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Continuous Synthesis of Main-Chain-type Fluorinated Graft Copolymers via Successive Flow START Polymerization and Cu(0)-Mediated RDRP

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Chinese Journal of Polymer Science 2023年第8期41卷 1155-1161,I0004页

作者： Peng Wang shuai-jie chen Jian-Nan cheng Wei-Wei He Li-Fen Zhang Zhen-Ping cheng State and Local Joint Engineering Laboratory for Novel Functional Polymeric Materials Jiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSuzhou key Laboratory of Macromolecular Design and Precision SynthesisCollege of ChemistryChemical Engineering and Materials ScienceSoochowUniversitySuzhou 215123China State Key Laboratory of Radiation Medicine and Protection School of Radiological and Interdisciplinary Sciences(RADX)Soochow UniversityCollaborative Innovation Center of Radiological Medicine of Jiangsu Higher Education InstitutionsSuzhou 215123China

Fluorinated polymers are receiving more and more attention worldwide due to their unique chemical properties,and modified fluorinated polymers with different topologies are persued for enriching and enhancing their performance in a variety of application *** this work,main-chain-type semifluorinated graft copolymers are produced steadily in continuous tube reactors via photocontrolled step transferaddition and radical-termination(START)polymerization and Cu(0)-mediated reversible deactivation radical polymerization(Cu(0)-RDRP)at room temperature for the first ***,semifluorinated alternating copolymer(AB)n B is prepared by START polymerization of 1,6-diiodoperfluorohexane(A)and 1,7-octadiene(B)in the first quartz pipeline under irradiation with purple LED light at 20℃.The(AB)nB with periodic C―I bonds is then flowed into the second copper pipeline directly and acts as the macroinitiators for Cu(0)-RDRP of methyl acrylate(MA)to obtain corresponding graft copolymer(AB)n *** work provides a new strategy for continuous synthesis of fluorinated graft copolymer materials.

关键词： Fluoropolymers Photopolymerization Graft Polymer Cu(O)-mediated RDRP START polymerization

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A short review of antibacterial Cu-bearing stainless steel:antibacterial mechanisms,corrosion resistance,and novel preparation techniques

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Journal of Iron and Steel Research International 2024年第1期31卷 24-45页

作者： shuai Liu Han-jie Guo School of Artificial Intelligence Beijing Technology and Business UniversityBeijing100048China Beijing Key Laboratory of Special Melting and Preparation of High-End Metal Materials University of Science and Technology BeijingBeijing100083China

Cu-bearing stainless steel is widely used in the fields of food,medical and household sanitary equipment because of its surface finish and corrosion ***,the growth of bacteria on stainless steel leads to the formation of biofilms,which causes ***,the antibacterial property of stainless steel is a worthy research *** of breakthroughs in the field of corrosion resistance and antimicrobial properties are still ***,due to the scarcity of publications on the antibacterial mechanisms and processing methods of antibacterial Cu-bearing stainless steel,we review the current state of relevant research and *** toxicity of Cu,corrosion resistance mechanism of stainless steel,and antibacterial mechanism and preparation method of antibacterial stainless steel are *** addition,alloying,surface modification and other methods are found to have limitations in balancing the toxicity and antibacterial properties of copper and the relationship between the antibacterial properties and corrosion resistance of Cu-bearing stainless steel.A new preparation method of antibacterial stainless steel associated with selective laser melting(SLM)is *** is becoming a powerful additive manufacturing technology that can be used to manufacture customized and complex *** research status of SLM applied in antibacterial stainless steel preparation is ***,the future research direction of Cu-bearing antibacterial stainless steel is discussed.

关键词： Cu-bearing stainless steel Antibacterial Processing Additive manufacturing Corrosion resistance

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Machine learning for prediction of retained austenite fraction and optimization of processing in quenched and partitioned steels

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Journal of Iron and Steel Research International 2024年第8期31卷 2002-2013页

作者： shuai Wang jie Li Li-yang Zeng Xun-wei Zuo Nai-lu chen Yong-hua Rongg Shanghai Key Laboratory of Materials Laser Processing and Modification School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China School of Materials Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China

The metastable retained austenite(RA)plays a significant role in the excellent mechanical performance of quenching and partitioning(Q&P)steels,while the volume fraction of RA(V_(RA))is challengeable to directly predict due to the complicated relationships between the chemical composition and process(like quenching temperature(Qr)).A Gaussian process regression model in machine learning was developed to predict V_(RA),and the model accuracy was further improved by introducing a metallurgical parameter of martensite fraction(fo)to accurately predict V_(RA) in Q&P *** developed machine learning model combined with Bayesian global optimization can serve as another selection strategy for the quenching temperature,and this strategy is very effcient as it found the"optimum"Qr with the maximum V_(RA) using only seven consecutive *** benchmark experiment also reveals that the developed machine learning model predicts V_(RA) more accurately than the popular constrained carbon equilibrium thermodynamic model,even better than a thermo-kinetic quenching-partitioning-tempering-local equilibrium model.

关键词： Q&P steel Retained austenite fraction Machine learning Quenching temperature Gaussian process regression model

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Innovations in metallurgical and materials processes:advancing liquid theory and honoring ***-jie Guo's contributions to physical chemistry in metallurgy

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Journal of Iron and Steel Research International 2024年第1期31卷 1-2页

作者： shuai Liu Jing Guo Han-jie Guo School of Artificial Intelligence Beijing Technology and Business UniversityBeijing100048China School of Metallurgical and Ecological Engineering University of Science and Technology Beijing(USTB)Beijing100083China

Spanning three decades,***-jie Guo's research group has dedicated itself to exploring the fundamental theories and practical applications of physical chemistry within the realm of *** under the assumption that molecul... 详细信息

关键词： chemistry liquid complexes

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Biological factors driving colorectal cancer metastasis

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World Journal of Gastrointestinal Oncology 2024年第2期16卷 259-272页

作者： shuai-Xing An Zhao-Jin Yu chen Fu Min-jie Wei Long-Hai Shen Department of Pharmacology School of PharmacyChina Medical UniversityShenyang 110122Liaoning ProvinceChina Liaoning Key Laboratory of Molecular Targeted Antitumor Drug Development and Evaluation Liaoning Cancer Immune Peptide Drug Engineering Technology Research CenterKey Laboratory of Precision Diagnosis and Treatment of Gastrointestinal Tumors(China Medical University)Ministry of EducationShenyang 110122Liaoning ProvinceChina BD Department Greenpine Pharma Group Co.LtdTianjin 300020China Center of Oncology Genertec Liaoyou Gem Flower HospitalPanJin 124010Liaoning ProvinceChina

Approximately 20%of colorectal cancer(CRC)patients present with metastasis at *** Stage I-III CRC patients who undergo surgical resection,18%typically suffer from distal metastasis within the first three years following initial *** median survival duration after the diagnosis of metastatic CRC(mCRC)is only 9 *** is traditionally considered to be an advanced stage malignancy or is thought to be caused by incomplete resection of tumor tissue,allowing cancer cells to spread from primary to distant organs;however,increa-sing evidence suggests that the mCRC process can begin early in tumor *** patients present with high heterogeneity and diverse cancer phenotypes that are classified on the basis of molecular and morphological *** genomic and nongenomic events can induce subclone diversity,which leads to cancer and *** the course of mCRC,metastatic cascades are associated with invasive cancer cell migration through the circulatory system,extravasation,distal seeding,dormancy,and reactivation,with each step requiring specific molecular ***,cancer cells presenting neoantigens can be recognized and eliminated by the immune *** this review,we explain the biological factors that drive CRC metastasis,namely,genomic instability,epigenetic instability,the metastatic cascade,the cancer-immunity cycle,and external lifestyle *** remarkable progress in CRC research,the role of molecular classification in therapeutic intervention remains *** review shows the driving factors of mCRC which may help in identifying potential candidate biomarkers that can improve the diagnosis and early detection of mCRC cases.

关键词： cancer Metastasis cascade Cancer immunity Genomic variation Epigenetic instability Lifestyle factor

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Hepatic perivascular epithelioid cell tumors:The importance of preoperative diagnosis

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World Journal of Gastroenterology 2024年第13期30卷 1926-1933页

作者： shuai Yan Jia-jie Lu Lin chen Wei-Hua Cai Jin-Zhu Wu Department of Medical School Nantong UniversityNantong 226300Jiangsu ProvinceChina Department of Hepatobiliary Surgery Affiliated Nantong Hospital 3 of Nantong UniversityNantong 226006Jiangsu ProvinceChina Nantong Institute of Liver Disease Affiliated Nantong Hospital 3 of Nantong UniversityNantong 226006Jiangsu ProvinceChina

Accurate preoperative diagnosis is highly important for the treatment of perivascular epithelioid cell tumors(PEComas)because PEComas are mainly benign tumors and may not require surgical *** analyzing the causes,properties and clinical manifestations of PEComas,we summarize the challenges and solutions in the diagnosis of PEComas.

关键词： Hepatic perivascular epithelioid cell tumors Liver Preoperative diagnosis Angiomyolipomas Mesenchymal tissue-derived tumors

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Quantum Curve and Bilinear Fermionic Form for the Orbifold Gromov–Witten Theory of P[r]

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Acta Mathematica Sinica,English Series 2024年第1期40卷 43-80页

作者： Chong Yao chen shuai GUO Mathematics Department Duke UniversityBox 90320DurhamNC 27708-0320USA School of Mathematical Sciences Peking UniversityBeijing 100871P.R.China

We construct the quantum curve for the Baker-Akhiezer function of the orbifold Gromov-Witten theory of the weighted projective line P[r].Furthermore,we deduce the explicit bilinear Fermionic formula for the(stationary... 详细信息

关键词： Quantum curve Free Fermions Gromov-Witten invariants Orbifold P^(1)

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UAV-assisted data collection for wireless sensor networks with dynamic working modes

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Digital Communications and Networks 2024年第3期10卷 805-812页

作者： jie chen Jianhua Tang Shien-Ming Wu School of Intelligent Engineering South China University of TechnologyGuangzhou511442China

Wireless Sensor Network(WSN)is a cornerstone of Internet of Things(IoT)and has rich application *** this work,we consider a heterogeneous WSN whose sensor nodes have a diversity in their Residual Energy(RE).In this work,to protect the sensor nodes with low RE,we investigate dynamic working modes for sensor nodes which are determined by their RE and an introduced energy ***,we employ an Unmanned Aerial Vehicle(UAV)to collect the stored data from the heterogeneous *** aim to jointly optimize the cluster head selection,energy threshold and sensor nodes’working mode to minimize the weighted sum of energy con-sumption from the WSN and UAV,subject to the data collection rate *** this end,we propose an efficient search method to search for an optimal energy threshold,and develop a penalty-based successive convex approximation algorithm to select the cluster *** we present a low-complexity iterative approach to solve the joint optimization problem and discuss the implementation *** results justify that our proposed approach is able to reduce the energy consumption of the sensor nodes with low RE significantly and also saves energy for the whole WSN.

关键词： Unmanned aerial vehicle Wireless sensor networks Cluster heads Dynamic working modes

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A review on current development of thermophotovoltaic technology in heat recovery

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International Journal of Extreme Manufacturing 2024年第2期6卷 297-323页

作者： Shuni chen Yanming Guo Qinghui Pan Yong shuai Ministry of Industry and Information Technology Key Laboratory of Aerospace Thermophysics School of Energy Science and EngineeringHarbin Institute of TechnologyHarbin 150001People’s Republic of China

The burning of fossil fuels in industry results in significant carbon emissions,and the heat generated is often not fully *** high-temperature industries,thermophotovoltaics(TPVs)is an effective method for waste heat *** review covers two aspects of high-efficiency TPV systems and industrial waste heat *** the system level,representative results of TPV complete the systems,while selective emitters and photovoltaic cells in the last decade are *** key points of components to improve the energy conversion efficiency are further analyzed,and the related micro/nano-fabrication methods are *** the application level,the feasibility of TPV applications in high-temperature industries is shown from the world waste heat utilization *** potential of TPV in waste heat recovery and carbon neutrality is illustrated with the steel industry as an example.

关键词： thermophotovoltaic waste heat recovery micro/nano-fabrication carbon neutrality

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Printable,flexible ceramic fiber paper based on electrospinning

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Rare Metals 2024年第6期43卷 2739-2746页

作者： Yong-shuai Xie Yuan cheng Yang Lyu Rui Li jie-Cai Han National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150001China State Key Laboratory of Intelligent Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan 430074China

Based on the fact that it is challenging for the polymer flexible circuit substrates to meet the requirements of serving in high-temperature environments,this work proposed the idea of using printable ceramic fiber paper as a high-temperature flexible circuit substrate.A ceramic fiber paper with all ceramic components had been developed via electrospinning,solving the problems of low strength and severe strength drop at high temperatures of traditional ceramic fiber *** tensile strength of the prepared ceramic fiber paper is 2.63 MPa,and the reliable service temperature is 1200℃.Its bulk density is about 1.5 times that of traditional ceramic fiber *** can be printed with patterns by commercial inkjet printers like ordinary printing paper and has excellent *** feasibility of ceramic fiber paper as a flexible circuit substrate was verified by constructing a simple *** the fiber paper is significantly bent,the circuit still forms a complete path,which proves that it has a strong application potential for high-temperature flexible circuit substrate and is expected to promote the development of flexible electronic devices serving at extreme high-temperature environments.

关键词： Ceramic fiber paper High temperature Inkjet printing Flexible electronic

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