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振荡来流下柔性立管涡激振动“分时特性”试验研究

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振动与冲击 2014年第21期33卷 1-7页

作者：王俊高付世晓许玉旺宋磊建上海交通大学海洋工程国家重点实验室上海200240

悬链线立管在顶部浮体的带动下,其动力响应会诱发其周围产生相对来流,而这种振荡来流将激励立管悬垂段产生"间歇性"的涡激振动。在海洋工程水池中对不同最大约化速度URmax、KC数组合下的振荡来流作用下的柔性立管进行模型试验研究,利用... 详细信息

悬链线立管在顶部浮体的带动下,其动力响应会诱发其周围产生相对来流,而这种振荡来流将激励立管悬垂段产生"间歇性"的涡激振动。在海洋工程水池中对不同最大约化速度URmax、KC数组合下的振荡来流作用下的柔性立管进行模型试验研究,利用光纤应变片测量柔性立管模型的涡激振动响应。结合模态分析与小波分析对试验数据进行分析,观察到一种区别于定常来流下的涡激振动响应形式,即具有"振幅调制"及"模态转换"的"分时特性"的涡激振动。最后讨论并总结了最大约化速度URmax以及KC数对涡激振动"分时特性"的影响规律。

关键词：振幅调制模态转换模态分析小波分析振荡来流涡激振动

g-C_(3)N_(4)nanosheets coupled with CoSe_(2)as co-catalyst for efficient photooxidation of xylose to xylonic acid

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Green Energy & Environment 2025年第1期10卷 231-238页

作者： Qi Hao Yijun Liu Ren Zou Ge shi shilian Yang Linxin Zhonga Wu Yang xiao Chi Yunpeng Liu shimelis Admassie Xinwen Peng State Key Laboratory of Pulp and Paper Engineering South China University of TechnologyGuangzhou510641GuangdongChina Hainan Key Laboratory of Storage&Processing of Fruits and Vegetables Agricultural Products Processing Research InstituteChinese Academy of Tropical Agricultural SciencesZhanjiangGuangdong524001China Department of Chemistry and Centre for Advanced 2D Materials(CA2DM)National University of Singapore 3 Science Drive 3 Singapore117543Singapore School of Materials Science and Hydrogen Energy Foshan UniversityFoshan528231GuangdongChina Department of Chemistry Addis Ababa UniversityPO BOX 1176Addis AbabaEthiopia

Photocatalysis has emerged as an effective approach to sustainably convert biomass into value-added ***_(2)is a promising nonprecious,efficient cocatalyst for photooxidation,which can facilitate the separation of photogenerated electron–holes,increase the reaction rates,and enhance photocatalytic *** this work,we synthesized a stable and efficient photocatalysis system of CoSe_(2)/g-C_(3)N_(4)through attaching CoSe_(2)on g-C_(3)N_(4)sheets,with a yield of 50.12%for the selective photooxidation of xylose to xylonic *** light illumination,the photogenerated electrons were prone to migrating from g-C_(3)N_(4)to CoSe_(2)due to the higher work function of CoSe_(2),resulting in the accelerated separation of photogenerated electron–holes and the promoted ***,this study reveals the unique function of CoSe_(2),which can significantly promote oxygen adsorption,work as an electron sink and accelerate the generation of$O2-,thereby improving the selectivity toward xylonic acid over other *** work provides useful insights into the design of selective photocatalysts by engineering g-C_(3)N_(4)for biomass high-value utilization.

关键词： Biomass photooxidation Hemicelluloses Xylose g-C_(3)N_(4) Xylonic acid

Tumor inflammation-specific self-amplifying fluorescent molecular probes induce an anti-tumor immune response

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Science China Chemistry 2025年第1期68卷 273-287页

作者： Shuguang Yang Lijun Hu Hong xiao Zecong xiao Xintao Shuai PCFM Lab of Ministry of Education School of Materials Science and Engineering Sun Yat-sen University Department of Ultrasound The Fifth Affiliated Hospital Sun Yat-sen University Department of Medical Ultrasound The Third Affiliated Hospital of Sun Yat-sen University Nanomedicine Research Center The Third Affiliated Hospital of Sun Yat-sen University

Enhancing the concentration of exogenous molecular drugs within the tumor microenvironment through enzyme-catalyzed polymerization presents a novel strategy for cancer therapy. Nonetheless, the optimization of the catalytic efficiency is often impeded by the inefficient expression of enzymes. Herein, we reported a self-amplifying fluorescent molecular probe, Bis-HTPICG, for photodynamic therapy(PDT) and subsequent PDT-induced immunoreaction. The Bis-HTP-ICG probe possesses a noticeable enzyme-catalyzed polymerization facilitated by myeloperoxidase(MPO), a crucial enzyme secreted by neutrophils at inflammation sites. Upon exposure to laser irradiation, Bis-HTP-ICG showed a high PDT efficacy, inducing an acute inflammatory response that stimulates further recruitment of neutrophils and then elevated MPO secretion. The heightened level of MPO enhances the accumulation of the Bis-HTP-ICG via self-polymerization or binding with intratumoral proteins following MPO enzyme catalysis, instigating a self-amplifying chain reaction cycle involving Bis-HTP-ICG, neutrophils and ***, PDT efficiently incites immunogenic cell death(ICD) in tumor cells, initiating an anti-tumor immune response including dendritic cells(DCs) maturation, T cell proliferation and reprogramming of tumor-associated neutrophils(TANs). This work portrays a promising strategy for self-amplification of fluorescent molecular probes through adjustable enzyme levels,potentially offering a unique avenue to enhance the tumor accumulation of molecular drugs for improved tumor therapy.

关键词： fluorescent molecular probes self-amplifying myeloperoxidase photodynamic therapy

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考虑海底边界影响的管道水动力特性研究

中国海洋平台 2011年第5期26卷 17-23页

作者：周青付世晓上海交通大学上海200030

利用雷诺平均方程,采用SSTk-ω湍流模式,建立了一个研究海底管道水动力特性的数值模型。利用该模型在Re为对不同间隙比下定常流通过海底悬跨管道进行了数值模拟,得到了管道的升阻力系数并分析了升阻力与间隙比的关系。通过与试验数据和... 详细信息

利用雷诺平均方程,采用SSTk-ω湍流模式,建立了一个研究海底管道水动力特性的数值模型。利用该模型在Re为对不同间隙比下定常流通过海底悬跨管道进行了数值模拟,得到了管道的升阻力系数并分析了升阻力与间隙比的关系。通过与试验数据和数值结果进行对比和对升阻力系数曲线作FFT变换,分析了该模型的可靠性,推测出临界间隙比,进而分析了尾涡形式及其产生与抑制机理。

关键词：数值模型海底管道海底边界水动力特性圆柱绕流边界层流

甲苯常压催化氧化制苯甲酸及其它芳烃的氧化反应的研究

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合成化学 1998年第4期 103-107页

作者： Zhang,Xiang fu shi,xiao Tian (Chengdu Institute of Organic Chemistry, Academia of Sinica, Chengdu,610041)

以２５％甲苯无水乙酸作反应液，钴、锰和铵的混合盐作催化剂，乙腈作促进剂，纯氧为氧化剂，在１１０℃±２℃下，常压反应１５ｈ，苯甲酸收率达８５％。用该催化剂体系氧化其它芳烃时，亦可获得类似结果。若芳烃侧链烷基Ｒ＝Ｃ１～Ｃ... 详细信息

以２５％甲苯无水乙酸作反应液，钴、锰和铵的混合盐作催化剂，乙腈作促进剂，纯氧为氧化剂，在１１０℃±２℃下，常压反应１５ｈ，苯甲酸收率达８５％。用该催化剂体系氧化其它芳烃时，亦可获得类似结果。若芳烃侧链烷基Ｒ＝Ｃ１～Ｃ６时，首先起反应的是与苯环相邻的碳原子，伯碳由醛变为酸；仲碳由酮升温后断链变酸；叔碳或烯键则直接断键变为酸。

关键词：甲苯苯甲酸芳烃促进剂乙腈催化氧化

Double [5]carbohelicene: facile synthesis, chiroptical properties,isomerization study, and lasing application

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Science China Chemistry 2025年第1期68卷 233-240页

作者： Peipei Liu Yantong Li Meng-Xiang Wu Hao Kang xiao-Li Zhao Lin Xu Linlin Liu xiaodong Li Junfeng Fang Zhiwei Fang Ya Cheng Hai-Bo Yang Huakang Yu Xueliang shi State Key Laboratory of Petroleum Molecular & Process Engineering Shanghai Key Laboratory of Green Chemistry and Chemical ProcessesSchool of Chemistry and Molecular Engineering East China Normal University School of Physics and Optoelectronics South China University of Technology Institute of Polymer Optoelectronic Materials & Devices State Key Laboratory of Luminescent Materials & Devices South China University of Technology School of Physics and Electronic Science Engineering Research Center of Nanophotonics & Advanced Instrument Ministry of EducationEast China Normal University State Key Laboratory of Precision Spectroscopy School of Physics and Electronic Science East China Normal University

Double carbohelicenes have attracted considerable attention due to their aesthetic structures, distinct π-conjugation extension, inherent chirality, and intriguing optical and electronic properties. Herein, the concise de novo synthesis of a new double[5]carbohelicene 1 together with its chiroptical properties, isomerization process and lasing application is presented. 1 was synthesized by a simple protocol involving the formation of a 6,6′-bipentacene as the key intermediate. It is worth noting that1 existed as two diastereomers 1-PP/MM and 1-PM, which were successfully isolated and unambiguously confirmed by Xray crystallography. The optical resolution of the racemic 1-PP/MM was successfully achieved by chiral-phase highperformance liquid chromatography（HPLC）, and 1-PP and 1-MM were characterized by circular dichroism. Interestingly, it was found that 1-PP/MM could be completely isomerized to 1-PM upon heating, and the detailed thermodynamics and kinetics of the isomerization process were systematically investigated. 1-PM exhibited deep-red luminescence with emission maximum at 723 nm and fluorescence quantum yield as high as 32.95%. Consequently, we can showcase the lasing application of 1-PM by doping with epoxy resin to assemble a bottle microlaser spontaneously, which the lasing wavelength is 796.6 nm at a threshold of 0.8 m J cm-2. We believe that our studies, including the facile synthesis methodology, detailed isomerization studies, and lasing application, will shed some light on the design and synthesis of novel carbohelical systems with more functions.

关键词： double carbohelicene optical resolution organic laser isomerization X-ray diffraction

D-DeepOCSORT: multi-object tracking algorithm based on LiDAR and monocular camera

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Optoelectronics Letters 2025年

作者： HE xiao REN Shuai LIU Chang shi Lei School of Information Engineering， Chang'an University School of Control of Robotic and Autonomous Systems， University of California Berkeley

Multi-object tracking is a fundamental problem in computer vision， and DeepOCSORT， due to its reliance on the 2D image position information of targets， tends to exhibit prediction drift. To enhance the tracking stability of DeepOCSORT， this paper proposes a novel multi-sensor data fusion-based multi-object tracking method. Specifically， we build upon the DeepOCSORT foundation and additionally integrate target velocity information directly measured by LiDAR. The introduction of this velocity information is conducted from three perspectives: firstly， during data association， a penalty term is constructed based on the differences in target velocities to constrain generating matches with consistent velocities; secondly， using LiDAR velocity for initialization and online updating of the velocity state within the tracker， making tracking predictions more stable; thirdly， controlling the degree of dependence on velocity information by adjusting the process noise covariance matrix. Evaluation results on the KITTI dataset demonstrate that compared to the original DeepOCSORT， the proposed improved multi-source heterogeneous information fusion method significantly enhances tracking performance， with maximum improvements of 3.35， 3.26， and 3.71 on the HOTA， MOTA， and IDF1 metrics， respectively. This study provides an effective approach to building a more stable and accurate multi-object tracking system.

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新型方舱大板胶粘剂的研制及其性能研究

国防制造技术 2009年第5期 48-51页

作者：周玲石小富中国电子科技集团公司第二十八研究所江苏南京210007

方舱是指控系统的主要装载平台,而胶粘剂是方舱生产中复合型关键原料,我所结合自身产品需要研制环氧类方舱大板胶粘剂,分析其固化机理,进行胶粘剂拉伸剪切强度、180°剥离强度、大板高低温贮存、整舱日照热效应试验,并将其与国外某些胶... 详细信息

方舱是指控系统的主要装载平台,而胶粘剂是方舱生产中复合型关键原料,我所结合自身产品需要研制环氧类方舱大板胶粘剂,分析其固化机理,进行胶粘剂拉伸剪切强度、180°剥离强度、大板高低温贮存、整舱日照热效应试验,并将其与国外某些胶粘剂相关性能进行比较,结果表明该胶粘剂具有良好的力学和环境适应性性能,适用于方舱生产。该胶黏剂具有良好的经济效益和社会效益,今后将进一步推广应用到民用市场。

关键词：方舱大板胶粘剂环境适应性

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柔性立管阻力特性试验数据处理技术

舰船科学技术 2021年第3期43卷 88-94页

作者：李曼徐永超单铁兵付世晓中国船舶及海洋工程设计研究所上海200011 上海交通大学海洋工程国家重点实验室上海200240

本文提出3种数据处理方法分析均匀来流中柔性立管的初始阻力特性。首先通过分析柔性立管在均匀来流中的变形及振动情况,分离出立管流向的初始变形对应的弯曲应变。根据复杂梁的弯曲变形理论,建立起弯曲应变与平均阻力之间的微分方程。随... 详细信息

本文提出3种数据处理方法分析均匀来流中柔性立管的初始阻力特性。首先通过分析柔性立管在均匀来流中的变形及振动情况,分离出立管流向的初始变形对应的弯曲应变。根据复杂梁的弯曲变形理论,建立起弯曲应变与平均阻力之间的微分方程。随后,针对试验中获取的立管轴向力及立管表面弯曲应变,提出计算平均阻力的数据处理方法,并进行算例验证与分析。最终使用提出的数据处理方法分析试验数据,得到立管表面各截面处的阻力分布。

关键词：柔性立管初始应变初始阻力数据处理