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Journal of Environmental Sciences 2024年第2期136卷 248-260页

作者： Ruipeng Wang Xiaoqi Wang shuiyuan cheng Jiaxian Zhu Xinyu Zhang Long cheng Kai Wang Key Laboratory of Beijing on Regional Air Pollution Control Faculty of Environment and LifeBeijing University of TechnologyBeijing 100124China

An evidence-based control strategy for emission reduction of VOC sources can effectively solve the regional PM2.5and O3compound pollution in China.We estimated the anthropogenic VOC emission inventory in China in 2018 and established a source profile database containing 129 sources based on localized detection and the latest research results.Then,the distribution of the ozone formation potential(OFP)and secondary organic aerosol formation potential(SOAFP)for emission sources was analyzed.Moreover,priority control routes for VOC emission sources were proposed for different periods.Anthropogenic VOC emissions in China reached 27,211.8 Gg in 2018,and small passenger cars,industrial protective coatings,biomass burning,heavy trucks,printing,asphalt paving,oil storage and transportation,coking,and oil refining were the main contributors.Industrial protective coatings,small passenger cars,and biomass burning all contributed significantly to OFP and SOAFP.Priority in emission reduction control should be given to industrial protective coatings,small passenger cars,heavy trucks,coking,printing,asphalt paving,chemical fibers,and basic organic chemical sources over the medium and long term in China.In addition,the priority control route for VOC emission sources should be adjusted according to the variations in VOC emission characteristics and regional differences,so as to obtain the maximum environmental benefits.

关键词： Volatile organic compounds Anthropogenic emission inventory Reactivity Emission projection Priority control route

A new scheme of PM_(2.5)and O_(3) control strategies with the integration of SOM,GA and WRF-CAMx

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Journal of Environmental Sciences 2024年第4期138卷 249-265页

作者： Wenjiao Duan Xiaoqi Wang shuiyuan cheng Ruipeng Wang Key Laboratory of Beijing on Regional Air Pollution Control Faculty of Environment and LifeBeijing University of TechnologyBeijing 100124China

Previous air pollution control strategies didn’t pay enough attention to regional collaboration and the spatial response sensitivities,resulting in limited control effects in China.This study proposed an effective PM_(2.5)and O_(3) control strategy scheme with the integration of Self-Organizing Map(SOM),Genetic Algorithm(GA)and WRF-CAMx,emphasizing regional collaborative control and the strengthening of control in sensitive areas.This scheme embodies the idea of hierarchical management and spatial-temporally differentiated management,with SOM identifying the collaborative subregions,GA providing the optimized subregion-level priority of precursor emission reductions,and WRF-CAMx providing response sensitivities for grid-level priority of precursor emission reductions.With Beijing-Tianjin-Hebei and the surrounding area(BTHSA,“2+26”cities)as the case study area,the optimized strategy required that regions along Taihang Mountains strengthen the emission reductions of all precursors in PM_(2.5)-dominant seasons,and strengthen VOCs reductions but moderate NOx reductions in O_(3)-dominant season.The spatiotemporally differentiated control strategy,without additional emission reduction burdens than the 14th Five-Year Plan proposed,reduced the average annual PM_(2.5)and MDA8 O_(3) concentrations in 28 cities by 3.2%-8.2% and 3.9%-9.7% respectively in comparison with non-differential control strategies,with the most prominent optimization effects occurring in the heavily polluted seasons(6.9%-18.0%for PM_(2.5)and 3.3%-14.2% for MDA8 O_(3),respectively).This study proposed an effective scheme for the collaborative control of PM_(2.5)and O_(3) in BTHSA,and shows important methodological implications for other regions suffering from similar air quality problems.

关键词： PM_(2.5)and O_(3)control SOM GA WRF-CAMx Bionic algorithm Machine learning

Aerosol-radiation interaction and its variation in North China within 2015–2019 period under continuous PM_(2.5)improvements

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Journal of Environmental Sciences 2024年第2期136卷 81-94页

作者： Zhe Lv Xiaoqi Wang Wei Wei Huahua Bai Xiaoyu Liu Guohao Li shuiyuan cheng Department of Environmental Science and Engineering Beijing University of TechnologyBeijing 100124China Key Laboratory of Beijing on Regional Air Pollution Control Beijing 100124China Beijing Municipal Research Institute of Eco-Environmental Protection Beijing 100037China Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Pollution Control and Application Beijing 100037China

A study was conducted on aerosol-radiation interactions over six cities in this region within the 2015–2019 period.WRF-Chem simulations on 2017 showed that based on the six-city average,the aerosol load(PM_(2.5)concentrations)of 121.9,49.6,43.3,and 66.3μg/m^(3)in January,April,July,and October,mainly lowered the level of downward shortwave radiation by 38.9,24.0,59.1,and 24.4 W/m~2and reduced the boundary layer height by 79.9,40.8,87.4,and 31.0 m,via scattering and absorbing solar radiation.The sensitivity of meteorological changes to identical aerosol loads varied in the order July>January>October and April.Then,the cooling and stabilizing effects of aerosols further led to increases in PM_(2.5),by23.0,3.4,4.6,and 7.3μg/m^(3)respectively in the four months.The sensitivity of the effect of aerosols on PM_(2.5)was greatest in January rather than in July,contrary to the effect on meteorology.Moreover,a negative linear relation was observed between daily BLH reductions and aerosol loads in fall and winter,and between PM_(2.5)increases and aerosol loads in all seasons.With the PM_(2.5)pollution improvements in this region,the aerosol radiative forcing was effectively reduced.This should result in daily BLH increases of 10–24 m in fall and winter,and the estimates in Beijing agreed well with the corresponding results based on AMDAR data.Additionally,the reduction in aerosol radiation effects brought about daily PM_(2.5)decreases of 1.6-2.8μg/m^(3),accounting for 7.0%–17.7%in PM_(2.5)improvements.

关键词： Radiative forcing Aerosol PM_(2.5) Boundary layer height(BLH) North China

Insights into multidimensional transport flux from vertical observation and numerical simulation in two cities in North China

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Journal of Environmental Sciences 2023年第3期125卷 831-842页

作者： Zhida Zhang Xiaoqi Wang shuiyuan cheng Guiqian Tang Yibin Fu Key Laboratory of Beijing on Regional Air Pollution Control Beijing University of TechnologyBeijing 100124China State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry(LAPC) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Key Laboratory of Environmental Optics and Technology Anhui Institute of Optics and Fine MechanicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China

This study represents the first quantitative evaluation of pollution transport budget within the boundary layer of typical cities in the Beijing-Tianjin-Hebei (BTH) region from the perspective of horizontal and vertical exchanges and further discusses the impact of the atmospheric boundary layer (ABL)-free troposphere (FT) exchange on concentration of fine particulate matter (PM_(2.5)) within the ABL during heavy pollution.From the perspective of the transport flux balance relationship,differences in pollution transport characteristics between the two cities is mainly reflected in the ABL-FT exchange effect.The FT mainly flowed into the ABL in BJ,while in SJZ,the outflow from the ABL to the FT was more intense.Combined with an analysis of vertical wind profile distribution,BJ was found to be more susceptible to the influence of northwest cold high prevailing in winter,while sinking of strong cold air allowed the FT flowing into the ABL influence the vertical exchange over BJ.In addition,we selected a typical pollution event for targeted analysis to understand mechanistic details of the influence of ABL-FT exchange on the pollution event.These results showed that ABL-FT interaction played an important role in PM_(2.5)concentration within the ABL during heavy pollution.Especially in the early stage of heavy pollution,FT transport contributed as much as 82.74% of PM_(2.5)within the ABL.These findings are significant for improving our understanding of pollution transport characteristics within the boundary layer and the effect of ABL-FT exchange on air quality.

关键词： Transport flux Horizontal transport Vertical exchange Atmospheric boundary layer Free troposphere Pollutant budget relationship

Exploring drivers of the aggravated surface O_(3) over North China Plain in summer of 2015–2019: Aerosols, precursors, and meteorology

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Journal of Environmental Sciences 2023年第5期127卷 453-464页

作者： Shengju Ou Wei Wei shuiyuan cheng Bin Cai Key Laboratory of Beijing on Regional Air Pollution Control Faculty of Environment and LifeBeijing University of TechnologyBeijing 100124China

Continuous aggravated surface O_(3) over North China Plain(NCP)has attracted widely public concern.Herein,we evaluated the effects of changes in aerosols,precursor emissions,and meteorology on O_(3) in summer(June)of 2015–2019 over NCP via 8 scenarios with WRF-Chem model.The simulated mean MDA8 O_(3) in urban areas of 13 major cities in NCP increased by 17.1%∼34.8%,which matched well with the observations(10.8%∼33.1%).Meanwhile,the model could faithfully reproduce the changes in aerosol loads,precursors,and meteorological conditions.A relatively-even O_(3) increase(+1.2%∼+3.9%for 24-h O_(3) and+1.0%∼+3.8%for MDA8 O_(3))was induced by PM_(2.5) dropping,which was consistent with the geographic distribution of regional PM_(2.5) reduction.Meanwhile,the NO_(2) reduction coupled with a nearconstant VOCs led to the elevated VOCs/NOx ratios,and then caused O_(3) rising in the areas under VOCs-limited regimes.Therein,the pronounced increases occurred in Handan,Xingtai,Shijiazhuang,Tangshan,and Langfang(+10.7%∼+13.6%for 24-h O_(3) and+10.2%∼+12.2%forMDA8 O_(3));while the increases in other citieswere 5.7%∼10.5%for 24-h O_(3) and 4.9%∼9.2%for MDA8 O_(3).Besides,the meteorological fluctuations brought about the more noticeable O_(3) increases in northern parts(+12.5%∼+13.5%for 24-h O_(3) and+11.2%∼+12.4%for MDA8 O_(3))than those in southern and central parts(+3.2%∼+9.3%for 24-h O_(3) and+3.7%∼+8.8%for MDA8 O_(3)).The sum of the impacts of the three drivers reached 16.7%∼21.9%,which were comparable to the changes of the observed O_(3).Therefore,exploring reasonable emissionsreduction strategies is essential for the ozone pollution mitigation over this region.

关键词： Surface ozone Driving force Aerosols Precursors Meteorology WRF-Chem model

A review of the technology and applications of methods for evaluating the transport of air pollutants

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Journal of Environmental Sciences 2023年第1期123卷 341-349页

作者： Xiaoqi Wang shuiyuan cheng Ying Zhou Hanyu Zhang Panbo Guan Zhida Zhang Weichao Bai Wujun Dai Key Laboratory of Beijing on Regional Air Pollution Control Beijing University of TechnologyBeijing 100124China School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China State Environmental Protection Key Laboratory of Food Chain Pollution Control Beijing Technology and Business UniversityBeijing 100048China

A variety of methods based on air quality models,including tracer methods,the bruteforce method(BFM),decoupled direct method(DDM),high-order decoupled direct method(HDDM),response surface models(RSMs)and so on forth,have been widely used to study the transport of air pollutants.These methods have good applicability for the transport of air pollutants with simple formation mechanisms.However,differences in research conclusions on secondary pollutants with obvious nonlinear characteristics have been reported.For example,the tracer method is suitable for the study of simpli?ed scenarios,while HDDM and RSMs are more suitable for the study for nonlinear pollutants.Multiple observation techniques,including conventional air pollutant observation,lidar observation,air sounding balloons,vehicle-mounted and ship-borne technology,aerial surveys,and remote sensing observations,have been utilized to investigate air pollutant transport characteristics with time resolution as high as 1 sec.In addition,based on a multi-regional input-output model combined with emission inventories,the transfer of air pollutant emissions can be evaluated and applied to study the air pollutant transport characteristics.Observational technologies have advantages in temporal resolution and accuracy,while modeling technologies are more?exible in spatial resolution and research plan setting.In order to accurately quantify the transport characteristics of pollutants,it is necessary to develop a research method for interactive veri?cation of observation and simulation.Quantitative evaluation of the transport of air pollutants from different angles can provide a scienti?c basis for regional joint prevention and control.

关键词： Air pollutant transport Simulation technology Observation technology Transport matrix Transport?ux

Selenium-enriched Cardamine violifolia protects against sepsis-induced intestinal injury by regulating mitochondrial fusion in weaned pigs

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中国科学:生命科学英文版 2023年第9期66卷 2099-2111页

作者： Dan Wang Yanling Kuang Qingqing Lv Wenshuai Xie Xiao Xu Huiling Zhu Yue Zhang Xin Cong shuiyuan cheng Yulan Liu Hubei Key Laboratory of Animal Nutrition and Feed Science Wuhan Polytechnic UniversityWuhan 430023China Enshi Se-Run Material Engineering Technology Co. Ltd.Enshi 445000China National R&D Center for Se-rich Agricultural Products Processing School of Modern Industry for Selenium Science and EngineeringWuhan Polytechnic UniversityWuhan 430023China

Sepsis is a life-threatening organ dysfunction caused by the dysregulated response of the host to an infection, and treatments are limited. Recently, a novel selenium source, selenium-enriched Cardamine violifolia(SEC) has attracted much attention due to its anti-inflammatory and antioxidant properties, but little is known about its role in the treatment of sepsis. Here, we found that SEC alleviated LPS-induced intestinal damage, as indicated by improved intestinal morphology, and increased disaccharidase activity and tight junction protein expression. Moreover, SEC ameliorated the LPS-induced release of pro-inflammatory cytokines, as indicated by decreased IL-6 level in the plasma and jejunum. Moreover, SEC improved intestinal antioxidant functions by regulating oxidative stress indicators and selenoproteins. In vitro, TNF-α-challenged IPEC-1 cells were examined and showed that selenium-enriched peptides, which are the main functional components extracted from Cardamine violifolia(CSP), increased cell viability, decreased lactate dehydrogenase activity and improved cell barrier function. Mechanistically, SEC ameliorated LPS/TNF-α-induced perturbations in mitochondrial dynamics in the jejunum and IPEC-1 cells. Moreover, CSPmediated cell barrier function is primarily dependent on the mitochondrial fusion protein MFN2 but not MFN1. Taken together,these results indicate that SEC mitigates sepsis-induced intestinal injury, which is associated with modulating mitochondrial fusion.

关键词： intestine MFN2 mitochondrial fusion piglets selenium sepsis

Temporal and spatial characteristics of PM_(2.5) transport fluxes of typical inland and coastal cities in China

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Journal of Environmental Sciences 2021年第5期33卷 229-245页

作者： Panbo Guan Xiaoqi Wicmg shuiyuan cheng Hanyu Zhang Key Laboratory of Beijing on Regional Air Pollution Control Beijing University of TechnologyBeijing100124China

Local pollution and the cross-boundary transmission of pollutants between cities have an inevitable impact on the atmosphere. Quantitative assessments of the contribution of transport to pollution in inland and coastal cities are necessary for the implementation of practical, regional, and joint emission control strategies. In this study, the Comprehensive Air Quality Model(CAMx), together with the Weather Research and Forecasting model(WRF), was used to simulate the contributions to pollution of different cities in 2016. The monthly inflow, outflow, and net flux from the ground to the extended layers served as the three main indicators for the analysis of the interactions of PM_(2.5) transport between adjacent cities. Between inland and coastal cities, the magnitude of inflow and outflow are larger in the former than in the latter. The inflow flux in the inland cities(Beijing and Shijiazhuang) was 10.6 and 10.7 kt/day, respectively, while that in the coastal cities(Tianjin, Shanghai, Hefei, Nanjing, and Hangzhou) was 9.1, 3.3, 5.8, 4.4, and 3.7 kt/day, respectively. In terms of variation over the year, the strongest inflow in the BTH region occurred in April, followed by October, July, and January, while that in the coastal cities in YRD occurred in January, followed by October, April, and July. Therefore, based on the flux intensity calculations and the transport flux pathways, effective joint control measures can be provided with scientific support, and a better understanding of the evolutionary mechanism among inland and coastal cities can be acquired.

关键词： PM_(2.5)flux modeling system regional transport inland cities coastal cities

A monitoring-modeling approach to SO_4^(2-) and NO_3^- secondary conversion ratio estimation during haze periods in Beijing, China

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Journal of Environmental Sciences 2019年第4期31卷 293-302页

作者： Xiaoqi Wang Wei Wei shuiyuan cheng Chong Zhang Wenjiao Duan Key Laboratory of Beijing on Regional Air Pollution Control Beijing University of Technology Collaborative Innovation Center of Beijing City Traffic Beijing University of Technology

SO_4^(2-) and NO_3^- are important chemical components of fine particulate matter(PM_(2.5)),especially during haze periods.This study selected two haze episodes in Beijing,China with similar meteorological conditions.A monitoring-modeling approach was developed to estimate the secondary conversion ratios of sulfur and nitrogen based on monitored and simulated concentrations.Measurements showed that in Episode 1(24th–25th October,2014),the concentrations(proportions)of SO_4^(2-) and NO_3^- reached 35.1μg/m^3(14.9%) and 55.0μg/m^3(22.9%),while they reached 14.4μg/m^3(9.3%) and 59.1μg/m^3(38.1%)in Episode 2(26th–27th October,2017).A modeling system was applied to apportion Beijing's SO_4^(2-) and NO_3^- in primary and secondary SO_4^(2-)/NO_3^- emitted from local and regional sources.Thus,secondary conversion contributions considering the local and regional level were defined.The former primarily focused on Beijing atmospheric oxidation ability and the latter mainly considered the existence form of Beijing SO_4^(2-)/NO_3^- under the regional transport impacts.Finally,secondary oxidation ratios were estimated through combining secondary conversion contribution coefficients for simulated and monitored concentrations.At regional level,sulfur oxidation ratios in polluted(clean)days during two sampling periods were0.57–0.72(0.07–0.52)and 0.74–0.80(0.08–0.61),nitrogen oxidation ratios were 0.20–0.29(0.05–0.15)and 0.34–0.38(0.02–0.29),indicating that atmospheric oxidation was enhanced when considering regional transport through 2014–2017.At the local level,sulfur oxidation ratios were 0.66–0.71(0.04–0.48)in haze(clean)days,while nitrogen oxidation ratios were0.16–0.29(0.02–0.16).The atmospheric oxidation ability markedly increased in PM_(2.5)pollution days,but changed only slightly between the two periods.

关键词： Haze periods SO42- and NO3- Secondary conversion Secondary oxidation ratio

On-board measurements of gaseous pollutant emission characteristics under real driving conditions from light-duty diesel vehicles in Chinese cities

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Journal of Environmental Sciences 2016年第8期28卷 28-37页

作者： Gang Wang shuiyuan cheng Jianlei Lang Song Li Liang Tian Key Laboratory of Beijing on Regional Air Pollution Control Beijing University of Technology Beijing 100124 China. Collaborative Innovation Center of Electric Vehicles Beijing 100081 China

A total of 15 light-duty diesel vehicles（LDDVs） were tested with the goal of understanding the emission factors of real-world vehicles by conducting on-board emission measurements. The emission characteristics of hydrocarbons（HC） and nitrogen oxides（NOx） at different speeds, chemical species profiles and ozone formation potential（OFP） of volatile organic compounds（VOCs） emitted from diesel vehicles with different emission standards were analyzed. The results demonstrated that emission reductions of HC and NOxhad been achieved as the control technology became more rigorous from Stage I to Stage IV. It was also found that the HC and NOxemissions and percentage of O2 dropped with the increase of speed, while the percentage of CO2 increased. The abundance of alkanes was significantly higher in diesel vehicle emissions, approximately accounting for 41.1%–45.2%, followed by aromatics and alkenes. The most abundant species were propene,ethane, n-decane, n-undecane, and n-dodecane. The maximum incremental reactivity（MIR）method was adopted to evaluate the contributions of individual VOCs to OFP. The results indicated that the largest contributors to O3 production were alkenes and aromatics, which accounted for 87.7%–91.5%. Propene, ethene, 1,2,4-trimethylbenzene, 1-butene, and1,2,3-trimethylbenzene were the top five VOC species based on their OFP, and accounted for 54.0%-64.8% of the total OFP. The threshold dilution factor was applied to analyze the possibility of VOC stench pollution. The majority of stench components emitted from vehicle exhaust were aromatics, especially p-diethylbenzene, propylbenzene, m-ethyltoluene, and p-ethyltoluene.

关键词： Light-duty diesel vehicles Emission factor Hydrocarbon Nitrogen oxide Volatile organic compounds Ozone formation potential