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Saturated hydraulic conductivity of compacted bentonite-sand mixtures before and after gas migration in artificial seawater

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Journal of Rock Mechanics and Geotechnical Engineering 2023年第1期15卷 216-226页

作者： Yasutaka Watanabe shingo yokoyama Misato Shimbashi Yoichi Yamamoto Takahiro Goto Sustainable System Research Laboratory Central Research Institute of Electric Power IndustryChibaJapan Science and Technology Department Nuclear Waste Management Organization of JapanTokyoJapan

To understand the self-healing property of an engineered barrier for radioactive waste disposal,the hydraulic conductivity of compacted bentoniteesand mixtures saturated with artificial seawater(SW)before and after gas migration was ***-and Ca-bentonites were mixed with fine sand at a ratio of 70%bentonite in dry *** aspects were considered during the experiment:the hydraulic conductivity of the specimen that was resaturated after gas migration and the distribution of water content immediately after gas migration to study gas migration *** gas migrated through the entire cross-section of the specimen,and gas breakthrough occurred in the equilibrium swelling pressure range ***,the gas flow rate reached a sufficient large value when the gas pressure was approximately twice the equilibrium axial pressure(the sum of swelling and confining pressures),which excluded the back *** the gas migration pathway was not visible when the specimen was observed immediately after gas migration,the water content distribution showed that several parts of the specimen with lower water content were connected in the direction of gas *** resaturation,the change in permeability was within a limited rangedtwo to three times larger than that before gas migration for each type of bentonite in *** slight change suggests that gas migration creates a pore structure that cannot be sealed via crystalline swelling of montmorillonite in SW,even if highly compacted bentonite is used under a constant-volume condition.

关键词： Bentonite Gas migration Hydraulic conductivity Seawater(SW) Self-healing

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Hydrothermal Formation of Lath-Shaped Trioctahedral Smectite with High Crystallinity

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Acta Geologica Sinica(English Edition) 2006年第2期80卷 290-295页

作者： Hirohisa YAMADA Kenji TAMURA shingo yokoyama Yujiro WATANABE Ecomaterials Center Nuclear Fuel Cycle Back-end Research Center College of Environmental Engineering and Architecture

Lath-shaped and highly crystalline trioctahedral smectites were synthesized under hydrothermal conditions. The quenched glasses with stoichiometrically dehydrated Na-smectite compositions were treated at （a） 500℃ and 100 MPa for 1 and 11 days; and （b） 300℃ and 100 MPa for 7 days. The crystallinity and particle size of products were dependent on the chemical composition of the starting glass, synthetic temperature and duration of hydrothermal treatment. The high structural ordering and large dimensions of the products were confirmed from the sharpness of XRD peaks; and hydration behavior under controlled relative humidity. Transmission electron microscopy was also performed for the characterization of the particle size of product. Particle sizes vary from ca. 10 nm to a few pm by changing the chemical compositions of the starting materials. The product with the highest structural ordering and largest dimension was obtained from Nao.33（Mg1.83Al0.67）Si4O11 glass treated at 500℃ and 100 MPa for 1 day. The obtained results also confirmed the metastability and compositional dependency in the formation of highly crystalline trioctahedral smectite at hydrothermal conditions.

关键词： high crystallinity hydration behavior hydrothermal formation lath-shaped trioctahedral smectite

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热液合成板状高结晶度三八面体蒙脱石

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地质学报 2006年第4期80卷 616-616页

作者： Hirohisa YAMADA Kenji TAMURA shingo yokoyama Yujiro WATANABE Ecomaterials Center National Institute for Materials Science1-1 NamikiTsukubaIbaraki 305-0044Japan Nuclear Fuel Cycle Back-end Research Center Central Research Institute of Electric Power Industry1646 AbikoChiba 270-1194Japan CollegeofEnvironmentalEngineeringandArchitecture

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