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Construction of Phosphorus-Functionalized Multichannel Carbon Interlayers for dendrite-Free Metallic Zn Anodes

energy & environmental Materials 2024年第05期7卷 99-107页

作者： Liang he Qingyin Zhang he Li Shiping Liu Ting Cheng Ruoxuan Zhang Yujia Wang Peng Zhang Zhiqiang Shi Tianjin Key Laboratory of Advanced Fibers and energy Storage School of Materials Science and Engineering Tiangong University Cangzhou Institute of Tiangong University School of Chemical engineering and Technology Tiangong University Tianjin Lishen Battery Joint-Stock CO. LTD

Zn metal anodes are usually subject to grave dendrite growth during platting/stripping, which dramatically curtails the lifespan of aqueous Zn-ion batteries and capacitors. To address above problems, in our work, a novel phosphorus-functionalized multichannel carbon interlayer was designed and covered on Zn anodes. The results demonstrated that the multichannel structure combined with the three-dimensional meshy skeleton can provide more sufficient space for Zn deposition, thereby effectively inhibiting the growth of zinc dendrites. Meanwhile, theoretical calculations also confirmed that the P–C and P=O functional groups from phosphorus-functionalized multichannel carbon interlayer have the decisive influence in reducing the zinc nucleation potential and depositing uniformly zinc. Concretely, the symmetrical battery assembled with phosphorus-functionalized multichannel carbon interlayer-covered Zn anodes possessed a long lifetime of 3300 h at2 mA cm-2with 1 mAh cm-2. Furthermore, the full cell with activated carbon cathodes exhibited a high specific capacity of 80.5 mAh g-1and outstanding cycling stability without capacity decay after 15 000 cycles at a high current density of 5 A g-1. The superior electrochemical performance exceeded that of most reported papers. Consequently, our synthesized zincophilic interlayer with the unique structure has superior prospects for application in stabilizing zinc anodes and prolonging the lifespan of batteries.

关键词： aqueous Zn-ion supercapacitors multichannel carbon fiber phosphorus functionalized Zn dendrite Zn metal anode

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Construction of core@double-shell structured energetic composites with simultaneously enhanced thermal stability and safety performance

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defence Technology（防务技术） 2024年第4期34卷 134-142页

作者： Peng Wang Wen Qian Ruolei Zhong Fangfang he Xin Li Jie Chen Li Meng Yinshuang Sun Guansong he Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900China State Key Laboratory of environment-friendly energy Materials School of Materials and ChemistrySouthwest University of Science and TechnologyMianyang 621010China

The poor thermal stability and high sensitivity severely hinder the practical application of hexanitrohexaazaisowurtzitane(CL-20).herein,a kind of novel core@double-shell CL-20 based energetic composites were fabricated to address the above *** coordination complexes which consist of natural polyphenol tannic acid(TA) and Fe~Ⅲ were chosen to construct the inner shell,while the graphene sheets were used to build the outer *** resulting CL-20/TA-Fe~Ⅲ/graphene composites exhibited simultaneously improved thermal stability and safety performance with only 1 wt% double-shell content,which should be ascribed to the intense physical encapsulation effect from inner shell combined with the desensitization effect of carbon nano-materials from outer *** phase transition(ε to γ) temperature increased from 173.70 ℃ of pure CL-20 to 191.87℃ of CL-20/TA-Fe~Ⅲ/graphene ***,the characteristic drop height(H_(50)) dramatically increased from 14.7 cm of pure CL-20 to112.8 cm of CL-20/TA-Fe~Ⅲ/graphene composites,indicating much superior safety performance after the construction of the double-shell *** general,this work has provided an effective and versatile strategy to conquer the thermal stability and safety issues of CL-20 and contributes to the future application of high energy density energetic materials.

关键词： CL-20 double-shell structure Thermal stability Safety performance Tannic acid Graphene sheets

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Global well-posedness for 2d inhomogeneous asymmetric fluids with large initial data

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Science China Mathematics 2024年第3期67卷 527-556页

作者： Chenyin Qian Beibei he Ting Zhang School of Mathematical Sciences Zhejiang Normal UniversityJinhua 321004China School of Mathematical Sciences Zhejiang UniversityHangzhou 310058China

In this paper, by using time-weighted global estimates and the Lagrangian approach, we first investigate the global existence and uniqueness of the solution for the 2d inhomogeneous incompressible asymmetric fluids with the initial(angular) velocity being located in sub-critical Sobolev spaces H^(s)(R^(2))(0d the initial density being bounded from above and below by some positive constants. The global unique solvability of the 2d incompressible inhomogeneous asymmetric fluids with the initial data in the critical Besov space(u_(0), w_(0))∈˙B^(0)_(2,1)(R^(2))andρ^(−1)−1∈˙B^(ε)_(2/ε),1(R^(2))is established. In particular, the uniqueness of the solution is also obtained without any more regularity assumptions on the initial density which is an improvement on the recent result of Abidi and Gui(2021) for the 2d inhomogeneous incompressible NavierStokes system.

关键词： inhomogeneous asymmetric fluids Littlewood-Paley theory Besov spaces global well-posedness

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Sulfated peptides and their receptors:Key regulators of plant development and stress adaptation

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Plant Communications 2024年第6期5卷 44-56页

作者： Liming he Liangfan Wu Jia Li Ministry of education Key Laboratory of Cell Activities and Stress Adaptations School of Life SciencesLanzhou UniversityLanzhou 730000China Guangdong Provincial Key Laboratory of Plant Adaptation and Molecular design School of Life SciencesGuangzhou UniversityGuangzhou 510006China

Four distinct types of sulfated peptides have been identiﬁed in Arabidopsis *** peptides play crucial roles in regulating plant development and stress *** studies have revealed that Xan-thomonas and Meloidogyne can secrete plant-like sulfated peptides,exploiting the plant sulfated peptide signaling pathway to suppress plant *** the past three decades,receptors for these four types of sulfated peptides have been identiﬁed,all of which belong to the leucine-rich repeat receptor-like protein kinase subfamily.A number of regulatory proteins have been demonstrated to play important roles in their corresponding signal transduction *** this review,we comprehensively summarize the discov-eries of sulfated peptides and their receptors,mainly in Arabidopsis *** also discuss their known biological functions in plant development and stress ***,we put forward a number of ques-tions for reference in future studies.

关键词： peptide hormone sulfated peptide receptor-like protein kinase plant development stress adaptation

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A Systematic Review and Performance evaluation of Open-Source Tools for Smart Contract Vulnerability detection

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Computers, Materials & Continua 2024年第7期80卷 995-1032页

作者： Yaqiong he Jinlin Fan Huaiguang Wu School of Computer Science and Technology Zhengzhou University of Light IndustryZhengzhou450001China

With the rise of blockchain technology,the security issues of smart contracts have become increasingly *** the availability of numerous smart contract vulnerability detection tools,many face challenges such as slow updates,usability issues,and limited installation *** challenges hinder the adoption and practicality of these *** paper examines smart contract vulnerability detection tools from 2016 to 2023,sourced from the Web of Science(WOS)and Google *** systematically collecting,screening,and synthesizing relevant research,38 open-source tools that provide installation methods were selected for further *** a developer’s perspective,this paper offers a comprehensive survey of these 38 open-source tools,discussing their operating principles,installation methods,environmental dependencies,update frequencies,and installation *** on this,we propose an ethereum smart contract vulnerability detection *** framework enables developers to easily utilize various detection tools and accurately analyze contract security *** validate the framework’s stability,over 1700 h of testing were ***,a comprehensive performance test was performed on the mainstream detection tools integrated within the framework,assessing their hardware requirements and vulnerability detection *** results indicate that the Slither tool demonstrates satisfactory performance in terms of system resource consumption and vulnerability detection *** study represents the first performance evaluation of testing tools in this domain,providing significant reference value.

关键词： Blockchain security ethereum smart contracts detection tools evaluation

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Image Segmentation-P300 Selector: A Brain–Computer Interface System for Target Selection

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Computers, Materials & Continua 2024年第5期79卷 2505-2522页

作者： Hang Sun Changsheng Li he Zhang Mechanical engineering Nanjing University of Science and TechnologyNanjing210018China

Brain–computer interface (BCI) systems, such as the P300 speller, enable patients to express intentions withoutnecessitating extensive ***, the complexity of operational instructions and the slow pace of characterspelling pose challenges for some patients. In this paper, an image segmentation P300 selector based on YOLOv7-mask and deepSORT is proposed. The proposed system utilizes a camera to capture real-world objects forclassification and tracking. By applying predefined stimulation rules and object-specificmasks, the proposed systemtriggers stimuli associated with the objects displayed on the screen, inducing the generation of P300 signals in thepatient’s brain. Its video processing mechanism enables the system to identify the target the patient is focusing oneven if the object is partially obscured, overlapped, moving, or changing in number. The system alters the target’scolor display, thereby conveying the patient’s intentions to caregivers. The data analysis revealed that the selfrecognitionaccuracy of the subjects using this method was between 92% and 100%, and the cross-subject P300recognition precision was 81.9%–92.1%. This means that simple instructions such as “do not worry, just focuson what you desire” effectively discerned the patient’s intentions using the Image Segmentation-P300 selector. Thisapproach provides cost-effective support and allows patients with communication difficulties to easily express theirneeds.

关键词： Brain-computer interface deep learning electroencephalogram P300 YOLOv7-mask

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Infinitely many dichotomous solutions for the Schrödinger-Poisson system

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Science China Mathematics 2024年第9期67卷 2049-2070页

作者： Yuke he Benniao Li Wei Long School of Mathematics and Statistics and Jiangxi Provincial Center for Applied Mathematics Jiangxi Normal UniversityNanchang 330022China

In this paper,we consider the following Schrodinger-Poisson system{-ε^(2)Δu+V(x)u+K(x)Φ(x)u=|u|^(p-1)u in R^(N),-ΔΦ(x)=K(x)u^(2)in RN,,where e is a small parameter,1d V(x)and K(x)are potential functions with different decay at *** first prove the non-degeneracy of a radial low-energy ***,by using the non-degenerate solution,we construct a new type of infinitely many solutions for the above system,which are called“dichotomous solutions”,i.e.,these solutions concentrate both in a bounded domain and near infinity.

关键词： dichotomous solutions non-degeneracy Schrodinger-Poisson system

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Quantum search with prior knowledge

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Science China(Information Sciences) 2024年第9期67卷 321-329页

作者： Xiaoyu he Xiaoming SUN Jialing ZHANG State Key Lab of Processors Institute of Computing Technology Chinese Academy of Sciences School of Computer Science and Technology University of Chinese Academy of Sciences

The combination of contextual side information and search is a powerful paradigm in the scope of artificial intelligence. The prior knowledge enables the identification of possible solutions but may be imperfect. Contextual information can arise naturally, for example in game AI where prior knowledge is used to bias move decisions. In this work we investigate the problem of taking quantum advantage of contextual information, especially searching with prior knowledge. We propose a new generalization of Grover's search algorithm that achieves the optimal expected success probability of finding the solution if the number of queries is fixed. experiments on small-scale quantum circuits verify the advantage of our algorithm. Since contextual information exists widely, our method has wide applications. We take game tree search as an example.

关键词： quantum computing quantum search quantum query algorithm prior knowledge

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Restoring cosmological concordance with axion-like early dark energy and dark matter characterized by a constant equation of state?

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Communications in Theoretical Physics 2024年第7期76卷 74-82页

作者： Yan-Hong Yao Xin-he Meng School of Physics and Astronomy Sun Yatsen University 2 Daxue RoadTangjiaZhuhaiChina School of Physics Nankai University 94 Weijin RoadNankaiTianjinChina

The Hubble tension persists as a challenge in *** early dark energy(ede)models,initially considered the most promising for alleviating the Hubble tension,fall short of addressing the issue without exacerbating other tensions,such as the S_(8)*** that a negative dark matter(dM)equation of state(eoS)parameter is conducive to reduce the value of the σ_(8)parameter,we extend the axion-like ede model in this paper by replacing the cold dark matter(CdM)with dM characterized by a constant eoS w_(dm)(referred to as WdM hereafter).We then impose constraints on this axion-like ede extension model,along with three other models:the axion-like ede model,ΛWdM,and Λ*** constraints are derived from a comprehensive analysis incorporating data from the Planck 2018 cosmic microwave background,baryon acoustic oscillations,and the Pantheon compilation,as well as a prior on H_(0)(i.e.H_(0)=73.04±1.04,based on the latest local measurement by Riess et al)and a Gaussianized prior on S_(8)(i.e.S_(8)=0.766±0.017,determined through the joint analysis of KId1000+BOSS+2dLenS).We find that although the new model maintains the ability to alleviate the Hubble tension to~1.4σ,it still exacerbates the S_(8)tension to a level similar to that of the axion-like ede model.

关键词： Hubble tension early dark energy noncold dark matter S8 tension

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Retrieval of high spatial resolution mountainous land surface temperature considering topographic and adjacency effects

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Science China earth Sciences 2024年第11期67卷 3610-3625页

作者： Zhiwei he Bohui TANG Zhaoliang LI Faculty of Land Resources engineering Kunming University of Science and Technology Key Laboratory of Plateau Remote Sensing Department of Education of Yunnan Province State Key Lab of Resources and environmental Information System Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of Sciences Key Laboratory of Agricultural Remote Sensing Ministry of Agriculture and Rural Affairs Institute of Agricultural Resources and Regional Planning Chinese Academy of Agricultural Sciences

Land surface temperature(LST) is a key parameter reflecting the interaction between land and atmosphere. Currently,thermal infrared(TIR) quantitative remote sensing technology is the only means to obtain large-scale, high spatial resolution LST. Accurately retrieving high spatial resolution mountainous LST(MLST) plays an important role in the study of mountain climate change. The complex terrain and strong spatial heterogeneity in mountainous areas change the geometric relationship between the surface and satellite sensors, affecting the radiation received by the sensors, and rendering the assumption of planar parallelism invalid. In this study, considering the influence of complex terrain in mountainous areas on atmospheric downward radiation and the thermal radiation contribution of adjacent pixels, a mountainous TIR radiative transfer model based on the sky view factor was developed. Combining with the atmospheric radiative transfer model MOdTRAN 5.2, a nonlinear generalized split-window algorithm suitable for high spatial resolution MLST retrieval was constructed and applied to Landsat-9 TIRS-2satellite TIR remote sensing data. The analysis results indicate that neglecting the topographic and adjacency effects would lead to significant discrepancies in LST retrieval, with simulated data showing LST differences of up to 2.5 K. Furthermore, due to the lack of measured MLST in the field, the MLST accuracy obtained by this retrieval method was indirectly validated using the currently recognized highest-accuracy forward 3d radiative transfer model dART. The MLST and emissivity were input into the dART model to simulate the brightness temperature at the top of the atmosphere(TOA) of Landsat-9 band 10, and compared with the brightness temperature at TOA of Landsat-9 band 10. The RMSe(Root Mean Square error) for the two subregions was0.50 and 0.61 K, respectively, indicating that the method proposed can retrieve high-precision MLST.

关键词： Mountainous land surface temperature Topographic and adjacency effects Nonlinear generalized split-window algorithm Landsat-9 data dART model

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