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Mn-based cathode materials for rechargeable batteries

Science China Chemistry 2024年第1期67卷 87-105页

作者： Xu Zhang shiqi liu Boya Wang Guoqing Wang Haozhe Du Xuanyu Wang Haidong Zhang Shu Zhao Lin Wang Haijun Yu Institute of Advanced Battery Materials and Devices Faculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124China Key Laboratory of Advanced Functional Materials Ministry of EducationBeijing University of TechnologyBeijing 100124China Create Energy&Benefit Future Co.Ltd. Beijing 100176China

The rapid expansion of renewable energies asks for great progress of energy-storage technologies for sustainable energy supplies,which raises the compelling demand of high-performance rechargeable batteries.To satisfy the huge demand from the coming energy-storage market,the resource and cost-effectiveness of rechargeable batteries become more and more important.Manganese(Mn)as a key transition element with advantages including high abundance,low cost,and low toxicity derives various kinds(spinels,layered oxides,polyanions,Prussian blue analogs,etc.)of high-performance Mn-based electrode materials,especially cathodes,for rechargeable batteries ranging from Li-ion batteries,Na-ion batteries,aqueous batteries,to multivalent metal-ion batteries.It is anticipated that Mn-based materials with Mn as the major transition-metal element will constitute a flourishing family of Mn-based rechargeable batteries(Mn RBs)for large-scale and differentiated energy-storage applications.On the other hand,several critical issues including Jahn-Teller effect,Mn dissolution,and O release greatly hinder the pace of Mn RBs,which require extensive material optimizations and battery/system improvements.This review aims to provide an investigation about Mn-based materials and batteries for the coming energy-storage demands,with compelling issues and challenges that must be overcome.

关键词： manganese cathode materials Mn-based rechargeable batteries energy storage

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Regulation of different light conditions for efficient biomass production and protein accumulation of Spirulina platensis

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Journal of Oceanology and Limnology 2024年第1期42卷 174-186页

作者： Yufei ZHANG Xianjun LI Yuhui LI shiqi liu Yanrui CHEN Miao JIA Xin WANG Lu ZHANG Qiping GAO Liang ZHANG Daoyong YU Baosheng GE State Key Laboratory of Heavy Oil Processing and Center for Bioengineering and Biotechnology China University of Petroleum(East China)Qingdao 266580China Tongwei Co. Ltd.Healthy Aquaculture Key Laboratory of Sichuan ProvinceChengdu 610093China

Light plays an important role in the photosynthesis and metabolic process of microalgae.However,how different light conditions regulate the biomass production and protein accumulation of microalgae is mostly unknown.In this study,the influence of different light conditions,including light colors,densities,and light:dark cycles on the cell growth and biochemical composition of Spirulina platensis was symmetrically characterized.Under different colored lights,S.platensis all shows an increase trend within the increased light intensity ranges;however,each showing different optimal light intensities.At the same light intensity,different colored lights show different growth rate of S.platensis following the sequence of red>white>green>yellow>blue.The maximum growth rate and protein accumulation were determined as 21.88 and 5.10 mg/(L·d)when illuminated under red LED.The energy efficiency of different light sources was calculated and ranked as red>white>blue≈green>yellow.Transcriptomic analysis suggests that red light can promote cell growth and protein accumulation by upregulating genes related to photosynthesis,carbon fixation,and C-N metabolism pathways.This study provides a conducive and efficient way to promote biomass production and protein accumulation of S.platensis by regulating light conditions.

关键词： microalgae light emitting diode protein accumulation biomass production transcriptomic analysis

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Research on Multi-Scale Feature Fusion Network Algorithm Based on Brain Tumor Medical Image Classification

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Computers, Materials & Continua 2024年第6期79卷 5313-5333页

作者： Yuting Zhou Xuemei Yang JunpingYin shiqi liu Graduate School China Academy of Engineering PhysicsBeijing100000China Department of Computational Mathematics Beijing Institute of Applied Physics and Computational MathematicsBeijing100000China National Key Laboratory of Computational Physics Beijing100088China Shanghai Zhangjiang Institute of Mathematics Shanghai201203China

Gliomas have the highest mortality rate of all brain tumors.Correctly classifying the glioma risk period can help doctors make reasonable treatment plans and improve patients’survival rates.This paper proposes a hierarchical multi-scale attention feature fusion medical image classification network(HMAC-Net),which effectively combines global features and local features.The network framework consists of three parallel layers:The global feature extraction layer,the local feature extraction layer,and the multi-scale feature fusion layer.A linear sparse attention mechanism is designed in the global feature extraction layer to reduce information redundancy.In the local feature extraction layer,a bilateral local attention mechanism is introduced to improve the extraction of relevant information between adjacent slices.In the multi-scale feature fusion layer,a channel fusion block combining convolutional attention mechanism and residual inverse multi-layer perceptron is proposed to prevent gradient disappearance and network degradation and improve feature representation capability.The double-branch iterative multi-scale classification block is used to improve the classification performance.On the brain glioma risk grading dataset,the results of the ablation experiment and comparison experiment show that the proposed HMAC-Net has the best performance in both qualitative analysis of heat maps and quantitative analysis of evaluation indicators.On the dataset of skin cancer classification,the generalization experiment results show that the proposed HMAC-Net has a good generalization effect.

关键词： Medical image classification feature fusion transformer

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Network pharmacology and experimental validation to reveal the pharmacological mechanisms of Sini decoction(四逆汤)against renal fibrosis

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Journal of Traditional Chinese Medicine 2024年第2期44卷 362-372页

作者： WANG Yan DENG Fanying liu shiqi WANG Yingli Department of Pharmacy Shanxi University of Chinese MedicineJinzhong 030619China Schools of Basic Medical Sciences Heilongjiang University of Chinese MedicineHaerbin 150040China

OBJECTIVE:To investigate the mechanism by which Sini decoction(四逆汤,SND)improves renal fibrosis(Rf)in rats based on transforming growth factor β1/Smad(TGF-β1/Smad)signaling pathway.METHODS:Network pharmacology was applied to obtain potentially involved signaling pathways in SND's improving effects on Rf.The targets of SND drug components and the targets of Rf were obtained by searching databases,such as the Traditional Chinese Medicine Systems Pharmacology Database and Analysis Platform(TCSMP)and GeenCard.The intersection targets of two searches were obtained and underwent signaling pathway analysis using a Venn diagram.Then experimental pharmacology was utilized to prove and investigate the effects of SND on target proteins in the TGF-β1/Smad signaling pathway.The Rf rat model was established by unilateral ureteral occlusion(UUO).The expression levels of transforming growth factor,matrix metalloproteinase-9(MMP-9),matrix metal protease-2(MMP-2),connective tissue growth factor(CTGF),and tissue inhibitor of metalloproteinase-1(TIMP-1)were determined by Masson staining of rat renal tissue,and immunohistochemical methods.The expression levels of Smad3,Smad2,and Smad7 in renal tissue were determined by Western blotting(WB).The mechanism of the improving effects of SND on Rf was investigated based on TGF-β1/Smad signaling pathway.RESULTS:A total of 12 drug components of Fuzi(Radix Aconiti Lateralis Preparata),5 drug components of Ganjiang(Rhizoma Zingiber),and 9 drug components of Gancao(Radix Glycy et Rhizoma)were obtained from the database search,and 207 shared targets were found.A total of 1063 Rf targets were found in the database search.According to the Venn diagram,in total,96 intersection targets were found in two database searches.The metabolic pathways involved included TGF-β signaling pathway,phosphatidylinositol-3-kinase/serine-threonine protein kinase signaling(PI3K/Akt)pathway,and hypoxia-inducible factor-1(HIF-1)signaling pathway.Masson staining analysis showed that compared with the model group,the renal

关键词： renal fibrosis network pharmacology transforming growth factor beta1 smad proteins Sini decoction

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Combining biological denitrification and electricity generation in methane-powered microbial fuel cells

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Journal of Environmental Sciences 2023年第8期130卷 212-222页

作者： Linpeng Yu Eryi Zhang Lin Yang shiqi liu Christopher Rensing Shungui Zhou Resources and Environment Fujian Agriculture and Forestry UniversityFuzhou 350002China Cranfield University CranfieldBedfordshire MK43 OALUK Biofuels Institute School of Environment and Safety EngineeringJiangsu UniversityZhenjiang 212013China

Methane has been demonstrated to be a feasible substrate for electricity generation in microbial fuel cells(MFCs)and denitrifying anaerobic methane oxidation(DAMO).However,these two processes were evaluated separately in previous studies and it has remained unknown whether methane is able to simultaneously drive these processes.Here we investigated the co-occurrence and performance of these two processes in the anodic chamber of MFCs.The results showed that methane successfully fueled both electrogenesis and denitrification.Importantly,the maximum nitrate removal rate was significantly enhanced from(1.4±0.8)to(18.4±1.2)mg N/(L·day)by an electrogenic process.In the presence of DAMO,the MFCs achieved a maximum voltage of 610 mV and a maximum power density of 143±12 mW/m^(2).Electrochemical analyses demonstrated that some redox substances(e.***.riboflavin)were likely involved in electrogenesis and also in the denitrification process.High-throughput sequencing indicated that the methanogen Methanobacterium,a close relative of Methanobacterium espanolae,catalyzed methane oxidation and cooperated with both exoelectrogens and denitrifiers(e.g.,Azoarcus).This work provides an effective strategy for improving DAMO in methane-powered MFCs,and suggests that methanogens and denitrifiers may jointly be able to provide an alternative to archaeal DAMO for methane-dependent denitrification.

关键词： Anaerobic methane oxidation Denitrification Microbial fuel cells Electricity generation Electroactive compounds Methanobacterium

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Erratum to:Regulation of different light conditions for efficient biomass production and protein accumulation of Spirulina platensis

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Journal of Oceanology and Limnology 2024年第2期42卷 695-695页

In this article,the legend for Fig.3 f&g was inadvertently mislabeled.The figure below shows the wrong one.The figure should have appeared as shown below.

关键词： figure wrong labeled

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3D reconstruction of coal pore network and its application in CO_(2)-ECBM process simulation at laboratory scale

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Frontiers of Earth Science 2022年第2期16卷 523-539页

作者： Huihuang FANG Hongjie XU Shuxun SANG shiqi liu Shuailiang SONG Huihu liu State Key Laboratory of Mining Response and Disaster Prevention and Control in Deep Coal Mines Anhui University of Science and TechnologyHuainan 232001China School of Earth and Environment Anhui University of Science and TechnologyHuainan 232001China Institute of Energy Hefei Comprehensive National Science CenterHefei 230000China Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization China University of Mining and TechnologyXuzhou 221008China Low Carbon Energy Institute China University of Mining and TechnologyXuzhou 221008China Shandong Provincial Lunan Geo-engineering Exploration Institute Jining 272100China

Three-dimensional(3D)reconstruction of the equivalent pore network model(PNM)using X-ray computed tomography(CT)data are of significance for studying the CO_(2)-enhanced coalbed methane recovery(CO_(2)-ECBM).The docking among X-ray CT technology,MATLAB,with COMSOL software not only can realize the 3D reconstruction of PNM,but also the CO_(2)-ECBM process simulation.The results show that the Median filtering algorithm enabled the de-noising of the original 2D CT slices,the image segmentation of all slices was realized based on the selected threshold,and the PNM can be constructed based on the Maximum Sphere algorithm.The mathematical model of CO_(2)-ECBM process fully coupled the expanded Langmuir equation.At the same time for CO_(2)injection,CH_(4)pressure tends to decrease with the increase of CO_(2)pressure,but its difference is not obvious.The CH_(4)pressure in the slice center changed a lot,while at the edge it changed a little under different CO_(2)pressures.The injected CO_(2)was transported to matrix along the macro and micro-fractures with continuous flow.The injected CO_(2)first replaced the adsorbed CH_(4)by covering the inner surface of macro-pores and meso-pores to form the single molecular layer adsorption of CO_(2).Then they migrated to micro-pores by Fick’s diffusion,sliding flow,and surface diffusion.Furthermore,the CO_(2)replaced CH_(4)adsorbed by volumetric filling in micro-pores,and formed the multi-molecular layer adsorption of CO_(2).The gas pressure and migration path between CO_(2)and CH_(4)are opposite.This study can provide a theoretical basis for studying digital rock physics technology and enrich the development of CO_(2)-ECBM technology.

关键词： CO_(2)-ECBM 3D reconstruction numerical simulation X-ray CT COMSOL Qinshui Basin

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Determination of representative elementary volume of digital coal based on fractal theory with X-ray CT data and its application in fractal permeability predication model

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Frontiers of Earth Science 2022年第3期16卷 657-670页

作者： Huihuang FANG Shuxun SANG shiqi liu Huihu liu Hongjie XU Yanhui HUANG School of Earth and Environment Anhui University of Science and TechnologyHuainan 232001China Institute of Energy Hefei Comprehensive National Science CenterHefei 230000China Low Carbon Energy Institute China University of Mining and TechnologyXuzhou 221008China School of Resources and Geosciences China University of Mining and TechnologyXuzhou 221116China Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization China University of Mining and TechnologyXuzhou 221008China State Key Laboratory of Petroleum Resources and Prospecting China University of PetroleumBeijing 102249China

Representative elementary volume(REV)is the key to study the heterogeneity of digital coal and characterize its macroscopic and microscopic properties.The permeability evolution law of digital coal based on REV analysis can provide theoretical support for the application of permeability prediction model in multi-scale reservoirs.This study takes typical coal samples from Bofang and Sihe coal mines in Qinshui Basin as research object.First,the nondestructive information of two samples is scanned and visualized.Secondly,the calculation methods of two-dimensional(2D)and threedimensional(3D)fractal dimensions of pores and fractures are illustrated.Then,the determination methods of REV based on porosity and fractal dimension are compared.Finally,the distribution pattern of fractal dimension and porosity curves is studied,the relationship between 2D and 3D fractal dimension is characterized,and the application of fractal permeability model in permeability analysis of multi-scale reservoir is further discussed.The REV size varies greatly in different vertex directions of the same sample and between samples,so REV analysis can only be performed in specific directions.When the REV based on fractal dimension is determined,the porosity curve continues to maintain a downward trend and then tends to be stable.The 2D fractal dimension has a positive linear correlation with the 3D fractal dimension,and the porosity can be expressed as a linear function of the fractal dimension.The permeability through REV analysis domain is mainly affected by fractal dimension,dip angle,azimuth angle and maximum fracture length,which is of great significance for exploring permeability evolution law of coal reservoir at different scales.This study is of great significance for enriching the determination methods of REV in digital coal and exploring the permeability evolution law of multi-scale reservoirs.

关键词： representative elementary volume fractal dimension permeability digital coal X-ray CT Qinshui Basin

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Expert consensus on treating esophageal stenosis in children by magnetic recanalization

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Chinese Medical Journal 2022年第7期135卷 796-798页

作者： shiqi liu Yi Lyu Scientific Committee of the Third International Conference of Magnetic Surgery Department of Neonatal Surgery Xi’an Children’s HospitalXi’an Jlaotong UniversityXi’anShaanxi 710003China Natlonal Local Joint Engineering Research Center for Precision Surgery and Regenerative Medicine The First Affiliated Hospital of Xi’an Jiaotong UniversityXi’anShaanxi 710061China Shaanxi Institute for Pediatric Diseases Xi’anShaanxi 710003China Xi’an Key Laboratory of Children’s Health and Diseases Xi’anShaanxi 710003China Department of Hepatobiliary Surgery Institute of Advanced Surgical Technology and EngineeringThe First Affiliated Hospital of Xi’an Jiaotong UniversityXi’anShaanxi 710061China Shaanxi Provincial Center for Regenerative Medicine and Surgical Engineering The First Affiliated Hospital of Xi’an Jiaotong UniversityXi’anShaanxi 710061China 不详

Postsurgical stricture is the most common cause of esophageal stenosis in children after congenital esophageal atresia repair,^([1,2])followed by congenital esophageal stenosis and chemical corrosion burns.^([3])Endoscopic or radiologic balloon dilation is the standard method for treatment of esophageal stenosis,but in some complicated cases with severe hyperplasia and severe restenosis and even occlusion,the effect of endoscopic treatment is limited.In 1993,Bulynin et al^([4])reported,for the first time.

关键词： esophageal stenosis balloon

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Experimental study on the deformation behaviour,energy evolution law and failure mechanism of tectonic coal subjected to cyclic loads

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International Journal of Mining Science and Technology 2022年第6期32卷 1301-1313页

作者： Deyi Gao Shuxun Sang shiqi liu Jian Wu Jishi Geng Wang Tao Tengmin Sun Key Laboratory of Coalbed Methane Resources and Reservoir Formation Process China University of Mining and TechnologyXuzhou 221116China School of Resources and Geosciences China University of Mining and TechnologyXuzhou 221116China Carbon Neutrality Institute China University of Mining and TechnologyXuzhou 221116China Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization China University of Mining and TechnologyXuzhou 221116China China United Coalbed Methane Co.Ltd.(CUCBM) Beijing 100083China

Compared to intact coal,tectonic coal exhibits unique characteristics.The deformation behaviours under cyclic loading with different confining pressures and loading rates are monitored by MTS815 test system,and the mechanical and energy properties are analysed using experimental data.The results show that the stress-strain curve could be divided into four stages in a single cycle.The elastic strain and elastic energy density increase linearly with deviatoric stress and are proportional to the confining pressure and loading rate;irreversible strain and dissipated energy density increase exponentially with deviatoric stress,inversely proportional to the confining pressure and loading rate.The internal structure of tectonic coal is divided into three types,all of which are damaged under different deviatoric stress levels,thereby explaining the segmentation phenomenon of stress-strain curve of tectonic coal in the cyclic loading process.Tectonic coal exhibits nonlinear energy storage characteristics,which verifies why the tectonic coal is prone to coal and gas outburst from the principle of energy dissipation.In addition,the damage mechanism of tectonic coal is described from the point of energy distribution by introducing the concepts of crushing energy and friction energy.

关键词： Tectonic coal Cyclic loading Deformation behaviour Energy evolution Failure mechanism

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