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Chinese Chemical Letters 2024年第10期35卷 420-424页

作者： Rongxin zhu Shengsheng yu Xuanzong Yang Ruyu zhu Hui Liu Kaikai Niu Lingbao Xing School of Chemistry and Chemical Engineering Shandong University of Technology

Using hydrogen-bonded organic frameworks（HOFs） as photosensitizers to perform photocatalytic oxidation reactions under green and mild conditions is still a challenge for the application of HOFs materials. This study presents a novel approach that exploits HOFs to enhance the efficiency of photocatalytic oxidation for achieving visible light catalytic oxidation of styrene and its derivatives in the aqueous environment. By using 1,3,6,8-tetrakis（p-benzoic acid）pyrene（H4TBAPy） as the monomer, a pyrene-based hydrogen-bonded organic framework（PFC-1） with a microporous structure was successfully *** with monomer H4TBAPy, due to the exciton effect and the interlayer confinement of HOFs, the singlet oxygen（1O2） production efficiency is significantly improved, which has great potential in photocatalytic oxidation reactions. Subsequently, the practicality of PFC-1 as a photocatalyst was studied,and the photocatalytic oxidation of styrene and its derivatives in aqueous solution was achieved under visible light with high catalytic efficiency, indicating that PFC-1 has significant potential to promote photocatalytic oxidation reactions under mild conditions. The utilization of HOFs as photosensitizers in this straightforward approach enables the attainment of green photocatalytic oxidation, hence expanding the potential applications of HOFs materials within the realm of photocatalysis.

关键词： Hydrogen-bonded organic frameworks Photocatalysis Pyrene singlet oxygen Styrene

Solving the subset sum problem by the quantum Ising model with variational quantum optimization based on conditional values at risk

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Science China(Physics,Mechanics & Astronomy) 2024年第8期67卷 43-55页

作者： Qilin Zheng Miaomiao yu Pingyu zhu Yan Wang Weihong Luo Ping Xu Institute for Quantum Information and State Key Laboratory of High Performance Computing College of Computer Science and TechnologyNational University of Defense TechnologyChangsha 410073China Hefei National Laboratory Hefei 230088China

The subset sum problem is a combinatorial optimization problem,and its complexity belongs to the nondeterministic polynomial time complete(NP-Complete)*** problem is widely used in encryption,planning or scheduling,and integer *** accurate search algorithm with polynomial time complexity has not been found,which makes it challenging to be solved on classical *** effectively solve this problem,we translate it into the quantum Ising model and solve it with a variational quantum optimization method based on conditional values at *** proposed model needs only n qubits to encode 2ndimensional search space,which can effectively save the encoding quantum *** model inherits the advantages of variational quantum algorithms and can obtain good performance at shallow circuit depths while being robust to noise,and it is convenient to be deployed in the Noisy Intermediate Scale Quantum *** investigate the effects of the scalability,the variational ansatz type,the variational depth,and noise on the ***,we also discuss the performance of the model under different conditional values at *** computer simulation,the scale can reach more than nine *** selecting the noise type,we construct simulators with different QVs and study the performance of the model with *** addition,we deploy the model on a superconducting quantum computer of the Origin Quantum Technology Company and successfully solve the subset sum *** model provides a new perspective for solving the subset sum problem.

关键词： subset sum problem quantum Ising model conditional values at risk variational quantum optimization

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Route selection for opportunity-sensing and prediction of waterlogging

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Frontiers of Computer Science 2024年第4期18卷 147-159页

作者： Jingbin WANG Weijie ZHANG Zhiyong yu Fangwan HUANG Weiping zhu Longbiao CHEN College of Computer and Data Science Fuzhou UniversityFuzhou 350108China Department of Computer Science and Technology Xiamen UniversityXiamen 361005China

Accurate monitoring of urban waterlogging contributes to the city’s normal operation and the safety of residents’daily ***,due to feedback delays or high costs,existing methods make large-scale,fine-grained waterlogging monitoring impossible.A common method is to forecast the city’s global waterlogging status using its partial waterlogging *** method has two challenges:first,existing predictive algorithms are either driven by knowledge or data alone;and second,the partial waterlogging data is not collected selectively,resulting in poor *** overcome the aforementioned challenges,this paper proposes a framework for large-scale and fine-grained spatiotemporal waterlogging monitoring based on the opportunistic sensing of limited bus *** framework follows the Sparse Crowdsensing and mainly comprises a pair of iterative predictor and *** predictor uses the collected waterlogging status and the predicted status of the uncollected area to train the graph convolutional neural *** combines both knowledge-driven and data-driven approaches and can be used to forecast waterlogging status in all regions for the upcoming *** selector consists of a two-stage selection procedure that can select valuable bus routes while satisfying budget *** experimental results on real waterlogging and bus routes in Shenzhen show that the proposed framework could easily perform urban waterlogging monitoring with low cost,high accuracy,wide coverage,and fine granularity.

关键词： waterlogging prediction sparse crowdsensing active learning route selection graph convolutional network

Carbon-based interface engineering and architecture design for high-performance lithium metal anodes

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Carbon Energy 2024年第1期6卷 207-235页

作者： Na zhu yuxiang Yang yu Li Ying Bai Junfeng Rong Chuan Wu siNOPEC Research Institute of Petroleum Processing Co. Ltd.BeijingChina Beijing Key Laboratory of Environmental Science and Engineering School of Materials Science and EngineeringBeijing Institute of TechnologyBeijingChina Yangtze Delta Region Academy of Beijing Institute of Technology JiaxingChina

Metallic lithium(Li)is considered the“Holy Grail”anode material for the nextgeneration of Li batteries with high energy density owing to the extraordinary theoretical specific capacity and the lowest negative electrochemical ***,owing to inhomogeneous Li-ion flux,Li anodes undergo uncontrollable Li deposition,leading to limited power output and practical *** materials and their composites with controllable structures and properties have received extensive attention to guide the homogeneous growth of Li to achieve high-performance Li *** this review,the correlation between the behavior of Li anode and the properties of carbon materials is ***,we review emerging strategies for rationally designing high-performance Li anodes with carbon materials,including interface engineering(stabilizing solid electrolyte interphase layer and other functionalized interfacial layer)and architecture design of host carbon(constructing three-dimension structure,preparing hollow structure,introducing lithiophilic sites,optimizing geometric effects,and compositing with Li).Based on the insights,some prospects on critical challenges and possible future research directions in this field are *** is anticipated that further innovative works on the fundamental chemistry and theoretical research of Li anodes are needed.

关键词： carbon materials dendrites hosts interfacial layers Li metal anodes

Monazite U-Th-Pb and sericite Rb-Sr dating of the Xiajiadian black shale-hosted gold deposit in the Qinling orogen,central China:Implications for regional gold metallogeny

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Science China Earth Sciences 2024年第8期67卷 2478-2494页

作者： Xueling yu Jianwei LI Xiaoye JIN Shaorui ZHAO Chongguo HE yunlong zhu State Key Laboratory of Geological Processes and Mineral Resources China University of GeosciencesWuhan 430074China School of Earth Resources China University of GeosciencesWuhan 430074China

The Qinling orogen in central China contains several black shale-hosted gold deposits,but the age of their formation and a possible relation between gold mineralization and regional tectonism remain *** we present results of in situ monazite U-Th-Pb dating and sericite Rb-Sr dating of the Xiajiadian black shale-hosted gold deposit to provide tight constraints on the time of gold deposition and information on the tectonic setting under which the deposit *** Xiajiadian gold deposit is mainly hosted in black shales of the Lower Cambrian Shuigoukou formation,with minor ores contained in sandy conglomerate of the Lower Devonian Xichahe *** ores in the black shales have been intensively oxidized and consist mainly of hematite,goethite,gypsum,quartz,calcite,native gold,and unrecognized iron ***,gold ores in the sandy conglomerate are free of oxidation and thus provide an opportunity to date the formation of the Xiajiadian gold *** ores consist of pyrite,marcasite,sericite,and quartz,which are associated with a variety of accessory minerals,including monazite,apatite,and *** is mainly present as structure-bound ions or nanoparticles in pyrite and marcasite,but minor native gold grains also occur as inclusions in *** is well developed in the ores,and has close textural association with Au-bearing pyrite and *** monazite grains have zoned textures consisting of a core area(Mnz1)and an overgrowth zone(Mnz2).Mnz1 contains 4.8–13 wt.%ThO_(2)and shows large variations in HREE and prominent negative Eu anomalies in the chondrite-normalized REE *** yields common lead-corrected^(208)Pb/^(232)Th dates ranging from 910±10 to416±4 Ma(2σ).These dates are interpreted in terms of a detrital origin for monazite in the core ***2 has much lower ThO_(2)contents of 0.8–1.7 wt.%and shows weak negative Eu anomalies in the chondrite-normalized REE *** yields common lead-corrected^(208)Pb/^(232

关键词： Monazite U-Th-Pb dating Sericite Rb-Sr dating Late Triassic(Norian) Orogenic gold deposit Xiajiadian

A Composite Transformer-Based Multi-Stage Defect Detection Architecture for Sewer Pipes

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Computers, Materials & Continua 2024年第1期78卷 435-451页

作者： Zifeng yu Xianfeng Li Lianpeng Sun Jinjun zhu Jianxin Lin School of Computer Science and Engineering Macao University of Science and TechnologyMacao999078China School of Environmental Science and Engineering Sun Yat-sen UniversityGuangzhou510275China Guangdong AIKE Environmental Science and Technology Co. Ltd.Zhongshan528400China

Urban sewer pipes are a vital infrastructure in modern cities,and their defects must be detected in time to prevent potential *** recent years,to relieve the manual efforts by human experts,models based on deep learning have been introduced to automatically identify potential ***,these models are insufficient in terms of dataset complexity,model versatility and *** work addresses these issues with amulti-stage defect detection architecture using a composite backbone Swin *** based on this architecture is trained using a more comprehensive dataset containingmore classes of *** ablation studies on the modules of combined backbone Swin Transformer,multi-stage detector,test-time data augmentation and model fusion,it is revealed that they all contribute to the improvement of detection accuracy from different *** model incorporating all these modules achieves the mean Average Precision(mAP)of 78.6% at an Intersection over Union(IoU)threshold of *** represents an improvement of 14.1% over the ResNet50 Faster Region-based Convolutional Neural Network(R-CNN)model and a 6.7% improvement over You Only Look Once version 6(YOLOv6)-large,the highest in the YOLO *** addition,for other defect detection models for sewer pipes,although direct comparison with themis infeasible due to the unavailability of their private datasets,our results are obtained from a more comprehensive dataset and have superior generalization capabilities.

关键词： Sewer pipe defect detection deep learning model optimization composite transformer

Microstructure evolution,mechanical properties and fracture behavior of Al-xsi/AZ91D bimetallic composites prepared by a compound casting

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Journal of Magnesium and Alloys 2024年第5期12卷 1944-1964页

作者： Guangyu Li Wenming Jiang Feng Guan Junwen zhu Yang yu Zitian Fan State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

In this paper,the effect of the si content on microstructure evolution,mechanical properties,and fracture behavior of the Al-xsi/AZ91D bimetallic composites prepared by compound casting was investigated *** obtained results showed that all the Al-xsi/AZ91D bimetallic composites had a metallurgical reaction layer(MRL),whose thickness increased with increasing si content for the hypoeutectic Al-si/AZ91D composites,while the hypereutectic Al-si/AZ91D composites were *** MRL included eutectic layer(E layer),intermetallic compound layer(IMC layer)and transition region layer(T layer).In the IMC layer,the hypereutectic Al-si/AZ91D composites contained some si solid solution and flocculent Mg_(2)si+Al-Mg IMCs phases not presented in the hypoeutectic Al-si/AZ91D ***,increasing si content,the thickness proportion of the T layer increased,forming an inconsistent preferred orientation of the *** shear strengths of the Al-xsi/AZ91D bimetallic composites enhanced with increasing si content,and the Al-15si/AZ91D composite obtained a maximum shear strength of 58.6 MPa,which was 73.4% higher than the Al-6si/AZ91D *** fractures of the Al-xsi/AZ91D bimetallic composites transformed from the T layer into the E layer with the increase of the si *** improvement of the shear strength of the Al-xsi/AZ91D bimetallic composites was attributed to the synergistic action of the Mg_(2)si particle reinforcement,the reduction of oxidizing inclusions and the ratio of Al-Mg IMCs as well as the orientation change of the MRL.

关键词： Al/Mg bimetallic composites si content Mg_(2)si reinforcement Microstructure Mechanical properties Fracture behavior

Association of age at diagnosis of diabetes with subsequent risk of age-related ocular diseases and vision acuity

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World Journal of Diabetes 2024年第4期15卷 697-711页

作者： si-Ting Ye Xian-Wen Shang yu Huang Susan zhu zhuo-Ting zhu Xue-Li Zhang Wei Wang Shu-Lin Tang Zong-yuan Ge Xiao-Hong Yang Ming-Guang He The Second Clinical College Guangzhou University of Chinese MedicineGuangzhou 510120Guangdong ProvinceChina Department of Ultrasound The Second Affiliated Hospital of Guangzhou University of Chinese MedicineGuangzhou 510120Guangdong ProvinceChina Guangdong Eye Institute Department of OphthalmologyGuangdong Provincial People’s HospitalGuangdong Academy of Medical SciencesGuangzhou 510080Guangdong ProvinceChina Guangdong Cardiovascular Institute Guangdong Provincial People's HospitalGuangdong Academy of Medical SciencesGuangzhou 510080Guangdong ProvinceChina Austin Hospital University of MelbourneMelbourne 3084VictoriaAustralia State Key Laboratory of Ophthalmology Zhongshan Ophthalmic CenterSun Yat-sen UniversityGuangzhou 510060Guangdong ProvinceChina Monash e-Research Center Faculty of EngineeringAirdoc ResearchNvidia AI Technology Research CenterMonash UniversityMelbourne 3080VictoriaAustralia Department of Ophthalmic Epidemiology Centre for Eye Research AustraliaMelbourne 3002VictoriaAustralia

BACKGROUND The importance of age on the development of ocular conditions has been reported by numerous *** may have different associations with different stages of ocular conditions,and the duration of diabetes may affect the development of diabetic eye *** there is a dose-response relationship between the age at diagnosis of diabetes and the risk of cardiovascular disease and mortality,whether the age at diagnosis of diabetes is associated with incident ocular conditions remains to be *** is unclear which types of diabetes are more predictive of ocular *** To examine associations between the age of diabetes diagnosis and the incidence of cataract,glaucoma,age-related macular degeneration(AMD),and vision *** Our analysis was using the UK *** cohort included 8709 diabetic participants and 17418 controls for ocular condition analysis,and 6689 diabetic participants and 13378 controls for vision *** diseases were identified using inpatient records until January *** acuity was assessed using a *** During a median follow-up of 11.0 years,3874,665,and 616 new cases of cataract,glaucoma,and AMD,respectively,were identified.A stronger association between diabetes and incident ocular conditions was observed where diabetes was diagnosed at a younger *** with type 2 diabetes(T2D)diagnosed at<45 years[HR(95%CI):2.71(1.49-4.93)],45-49 years[2.57(1.17-5.65)],50-54 years[1.85(1.13-3.04)],or 50-59 years of age[1.53(1.00-2.34)]had a higher risk of AMD independent of glycated haemoglobin.T2D diagnosed<45 years[HR(95%CI):2.18(1.71-2.79)],45-49 years[1.54(1.19-2.01)],50-54 years[1.60(1.31-1.96)],or 55-59 years of age[1.21(1.02-1.43)]was associated with an increased cataract risk.T2D diagnosed<45 years of age only was associated with an increased risk of glaucoma[HR(95%CI):1.76(1.00-3.12)].HRs(95%CIs)for AMD,cataract,and glaucoma associated with type 1 diabetes(T1D)were 4.12(1.99-8.53),

关键词： Diabetes Age at diagnosis Cataract Glaucoma Age-related macular disease Vision acuity

High spectral efficiency 4-mode 400-km transmission using hybrid probabilistically and geometrically shaped 128QAM

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Science China(Technological Sciences) 2024年第5期67卷 1628-1630页

作者： DING JunJie yu JianJun WANG Chen LONG Jianyu zhu Min ZHANG Jiao Pervasive Communication Research Center Purple Mountain LaboratoriesNanjing 211111China Key Laboratory for Information Science of Electromagnetic Waves(MoE) Fudan UniversityShanghai 200433China

Wavelength division multiplexing(WDM)and space division multiplexing(SDM)based on few-mode fiber(FMF)and multi-core fiber(MCF)have been vigorously developed to increase the transmission capacity of optical communication networks[1–5].However,the mode crosstalk generated in the mode division multiplexing(MDM)system causes the correlation between different mode signals,which seriously damages the transmission ***,an effective multiple-input-multiple-output(MIMO)time domain or frequency domain equalizer should be used to eliminate the crosstalk between different mode signals.

关键词： crosstalk fiber multiplexing

Nanodiamond:a promising metal-free nanoscale material in photocatalysis and electrocatalysis

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Rare Metals 2024年第8期43卷 3501-3552页

作者： Xiao-Wu Gao Zi-Wei Zhao Yang He Sai-Fei Fan Ke-Ran Jiao si-yu Lou Xin-yue Han Peng-Fei Song Rong Cai zhun Hu Zhong-Jie Jiang Yong-Jie Wang Jia-Qi zhu Guangdong Provincial Key Laboratory of Semiconductor Optoelectronic Materials and Intelligent Photonic Systems School of ScienceHarbin Institute of TechnologyShenzhen 518055China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150080China School of Advanced Technology Xi'an Jiaotong-Liverpool UniversitySuzhou215000China Department of Biosciences Rice UniversityHoustonTX 77251USA Institute of Industrial Catalysis School of Chemical Engineering and TechnologyXi'an Jiaotong UniversityXi'an 710049China Guangzhou Key Laboratory for Surface Chemistry of Energy Materials New Energy Research Institute&Guangdong Engineering and Technology Research Center for Surface Chemistry of Energy MaterialsCollege of Environment and EnergySouth China University of TechnologyGuangzhou 510006China

Benefiting from its surface-rich functional groups,eco-friendliness,impressive electrochemical properties,excellent light absorption,structural tunability at the atomic/morphological level,and ultra-high stability under harsh conditions,nanodiamond has emerged as a promising carbon-based non-metallic material in the field of energy conversion such as electrocatalysis and ***,nanodiamond,as a new generation of green catalysts,can overcome the poisoning of catalysts by complex pollutants in advanced oxidation processes,thus effectively removing organic matter from water,which is unparalleled in reducing the cost of water purification and avoiding secondary cross-contamination of water by traditional heavy metal-based ***,we review the research and development of nanodiamonds as major electrocatalysts and photocatalysts for energy conversion and for air/water treatment for environmental *** relevant properties,trimming strategy,mechanistic understanding,and design principles of nanodiamond as a catalyst are described,as well as the challenges and prospects of this emerging field.

关键词： Carbon materials Nanodiamond Electrocatalysis Photocatalysis Energy conversion Pollutant treatment