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Non-fullerene Acceptors with a Thieno[3,4-c]pyrrole-4,6-dione(TPD) Core for Efficient Organic Solar Cells

Chinese Journal of Polymer Science 2019年第10期37卷 1005-1014,I0005页

作者： shi-zhe geng Wei-Tao Yang Jian Gao Shui-Xing Li Min-Min shi Tsz-Ki Lau Xin-Hui Lu Chang-Zhi Li Hong-zheng Chen Key Laboratory of Macromolecular Synthesis and Functionalization(Ministry of Education) State Key Laboratory of Silicon MaterialsDepartment of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027China Department of Physics The Chinese University of Hong KongNew TerritoriesHong KongChina

To achieve the red-shifted absorptions and appropriate energy levels of A-D-A type non-fullerene acceptors(NFAs), in this work, we design and synthesize two new NFAs, named TPDCIC and TPDCNC, whose electron-donating(D) unit is constructed by a thieno[3,4-c]pyrrole-4,6-dione(TPD) core attached to two cyclopentadithiophene(CPDT) moieties at both sides, and the electronaccepting(A) end-groups are 2-(3-oxo-2,3-dihydroinden-1-ylidene)malononitrile(IC) and 2-(3-oxo-2,3-dihydro-1 H-cyclopenta[b]naphthalen-1-ylidene)malononitrile(NC), respectively. Benefiting from TPD core, which easily forms quinoid structure and O···H or O···S intramolecular noncovalent interactions, TPDCIC and TPDCNC show more delocalization of π-electrons and perfect planar molecular geometries, giving the absorption ranges extended to 822 and 852 nm, respectively. Furthermore, the highest occupied molecular orbital(HOMO) levels of TPDCIC and TPDCNC remain relatively low-lying due to the electronegativity of the carbonyl groups on TPD core. Considering that the absorptions and energy levels of the two NFAs match well with those of a widely used polymer donor, PBDB-T, we fabricate two kinds of organic solar cells(OSCs) based on the PBDB-T:TPDCIC and PBDB-T:TPDCNC blended films, respectively. Through a series of optimizations, the TPDCIC-based devices yield an impressing power conversion efficiency(PCE)of 10.12% with a large short-circuit current density(JSC) of 18.16 mA·cm-2, and the TPDCNC-based ones exhibit a comparable PCE of9.80% with a JSC of 17.40 mA·cm-2. Our work is the first report of the TPD-core-based A-D-A type NFAs, providing a good reference for the molecular design of high-performance NFAs.

关键词： Non-fullerene acceptors (NFAs) Organic solar cells (OSCs) Thieno[3,4-c]pyrrole-4,6-dione (TPD) Narrow bandgap Energy levels

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Command filtered integrated estimation guidance and control for strapdown missiles with circular field of view

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Defence Technology（防务技术） 2024年第5期35卷 211-221页

作者： Wei Wang Jiaqi Liu shiyao Lin Baokui geng Zhongjiao shi School of Aerospace Engineering Beijing Institute of TechnologyBeijing 10081China China Research and Development Academy of Machinery Equipment Beijing 100089China Northwest Industries Group CO. Ltd.Xi'an 710043China

In this paper,an integrated estimation guidance and control(IEGC)system is designed based on the command filtered backstepping approach for circular field-of-view(FOV)strapdown *** threedimensional integrated estimation guidance and control nonlinear model with limited actuator deflection angle is established considering the seeker's FOV *** boundary time-varying integral barrier Lyapunov function(IBLF)is employed in backstepping design to constrain the body line-of-sight(BLOS)in IEGC system to fit a circular ***,the nonlinear adaptive controller is designed to estimate the changing aerodynamic *** generalized extended state observer(GESO)is designed to estimate the acceleration of the maneuvering targets and the unmatched time-varying disturbances for improving tracking ***,the command filters are used to solve the"differential expansion"problem during the backstepping *** Lyapunov theory is used to prove the stability of the overall closed-loop IEGC ***,the simulation results validate the integrated system's effectiveness,achieving high accuracy strikes against maneuvering targets.

关键词： Integrated estimation guidance and control Circular field-of-view Time-varying integral barrier Lyapunov function Command filtered backstepping control Nonlinear adaptive control Extended state observer

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Locally and globally uniform approximations for ruin probabilities of a nonstandard bidimensional risk model with subexponential claims

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Applied Mathematics(A Journal of Chinese Universities) 2024年第1期39卷 98-113页

作者： LIU Zai-ming geng Bing-zhen WANG shi-jie School of Mathematics and Statistics Central South UniversityChangsha 410083China School of Big Data and Statistics Anhui UniversityHefei 230601China

Consider a nonstandard continuous-time bidimensional risk model with constant force of interest,in which the two classes of claims with subexponential distributions satisfy a general dependence structure and each pair of the claim-inter-arrival times is arbitrarily *** some mild conditions,we achieve a locally uniform approximation of the finite-time ruin probability for all time horizon within a finite *** we further assume that each pair of the claim-inter-arrival times is negative quadrant dependent and the two classes of claims are consistently-varying-tailed,it shows that the above obtained approximation is also globally uniform for all time horizon within an infinite interval.

关键词： bidimensional risk model asymptotic formula subexponential distribution consistently varying tail ruin probability

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A continuous-wave Nd:YVO_(4)-KGW intracavity Raman laser with over 34% diode-to-Stokes optical efficiency

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High Power Laser Science and Engineering 2024年第2期12卷 62-68页

作者： Quan Sheng Jingni geng Tianchang Liu shijie Fu Wei shi Jianquan Yao Institute of Laser and Optoelectronics School of Precision Instrument and Optoelectronics EngineeringTianjin UniversityTianjinChina Key Laboratory of Optoelectronic Information Technology(Ministry of Education) Tianjin UniversityTianjinChina

We demonstrate a continuous-wave(CW)Nd:YVO_(4)-potassium gadolinium tungstate(KGW)intracavity Raman laser with a diode-to-Stokes optical efficiency of 34.2%.By optimizing the cavity arrangement and reducing the cavity losses,8.47 W Stokes output at 1177 nm was obtained under an incident 878.6 nm diode pump power of 24.8 *** influence of cavity losses on the power and efficiency of the CW Raman laser,as well as the potential for further optimization,was investigated based on the numerical *** observation of thermally-induced output rollover was well explained by the calculation of the thermal lensing and cavity stability,indicating that the end-face curvature played an important role when the end-face of the crystal was highly reflective coated to make the cavity.A 10.9 W Stokes output under 40.9 W incident pump was also demonstrated with a cavity arrangement less sensitive to the end-face curvature,which is the highest output power of CW intracavity Raman lasers reported.

关键词： continuous wave intracavity Raman laser KGW crystal thermal lens

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CPT: a pre-trained unbalanced transformer for both Chinese language understanding and generation

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Science China(Information Sciences) 2024年第5期67卷 43-55页

作者： Yunfan SHAO Zhichao geng Yitao LIU Junqi DAI Hang YAN Fei YANG zhe LI Hujun BAO Xipeng QIU School of Computer Science Fudan University Shanghai Key Laboratory of Intelligent Information Processing Fudan University zhejiang Lab

In this paper, we take the advantage of previous pre-trained models(PTMs) and propose a novel Chinese pre-trained unbalanced transformer(CPT). Different from previous Chinese PTMs, CPT is designed to utilize the shared knowledge between natural language understanding(NLU) and natural language generation(NLG) to boost the performance. CPT consists of three parts: a shared encoder, an understanding decoder, and a generation decoder. Two specific decoders with a shared encoder are pretrained with masked language modeling(MLM) and denoising auto-encoding(DAE) tasks, *** the partially shared architecture and multi-task pre-training, CPT can(1) learn specific knowledge of both NLU or NLG tasks with two decoders and(2) be fine-tuned flexibly that fully exploits the potential of the model. Moreover, the unbalanced transformer saves the computational and storage cost, which makes CPT competitive and greatly accelerates the inference of text generation. Experimental results on a wide range of Chinese NLU and NLG tasks show the effectiveness of CPT.

关键词： pre-trained model transformer language model generation unified model

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Study on the catch,bycatch and discard of Chinese pelagic longline fisheries in the Atlantic Ocean

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Aquaculture and Fisheries 2024年第2期9卷 280-286页

作者： Boyi Pan Jiangfeng Zhu Qinqin Lin zhe geng Feng Wu Yuying Zhang College of Marine Sciences Shanghai Ocean UniversityShanghai201306China Key Laboratory of Sustainable Exploitation of Oceanic Fisheries Resources Ministry of EducationShanghai Ocean UniversityShanghai201306China Department of Biological Sciences Florida International UniversityNorth MiamiFL33181USA

Catch,bycatch and discard information is important for the assessment and management of *** Chinese pelagic tuna longline observer data from 2010 to 2018,we studied the catch composition in the Chinese pelagic tuna longline fisheries in Atlantic targeting bigeye tuna(Thunnus obesus)and bluefin tuna(Thunnus thynnus),and analyzed the survival status and discard rates of common bycatch species.A total of 55 species,including tunas,billfishes,sharks,sea turtles,cetaceans,seabirds,and other pelagic species,were *** results indicated that the catch composition of the Chinese pelagic tuna longline fishery targeting bigeye tuna was significantly different from that targeting bluefin *** annual discard rates of common species decreased over this *** rate by length and discard mortality for common species were varied among *** is the first study to estimate catch,bycatch,and discard using Chinese pelagic tuna longline observer data in the Atlantic Ocean,which is important for the management of Chinese tuna longline fisheries in Atlantic Ocean.

关键词： Longline fishery Catch composition Discard Size distribution Atlantic

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Manipulator tracking technology based on FSRUKF

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Journal of Systems Engineering and Electronics 2024年第2期35卷 473-484页

作者： shi Guoqing ZHANG Boyan ZHANG Jiandong YANG Qiming HUANG Xiaofeng QUE Jianyao PU Junwei geng Xiutang School of Electronics and Information Northwestern Polytechnical UniversityXi’an 710072China Northwest Institute of Mechanical&Electrical Engineering Xianyang 712000China

Aiming at the shortcoming that the traditional industrial manipulator using off-line programming cannot change along with the change of external environment,the key technologies such as machine vision and manipulator control are studied,and a complete manipulator vision tracking system is ***,Denavit-Hartenberg(D-H)parameters method is used to construct the model of the manipulator and analyze the forward and inverse kinematics equations of the *** the same time,a binocular camera is used to obtain the threedimensional position of the ***,in order to make the manipulator track the target more accurately,the fuzzy adaptive square root unscented Kalman filter(FSRUKF)is proposed to estimate the target ***,the manipulator tracking system is built by using the position-based visual *** simulation experiments show that FSRUKF converges faster and with less error than the square root unscented Kalman filter(SRUKF),which meets the application requirements of the manipulator tracking system,and basically meets the application requirements of the manipulator tracking system in the practical experiments.

关键词： square root unscented Kalman filter(SRUKF) fuzzy inference manipulator visual servo

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The effects of in ovo feeding of selenized glucose on liver selenium concentration and antioxidant capacity in neonatal broilers

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Chinese Chemical Letters 2024年第6期35卷 312-315页

作者： Jiahui Li Qiao shi Ying Xue Mingde zheng Long Liu Tuoyu geng Daoqing Gong Minmeng Zhao Jiangsu Key Laboratory of Animal genetic Breeding and Molecular Design College of Animal Science and TechnologyYangzhou UniversityYangzhou 225009China Joint International Research Laboratory of Agriculture and Agri-Product Safety of Ministry of Education of China Yangzhou UniversityYangzhou 225009China

Selenium is an essential trace element for humans and *** the active center of selenoproteins,the addition of selenium is beneficial to enhance the antioxidant ***,the high cost limits the application of organic Se in agriculture animal *** glucose(SeGlu)is a newly invented organoselenium material with good stability,low toxicity and low *** assay found that SeGlu was able to increase selenium deposition in liver of newborn broilers,and enhance the antioxidant capacity of liver by elevating the activities of antioxidant enzymes such as total superoxide dismutase and glutathione *** paper as the first example clarifying the mechanism of SeGlu to enhance the antioxidant ability of chicks,shows that SeGlu can be used as an organic selenium enrichment additive for early nutrition of *** a cross-discipline study involving chemistry,biology and agriculture animal science,the work may be beneficial for studies in related fields and prompt the development of the selenium science.

关键词： Selenized glucose In ovo feeding Antioxidant capacity Selenium Broiler

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Mixed Dead-time Effect Suppression Strategy for Modular Multilevel Converters

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CSEE Journal of Power and Energy Systems 2024年第3期10卷 1075-1084页

作者： Zhi geng Minxiao Han School of Electrical and Electronic Engineering North China Electric Power UniversityBeijing 102206China IEEE

Dead time is necessary for the coupled power switches to prevent shoot-through,especially in the modular multilevel converters(MMCs)with a large number of power *** paper proposes a dead-time effect suppression strategy for MMCs with nearest level *** operational principles of MMCs are first *** to the operational features of MMCs,the method that removes a switching signal from the coupled switches and the reduced switching frequency voltage balancing algorithms(RSFVBAs)are mixed in the proposed *** the intervals that are furthest away from the zerocrossing points(ZCP)of arm currents,the single switching signal method can completely eliminate the dead-time effect(DTE).Alternatively,the DTE is suppressed by the RSFVBA in intervals that are close to the *** the combination of the two methods,the dependence of the DTE suppression method on currents is reduced and the influences of ZCP are also released without degrading the normal operation performance of ***,the output performance of MMCs is improved and the voltage stress on the arm inductor dramatically ***,the validation of the method is verified by the simulation results with the professional tool Matlab/Simulink.

关键词： Dead-time effect modular multilevel converters switching frequency voltage balancing algorithm

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Interstitial carbon induces enriched Cu^(δ+) sites in Cu_(2)O nanoparticles to facilitate CO_(2) electroreduction to C_(2+) products

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Nano Research 2024年第8期17卷 7013-7019页

作者： Haoran Wang Rongbo Sun Peigen Liu Haohui Hu Chen Ling Xiao Han Yi shi Xusheng zheng geng Wu Xun Hong Center of Advanced Nanocatalysis(CAN) Department of Applied ChemistryHefei National Laboratory for Physical Sciences at the MicroscaleUniversity of Science and Technology of ChinaHefei 230026China Sinochem Holdings Co Ltd Xiongan New AreaHebei 071700China National Synchrotron Radiation Laboratory(NSRL) University of Science and Technology of ChinaHefei 230029China

The electrochemical CO_(2) reduction reaction(CO_(2)RR)holds significant promise in advancing carbon *** catalysts for the electrochemical CO_(2)RR to multi-carbon(C_(2+))products(e.g.,C_(2)H_(4))under industrial-level current density is urgently needed and ***,we report the Cu_(2)O nanoparticles doped with interstitial carbon atoms(denoted as C-Cu_(2)O NPs)for the conversion of CO_(2) to C_(2+)*** interstitial carbon promotes the C-Cu_(2)O NPs to possess abundant unsaturated Cu–O bonds,leading to a high-density Cu^(δ+)(0<δ<1)*** obtained C-Cu_(2)O NPs exhibited significant Faradic efficiency(FE)of C_(2+) products approaching 76.9%and a partial current density reaching 615.2 mA·cm^(–2)under an industrial-level current density of 800 mA·cm^(–2).Furthermore,the efficient electrosynthesis of C_(2)H_(4) achieved an FE of 57.4%with a partial current density of 459.2 mA·cm^(–2).In situ electrochemical attenuated total reflection Fourier transform infrared spectroscopy and in situ Raman spectroscopy analyses revealed that C-Cu_(2)O NPs stabilized the intermediate*CO and facilitated C–C coupling,leading to increased selectivity towards C_(2+) products.

关键词： CO_(2) electroreduction C-C coupling interstitial carbon *CO coverage industrial-level current density

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