Li Junjie zhao Mimi Wang Xing su Aohui Zhou School of Resources and Safety Engineering Central South UniversityChangsha 410083China

This study introduces a coupled electromagnetic–thermal–mechanical model to reveal the mechanisms of microcracking and mineral melting of polymineralic rocks under microwave *** tests validate the rationality of the proposed *** microscopic mineral sections into the granite model for simulation shows that uneven temperature gradients create distinct molten,porous,and nonmolten zones on the fracture ***,the varying thermal expansion coefficients and Young's moduli among the minerals induce significant thermal stress at the mineral *** and biotite with higher thermal expansion coefficients are subjected to compression,whereas plagioclase with smaller coefficients experiences tensile *** the molten zone,quartz undergoes transgranular cracking due to theα–βphase *** local high temperatures also induce melting phase transitions in biotite and *** numerical study provides new insights into the distribution of thermal stress and mineral phase changes in rocks under microwave irradiation.

关键词： microwave numerical modeling microcracking phase change granite

A multi-agent collaboration scheme for energy-efficient task scheduling in a 3D UAV-MEC space

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Frontiers of Information Technology & Electronic Engineering 2024年第6期25卷 824-838页

作者： Yang LI Ziling WEI Jinshu su Baokang zhao College of Computer National University of Defense TechnologyChangsha 410073China Academy of Military Sciences Beijing 100091China

Multi-access edge computing(MEC)presents computing services at the edge of networks to address the enormous processing requirements of intelligent *** to the maneuverability of unmanned aerial vehicles(UAVs),they can be used as temporal aerial edge nodes for providing edge services to ground users in ***,MEC environment is usually dynamic and *** is a challenge for multiple UAVs to select appropriate service ***,most of existing works study UAV-MEC with the assumption that the flight heights of UAVs are fixed;i.e.,the flying is considered to occur with reference to a two-dimensional plane,which neglects the importance of the *** this paper,with consideration of the co-channel interference,an optimization problem of energy efficiency is investigated to maximize the number of fulfilled tasks,where multiple UAVs in a threedimensional space collaboratively fulfill the task computation of ground *** the formulated problem,we try to obtain the optimal flight and sub-channel selection strategies for UAVs and schedule strategies for *** on the multi-agent deep deterministic policy gradient(MADDPG)algorithm,we propose a curiosity-driven and twin-networks-structured MADDPG(CTMADDPG)algorithm to solve the formulated *** uses the inner reward to facilitate the state exploration of agents,avoiding convergence at the sub-optimal ***,we adopt the twin critic networks for update stabilization to reduce the probability of Q value *** simulation results show that CTMADDPG is outstanding in maximizing the energy efficiency of the whole system and outperforms the other benchmarks.

关键词： Multi-access edge computing Multi-agent reinforcement learning Unmanned aerial vehicles Task scheduling

On the Infinite-Dimensional Modular Lie superalgebras of O-Type

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Algebra Colloquium 2024年第2期31卷 347-360页

作者： Xiaoning Xu Jing zhao Yucai su School of Mathematics and Statistics Liaoning UniversityShenyang 110036China 不详

The natural filtrations of infinite-dimensional Lie superalgebras of O-type over a field of positive characteristic are proved to be invariant under automorphisms by studying ad-nilpotent *** observe that two Lie superalgebras of O-type are isomorphic if and only if the integers in the definition of these Lie superalgebras are ***,all the Lie superalgebras of O-type are classified in the sense of isomorphism.

关键词： filtration isomorphism classification

Tracking lithiation with transmission electron microscopy

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Science China Chemistry 2024年第1期67卷 291-311页

作者： Xincheng Lei Jianxiong zhao Jiayi Wang Dong su Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China South China Academy of Advanced Optoelectronics&International Academy of Optoelectronics at zhaoqing South China Normal UniversityGuangzhou 510006China

Li-ion batteries(LIBs)have dominated energy-storage techniques for portable electronic devices and electric cars,and are expanding their territory into the large-scale energy *** energy storage of LIBs is realized by the reversible shuttle of lithium ions between *** is essential to track the lithium diffusion and obtain a profound insight into the lithiation mechanism during the work cycle of *** electron microscopy(TEM)is a powerful tool for the structural characterization,which can provide the information about the lithiation at the atomic *** this review,we summarize the research frontiers of TEM applications on *** introduce the techniques for the direct observation of Li species in LIB-related ***,the application of cryo-TEM is ***,in-situ TEM technique is further discussed since it shows great advantages in studying the dynamical structure changes of *** perspectives and strategies in this review offer feasible guidance for researchers to further improve the performance of LIBs.

关键词： lithium-ion battery electrode materials transmission electron microscopy cryo-TEM in-situ TEM

Power equipment vibration visualization using intelligent sensing method based on event-sensing principle

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Global Energy Interconnection 2024年第2期7卷 228-240页

作者： Mingzhe zhao Xiaojun Shen Lei su Zihang Dong Tongji University No.1239 Siping RoadYangpu DistrictShanghai 200092P.R.China State Grid Shanghai Municipal Electric Power Company Electric Power Science Research Institute Shanghai 200437P.R.China Department of Electrical and Electronic Engineering Imperial College LondonLondonSW72AZU.K.

Vibration measurements can be used to evaluate the operation status of power equipment and are widely applied in equipment quality inspection and fault ***-sensing technology can sense the change in surface light intensity caused by object vibration and provide a visual description of vibration *** on the analysis of the principle underlying the transformation of vibration behavior into event flow data by an event sensor,this paper proposes an algorithm to reconstruct event flow data into a relationship correlating vibration displacement and time to extract the amplitude-frequency characteristics of the vibration signal.A vibration measurement test platform is constructed,and feasibility and effectiveness tests are performed for the vibration motor and other power *** results show that event-sensing technology can effectively perceive the surface vibration behavior of power and provide a wide dynamic ***,the vibration measurement and visualization algorithm for power equipment constructed using this technology offers high measurement accuracy and *** results of this study provide a new noncontact and visual method for locating vibrations and performing amplitude-frequency analysis on power equipment.

关键词： Power equipment Event sensing Non contact measurement Graphic display Feasibility

E2E-MFERC:AMulti-Face Expression Recognition Model for Group Emotion Assessment

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Computers, Materials & Continua 2024年第4期79卷 1105-1135页

作者： Lin Wang juan zhao Hu Song Xiaolong Xu Jiangsu Key Laboratory of Big Data Security&Intelligent Processing Nanjing University of Posts and TelecommunicationsNanjing210042China School of Network Security Jinling Institute of TechnologyNanjing211169China State Grid Jiangsu Electric Power Company Limited Nanjing210000China School of Computer Science Nanjing University of Posts and TelecommunicationsNanjing210042China

In smart classrooms, conducting multi-face expression recognition based on existing hardware devices to assessstudents’ group emotions can provide educators with more comprehensive and intuitive classroom effect analysis,thereby continuouslypromotingthe improvementof teaching ***,most existingmulti-face expressionrecognition methods adopt a multi-stage approach, with an overall complex process, poor real-time performance,and insufficient generalization ability. In addition, the existing facial expression datasets are mostly single faceimages, which are of low quality and lack specificity, also restricting the development of this research. This paperaims to propose an end-to-end high-performance multi-face expression recognition algorithm model suitable forsmart classrooms, construct a high-quality multi-face expression dataset to support algorithm research, and applythe model to group emotion assessment to expand its application value. To this end, we propose an end-to-endmulti-face expression recognition algorithm model for smart classrooms (E2E-MFERC). In order to provide highqualityand highly targeted data support for model research, we constructed a multi-face expression dataset inreal classrooms (MFED), containing 2,385 images and a total of 18,712 expression labels, collected from smartclassrooms. In constructing E2E-MFERC, by introducing Re-parameterization visual geometry group (RepVGG)block and symmetric positive definite convolution (SPD-Conv) modules to enhance representational capability;combined with the cross stage partial network fusion module optimized by attention mechanism (C2f_Attention),it strengthens the ability to extract key information;adopts asymptotic feature pyramid network (AFPN) featurefusion tailored to classroomscenes and optimizes the head prediction output size;achieves high-performance endto-end multi-face expression detection. Finally, we apply the model to smart classroom group emotion assessmentand provide design refe

关键词： Multi-face expression recognition smart classroom end-to-end detection group emotion assessment

Asperuloside Promotes Apoptosis of Cervical Cancer Cells through Endoplasmic Reticulum Stress-Mitochondrial Pathway

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Chinese Journal of Integrative Medicine 2024年第1期30卷 34-41页

作者： QI Zhi-min WANG Xia LIU Xia zhao juan Medical Examination Center Hebei Province Hospital of Chinese MedicineShijiazhuang(050011)China Department of Gynaecology and Obstetrics Hebei Province Hospital of Chinese MedicineShijiazhuang(050011)China Experimental Center for Teaching Hebei Medical UniversityShijiazhuang(050017)China

Objective: To investigate the effects of asperuloside on cervical cancer based on endoplasmic reticulum(ER) stress and mitochondrial pathway. Methods: Different doses(12.5–800 μg/mL) of asperuloside were used to treat cervical cancer cell lines Hela and CaSki to calculate the half maximal inhibitory concentration(IC_(50)) of asperuloside. The cell proliferation was analyzed by clone formation assay. Cell apoptosis, intracellular reactive oxygen species(ROS) and mitochondrial membrane potential were determined by flow cytometry. The protein expressions of cleaved-caspase-3, Bcl-2, Bax, Cyt-c, cleaved-caspase-4 and glucose-regulated protein 78(GRP78) were analyzed by Western blot. And the inhibitor of ER stress, 4-phenyl butyric acid(4-PBA) was used to treat cervical cancer cells to further verify the role of ER stress in the apoptosis of cervical cancer cells induced by asperuloside. Results: Asperuloside of 325, 650, and 1300 μg/mL significantly inhibited the proliferation and promoted apoptosis of Hela and CaSki cells(Psuggesting that asperuloside promotes apoptosis of cervical cancer cells through ER stress-mitochondrial pathway.

关键词： asperuloside Chinese medicine cervical cancer endoplasmic reticulum stress mitochondrial damage apoptosis

Reversible isomerization of donor-acceptor Stenhouse adduct derivatives in water through dendritic confinement

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Science China Chemistry 2024年第5期67卷 1636-1646页

作者： Jiaxing Zhang Qingyun zhao Xinyan su Afang Zhang Wen Li International Joint Laboratory of Biomimetic and Smart Polymers School of Materials Science and EngineeringShanghai UniversityShanghai 200444China

Modulating reversible isomerization of hydrophobic dyes in aqueous solutions is greatly desired. Here we report on reversible isomerization of solvatochromic donor-acceptor Stenhouse adducts(DASAs) in water through the confinement from dendritic oligoethylene glycols(OEGs). Dendronization of DASAs with dendritic OEGs affords them characteristic thermoresponsiveness. These dendronized DASAs spontaneously isomerize in water from hydrophobic linear state into hydrophilic cyclic state at room temperature due to the strong hydration. However, hydrophobic microenvironment through thermally dehydration and collapse of the dendritic OEGs at elevated temperatures confines hydration of the DASA moieties and mediates their interactions with the collapsed hydrophobic OEG domains, affording their isomerization recovery in water efficiently from the hydrophilic cyclic state into the hydrophobic linear state. The confinement-mediated reversible isomerization of DASA moieties in water can be repeated through alternative photo-irradiation and thermal dehydrations, exhibiting excellent fatigue resistance.

关键词： dendrimers donor-acceptor Stenhouse adducts isomerization confinement thermoresponsiveness