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Subconjunctival trypsin injection for anterior chamber fibrin exudates in eyes with globe rupture following vitrectomy

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International Journal of Ophthalmology(English edition) 2024年第11期17卷 2037-2044页

作者： shu-wen lu Hao-Yu Li Xin-Min Li Chao Ma Xian Li Qiu-Ming Hu Department of Ophthalmology the First Affiliated Hospital of Henan University of Chinese MedicineZhengzhou 450000Henan ProvinceChina Department of Ophthalmology the Second Xiangya HospitalCentral South UniversityChangsha 410021Hunan ProvinceChina Hunan Clinical Research Centre of Ophthalmic Disease Changsha 410021Hunan ProvinceChina Department of Ophthalmology the First Affiliated Hospital of Xinxiang Medical UniversityXinxiang 453100Henan ProvinceChina Department of Ophthalmology the First Affiliated Hospital of Zhengzhou UniversityZhengzhou 450052Henan ProvinceChina School of Pharmacy and Optometry Faculty of BiologyMedicine and HealthThe University of ManchesterManchester M139PLUnited Kingdom Department of Retina and Vitreous Jingliang Eye HospitalGuangxi Medical UniversityNanning 530021Guangxi Zhuang Autonomous RegionChina

AIM:To compare the safety and clinical outcomes of subconjunctival trypsin and dexamethasone(DEX)injections in the treatment of anterior chamber fibrin exudates in eyes with globe rupture following primary wound repair and ***:A retrospective analysis included 42 males and 10 females(mean age 46.0±6.0y,range 34 to 58y)who underwent primary wound sutures and vitrectomy for globe *** with pupil-covered fibrinous exudate or/and membrane in the anterior chamber were *** the first postoperative day,subconjunctival injections of either 5000 units(0.4 mL)of trypsin solution(n=25)or 0.5 mL(1 mg)DEX(n=27)were administered to accelerate exudate *** was assessed by observing break time and partial absorption of the fibrin exudate *** and comfort were evaluated by monitoring intraocular pressure(IOP),allergy,pain,and foreign body ***:Both groups achieved 1/3 absorption of the anterior chamber fibrin exudate membrane,but the trypsin group exhibited shorter break time and partial absorption time compared to the DEX group(P<0.05).Trypsin treatment was also less irritating to *** adverse reactions were reported,and IOP remained *** acuity improved in both groups without statistical ***:Compared to DEX,trypsin demonstrates a shorter absorption time for the fibrin exudate membrane with a more comfortable process in treating pupil-covered fibrinous exudate or/and membrane after vitrectomy for globe rupture.

关键词： globe rupture vitrectomy exudative fibrin membrane trypsin dexamethasone

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下地幔压力条件下(Mg0.97，Fe0.03)O方镁铁矿的光学性质

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物理学报 2015年第11期64卷 436-441页

作者：高敏舒文路叶强何林祝文军四川师范大学物理与电子工程学院固体物理研究所成都610068 中国工程物理研究院流体物理研究所冲击波物理与爆轰物理重点实验室绵阳621900

本文采用第一性原理方法,计算了(Mg0.97,Fe0.03)O方镁铁矿的理想晶体和含镁-氧离子双空位点缺陷晶体在下地幔压力条件下的光学性质.吸收光谱数据表明,方镁铁矿理想晶体的结果与晶体场等理论预测的结果相似:压力诱导铁自旋态的转变将导... 详细信息

本文采用第一性原理方法,计算了(Mg0.97,Fe0.03)O方镁铁矿的理想晶体和含镁-氧离子双空位点缺陷晶体在下地幔压力条件下的光学性质.吸收光谱数据表明,方镁铁矿理想晶体的结果与晶体场等理论预测的结果相似:压力诱导铁自旋态的转变将导致方镁铁矿吸收谱有巨大蓝移,并在近红外光区出现了透明现象.然而,在方镁铁矿中含有点缺陷时,其结果与晶体场等理论预测结果存在本质差异:铁自旋态的转变将导致在近红外光区的吸收性显著增强.含点缺陷晶体折射率的计算结果表明,压力、波数及铁自旋态的转变对(Mg0.97,Fe0.03)O方镁铁矿的折射率有较明显地影响.本文结果不仅对探索下地幔方镁铁矿在高压下的光学性质有重要的参考价值,而且还指明高压吸收光谱的测量可能是准确获得铁自旋态信息一个好的手段.

关键词：高压第一性原理计算光学性质方镁铁矿

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Metal-organic frameworks with dinuclear metal centers for synergistically boosting CO2 photoreduction

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Science China Chemistry 2025年第1期68卷 201-208页

作者： Hui-Feng Wang wen-Jie Shi Yu-Xin Yang Bao-Xia Dong Tong-Bu lu Di-Chang Zhong School of Chemistry and Chemical Engineering Yangzhou University Institute for New Energy Materials and Low Carbon Technologies School of Materials Science and Engineering Tianjin University of Technology

Dinuclear metal synergistic catalysis （DMSC） has been proved powerful in boosting CO2reduction,while this has not been achieved in heterogeneous catalysts with long-range order *** this study,we,by introduction of metal catalytic centers into an indium-based metal-organic framework （MOF）,obtained a series of isostructural In-MOFs,including three MOFs with mononuclear metal catalytic center （M-In）,three MOFs with dinuclear homometallic catalytic centers （MM-In）,and three MOFs with dinuclear heterometallic catalytic centers (MM’-In,M/M’=Co（II）,Ni（II）,Zn（II）).It was found that all these MOFs can serve as catalysts for photochemical CO2reduction to *** with M-In,the catalytic activities of MM-In were obviously enhanced,and that of MM’-In was further significantly *** example,the CO yield of Co Zn-In reaches a record value of 12,700μmol g-1h-1,which is 4.0,8.1,9.4,and 18.6-fold higher than that of Co Co-In,Zn Zn-In,Co-In,and Zn-In,***,the catalytic activities of Co Ni-In and Ni Zn-In also show different fold increase than those of corresponding dinuclear homometallic and mononuclear metallic *** results of control experiments and theoretical calculation reveal that the higher catalytic activities of MM-In over M-In can be ascribed to the DMSC effect,and the higher catalytic activity of MM’-In over MM-In can be ascribed to the strengthened DMSC *** work reveals the relationship between DMSC effect and bimetal centers in CO2reduction,which provides new insights into the DMSC and paves a new way to design highly active catalysts for photochemical CO2reduction.

关键词： metal-organic frameworks dinuclear metal centers synergistic catalysis CO2 reduction photocatalysis

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铁的电子自旋相变对下地幔方镁铁矿光学性质的影响

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四川大学学报（自然科学版） 2018年第3期55卷 554-558页

作者：曾明凤舒文路何林成都职业技术学院基础部成都610041 四川师范大学物理与电子工程学院固体物理研究所成都610068

本文采用第一性原理方法,计算了(Mg0.8125,Fe0.1875)O方镁铁矿理想晶体和含氧离子空位点缺陷晶体在下地幔压力范围内的光学性质.理想晶体吸收谱数据表明,与晶体场理论预测的结果一致,铁在高压下的电子自旋相变将导致方镁铁矿吸收光谱显... 详细信息

本文采用第一性原理方法,计算了(Mg0.8125,Fe0.1875)O方镁铁矿理想晶体和含氧离子空位点缺陷晶体在下地幔压力范围内的光学性质.理想晶体吸收谱数据表明,与晶体场理论预测的结果一致,铁在高压下的电子自旋相变将导致方镁铁矿吸收光谱显著蓝移,从而使得近红外区域出现了透明的现象.然而,令人感兴趣的是,含空位缺陷晶体的结果与晶体场理论的结果有本质差别,却与实验观测一致:电子自旋相变将使得近红外区的吸收性显著增强.同时,含空位缺陷晶体的折射率结果显示,压力、波长以及电子自旋相变对下地幔方镁铁矿的折射率有较明显地影响.

关键词：下地幔方镁铁矿高压第一性原理计算光学性质

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Thermoresponsive helical dendronized poly(arylacetylene)s:modulating the dynamic chirality

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Science China Chemistry 2025年

作者： Xueting lu Lei Wang Liangxuan Ren wen Li Afang Zhang International Joint Laboratory of Biomimetic&Smart Polymers School of Materials Science and EngineeringShanghai University

Helical poly(arylacetylene)s have formed an intriguing class of polymers,whose chiralities are dynamic and liable to external *** combining dendronized polymer topology with dendritic oligoethylene glycols (OEGs),we here report on synthesis of a homologous series of thermoresponsive dendronized poly(arylacetylene)s with either poly(phenyl acetylene) or poly(naphthalene acetylene) as the backbones,and investigate tunability of their helical *** polymers carry dendritic OEG pendants with either methoxyl-or ethoxyl-terminals to tune their unprecedent thermoresponsive behaviors,and at the same time,dendritic shielding plays an important role in mediating their thermal phase transition *** of these polymers is originated from the chiral alanine or phenylalanine moieties within the dendritic pendants,which can be tailored through manipulating solvation in different organic solvents or via thermal dehydration and collapse in ***,achiral additives such as linear or dendritic OEGs and benzene derivatives can act similarly as thermal dehydration to induce chirality transitions of these polymers in aqueous phase through interplay competitions between the additives and the polymers against their hydration.

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Repetitive traumatic brain injury–induced complement C1–related inflammation impairs long-term hippocampal neurogenesis

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Neural Regeneration Research 2025年第3期20卷 821-835页

作者： Jing Wang Bing Zhang Lanfang Li Xiaomei Tang Jinyu Zeng Yige Song Chao Xu Kai Zhao Guoqiang Liu Youming lu Xinyan Li Kai shu Department of Neurosurgery Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei ProvinceChina Department of Neurosurgery Shanxi Bethune HospitalShanxi Academy of Medical SciencesTongji Shanxi HospitalThird Hospital of Shanxi Medical UniversityTaiyuanShanxi ProvinceChina Department of Pathophysiology School of Basic Medicine and Tongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei ProvinceChina Institute for Brain Research Wuhan Center of Brain ScienceHuazhong University of Science and TechnologyWuhanHubei ProvinceChina Department of Graduate Student Chongqing Medical UniversityChongqingChina Department of Basic Medicine School of Medical ScienceHubei University for NationalitiesEnshiHubei ProvinceChina Department of Anatomy School of Basic Medicine and Tongji Medical CollegeHuazhong University of Science and TechnologyWuhanHubei ProvinceChina

Repetitive traumatic brain injury impacts adult neurogenesis in the hippocampal dentate gyrus,leading to long-term cognitive ***,the mechanism underlying this neurogenesis impairment remains *** this study,we established a male mouse model of repetitive traumatic brain injury and performed long-term evaluation of neurogenesis of the hippocampal dentate gyrus after repetitive traumatic brain *** results showed that repetitive traumatic brain injury inhibited neural stem cell proliferation and development,delayed neuronal maturation,and reduced the complexity of neuronal dendrites and *** with repetitive traumatic brain injuryalso showed deficits in spatial memory ***,following repetitive traumatic brain injury,neuroinflammation was enhanced in the neurogenesis microenvironment where C1q levels were increased,C1q binding protein levels were decreased,and canonical Wnt/β-catenin signaling was *** inhibitor of C1 reversed the long-term impairment of neurogenesis induced by repetitive traumatic brain injury and improved neurological *** findings suggest that repetitive traumatic brain injury–induced C1-related inflammation impairs long-term neurogenesis in the dentate gyrus and contributes to spatial memory retrieval dysfunction.

关键词： complement C1 dendrite dentate gyrus hippocampus neural stem cell neurogenesis neuroinflammation neurological function neuron traumatic brain injury

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铜陵矿集区深部发现126Ma的正长花岗岩:来自3000m科学钻探的证据

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中国地质 2016年第5期43卷 1495-1513页

作者：吴才来董树文王陆太王次松雷敏吴迪中国地质科学院地质研究大陆构造与动力学重点研究室北京100037 中国地质科学院北京100037 安徽地矿局321地质队安徽铜陵244033 中国地质大学地球科学学院北京100083

铜陵矿集区3000 m科学钻揭示,舒家店地区在1775 m以下存在红色的正长花岗岩,从该深度继续钻进约700 m后仍为这种岩石,而这种岩石在地表或其他钻孔中从未见到过。研究表明,正长花岗岩以富硅、富碱,富含高场强元素如Zr、Nb、Y和轻稀土元素... 详细信息

铜陵矿集区3000 m科学钻揭示,舒家店地区在1775 m以下存在红色的正长花岗岩,从该深度继续钻进约700 m后仍为这种岩石,而这种岩石在地表或其他钻孔中从未见到过。研究表明,正长花岗岩以富硅、富碱,富含高场强元素如Zr、Nb、Y和轻稀土元素(Eu除外)和较低的Mg O、Ba和Sr的含量为特征,全岩的10000Ga/Al比值为>2.6,Zr+Nb+Ce+Y>350×10-6,稀土元素配分模型具有明显的Eu负异常,微量元素原始地幔标准化曲线具有明显的Ba、Sr、P、Ti亏损,表现出A型花岗岩的地球化学属性。锆石LA-MC-ICP-MS U-Pb定年结果表明,该A型花岗岩的年龄为126 Ma,与长江中下游地区其他A型花岗岩的时代一致,属于长江中下游地区三期岩浆活动当中的第二期岩浆活动的产物。研究表明,长江中下游地区3次岩浆作用与岩石圈的多次拆沉作用密切相关,而且每一次拆沉作用都会使壳幔附近的深位岩浆房向地壳浅部迁移,而A型花岗岩则是迁移到浅部的深位岩浆房诱发的地壳部分熔融形成的岩浆,沿断裂带侵位而形成,也标志着本区的构造背景在126 Ma时处于拉张的高峰期。

关键词：锆石U-Pb定年 A型花岗岩铜陵舒家店

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Understanding the local structure and thermophysical behavior of Mg-La liquid alloys via machine learning potential

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 439-449页

作者： Jia Zhao Taixi Feng Guimin lu National Engineering Research Center for Integrated Utilization of Salt Lake Resource East China University of Science and TechnologyShanghai 200237China Joint International Laboratory for Potassium and Lithium Strategic Resources East China University of Science and TechnologyShanghai 200237China

The local structure and thermophysical behavior of Mg-La liquid alloys were in-depth understood using deep potential molecular dynamic(DPMD) simulation driven via machine learning to promote the development of Mg-La alloys. The robustness of the trained deep potential(DP) model was thoroughly evaluated through several aspects, including root-mean-square errors(RMSEs), energy and force data, and structural information comparison results;the results indicate the carefully trained DP model is reliable. The component and temperature dependence of the local structure in the Mg-La liquid alloy was analyzed. The effect of Mg content in the system on the first coordination shell of the atomic pairs is the same as that of temperature. The pre-peak demonstrated in the structure factor indicates the presence of a medium-range ordered structure in the Mg-La liquid alloy, which is particularly pronounced in the 80at% Mg system and disappears at elevated temperatures. The density, self-diffusion coefficient, and shear viscosity for the Mg-La liquid alloy were predicted via DPMD simulation, the evolution patterns with Mg content and temperature were subsequently discussed, and a database was established accordingly. Finally, the mixing enthalpy and elemental activity of the Mg-La liquid alloy at 1200 K were reliably evaluated,which provides new guidance for related studies.

关键词： magnesium-lanthanum liquid alloys local structure macroscopic properties thermodynamic behavior deep potential mo-lecular dynamic simulation

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A self-adaptive inorganic in-situ separator by particle crosslinking for nonflammable lithium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 469-480页

作者： Jiarui Yang Jiuzhou Liu wenrui Cai Ziyu Zhao Shan Wang lu He Shanshan Lv Zhiwei Zhu Zhongfeng Ji Guojiang wen Hua Li Yuanming Zhai Xuewei Fu Wei Yang Yu Wang College of Polymer Science and Engineering State Key Laboratory of Polymer Materials Engineering Sichuan University

All-safe liquid-state lithium-ion batteries(ASLS-LIBs) is of great interest as they can potentially combine the safety of all-solid-state batteries with the high performance and low manufacturing cost of traditional liquid-state LIBs. However, the practical success of ASLS-LIBs is bottlenecked by the lack of advanced separator technology that can simultaneously realize high performances in puncturing-tolerability,fire-resistance, and importantly, wetting-capability with non-flammable liquid-electrolytes. Here, we propose a concept of inorganic in-situ separator(IISS) by hybrid-sol physical crosslinking directly onto the electrode surface to address the above challenges. Particularly, the hybrid-sol is designed with silica nanoparticles as the building block and poly(vinylidene difluoride) nanoparticles as the crosslinking agent. The critical factors for controlling the IISS microstructures and properties have been systematically investigated. The advantages of the IISS have been confirmed by its fast wetting with various fireresistant liquid-electrolytes, customizable thickness and porous structures, robust interface with planar or three-dimensional(3D)-structured electrodes, and importantly, unexpected self-adaptability against puncturing. Enabled by the above merits, a fire-resistant ASLS-LIB is successfully assembled and demonstrated with stable electrochemical performance. This sol-crosslinked IISS may open an avenue for the studies on the next-generation separator technology, cell assembling, solid electrolyte processing as well as non-flammable secondary batteries.

关键词： Silica nanoparticles

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Efficient large-area flexible organic photovoltaic modules on transparent thin silver electrodes

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Science China Chemistry 2025年

作者： Cong Xie Zedong Xiong Xinlu Liu wen Wang Yang Liu Xueshi Jiang Xin lu lulu Sun Yinhua Zhou Wuhan National Laboratory for Optoelectronics Huazhong University of Science and Technology Kunming Institute of Physics

Large-area flexible organic photovoltaic（OPV） modules are challenging to achieve high power conversion efficiency（PCE）.Electrical shunts or shortages generally occur in large-area OPV modules due to the ultrathin（100–200 nm） and soft active layers. Improving the surface smoothness of bottom transparent electrode will be able to suppress the shunts and shortages. In this work, we report a method to fabricate smooth and flexible transparent electrodes based on thin silver film, and further to fabricate efficient large-area flexible OPV modules. The fabricated thin silver transparent electrodes simultaneously have high conductivity, high optical transmittance, good mechanical flexibility and low surface roughness. Humidity exposure（h.e.）treatment on MoO3effectively facilitates the continuous growth of the thin transparent silver electrode. 6 nm silver film on MoO3（h.e.） on plastic substrate shows a transmittance up to 89%, a sheet resistance of 15 Ω/sq, and a low surface roughness with a rootmean-square value of 0.276 nm. Furthermore, 52-cm2flexible organic solar modules（15 subcells） showed a certified PCE of12.66%. Furthermore, a 1350 cm2flexible component assembled by 25 pieces of 52–55 cm2modules showed certified PCE of12.10% with an open-circuit voltage of 62.85 V.

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