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Journal of Energy Chemistry 2024年第5期92卷 216-223页

作者： Xuexiu gu Xuan-Wen Gao Dongrun Yang Qinfen gu YSong Hong Chen Tianzhen Ren Wen-Bin Luo Institute for Energy Electrochemistry and Urban Mines Metallurgy School of MetallurgyNortheastern UniversityShenyang 110819LiaoningChina Australian Synchrotron(ANSTO) 800 Blackburn RdClaytonVictoria 3168Australia School of Science and Engineering University of DundeeNethergateDundee DD14HNScotlandUK

As the primary suppliers of cyclable sodium ions,O3-type layer-structured manganese-based oxides are recognized as highly competitive cathode candidates for sodium-ion *** advance the development of high-energy sodium-ion batteries,it is crucial to explore cathode materials operating at high voltages while maintaining a stable cycling *** orbital and electronic structure of the octahedral center metal element plays a crucial role in maintaining the octahedra structural integrity and improving Na^(+)ion diffusion by introducing heterogeneous chemical *** by the abundant configuration of extra nuclear electrons and large ion radius,we employed trace amounts of tungsten in this *** obtained cathode material can promote the reversibility of oxygen redox reactions in the high-voltage region and inhibit the loss of lattice ***,the formation of a Na_(2)WO_(4) coating on the material surface can improve the interfacial stability and interface ions *** demonstrates an initial Coulombic efficiency(ICE)of 94.6%along with 168.5 mA h g^(-1 )discharge capacity within the voltage range of 1.9-4.35 *** findings contribute to the advancement of high-energy sodium-ion batteries by providing insights into the benefits of tungsten doping and Na_(2)WO_(4) coating on cathode materials.

关键词： Sodium ion battery Layer-structured manganese-based oxides Cathodematerial Surface modification Elements doping

Health diagnosis of ultrahigh arch dam performance using heterogeneous spatial panel vector model

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Water Science and Engineering 2024年第2期17卷 177-186页

作者： Er-feng Zhao Xin Li Chong-shi gu The National Key Laboratory of Water Disaster Prevention Hohai UniversityNanjing 210098China NationalEngineering Research Centerof Water Resources Eficient Utilization and Engineering Safety Hohai UniversityNanjing 20098China

Currently,more than ten ultrahigh arch dams have been constructed or are being constructed in *** control is essential to long-term operation of these *** study employed the flexibility coefficient and plastic complementary energy norm to assess the structural safety of arch dams.A comprehensive analysis was conducted,focusing on differences among conventional methods in characterizing the structural behavior of the Xiaowan arch dam in ***,the spatiotemporal characteristics of the measured performance of the Xiaowan dam were explored,including periodicity,convergence,and time-effect *** findings revealed the governing mechanism of main ***,a heterogeneous spatial panel vector model was developed,considering both common factors and specific factors affecting the safety and performance of arch *** model aims to comprehensively illustrate spatial heterogeneity between the entire structure and local regions,introducing a specific effect quantity to characterize local deformation ***,the proposed model was applied to the Xiaowan arch dam,accurately quantifying the spatiotemporal heterogeneity of dam ***,the spatiotemporal distri-bution characteristics of environmental load effects on different parts of the dam were reasonably *** of the model prediction enhances its credibility,leading to the formulation of health diagnosis criteria for future long-term operation of the Xiaowan *** findings not only enhance the predictive ability and timely control of ultrahigh arch dams'performance but also provide a crucial basis for assessing the effectiveness of engineering treatment measures.

关键词： Ultrahigh arch dam Structural performance Deformation behavior Diagnosis criterion Panel data model

Compressed Data Separation via ℓ_(q)-Split Analysis with ℓ_(∞)-Constraint

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Acta Mathematica Sinica,English Series 2024年第7期40卷 1655-1673页

作者： Ming Yang gu Song Li Jun Hong Lin School of Mathematical Science Zhejiang UniversityHangzhou310027P.R.China Center for Data Science Zhejiang UniversityHangzhou310027P.R.China

In this paper,we study compressed data separation(CDS)problem,i.e.,sparse data separation from a few linear random *** propose the nonconvex ℓ_(q)-split analysis with ℓ_(∞)-constraint and 0 详细信息

In this paper,we study compressed data separation(CDS)problem,i.e.,sparse data separation from a few linear random *** propose the nonconvex ℓ_(q)-split analysis with ℓ_(∞)-constraint and 0

关键词： Data separation ℓ_(q)-split analysis Dantzig selector frames restricted isometry property compressed sensing

The essential roles of m^(6)A modification in osteogenesis and common bone diseases

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Genes & Diseases 2024年第1期11卷 335-345页

作者： Yuxi gu Yidan Song Yihua Pan Jun Liu State Key Laboratory of Oral Diseases&National Clinical Research Center for Oral Diseases Department of OrthodonticsWest China Hospital of StomatologySichuan UniversityChengduSichuan 610041China

N6-methyladenosine(m^(6)A)is the most prevalent modification in the eukaryotic transcriptome and has a wide range of functions in coding and noncoding *** affects the fate of the modified RNA,including its stability,splicing,and translation,and plays an important role in post-transcriptional *** play a key role in supporting and pro-tecting muscles and other organs,facilitating the movement of the organism,ensuring blood production,*** diseases such as osteoarthritis,osteoporosis,and bone tumors are serious public health *** processes of bone development and osteogenic differen-tiation require the precise regulation of gene expression through epigenetic mechanisms including histone,DNA,and RNA *** a reversible dynamic epigenetic mark,m^(6)A modifications affect nearly every important biological process,cellular component,and molecular function,including skeletal development and *** recent years,studies have shown that m^(6)A modification is involved in osteogenesis and bone-related *** this review,we summarized the proteins involved in RNA m^(6)A modification and the latest progress in elucidating the regulatory role of m^(6)A modification in bone formation and stem cell direc-tional *** also discussed the pathological roles and potential molecular mech-anisms of m^(6)A modification in bone-related diseases like osteoporosis and osteosarcoma and suggested potential areas for new strategies that could be used to prevent or treat bone de-fects and bone diseases.

关键词： Bone diseases m^(6)A modification Osteogenesis Regulatory role Stem cells

Progresses and Prospects of Asymmetrically Coordinated Single Atom Catalysts for Lithium-Sulfur Batteries

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Energy & Environmental Materials 2024年第4期7卷 48-63页

作者： Rong Zhou Shaonan gu Meng guo shuzheng Xu guowei Zhou Key Laboratory of Fine Chemicals in Universities of Shandong Jinan Engineering Laboratory for Multi-scale Functional Materials School of Chemistry and Chemical Engineering Qilu University of Technology(Shandong Academy of Sciences)

Lithium-sulfur batteries (LSBs) are widely regarded as promising next-generation batteries due to their high theoretical specific capacity and low material ***,the practical applications of LSBs are limited by the shuttle effect of lithium polysulfides (LiPSs),electronic insulation of charge and discharge products,and slow LiPSs conversion reaction kinetics.

关键词： asymmetrical coordination conversion catalysis Li-S batteries shuttle effect single atom catalysts

Numerical simulation of granular silicon growth and silicon fines formation process in polysilicon fluidized bed

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Particuology 2024年第4期87卷 74-86页

作者： guangkai gu guoqiang Lv Wenhui Ma Shanlin Du Boqiang Fu Faculty of Metallurgical and Energy Engineering Kunming University of Science and TechnologyKunming 650093China State Key Laboratory of Complex Nonferrous Metal Resources Cleaning Utilization in Yunnan Province Kunming 650093China

Operating conditions strongly affect the yield and quality of polysilicon in a polysilicon fluidized *** this study,a new model of polysilicon fluidized bed was established using the Euler-Euler model coupled with population balance model(PBM),which was combined with fluid flow,heat,and mass transfer models,while considering the scavenging effect of silicon *** effects of different operating conditions on the deposition and formation rates of silicon fines were *** show that the model can correctly describe the particle growth process in the fluidized bed of *** silicon fines and the interphase velocity difference show"N"-and"M"-shaped distributions along the axial direction,*** particle temperature and concentration near the wall are higher than those in the central *** decomposition of silane in the bottom region of the bed is dominated by het-erogeneous *** scavenging of silicon fines occurs in the dilute-phase *** effects of operating conditions,*** gas temperature,silane composition,and gas velocity,on the reactor performance were also explored *** the inlet gas composition and velocity enhances the formation rates of solid silicon and *** the inlet gas temperature promotes the growth of solid silicon and inhibits the formation of silicon *** fluidization ratio,low inlet silane concentration,and high inlet gas temperature enhance the selectivity of silicon growth.

关键词： Polysilicon fluidized bed Particle growth Fines CFD Population balance model(PBM)

Layered Structural PBAT Composite Foams for Efficient Electromagnetic Interference Shielding

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Nano-Micro Letters 2024年第2期16卷 273-286页

作者： Jianming Yang Hu Wang Yali Zhang Hexin Zhang Junwei gu School of Chemistry and Chemical Engineering Anhui University of TechnologyMa’anshanAnhui 243032People’s Republic of China Shaanxi Key Laboratory of Macromolecular Science and Technology School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072ShaanxiPeople’s Republic of China School of Materials Science and Engineering Jiangsu University of Science and TechnologyZhenjiang 212003JiangsuPeople’s Republic of China

The utilization of eco-friendly,lightweight,high-efficiency and high-absorbing electromagnetic interference(EMI)shielding composites is imperative in light of the worldwide promotion of sustainable *** this work,magnetic poly(butyleneadipate-coterephthalate)(PBAT)microspheres were firstly synthesized via phase separation method,then PBAT composite foams with layered structure was constructed through the supercritical carbon dioxide foaming and scraping *** merits of integrating ferroferric oxideloaded multi-walled carbon nanotubes(Fe3O4@MWCNTs)nanoparticles,a microcellular framework,and a highly conductive silver layer have been judiciously orchestrated within this distinctive layered *** are consumed throughout the process of“absorption-reflection-reabsorption”as much as possible,which greatly declines the secondary radiation *** biodegradable PBAT composite foams achieved an EMI shielding effectiveness of up to 68 dB and an absorptivity of 77%,and authenticated favorable stabilization after the tape adhesion experiment.

关键词： Electromagnetic interference shielding Layered structure Supercritical carbon dioxide foaming Poly(butyleneadipateco-terephthalate) Microcellular

Ultrahigh performance passive radiative cooling by hybrid polar dielectric metasurface thermal emitters

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Opto-Electronic Advances 2024年第4期7卷 17-25页

作者： Yinan Zhang yinggang Chen Tong Wang Qian Zhu Min gu Institute of Photonic Chips University of Shanghai for Science and TechnologyShanghai 200093China Centre for Artificial-Intelligence Nanophotonics School of Optical-Electrical and Computer EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China

Real-world passive radiative cooling requires highly emissive,selective,and omnidirectional thermal emitters to maintain the radiative cooler at a certain temperature below the ambient temperature while maximizing the net cooling *** various selective thermal emitters have been demonstrated,it is still challenging to achieve these conditions sim-ultaneously because of the extreme difficulty in controlling thermal emission of photonic structures in *** we demonstrated hybrid polar dielectric metasurface thermal emitters with machine learning inverse design,en-abling a high emissivity of~0.92 within the atmospheric transparency window 8-13μm,a large spectral selectivity of~1.8 and a wide emission angle up to 80 degrees,*** selective and omnidirectional thermal emitter has led to a new record of temperature reduction as large as~15.4°C under strong solar irradiation of~800 W/m2,signific-antly surpassing the state-of-the-art *** designed structures also show great potential in tackling the urban heat island effect,with modelling results suggesting a large energy saving and deployment area *** research will make significant impact on passive radiative cooling,thermal energy photonics and tackling global climate change.

关键词： radiative cooling dielectric metasurfaces machine learning thermal emitters

Effect of fore/aft-loaded rotor on compressor stability under inlet circumferential distortion

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Chinese Journal of Aeronautics 2024年第5期37卷 199-213页

作者： Dakun SUN Benhao gu Fangfei NING Dengke XU Xiaofeng SUN School of Energy and Power Engineering Beihang UniversityBeijing 102206China Research Institute of Aero-engine Beihang UniversityBeijing 102206China

A modified small perturbation stability prediction model for axial compressors with circumferential inlet distortions is established and applied to investigate the effect of fore/aft-loaded rotor on compressor stability under circumferentially distorted inlet *** inlet total pressure distribution downstream of the distortion screen is measured in experiments and employed for simulations which are implemented via time-space spectral *** stall inception prediction results via the stability model indicate that the compressor with aft-loaded rotor not only performs better in terms of stability under uniform inlet,but also maintains a larger stability margin under circumferentially distorted *** experiments for compressors with fore-loaded and aft-loaded rotor are respectively carried *** results validate the reliability of numerical simulations and the predicted conclusion that the aft-loaded rotor is beneficial for compressor ***,the ability of the developed theoretical model for compressor stability prediction under circumferential distortions is *** addition,dynamic pressure signals at rotor tip measured in experiments illustrate that the circumferential distortion has little effect on the compressor stall pattern.

关键词： Axial compressor stability Inlet distortion Blade loading Small perturbation Time-space spectral method

High Dynamic Bounding and Jumping Motion of Quadruped Robot Based on Stable Optimization Control

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Journal of Bionic Engineering 2024年第1期21卷 101-111页

作者： Sai gu Fei Meng Botao Liu Junyao Gao Qiang Huang School of Mechatronical Engineering Beijing Institute of Technology100081 BeijingChina Key Laboratory of Biomimetic Robots and Systems Ministry of EducationBeijing 100081China

Aiming at the environment such as ravines and obstacles that may be encountered in the actual movement,this paper proposes a method for optimizing the bounding and jumping motion based on the ground touching force trajectory and the air motion trajectory of the quadruped *** method of optimizing the ground reaction force according to the speed of the demand and the height of the jump,and adjusting the stance and swing time according to the relationship of dynamics and momentum *** the same time,under the constraints of dynamics and energy consumption of the robot system,considering the jumping distance and height,a method for optimizing the air trajectory of bounding and jumping is *** switching and landing stability control are also ***,the experimental results show that the quadruped robot has strong bounding and jumping ability,and has achieved stable bounding movement and forward jump movement of 0.8 m.

关键词： Quadruped robot High dynamic motion control-Periodic limit cycle Trajectory optimization