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High-performance,stable CoNi LDH@Ni foam composite membrane with innovative peroxymonosulfate activation for 2,4-dichlorophenol destruction

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Journal of Environmental Sciences 2024年第7期141卷 235-248页

作者： yu liu Weibao liu Xinrui Gan Jiangwei shang Xiuwen Cheng College of Chemistry and Environmental Science Xinjiang Laboratory of Phase Transitions and Microstructures of Condensed Matter PhysicsYili Normal UniversityYining 835000China Key Laboratory for Environmental Pollution Prediction and Control Gansu ProvinceCollege of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China

In this study,the cobalt-nickel layered double hydroxides(CoNi LDH)were synthesized with a variety of Co/Ni mass ratio,as *** comparison,Co1Ni3LDH presented the best peroxymonosulfate(PMS)activation efficiency for 2,4-dichlorophenol ***,CoNi LDH@Nickel foam(CoNi LDH@NF)composite membrane was constructed for enhancing the stability of catalytic ***,CoNi LDH@NF-PMS system exerted high degradation efficiency of 99.22%within 90 min for 2,4-DCP when[PMS]_(0)=0.4 g/L,Co^(1)Ni^(3)LDH@NF=2 cm×2 cm(0.2 g/L),reaction temperature=298 *** the surface morphology and structure of the catalyst,it was demonstrated that the CoNi LDH@NF composite membrane possessed abundant cavity structure,good specific surface area and sufficient active ***,·OH,SO_(4)·^(-)and^(1)O_(2)played the primary role in the CoNi LDH@NF-PMS system for 2,4-DCP decomposition,which revealed the PMS activation mechanism in CoNi LDH@NF-PMS ***,this study eliminated the stability and adaptability of CoNi LDH@NF composite membrane,proposing a new theoretical basis of PMS heterogeneous catalysts selection.

关键词： CoNi LDH@NF composite membrane Peroxymonosulfate 2,4-dichlorophenol Reactive radicals

AstroPose:Astronaut pose estimation using a monocular camera during extravehicular activities

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Science China(Technological Sciences) 2024年第6期67卷 1933-1945页

作者： liu ZiBin LI You WANG ChunHui liu Liang GUAN BangLei shang Yang yu QiFeng College of Aerospace Science and Engineering National University of Defense TechnologyChangsha410073China Key Laboratory of Human Factors Engineering China Astronaut Research and Training CenterBeijing100094China

With the completion of the Chinese space station,an increasing number of extravehicular activities will be executed by astronauts,which is regarded as one of the most dangerous activities in human space *** guarantee the safety of astronauts and the successful accomplishment of missions,it is vital to determine the pose of astronauts during extravehicular *** article presents a monocular vision-based pose estimation method of astronauts during extravehicular activities,making full use of the available observation ***,the camera is calibrated using objects of known structures,such as the spacesuit backpack or the circular handrail outside the space ***,the pose estimation is performed utilizing the feature points on the *** proposed methods are validated both on synthetic and semi-physical simulation experiments,demonstrating the high precision of the camera calibration and pose *** further evaluate the performance of the methods in real-world scenarios,we utilize image sequences of Shenzhou-13 astronauts during extravehicular *** experiments validate that camera calibration and pose estimation can be accomplished solely with the existing observation resources,without requiring additional complicated *** motion parameters of astronauts lay the technological foundation for subsequent applications such as mechanical analysis,task planning,and ground training of astronauts.

关键词： monocular camera astronaut pose estimation camera calibration

Porous nanocomposites with enhanced intrinsic piezoresistive sensitivity for bioinspired multimodal tactile sensors

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Microsystems & Nanoengineering 2024年第1期10卷 243-256页

作者： Jianpeng Zhang Song Wei Caichao liu Chao shang Zhaoqiang He yu Duan Zhengchun Peng State Key Laboratory of Radio Frequency Heterogeneous Integration(Shenzhen University) School of Physics and Optoelectronic EngineeringShenzhen University518060 ShenzhenGuangdong ProvinceP.R.China Linksense Technology Ltd. 518060 ShenzhenGuangdong ProvinceP.R.China

In this work,we propose porous fluororubber/thermoplastic urethane nanocomposites(PFTNs)and explore their intrinsic piezoresistive sensitivity to *** experiments reveal that the intrinsic sensitivity of the PFTN-based sensor to pressure up to 10 kPa increases up to 900%compared to the porous thermoplastic urethane nanocomposite(PTN)counterpart and up to 275%compared to the porous fluororubber nanocomposite(PFN)*** pressures exceeding 10 kPa,the resistance-pressure relationship of PFTN follows a logarithmic function,and the sensitivity is 221%and 125%higher than that of PTN and PFN,*** the excellent intrinsic sensitivity of the thick PFTN film,a single sensing unit with integrated electrode design can imitate human skin for touch detection,pressure perception and traction *** sensing range of our multimodal tactile sensor reaches~150 Pa,and it exhibits a linear fit over 97%for both normal pressure and shear *** also demonstrate that an electronic skin,made of an array of sensing units,is capable of accurately recognizing complex tactile interactions including pinch,spread,and tweak motions.

关键词： sensation intrinsic modal

Simplified p-i-n Perovskite Solar Cells with a Multifunctional Polyfullerene Electron Transporter

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Chinese Journal of Polymer Science 2024年第8期42卷 1060-1066页

作者： Fei-Fei Wang Tian-Xiao liu Ze-Wei Cui Ling-yuan Wang yun-Jie Dou Xiao-yu Shi Si-Wei Luo Xiao-Dong Hu Zhi-Jun Ren Yang-Yang liu yu Zhao shang-shang Chen State Key Laboratory of Coordination Chemistry MOE Key Laboratory of High Performance Polymer Materials&TechnologySchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing 21003China

In prevailing p-i-n perovskite solar cells(PSCs),solution-processible fullerene molecules are widely used as electron-transporting layers(ETLs)but they typically suffer from poor uniformity and undesirable stability ***,a separate bathocuproine(BCP)layer is needed to block hole tran sfer,increasing fabrication complexity and ***,we address these limitations by develo ping a novel polymeric ETL(named PF BCP)synthesized by polymerizing C_(60)with *** innovative material achieves both efficient electron transport and hole blocking,while its excellent uniformity minimizes interface recombination and enhances ***,our blade-coated PSCs utilizing PFBCP achieve a high power conversion efficiency exceeding 22%and retain 91%of initial efficiency after 1200 h of light *** development not only paves the way for commercially viable PSCs but also opens avenues for future ETL design to realize even more efficient and stable PSCs.

关键词： Polyfullerene Perovskite solar cells Electron transporter Stability

Differences in and factors controlling organic matter enrichment in the Ziliujing Formation shale in the Sichuan Basin

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Petroleum Science 2024年第1期21卷 77-86页

作者： Peng Li Zhong-Bao liu He Bi Tao Jiang Rui-Kang Bian Peng-Wei Wang Xiao-yu shang State Key Laboratory of Shale Oil and Gas Enrichment Mechanisms and Efficient Development Beijing102206China Key Laboratory of Shale Oil/Gas Exploration and Production Technology SINOPECBeijing102206China Petroleum Exploration and Production Research Institute SINOPECBeijing102206China Research Institute of Petroleum Exploration and Development PetroChinaBeijing100083China Chinese Academy of Geological Sciences Beijing100037China No.4 Oil Production Plant in Daqing Oilfield Co Ltd. Daqing163511HeilongjiangChina

Lacustrine shale oil and gas are important fields for unconventional exploration and development in China,and organic-rich shale deposition lays down the critical foundation for hydrocarbon *** are two sets of shale,the Dongyuemiao and Da’anzhai Members,in the Ziliujing Formation in the Sichuan *** identify the differential enrichment characteristics of organic matter and clarify its controlling factors,geochemical analyses of organic and inorganic geochemical analyses were *** results showed that the total organic carbon content of the Dongyuemiao shale(1.36%)is slightly higher than that of the Da’anzhai shale(0.95%).The enrichment of organic matter in the two shales resulted from the comprehensive controls of paleoproductivity,paleoenvironment,and terrigenous input,but different factors have different *** addition,driven by climate,the change in the sulfate concentration in the bottom water further led to the different intensities of bacterial sulfate reduction in early *** made a great difference regarding organic matter accumulation in the two *** general,climate may have played a dominant role in organic matter enrichment in the two sets of shale.

关键词： Lacustrine shale Ziliujing Formation Sichuan Basin Enrichment mechanism of organic matter

Data-driven evacuation and rescue traffic optimization with rescue contraflow control

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Journal of Safety Science and Resilience 2024年第1期5卷 1-12页

作者： Zheng liu Jialin liu Xuecheng shang Xingang Li School of Management Engineering Zhengzhou University of AeronauticsZhengzhou 450046China Collaborative Innovation Center for Aviation Economy Development of Henan Province Zhengzhou University of AeronauticsZhengzhou 450046China School of Systems science Beijing Jiaotong UniversityBeijing 100044China Key Laboratory of Transport Industry of Big Data Application Technologies for Comprehensive Transport Beijing Jiaotong UniversityBeijing 100044China School of Transportation Engineering Shandong Jianzhu UniversityJinan 250101China

In response to local sudden disasters,e.g.,high-rise office or residential building fire disasters,road occupation can cause conflicts,and traffic directions may be opposite between evacuation vehicles and rescue vehicles;moreover,lane contraflow can be adopted to meet these surge traffic ***,lane contraflow that provides more roads for rescue vehicles reduces the traffic supply in the evacuation *** is unclear how to control the number of contraflow roads used by rescue vehicles to coordinate evacuation and rescue traffic ***,we adjust the critical rescue traffic volume of reversing the normal road traffic direction to control rescue ***,we propose a multiobjective mixed integer linear programming formulation for evacuation and rescue traffic ***,considering that the upper limit of the critical rescue traffic volume is unknown and that the proposed formulation includes multiple objectives and multi-priority vehicle classes,a three-stage solving algorithm is ***,a large-scale evacuation and rescue traffic optimization result dataset is obtained for the Nguyen–Dupuis road network,and the impact of different rescue contraflow control plans on evacuation and rescue traffic is studied based on data-driven sta-tistical *** results show that by adjusting the optimal rescue traffic route,the critical rescue traffic volume for reversing the normal road traffic direction can reduce the interference of rescue traffic to evacuation traffic operation performance without reducing rescue traffic operation performance,and can be used to coor-dinate evacuation and rescue traffic operation under rescue contraflow.

关键词： Evacuation and rescue traffic optimization Rescue contraflow control Multiobjective mixed integer linear programming Three-stage solving algorithm Data-driven statistical analysis

Design of digital calibration based on variable step size of sub-binary SAR ADC

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The Journal of China Universities of Posts and Telecommunications 2024年第2期31卷 62-71页

作者： liu Wei Zhao Yanke shang Shiguang School of Electronic Engineering Xi'an University of Posts and TelecommunicationsXi'an 710121China

Addressing the impact of capacitor mismatch on the conversion accuracy of successive approximation register analog-to-digital converter(SAR ADC),a 12-bit 1 MS/s sub-binary SAR ADC designed using variable step size digital calibration was *** least mean square(LMS)calibration algorithm was employed with a ramp signal used as the calibration *** errors,extracted under injected disturbances,underwent iterative training to optimize weight *** address the trade-off between conversion accuracy and speed caused by a fixed step size,a novel variable step size algorithm tailored for SAR ADC calibration was *** core circuit and layout of the SAR ADC were implemented using the Taiwan Semiconductor Manufacturing Company(TSMC)0.35μm complementary metal-oxide-semiconductor(CMOS)commercial *** of the SAR ADC calibration algorithm was conducted using Simulink,demonstrating quick convergence and meeting conversion accuracy requirements compared to fixed step size *** results indicated that the convergence speed of the LMS digital calibration algorithm with variable step size was approximately eight times faster than that with a fixed step size,also yielding a lower mean square error(MSE).After calibration,the simulation results for the SAR ADC exhibited an effective number of bit(ENOB)of 11.79 bit and a signal-to-noise and distortion ratio(SNDR)of 72.72 dB,signifying a notable enhancement in the SAR ADC performance.

关键词： successive approximation register analog-to-digital converter(SAR ADC) variable step size digital calibration disturbance technique

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Accurate and efficient floor localization with scalable spiking graph neural networks

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Satellite Navigation 2024年第1期5卷 191-206页

作者： Fuqiang Gu Fangming Guo Fangwen yu Xianlei Long Chao Chen Kai liu Xuke Hu Jianga shang Songtao Guo College of Computer Science Chongqing UniversityChongqingChina Department of Precision Instrument Tsinghua UniversityBeijingChina Institute of Data Science German Aerospace Center(DLR)JenaGermany School of Computer Science China University of GeosciencesWuhanChina

Floor localization is crucial for various applications such as emergency response and rescue,indoor positioning,and recommender *** existing floor localization systems have many drawbacks,like low accuracy,poor scalability,and high computational *** this paper,we first frame the problem of floor localization as one of learning node embeddings to predict the floor label of a ***,we introduce FloorLocator,a deep learning-based method for floor localization that integrates efficient spiking neural networks with powerful graph neural *** approach offers high accuracy,easy scalability to new buildings,and computational *** results on using several public datasets demonstrate that FloorLocator outperforms state-of-the-art ***,in building B0,FloorLocator achieved recognition accuracy of 95.9%,exceeding state-of-the-art methods by at least 10%.In building B1,it reached an accuracy of 82.1%,surpassing the latest methods by at least 4%.These results indicate FloorLocator’s superiority in multi-floor building environment localization.

关键词： Indoor positioning Deep learning Floor localization Spiking neural networks Graph neural networks

Alternative splicing of the PECTINESTERASE gene encoding a cell wall-degrading enzyme affects postharvest softening in grape

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Journal of Integrative Agriculture 2024年第3期23卷 863-875页

作者： Hainan liu Maosong Pei Charles Ampomah-Dwamena Yaxin shang Yihe yu Tonglu Wei Qiaofang Shi Dalong Guo College of Horticulture and Plant Protection Henan University of Science and TechnologyLuoyang 471000China Henan Engineering Technology Research Center of Quality Regulation and Control of Horticultural Plants Luoyang 471000China The New Zealand Institute for Plant&Food Research Limited(PFR) Auckland 1010New Zealand

The firmness of table grape berries is a crucial quality parameter. Despite extensive research on postharvest fruit softening, its precise molecular mechanisms remain elusive. To enhance our comprehension of the underlying molecular factors, we initially identified differentially expressed genes(DEGs) by comparing the transcriptomes of folic acid(FA)-treated and water-treated(CK) berries at different time points. We then analyzed the sequences to detect alternatively spliced(AS) genes associated with postharvest softening. A total of 2,559 DEGs were identified and categorized into four subclusters based on their expression patterns, with subcluster-4 genes exhibiting higher expression in the CK group compared with the FA treatment group. There were 1,045 AS-associated genes specific to FA-treated berries and 1,042 in the CK-treated berries, respectively. Gene Ontology(GO) annotation indicated that the AS-associated genes in CK-treated berries were predominantly enriched in cell wall metabolic processes,particularly cell wall degradation processes. Through a comparison between treatment-associated AS genes and subcluster-4 DEGs, we identified eight genes, including Pectinesterase 2(VvPE2, Vitvi15g00704), which encodes a cell wall-degrading enzyme and was predicted to undergo an A3SS event. The reverse transcription polymerase chain reaction further confirmed the presence of a truncated transcript variant of VvPE2 in the FA-treated *** study provides a comprehensive analysis of AS events in postharvest grape berries using transcriptome sequencing and underscores the pivotal role of VvPE2 during the postharvest storage of grape berries.

关键词： grape postharvest softening folic acid alternative splicing Pectinesterase 2 alternative 3'splice site(A3SS)