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Mobilization of arsenic from contaminated sediment by anionic and nonionic surfactants

Journal of Environmental Sciences 2017年第6期29卷 281-289页

作者： Chuan liang Xianjia peng Beijing Key Laboratory of Industrial Wastewater Treatment and Reuse Research Center for Eco-Environmental SciencesChinese Academy of SciencesBelting 100085China Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

The increasing manufacture of surfactants and their wide application in industry, agriculture and household detergents have resulted in large amounts of surfactant residuals being discharged into water and distributed into sediment. Surfactants have the potential to enhance arsenic mobility, leading to risks to the environment and even human beings. In this study, batch and column experiments were conducted to investigate arsenic mobilization from contaminated sediment by the commercial anionic surfactants sodium dodecylbenzenesulfonate （SDBS）, sodium dodecyi sulfate （SDS）, sodium laureth sulfate （AES） and nonionic surfactants phenyl-polyethylene glycol （Triton X-100） and polyethylene glycol sorbitan monooleate （Tween-80）. The ability of surfactants to mobilize arsenic followed the order AES 〉 SDBS 〉 SDS = Triton X-100 〉 Tween 80. Arsenic mobilization by AES and Triton X-100 increased greatly with the increase of surfactant concentration and pH, while arsenic release by SDBS, SDS and Tween-80 slightly increased. The divalent ion Ca2＋ caused greater reduction of arsenic mobilization than Na＋. Sequential extraction experiments showed that the main fraction of arsenic mobilized was the specifically adsorbed fraction. Solid phase extraction showed that arsenate （As（V）） was the main species mobilized by surfactants, accounting for 65.05%-77.68% of the total mobilized arsenic. The mobilization of arsenic was positively correlated with the mobilization of iron species. The main fraction of mobilized arsenic was the dissolved fraction, accounting for 70% of total mobilized arsenic.

关键词： Surfactants Arsenic Iron Sediment Mobilization

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华北克拉通和巴西圣弗朗西斯科-刚果克拉通新元古代早期岩浆作用(ca.940~890Ma)序列与成因

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岩石学报 2025年第1期41卷 167-182页

作者：苏向东彭澎郑州大学生态与环境学院地热与生态地质研究中心郑州450001 中国科学院地质与地球物理研究所中国-巴西联合地学研究中心北京100029

华北克拉通和巴西圣弗朗西斯科-刚果克拉通新元古代早期的岩墙和岩床及玄武岩(ca.940~890Ma)岩浆活动时间对比和古地磁研究结果表明,上述克拉通在新元古代可能相邻。这些阶段性岩浆作用的演化趋势和源区特征及其所反映的地质过程与构造... 详细信息

华北克拉通和巴西圣弗朗西斯科-刚果克拉通新元古代早期的岩墙和岩床及玄武岩(ca.940~890Ma)岩浆活动时间对比和古地磁研究结果表明,上述克拉通在新元古代可能相邻。这些阶段性岩浆作用的演化趋势和源区特征及其所反映的地质过程与构造背景对进一步开展大陆重建有重要意义。本文系统总结和对比分析了两个克拉通新元古代镁铁质岩石的岩相学、地球化学和同位素年代学数据。研究发现,这些岩石大致可分为两类多期:(1)年龄较老(ca.940~920Ma)且演化的高Ti岩石(MgO2%),负Eu异常明显(Eu/Eu^(*)=0.7~1.0);(2)年龄较年轻(ca.915~890Ma)且较为原始的低Ti岩石(MgO>6.5%,TiO_(2)<2%),具有正Eu异常(Eu/Eu^(*)=1~1.2)或者没有Eu异常(Eu/Eu=1)。早期高Ti岩浆源区类似于EMⅠ型地幔端元(ε_(Nd)(t)=-8~+3),Sr-Nd同位素特征表明其可能是软流圈上涌熔融产生的岩浆与岩石圈地幔相互作用的结果;而晚期低Ti岩石Nd同位素与球粒陨石值类似(ε_(Nd)(t)=-2~+3),可能来源于软流圈地幔。这两类岩石在华北克拉通和巴西圣弗朗西斯科-刚果克拉通几乎同时出现,且可类比。岩浆演化趋势、微量元素和Sr-Nd同位素等特征及单斜辉石-熔体平衡深度计算表明,早期高Ti岩浆产生于大陆岩石圈破裂初期,经历了较高程度的结晶分异作用;而晚期低Ti岩浆的持续作用(~30Myr)可能与岩石圈破裂过程中不断增强的软流圈岩浆活动相关。该裂谷演化进程在Sr同位素特征变化上也有体现,即与早期高Ti岩石相比,晚期低Ti岩石的Sr同位素更为富集但Nd同位素保持不变,表明该类岩石的产生可能在大陆裂谷发育过程中受到海水蚀变的影响。以上证据表明,华北克拉通和巴西圣弗朗西斯科-刚果克拉通在新元古代早期具有可类比的岩石圈应力演化状态,且经历了相似的地幔地球化学动力学过程,支持两个克拉通在该时期相邻。

关键词：华北克拉通圣弗朗西斯科-刚果克拉通新元古代大火成岩省

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Establishing a new testing protocol of the electrochemical stability window for electric double-layer capacitors

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Science China Chemistry 2025年第01期 217-225页

作者： Ruilin Hou Xiaoxi Zhao Tingting liang Qingyun Dou Shan Xu Xingbin Yan School of Materials Science and Engineering Sun Yat-sen University Laboratory of Clean Energy Chemistry and Materials Lanzhou Institute of Chemical Physics Chinese Academy of Sciences College of Engineering and Applied Sciences Nanjing University Center of Industrial Analysis and Testing Guangdong Academy of Science

The electrochemical stability window(ESW) is crucial for determining the energy density of electric double-layer capacitors(EDLCs). However, current ESW testing protocols of EDLCs are strongly affected by artificial factors, thereby leading to unreliable result. To solve this problem, we first identify the key shortcomings of the traditional protocols by analyzing their test principles. Subsequently, taking an aqueous carbon-based EDLC as an example, we design a side reaction descriptor to represent the response difference in the charging capacitance to side reactions between the cyclic voltammetry and galvanostatic chargedischarge methods. With the aid of this descriptor, we propose a new ESW testing protocol, which is not only able to completely avoid the adverse influence of subjective factors but also fully consider the operating condition limitations. The protocol can be extended from the single electrode to the full device. This work proposes a more rigorous definition of ESW and provides a reliable protocol for evaluating the ESW of EDLCs.

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Yield potential and nitrogen use efficiency of China's super rice

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Journal of Integrative Agriculture 2017年第5期16卷 1000-1008页

作者： WANG Fei peng shao-bing National Key Laboratory of Crop Improvement Huazhong Agricultural UniversityWuhan 430070P.R.China Key Laboratory of Crop Ecophysiology and Farming System in the Middle Reaches of the Yangtze River Ministry of Agriculture/College of Plant Science and TechnologyHuazhong Agricultural UniversityWuhan 430070P.R.China

In 1996, a mega project that aimed to develop rice varieties with super-high yield potential （super rice） was launched by the Ministry of Agriculture （MOA） in China using a combination of the ideotype approach and intersubspecific heterosis. Significant progress has been made in the last two decades, with a large number of super rice varieties being approved by the MOA and the national average grain yield being increased from 6.21 t ha^-1 in 1996 to 6.89 t ha^-1 in 2015. The increase in yield potential of super rice was mainly due to the larger sink size which resulted from larger panicles. Moreover, higher photosynthetic capacity and improved root physiological traits before heading contributed to the increase in sink size. However, the poor grain filling of the later-flowering inferior spikelets and the quickly decreased root activity of super rice during grain filling period restrict the achievement of high yield potential of super rice. Furthermore, it is widely accepted that the high yield potential of super rice requires a large amount of N fertilizer input, which has resulted in an increase in N consumption and a decrease in nitrogen use efficiency （NUE）, although it remains unclear whether super rice per se is responsible for the latter. In the present paper, we review the history and success of China＇s Super Rice Breeding Pro- gram, summarize the advances in agronomic and physiological mechanisms underlying the high yield potential of super rice, and examine NUE differences between super rice and ordinary rice varieties. We also provide a brief introduction to the Green Super Rice Project, which aims to diversify breeding targets beyond yield improvement alone to address global concerns around resource use and environmental change. It is hoped that this review will facilitate further improvement of rice production into the future.

关键词： super rice yield potential nitrogen use efficiency Green Super Rice

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Persistent alterations in gray matter in COVID-19 patients experiencing sleep disturbances:a 3-month longitudinal study

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Neural Regeneration Research 2025年第10期20卷 3013-3024页

作者： Kaixuan Zhou Gaoxiong Duan Ying Liu Bei peng Xiaoyan Zhou Lixia Qin Lingyan liang Yichen Wei Qingping Zhang Xiaocheng Li Haixia Qin Yinqi Lai Yian Lu Yan Zhang Jiazhu Huang Jinli Huang Yinfei Ouyang Bolin Bin Mingming Zhao Jun Liu Jianrong Yang Demao Deng Guangxi Key Laboratory of Special Biomedicine School of MedicineGuangxi UniversityNanningGuangxi Zhuang Autonomous RegionChina Department of Radiology the People’s Hospital of Guangxi Zhuang Autonomous RegionGuangxi Academy of Medical SciencesNanningGuangxi Zhuang Autonomous RegionChina Department of Sleep Medicine the People’s Hospital of Guangxi Zhuang Autonomous RegionNanningGuangxi Zhuang Autonomous RegionChina Department of Radiology The Second Xiangya HospitalCentral South UniversityChangshaHunan ProvinceChina Guangxi Clinical Research Center for Sleep Medicine the People’s Hospital of Guangxi Zhuang Autonomous RegionNanningGuangxi Zhuang Autonomous RegionChina

Sleep disturbances are among the most prevalent neuropsychiatric symptoms in individuals who have recovered from severe acute respiratory syndrome coronavirus 2 *** studies have demonstrated abnormal brain structures in patients with sleep disturbances who have recovered from coronavirus disease 2019(COVID-19).However,neuroimaging studies on sleep disturbances caused by COVID-19 are scarce,and existing studies have primarily focused on the long-term effects of the virus,with minimal acute phase *** a result,little is known about the pathophysiology of sleep disturbances in the acute phase of *** address this issue,we designed a longitudinal study to investigate whether alterations in brain structure occur during the acute phase of infection,and verified the results using 3-month follow-up data.A total of 26 COVID-19 patients with sleep disturbances(aged 51.5±13.57 years,8 women and 18 men),27 COVID-19 patients without sleep disturbances(aged 47.33±15.98 years,9 women and 18 men),and 31 age-and gender-matched healthy controls(aged 49.19±17.51 years,9 women and 22 men)were included in this *** COVID-19 patients with sleep disturbances were included in a longitudinal *** found that COVID-19 patients with sleep disturbances exhibited brain structural changes in almost all brain *** cortical thicknesses of the left pars opercularis and left precuneus were significantly negatively correlated with Pittsburgh Sleep Quality Index ***,we observed changes in the volume of the hippocampus and its subfield regions in COVID-19 patients compared with the healthy *** 3-month follow-up data revealed indices of altered cerebral structure(cortical thickness,cortical grey matter volume,and cortical surface area)in the frontal-parietal cortex compared with the baseline in COVID-19 patients with sleep *** findings indicate that the sleep disturbances patients had altered morphology in the cortical an

关键词： brain structure cortical gray matter volume cortical surface area cortical thickness hippocampus magnetic resonance imaging Pittsburgh Sleep Quality Index severe acute respiratory syndrome coronavirus 2 infections sleep disturbances sub-cortical volume

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Interfacial Zn2+-solvation regulator towards reversible and stable Zn anode

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Journal of Energy Chemistry 2025年第1期100卷 684-692页

作者： Miao Zhou Xiongbin Luo Hang Li Shan Guo Zhuang Tong Xiaotao Zhou Xu Li Zhaohui Hou Shuquan liang Guozhao Fang College of Mechanical Engineering Key Laboratory of Hunan Province for Advanced Carbon-based Functional Materials Hunan Institute of Science and Technology School of Materials Science and Engineering Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province Central South University College of Materials and Metallurgy Guizhou University National Energy Metal Resources and New Materials Key Laboratory Central South University

Aqueous zinc-ion batteries （AZIBs） are fundamentally challenged by the instability of the electrode/electrolyte interface,predominantly due to irreversible zinc （Zn） deposition and hydrogen ***,the intricate mechanisms behind the electrochemical discrepancies induced by interfacial Zn2+-solvation and deposition behavior demand comprehensive *** molecules endowed with special functional groups （such as hydroxyl,carboxyl,etc.） have the potential to significantly optimize the solvation structure of Zn2+and regulate the interfacial electric double layer （EDL）.By increasing nucleation overpotential and decreasing interfacial free energy,these functional groups facilitate a lower critical nucleation radius,thereby forming an asymptotic nucleation model to promote uniform Zn ***,this study presents a pioneering approach by introducing trace amounts of n-butanol as solvation regulators to engineer the homogenized Zn （H-Zn） anode with a uniform and dense *** interfacial reaction and structure evolution are explored by in/ex-situ experimental techniques,indicating that the H-Zn anode exhibits dendrite-free growth,no by-products,and weak hydrogen evolution,in sharp contrast to the bare ***,the H-Zn anode achieves a remarkable Zn utilization rate of approximately 20% and simultaneously sustains a prolonged cycle life exceeding 500 ***,the H-Zn//NH4V4O10（NVO） full battery showcases exceptional cycle stability,retaining 95.04%capacity retention after 400 cycles at a large current density of 5 A *** study enlightens solvation-regulated additives to develop Zn anode with superior utilization efficiency and extended operational lifespan.

关键词： Aqueous zinc-ion batteries Interfacial reaction Asymptotic nucleation model Reversible and stable Zn anode

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Development and validation of machine learning models for nonalcoholic fatty liver disease

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Hepatobiliary & Pancreatic Diseases International 2023年第6期22卷 615-621页

作者： Hong-Ye peng shao-Jie Duan liang Pan Mi-Yuan Wang Jia-liang Chen Yi-Chong Wang Shu-Kun Yao Graduate School of Beijing University of Chinese Medicine Beijing 100029China Department of Gastroenterology China-Japan Friendship HospitalBeijing 100029China Phase 1 Clinical Trial Center Deyang People’s HospitalDeyang 618000China School of Public Health Tongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430030China Center of Integrated Traditional Chinese and Western Medicine Beijing Ditan HospitalCapital Medical UniversityBeijing 100102China

Background: Nonalcoholic fatty liver disease(NAFLD) had become the most prevalent liver disease worldwide. Early diagnosis could effectively reduce NAFLD-related morbidity and mortality. This study aimed to combine the risk factors to develop and validate a novel model for predicting NAFLD. Methods: We enrolled 578 participants completing abdominal ultrasound into the training set. The least absolute shrinkage and selection operator(LASSO) regression combined with random forest(RF) was conducted to screen significant predictors for NAFLD risk. Five machine learning models including logistic regression(LR), RF, extreme gradient boosting(XGBoost), gradient boosting machine(GBM), and support vector machine(SVM) were developed. To further improve model performance, we conducted hyperparameter tuning with train function in Python package ‘sklearn’. We included 131 participants completing magnetic resonance imaging into the testing set for external validation. Results: There were 329 participants with NAFLD and 249 without in the training set, while 96 with NAFLD and 35 without were in the testing set. Visceral adiposity index, abdominal circumference, body mass index, alanine aminotransferase(ALT), ALT/AST(aspartate aminotransferase), age, high-density lipoprotein cholesterol(HDL-C) and elevated triglyceride(TG) were important predictors for NAFLD risk. The area under curve(AUC) of LR, RF, XGBoost, GBM, SVM were 0.915 [95% confidence interval(CI): 0.886–0.937], 0.907(95% CI: 0.856–0.938), 0.928(95% CI: 0.873–0.944), 0.924(95% CI: 0.875–0.939), and 0.900(95% CI: 0.883–0.913), respectively. XGBoost model presented the best predictive performance, and its AUC was enhanced to 0.938(95% CI: 0.870–0.950) with further parameter tuning. Conclusions: This study developed and validated five novel machine learning models for NAFLD prediction, among which XGBoost presented the best performance and was considered a reliable reference for early identification of high-risk patients wit

关键词： Nonalcoholic fatty liver disease Machine learning Predictive factors

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Multicolored Bipartite Ramsey Numbers of Large Cycles

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 347-357页

作者： shao-qiang LIU Yue-jian peng College of Mathematics and Statistics Hanshan Normal UniversityChaozhou 521041China School of Mathematics Hunan UniversityChangsha 410082China

For an integer r≥2 and bipartite graphs Hi,where 1≤i≤r,the bipartite Ramsey number br(H1,H2,…,Hr)is the minimum integer N such that any r-edge coloring of the complete bipartite graph KN;N contains a monochromatic subgraph isomorphic to Hi in color i for some 1≤i≤*** show that if r≥3;α1,α2>0,αj+2≥[(j+2)!-1]Σi=1^(j+1)α1 for j=1,2…r-2,then br(C2[α1n],C2[α2n],…,C2[αrn]=(Σ=j=1^(r)a j+o(1))n.

关键词： ramsey number bipartite ramsey number regularity lemma

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Multi-receptive field interaction network for shape from polarization

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Science China(Information Sciences) 2025年第1期 394-395页

作者： Yini peng Rui LIU Zhiyuan ZHANG Zhongyuan WANG Jiayi MA Xin TIAN Electronic Information School Wuhan University Computer Science School Wuhan University Wuhan Institute of Quantum Technology

Shape from polarization (SfP) method can use the polarization information in reflected light to estimate the surface normal of the target,which can further reconstruct the shape of the *** a simple image capture process,it can use low-cost equipment to meet a high precision imaging requirement,which can be used in remote scenes and other applications.

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Liver as a new target organ in Alzheimer's disease:insight from cholesterol metabolism and its role in amyloid-beta clearance

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Neural Regeneration Research 2025年第3期20卷 695-714页

作者： Beibei Wu Yuqing Liu Hongli Li Lemei Zhu Lingfeng Zeng Zhen Zhang Weijun peng Department of Integrated Traditional Chinese&Western Medicine The Second Xiangya HospitalCentral South UniversityChangshaHunan ProvinceChina Academician Workstation Changsha Medical UniversityChangshaHunan ProvinceChina Yangsheng College of Traditional Chinese Medicine Guizhou University of Traditional Chinese MedicineGuiyangGuizhou ProvinceChina Qinhuangdao Shanhaiguan Pharmaceutical Co. LtdQinhuangdaoHebei ProvinceChina National Clinical Research Center for Mental Disorder The Second Xiangya HospitalCentral South UniversityChangshaHunan ProvinceChina

Alzheimer's disease,the primary cause of dementia,is characterized by neuropathologies,such as amyloid plaques,synaptic and neuronal degeneration,and neurofibrillary *** amyloid plaques are the primary characteristic of Alzheimer's disease in the central nervous system and peripheral organs,targeting amyloid-beta clearance in the central nervous system has shown limited clinical efficacy in Alzheimer's disease *** abnormalities are commonly observed in patients with Alzheimer's *** liver is the primary peripheral organ involved in amyloid-beta metabolism,playing a crucial role in the pathophysiology of Alzheimer's ***,impaired cholesterol metabolism in the liver may exacerbate the development of Alzheimer's *** this review,we explore the underlying causes of Alzheimer's disease and elucidate the role of the liver in amyloid-beta clearance and cholesterol ***,we propose that restoring normal cholesterol metabolism in the liver could represent a promising therapeutic strategy for addressing Alzheimer's disease.

关键词： ABCA1 Alzheimer's disease amyloid-beta apolipoprotein E cholesterol metabolism liver liver X receptor low-density lipoprotein receptor-related protein 1 peripheral clearance tauroursodeoxycholic acid

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