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Multifunctional interfacial molecular bridge enabled by an aggregation-induced emission strategy for enhancing efficiency and UV stability of perovskite solar cells

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Journal of Energy Chemistry 2024年第8期95卷 588-595,I0013页

作者： shuhang bian Yuqi Wang Fancong Zeng Zhongqi Liu Bin Liu Yanjie Wu Long Shao Yongzhi Shao Huan Zhang Shuainan Liu Jin Liang Xue Bai Lin Xu Donglei Zhou Biao Dong Hongwei Song State Key Laboratory on Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012JilinChina College of Science Shanghai UniversityShanghai 200444China

The interface defects between the electron transport layer(ETL)and the perovskite layer,as well as the low ultraviolet(UV)light utilization rate of the perovskite absorption layer,pose significant challenges for the commercialization of perovskite solar cells(PSCs).To address this issue,this paper proposes an innovative multifunctional interface modulation strategy by introducing aggregation-induced emission(AIE)molecule 5-[4-[1,2,2-tri[4-(3,5-dicarboxyphenyl)phenyl]ethylene]phenyl]benzene-1,3-dicarboxylic acid(H_(8)ETTB)at the SnO_(2)ETL/perovskite ***,the interaction of H_(8)ETTB with the SnO_(2)surface,facilitated by its carboxyl groups,is effective in passivating surface defects caused by noncoord inated Sn and O *** interaction enhances the conductivity of the SnO_(2)film and adjusts energy levels,leading to enhanced charge carrier ***,H_(8)ETTB can passivate noncoord inated Pb^(2+)ions at the perovskite interface,promoting perovskite crystallization and reducing the interface energy barrier,resulting in a perovskite film with low defects and high crystalline *** importantly,the H_(8)ETTB molecule,can convert UV light into light absorbable by the perovskite,thereby reducing damage caused by UV light and improving the device's utilization of ***,the champion PSC based on SnO_(2)-H_(8)ETTB achieves an impressing efficiency of 23.32%and significantly improved photostability compared with the control device after continuous exposure to intense UV *** addition,the Cs_(0.05)(FA_(0.95)MA_(0.05))_(0.95)Pb(I_(0.95)Br_(0.05))_(3)based device can achieve maximum efficiency of 24.01%,demonstrating the effectiveness and universality of this ***,this innovative interface bridging strategy effectively tackles interface defects and low UV light utilization in PSCs,presenting a promising approach for achieving highly efficient and stable PSCs.

关键词： Perovskite solar cells Aggregation-induced emission Defect passivation Efficiency UV stability

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Trustworthy semi-supervised anomaly detection for online‐tooffline logistics business in merchant identification

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CAAI Transactions on Intelligence Technology 2024年第3期9卷 544-556页

作者： Yong Li shuhang Wang Shijie Xu Jiao Yin Business School China University of Political Science and LawBeijingChina JD Logistics BeijingChina Southeast University NanjingChina Institute for Sustainable Industries and Liveable Cities Victoria UniversityMelbourneVictoriaAustralia

The rise of online-to-offline(O2O)e-commerce business has brought tremendous opportunities to the logistics *** the online-to-offline logistics business,it is essential to detect anomaly merchants with fraudulent shipping behaviours,such as sending other merchants'packages for profit with their low *** can help reduce the financial losses of platforms and ensure a healthy *** anomaly detection studies have mainly focused on online fraud behaviour detection,such as fraudulent purchase and comment behaviours in ***,these methods are not suitable for anomaly merchant detection in logistics due to the more complex online and offline operation of package-sending behaviours and the interpretable requirements of offline deployment in ***,a semi-supervised multiview fusion-based Anomaly Detection framework in online-to-offline logistics is proposed,which consists of a basic version SemiDet and an attention-enhanced multi-view fusion *** SemiDet,pair-wise data augmentation is first conducted to promote model robustness and address the challenge of limited labelled anomaly ***,SemiDet calculates the anomaly scoring of each merchant with an auto-encoder *** the multi-relationships among logistics merchants,a multi-view attention fusion-based anomaly detection network is further designed to capture merchants'mutual influences and improve the anomaly merchant detection performance.A post-hoc perturbation-based interpretation model is designed to output the importance of different views and ensure the trustworthiness of end-to-end anomaly *** framework based on an eight-month real-world dataset collected from one of the largest logistics platforms in China is evaluated,involving 6128 merchants and 16 million historical order consignor records in *** results show that the proposed model outperforms other baselines in both AUC-ROC and AUC-PR metrics.

关键词： artificial intelligence techniques data fusion deep learning

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A"messenger zone hypothesis"based on the visual three-dimensional spatial distribution of motoneurons innervating deep limb muscles

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Neural Regeneration Research 2024年第7期19卷 1559-1567页

作者： Chen Huang Shen Wang Jin Deng Xinyi Gu shuhang Guo Xiaofeng Yin MoE Key Laboratory for Trauma Treatment and Nerve Regeneration Peking UniversityBeijingChina Department of Orthopedics and Trauma Peking University People’s HospitalBeijingChina

Coordinated contraction of skeletal muscles relies on selective connections between the muscles and multiple classes of the spinal motoneuro *** r,current research on the spatial location of the spinal motoneurons innervating differe nt muscles is *** this study,we investigated the spatial distribution and relative position of different motoneurons that control the deep muscles of the mouse hindlimbs,which were innervated by the obturator nerve,femoral nerve,inferior gluteal nerve,deep pe roneal nerve,and tibial *** were visualized by combining a multiplex retrograde tracking technique compatible with three-dimensional imaging of solvent-cleared o rgans(3DISCO)and 3-D imaging technology based on lightsheet fluorescence microscopy(LSFM).Additionally,we propose the hypothesis that"messenger zones"exist as interlaced areas between the motoneuron pools that dominate the synergistic or antagonist muscle *** hypothesize that these interlaced neurons may participate in muscle coordination as messenger *** revealed the precise mutual positional relationships among the many motoneurons that innervate different deep muscles of the *** only do these findings update and supplement our knowledge regarding the overall spatial layout of spinal motoneurons that control mouse limb muscles,but they also provide insights into the mechanisms through which muscle activity is coordinated and the architecture of motor circuits.

关键词： 3-D imaging motoneurons multiple retrograde tracing muscle coordination skeletal muscle spatial distribution optical tissue clearing

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Radar Signal Intra-Pulse Modulation Recognition Based on Deep Residual Network

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Journal of Beijing Institute of Technology 2024年第2期33卷 155-162页

作者： Fuyuan Xu Guangqing Shao Jiazhan Lu Zhiyin Wang Zhipeng Wu shuhang Xia No.8511 Research Institute of China Aerospace Science&Industry Corp(CASIC) Nanjing 210007China

In view of low recognition rate of complex radar intra-pulse modulation signal type by traditional methods under low signal-to-noise ratio(SNR),the paper proposes an automatic recog-nition method of complex radar intra-pulse modulation signal type based on deep residual *** basic principle of the recognition method is to obtain the transformation relationship between the time and frequency of complex radar intra-pulse modulation signal through short-time Fourier transform(STFT),and then design an appropriate deep residual network to extract the features of the time-frequency map and complete a variety of complex intra-pulse modulation signal type *** addition,in order to improve the generalization ability of the proposed method,label smoothing and L2 regularization are *** simulation results show that the proposed method has a recognition accuracy of more than 95%for complex radar intra-pulse modulation sig-nal types under low SNR(2 dB).

关键词： intra-pulse modulation low signal-to-noise deep residual network automatic recognition

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Comprehensive characterization of cell disulfidptosis in human cancers:An integrated pan-cancer analysis

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Genes & Diseases 2024年第4期11卷 5-8页

作者： Guo Zhao Yale Jiang Yuning Wang shuhang Wang Ning Li Clinical Trial Center National Cancer Center/National Clinical Research Center for Cancer/Cancer HospitalChinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100021China

Excessive accumulation of disulfide molecules,like cystine,can induce disulfide stress and high toxicity in cells,but the reduced form of nicotinamide adenine dinucleotide phosphate can reverse this process and mitiga... 详细信息

关键词： disulfide cancer characterization

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Control Techniques of Chinese Chestnut Yellow Crinkle

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Plant Diseases and Pests 2024年第3期15卷 12-13页

作者： shuhang ZHANG Yongbin XIONG Liying FAN Changli Institute of Pomology Hebei Academy of Agriculture and Forestry SciencesChangli 066600China Hebei Academy of Agriculture and Forestry Sciences Shijiazhuang 050031China

This paper initially delineates the symptoms,characteristics,and hazards associated with Chinese chestnut yellow crinkle,as well as the transmission and infection pathways of the ***,it proposes the prevention and control strategies of the disease,including rigorous investigation and monitoring of the disease,enhanced monitoring of seedlings and scions,and integrated disease management techniques to promote the tree s health and *** strategies serve to inform the prevention and control of Chinese chestnut yellow crinkle in production.

关键词： Chestnut Chinese chestnut yellow crinkle Symptom Prevention and control

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Nanoparticle drug delivery system for the treatment of brain tumors:Breaching the blood–brain barrier

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Acta Pharmaceutica Sinica B 2024年第6期14卷 2786-2789页

作者： Qiyu Tang Guo Zhao Hong Fang Yale Jiang Peiwen Ma Jiawei Zhoua Dongyan Liu Shujun Xing Gaoquan Li Nian Liu Huiyu Chen shuhang Wang Ning Li Clinical Trial Center National Cancer Center/National Clinical Research Center for Cancer/Cancer HospitalChinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100021China Chongqing Upgra Biotechnology Co. Ltd.Chongqing 401331China

To the Editor:Malignant brain tumors represent a substantial morbidity and mortality burden globally,with 308,102 new cases and 251,329 cancer-related deaths in *** tumors encompass primary tumors originating in the brain and brain metastases(BM)that have been spread from cancer lesions of other ***,BM are the most prevalent intracranial malignant tumor affecting approximately 20%-40%of cancer patients2.

关键词： Nanoparticle Drug delivery system Blood-brain barrier Tumor Glioma

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Numerical analysis for the free-boundary current reversal equilibrium in the AC plasma current operation in a tokamak

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Plasma Science and Technology 2024年第2期26卷 22-30页

作者：胡业民王柳青白书航于治夏天阳 Institute of Plasma Physics Chinese Academy of SciencesHefei 230031People's Republic of China University of Science and Technology of China Hefei 230026People's Republic of China Institutes of Physical Science and Information Technology Anhui UniversityHefei 230601People's Republic of China

In recent decades, tokamak discharges with zero total toroidal current have been reported in tokamak experiments, and this is one of the key problems in alternating current(AC) *** efficient free-boundary equilibrium code is developed to investigate such advanced tokamak discharges with current reversal equilibrium configuration. The calculation results show that the reversal current equilibrium can maintain finite pressure and also has considerable effects on the position of the X-point and the magnetic separatrix shape, and hence also on the position of the strike point on the divertor plates, which is extremely useful for magnetic design, MHD stability analysis, and experimental data analysis etc. for the AC plasma current operation on tokamaks.

关键词： current reversal equilibrium AC operation free-boundary equilibrium tokamak

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盐溶液饱和岩土的本构理论及在黏土中的应用

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岩土工程学报 2024年第2期46卷 223-234页

作者：胡亚元袁书行浙江大学滨海和城市岩土工程研究中心浙江杭州310058

盐溶液中离子的化学活性会改变饱和岩土的力学性质,诱发其工程性能出现劣化甚至失效等岩土工程问题。为了研究化学活性对饱和岩土水力与变形特性的影响,基于混合物理论与热力学溶液理论,建立了盐溶液饱和岩土材料的本构理论框架。与以... 详细信息

盐溶液中离子的化学活性会改变饱和岩土的力学性质,诱发其工程性能出现劣化甚至失效等岩土工程问题。为了研究化学活性对饱和岩土水力与变形特性的影响,基于混合物理论与热力学溶液理论,建立了盐溶液饱和岩土材料的本构理论框架。与以往研究不同,该理论将固相应变分解为孔隙率变化引起的骨架应变、固相材料变形引起的基质应变以及化学反应等物质交换引起的质量交换应变,用以凸显孔隙率在水-力-化学多场耦合机制中的关键作用;采用溶质的现时质量分数作为化学状态变量来反映化学活性的影响;利用自由能和耗散势分别建立弹性和塑性本构关系。根据该理论框架建立了NaCl溶液饱和黏土的固相、流相本构关系以及溶质的渗流-扩散方程,并得到了已有试验数据的验证,表明该框架可以指导盐溶液饱和岩土的本构建模工作。

关键词：混合物理论盐溶液饱和岩土材料化学活性本构理论等向压缩

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基于主线密度预测的快速路入口匝道控制方法

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交通运输系统工程与信息 2024年第4期24卷 94-104,126页

作者：邓明君李书行李响张兵薛运强华东交通大学交通运输工程学院南昌330013

针对快速路入口匝道区域拥堵问题,本文提出一种基于交通密度预测的入口匝道控制方法。通过分析快速路匝道区域的交通特性,定义交通流缓行状态,利用经典宏观交通流模型对快速路主线的历史密度进行统计,基于速度、密度参数进行聚类分析量... 详细信息

针对快速路入口匝道区域拥堵问题,本文提出一种基于交通密度预测的入口匝道控制方法。通过分析快速路匝道区域的交通特性,定义交通流缓行状态,利用经典宏观交通流模型对快速路主线的历史密度进行统计,基于速度、密度参数进行聚类分析量化缓行状态交通参数特征。基于城市交通流的日变化特性,利用时间序列模型对交通密度进行短期预测,基于预测结果识别缓行状态。针对交通缓行状态,提出一种快速路主线交通密度与入口匝道排队长度的协同控制模型,通过控制入口匝道进而控制主线下游密度不超过临界密度,利用PSO-PID(Particle Swarm Optimization-Proportional Integral Derivative Control)算法对控制模型进行求解。以南昌市洪都大道快速路为例,对晚高峰缓行时段进行仿真分析,并与经典的匝道控制方案进行对比分析。结果表明:本文模型相较ALINEA模型,将匝道调节率提高11.0%,匝道平均排队长度和平均延误分别降低了14.8%和13.5%。

关键词：城市交通预测控制信号配时优化快速路入口匝道 PID算法

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