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In-situ constructed polymer/alloy composite with high ionic conductivity as an artificial solid electrolyte interphase to stabilize lithium metal anode

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Nano Research 2023年第3期16卷 3888-3894页

作者： Ai-Long Chen Yushan Qian shujun zheng Yuyang Chen Yue Ouyang Lulu Mo zheng-Long Xu Yue-E Miao Tianxi Liu State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China Department of Industrial and Systems Engineering The Hong Kong Polytechnic UniversityHong HumKowloonHong Kong 999077China Key Laboratory of Synthetic and Biological Colloids Ministry of EducationSchool of Chemical and Material EngineeringJiangnan UniversityWuxi 214122China

Lithium(Li)metal is regarded as the best anode material for lithium metal batteries(LMBs)due to its high theoretical specific capacity and low redox ***,the notorious dendrites growth and extreme instability of the solid electrolyte interphase(SEI)layers have severely retarded the commercialization process of ***,a double-layered polymer/alloy composite artificial SEI composed of a robust poly(1,3-dioxolane)(PDOL)protective layer,Sn and LiCl nanoparticles,denoted as PDOL@Sn-LiCl,is fabricated by the combination of in-situ substitution and polymerization processes on the surface of Li metal *** lithiophilic Sn-LiCl multiphase can supply plenty of Li-ion transport channels,contributing to the homogeneous nucleation and dense accumulation of Li *** mechanically tough PDOL layer can maintain the stability and compact structure of the inorganic layer in the long-term cycling,and suppress the volume fluctuation and dendrites formation of the Li metal *** a result,the symmetrical cell under the double-layered artificial SEI protection shows excellent cycling stability of 300 h at 5.0 mA·cm^(−2)for 1 mAh·cm^(−2).Notably,the Li||LiFePO_(4)full cell also exhibits enhanced capacity retention of 150.1 mAh·g^(−1)after 600 cycles at 1.0 ***,the protected Li foil can effectively resist the air and water corrosion,signifying the safe operation of Li metal in practical *** present finding proposed a different tactic to achieve safe and dendrite-free Li metal anodes with excellent cycling stability.

关键词： polymer/alloy composite in-situ polymerization artificial solid electrolyte interphase(SEI) double-layered structure lithium metal battery.

分层评价指导治疗对改善亚急性甲状腺炎复发率和甲减发生率的临床研究

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中国煤炭工业医学杂志 2024年第2期27卷 122-127页

作者：郑淑君句卫玲高丽红张娟甄璐代新华郭彩云太原钢铁(集团)有限公司总医院内分泌科山西省太原市030003

目的探究分层评价指导治疗对亚急性甲状腺炎(SAT)患者甲减发生率和复发率、不良反应发生情况的影响。方法随机选取2020年6月—2023年6月该院门诊及病房收治的168例SAT患者,按照SPSS随机数字表,采用1:1:1随机分组,其中局部注射组(n=56... 详细信息

目的探究分层评价指导治疗对亚急性甲状腺炎(SAT)患者甲减发生率和复发率、不良反应发生情况的影响。方法随机选取2020年6月—2023年6月该院门诊及病房收治的168例SAT患者,按照SPSS随机数字表,采用1:1:1随机分组,其中局部注射组(n=56)和口服治疗组(n=56)为对照组,分层评价组(n=56)为治疗组。通过基于临床实践经验自主设计的甲状腺损害程度和复发风险评分表进行分层评价。分析三组患者的一般资料、甲减发生率、复发率、临床疗效(疼痛缓解时间、发热缓解时间、1个月后血沉及甲功恢复情况)及不良反应发生情况。结果三组患者性别、年龄、发病至就诊时间、症状特点、炎症指标、甲功情况间比较,差异无统计学意义(P>0.05)。与局部注射组、口服治疗组比较,分层评价组甲减发生率和复发率均降低(P<0.05);与口服治疗组比较,分层评价组和局部注射组疼痛、发热症状缓解时间缩短(P<0.05);与口服治疗组比较,局部注射组、分层评价组1个月后血沉、甲功恢复正常率情况差异有统计学意义(P<0.05),分层评价组比局部注射组1个月后甲功恢复正常率高,差异有统计学意义(P<0.05);与口服治疗组比较,分层评价组和局部注射组空腹血糖、果糖胺、体重变化等差异有统计学意义(P<0.05)。结论通过分层评价方式选择合适的SAT针对性治疗方案,可令甲减发生率降低,复发率降低,症状缓解快,血沉、甲功恢复效果较好。

关键词：亚急性甲状腺炎复发率甲减发生率分层评价指导治疗

Study on hydrodynamic diffusion law of the swelling particle slurry in karst pipeline

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Particuology 2024年第4期87卷 218-231页

作者： Bingchuan Cheng Haibo Li Guangming Pan Runhuai Deng Yu'an Gong shujun Xu Kun Zhou Zhuo zheng School of Civil Engineering Geotechnical and Structural Engineering Research CenterShandong UniversityJinan250061China The Fourth Prospecting of Shandong Coal Geology Bureau Weifang261000China China Railway 14th Bureau Group Corporation Limited Jinan250101China School of Trafic Engineering Shandong Jianzhu University.Fengming RoadLingang Development ZoneJinan250101China

The swelling particle grouting material has demonstrated remarkable plugging effectiveness in high-pressure and large-flow burst water within karst ***,current research on the rheolog-ical model,flow computation theory,and plugging mechanism of this material is *** conven-tional grouting slurry diffusion process,using the liquid-liquid two-phase flow method,fails to accurately simulate high solubility slurry and particle *** address these limitations,this study established a precise constitutive model to describe the swelling particle slurry diffusion process in dynamic ***,a coupling calculation method was proposed to analyze the spatiotemporal heterogeneity of viscosity during slurry diffusion by considering the migration of slurry and the changes in *** investigate the interaction between particle swelling and flow field changes,a Compu-tational Fluid Dynamics-Discrete Element Method(CFD-DEM)coupling model was developed for the diffusion of swelling particle *** is demonstrated that slurry viscosity increases exponentially within the diffusion front as the particle swelling rate rises,and the drag force exhibits an intriguing behavior of initially increasing and then decreasing as the slurry flows through the ***-more,the CFD-DEM coupling model proved to be more accurate in describing viscosity distribution and diffusion distance compared to the finite element *** primary objective of this paper is to reveal the plugging mechanism and provide theoretical support for the engineering application of the swelling particle grouting material.

关键词： Karst pipeline Swelling particle grouting material Dynamic water diffusion Spatiotemporal variation of viscosity CFD-DEM coupling model

Influence of Component Size on the Corrosion Behavior of Ti6Al4V Alloy Fabricated by Electron Beam Powder Bed Fusion

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Acta Metallurgica Sinica(English Letters) 2024年第1期37卷 159-168页

作者： Hongyu zheng Xin Gai Yun Bai Wentao Hou shujun Li Yulin Hao R.D.K.Misra Rui Yang Institute of Metal Research Chinese Academy of SciencesShenyang110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang110016China Nuclear Power Institute of China Chengdu610213China Department of Metallurgical Materialsand Biomedical EngineeringThe University of Texas at El Paso500WUniversity AvenueEl PasoTX79968USA

The electrochemical behavior of Ti-6Al-4V with 1 mm and 16 mm thickness prepared by electron beam powder bed fusion(EB-PBF)was investigated in phosphate buffered *** results showed that EB-PBF Ti-6Al-4V with a larger component size was more resistant to corrosion compared to the smaller component,because of less acicularαʹphase content and moreβphase *** a non-equilibrium phase in the“high-energy state”,αʹphase has a greater susceptibility to corrode and reduces the corrosion resistance of the material,whileβphase improves corrosion resistance of titanium *** results show that the phase composition has a more significant effect on the corrosion performance than the grain size.

关键词： Electron beam powder bed fusion Ti6Al4V alloy Corrosion resistance Component size Polarisation

A Mean-Field Game for a Forward-Backward Stochastic System With Partial Observation and Common Noise

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IEEE/CAA Journal of Automatica Sinica 2024年第3期11卷 746-759页

作者： Pengyan Huang Guangchen Wang shujun Wang Hua Xiao the School of Control Science and Engineering Shandong University the School of Statistics and Mathematics Shandong University of Finance and Economics IEEE the School of Management Shandong University the School of Mathematics and Statistics Shandong University

This paper considers a linear-quadratic(LQ) meanfield game governed by a forward-backward stochastic system with partial observation and common noise,where a coupling structure enters state equations,cost functionals and observation ***,to reduce the complexity of solving the meanfield game,a limiting control problem is *** virtue of the decomposition approach,an admissible control set is *** a filter technique and dimensional-expansion technique,a decentralized control strategy and a consistency condition system are derived,and the related solvability is also ***,we discuss an approximate Nash equilibrium property of the decentralized control ***,we work out a financial problem with some numerical simulations.

关键词： Decentralized control strategy ϵ-Nash equilibrium forward-backward stochastic system mean-field game partial observation

Compressed Least Squares Algorithm of Continuous-Time Linear Stochastic Regression Model Using Sampling Data

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Journal of Systems Science & Complexity 2024年第4期37卷 1488-1506页

作者： XIE Siyu ZHANG shujun WANG Ziming GAN Die School of Aeronautics and Astronautics University of Electronic Science and Technology of ChinaChengdu 611731China China Academy of Aerospace Science and Innovation Beijing 100176China Zhongguancun Laboratory Beijing 100094China

In this paper,the authors consider a sparse parameter estimation problem in continuoustime linear stochastic regression models using sampling *** on the compressed sensing(CS)method,the authors propose a compressed least squares(LS) algorithm to deal with the challenges of parameter *** each sampling time instant,the proposed compressed LS algorithm first compresses the original high-dimensional regressor using a sensing matrix and obtains a low-dimensional LS estimate for the compressed unknown ***,the original high-dimensional sparse unknown parameter is recovered by a reconstruction *** introducing a compressed excitation assumption and employing stochastic Lyapunov function and martingale estimate methods,the authors establish the performance analysis of the compressed LS algorithm under the condition on the sampling time interval without using independence or stationarity conditions on the system *** last,a simulation example is provided to verify the theoretical results by comparing the standard and the compressed LS algorithms for estimating a high-dimensional sparse unknown parameter.

关键词： Compressed excitation condition compressed sensing continuous-time model least squares linear stochastic regression parameter identification sampling data

Dynamic response of buildings under debris flow impact

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Journal of Mountain Science 2024年第5期21卷 1581-1597页

作者： LIU Huan FAN Xiaoyi TIAN shujun DENG Xin School of Mechanical and Electrical Engineering Southwest Petroleum UniversityChengdu 610500China School of Civil Engineering and Geomatics Southwest Petroleum UniversityChengdu 610500China Housing and Urban-Rural Development Bureau of Mingshan District Ya’an 625100China Engineering Safety Assessment and Protection Research Southwest Petroleum UniversityChengdu 610500China School of Civil Engineering and Architecture Southwest University of Science and TechnologyMianyang 621010China

This study employs the smoothed particle hydrodynamics–finite element method(SPH–FEM) coupling numerical method to investigate the impact of debris flow on reinforced concrete(RC)-frame buildings. The methodology considers the variables of debris flow depth and velocity and introduces the intensity index IDV(IDV = DV) to evaluate three different levels of debris flow impact intensity. The primary focus of this study is to investigate the dynamic response and failure mechanism of RC-frame buildings under debris flow impact, including structural failure patterns, impact force and column displacement. The results show that under a highintensity impact, a gradual collapse process of the RCframe building can be observed, and the damage mode of the frame column reflects shear failure or plastic hinge failure mechanism. First, the longitudinal infill walls are damaged owing to their low out-of-plane flexural capacity;the critical failure intensity index IDV value is approximately 7.5 m2/s. The structure cannot withstand debris flows with an intensity index IDV greater than 16 m2/s, and it is recommended that the peak impact force should not exceed 2100 k N. The impact damage ability of debris flow on buildings mostly originates from the impact force of the frontal debris flow, with the impact force of the debris flow body being approximately 42% lower than that of the debris flow head. Finally, a five-level classification system for evaluating the damage status of buildings is proposed based on the numerical simulation and investigation results of the disaster site.

关键词： SPH–FEM method Debris flow Buildings The intensity index Dynamic response

Effects of Interaction between Axial and Radial Secondary Air and Reductive Intensity in Reduction Region on Combustion Characteristics and NO_(x) Emission of Coal Preheated by a Self-Preheating Burner

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Journal of Thermal Science 2024年第1期33卷 249-267页

作者： SU Kun DING Hongliang OUYANG Ziqu ZHANG Jinyang ZHU shujun Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China School of Energy and Power Engineering Jiangsu UniversityZhenjiang 212013China

The study focused on the effects of the interaction between axial and radial secondary air and the reductive intensity in reduction region on combustion characteristics and NO_(x) emission in a 30 kW preheating combustion *** results revealed that the interaction and reductive intensity influenced the combustion in the down-fired combustor(DFC) and NO_(x) emission *** the temperature distribution,the interaction caused the position of the main combustion region to shift down as R_(2-12)(ratio of axial secondary air flow to radial secondary air flow) decreased or λ_(2)(total secondary air ratio) increased,and there was the interplay between both of their *** R_(3-12)(ratio of first-staged tertiary air flow to second-staged tertiary air flow)increased,the decrease in the reductive intensity also caused the above phenomenon,and the peak temperature increased in this *** the NO_(x) emission,the interaction affected the NO_(x) reduction adversely when λ_(2) or R_(2-12) was higher,and the range of this effect was larger,so that the NO_x emission increased obviously as they *** decrease in the reductive intensity caused the NO_(x) emission increased under the homogeneous reduction mechanism,while was unchanged at a high level under the heterogeneous reduction *** the combustion efficiency,the interaction improved the combustion efficiency as λ_(2) increased when R_(2-12) was lower,while reduced it as λ_(2) increased excessively when R_(2-12) was *** proper decrease in the reductive intensity caused the combustion efficiency increased obviously,while was hardly improved further when the intensity decreased *** this study,the lowest NO_(x) emission was only 41.75 mg/m^(3) without sacrificing the combustion efficiency by optimizing the interaction and reductive intensity.

关键词： self-preheating interaction of axial and radial secondary air reductive intensity combustion characteristic NO_(x)emission

Low-rank spectral estimation algorithm of learning Markov model

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Frontiers of Mathematics in China 2024年第3期19卷 137-155页

作者： Yongye ZHAO shujun BI Department of Basic Courses Guangzhou Maritime UniversityGuangzhou 510725China Department of Mathematics South China University of TechnologyGuangzhou 510640China

This paper proposes a low-rank spectral estimation algorithm of learning Markov ***,an approximate projection algorithm for the rank-constrained frequency matrix set is proposed,and thereafter its local Lipschitzian error bound ***,we propose a low-rank spectral estimation algorithm for estimating the state transition frequency matrix and the probability matrix of Markov model by applying the approximate projection algorithm to correct the maximum likelihood estimation of the frequency matrix,and prove that there is only a multiplying constant difference in estimation errors between the low-rank spectral estimation and the maximum likelihood estimation under appropriate ***,numerical comparisons with the prevailing maximum likelihood estimation,spectral estimation,and rank-constrained maxi-mum likelihood estimation show that the low-rank spectral estimation algorithm is effective.

关键词： Markov model low-rank spectral estimation error bound approximate projection