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A high-performance lithium anode based on N-doped composite graphene

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Rare Metals 2024年第3期43卷 1030-1036页

作者： Can Jiao Hao-Bo Sun Li Zhang shang-qian zhao Guo-Yao Pang Chun-Rong zhao Shi-Gang Lu General Research Institute for Nonferrous Metals Beijing100088China China Automotive Battery Research Institute Co.Ltd Beijing101407China

Lithium(Li)metal is the most promising electrode for next-gene ration rechargeable *** order to push the commercialization of the lithium metal batteries,a kind of nitrogen(N)-doped composite graphene(NCG)adopted as the Li plating host was prepared to regulate Li metal nucleation and suppress dendrite ***,a new kind of sandwich-type composite lithium metal(STCL)electrode was developed to improve its *** STCL electrode can be used as convenient as a piece of Li foil but no dendrite *** a symmetric battery,the STCL electrode cycled for more than 4500 h with the overpotential of less than 40 *** due to the creative design,the STCL promises the Li-S battery with a prolonged cycling lifespan.

关键词： Lithium metal anode Lithiophilic N-doped composite graphene Sandwich-type composite lithium metal electrode

Unraveling the significance of cobalt on transformation kinetics,crystallography and impact toughness in high-strength steels

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 380-390页

作者： Yishuang Yu Jingxiao zhao Xuelin Wang Hui Guo Zhenjia Xie Chengjia shang Collaborative Innovation Center of Steel Technology University of Science and Technology BeijingBeijing 100083China School of Materials Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China State Key Laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing 100083China

This work reveals the significant effects of cobalt(Co)on the microstructure and impact toughness of as-quenched highstrength steels by experimental characterizations and thermo-kinetic *** results show that the Co-bearing steel exhibits finer blocks and a lower ductile-brittle transition temperature than the steel without ***,the Co-bearing steel reveals higher transformation rates at the intermediate stage with bainite volume fraction ranging from around 0.1 to *** improved impact toughness of the Co-bearing steel results from the higher dense block boundaries dominated by the V1/V2 variant ***,the addition of Co induces a larger transformation driving force and a lower bainite start temperature(BS),thereby contributing to the refinement of blocks and the increase of the V1/V2 variant *** findings would be instructive for the composition,microstructure design,and property optimization of high-strength steels.

关键词： high-strength steel cobalt transformation kinetics crystallography impact toughness

Revolutionizing photothermal CO_(2)hydrogenation with ceria-based catalysts

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Nano Research 2025年第1期18卷 30-49页

作者： zhaorui Zhang Xiao Han Junhong Zhang Yunyun Dong Jinsheng zhao qian Xu ingqiang Zhang School of Chemistry and Chemical Engineering Liaocheng UniversityLiaocheng 252059China Institute for Catalysis Hokkaido UniversityN-21W-10Sapporo 001-0021Japan National Synchrotron Radiation Laboratory University of Science and Technology of ChinaHefei 230029China

In the context of achieving carbon neutrality,CO_(2)catalytic conversion technologies are effective in reducing atmospheric CO_(2)concentrations while simultaneously producing renewable *** approach is seen as a viable method for constructing a new carbon cycle,thereby effectively addressing the issue of global *** CO_(2)conversion has recently emerged as a promising research focus due to its high energy utilization efficiency,superior CO_(2)conversion,excellent product selectivity,mild operating conditions,low energy consumption and minimal operating *** oxide(CeO_(2))has been widely used in photothermal catalysis due to its unique chemical properties,particularly when used as a support material with supported metals,creating distinctive interfacial sites for catalytic *** an emerging star support in photothermal CO_(2)conversion,its contributions are equally significant and should not be ***,to our knowledge,there has been no comprehensive review of CeO_(2)applications in catalytic hydrogenation of CO_(2).In this paper,we summarize and discuss CeO_(2)-based materials for photothermal CO_(2)conversion to value-added *** research particularly focuses on the synthesis methods of CeO_(2)-supported catalysts,the history of CeO_(2)in photothermal catalysis,types of photothermal catalytic reactors,unique characterization methods for the photothermal catalysts and the photothermal CO_(2)hydrogenation reactions by CeO_(2)-based *** related to further challenges and future directions for photothermal CO_(2)hydrogenation are also provided.

关键词： CO_(2)neutrality hydrogenation photothermal catalysis ceria C1 chemistry

Efficient Computational Approach for Predicting the 3D Acoustic Radiation of the Elastic Structure in Pekeris Waveguides

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Journal of Ocean University of China 2022年第4期21卷 903-916页

作者： qian Zhiwen HE Yuanan shang Dejiang zhao Haihan ZHAI Jingsheng School of Marine Science and Technology Tianjin UniversityTianjin 300072China Systems Engineering Research Institute Beijing 100036China College of Underwater Acoustics Engineering Harbin Engineering UniversityHarbin 150001China

Ocean boundaries present a significant effect on the vibroacoustic characteristics and sound propagation of an elastic structure in *** this study,an efficient finite element/wave superposition method(FE/WSM)for predicting the three-dimen-sional acoustic radiation from an arbitrary-shaped radiator in Pekeris waveguides with a lossy seabed is *** method is based on the FE method(FEM),WSM,and sound propagation ***,a near-field vibroacoustic model is established by the FEM to obtain vibration information on a radiator ***,the WSM based on the Helmholtz boundary integral is used to pre-dict the far-field acoustic radiation and ***,the rigorous image source method and complex normal mode are employed to obtain the near-and far-field Green’s function(GF),*** former,which is based on the spherical wave decomposition,is adopted to accurately solve the near-field source strength,and the far-field acoustic radiation is calculated by the latter and perturbation *** simulations of both models are compared to theoretical wavenumber integration ***,numerical experiments on elastic spherical and cylindrical shells in Pekeris waveguides are presented to validate the accuracy and efficiency of the proposed *** results show that the FE/WSM is adaptable to complex radiators and ocean-acoustic envi-ronments,and are easy to implement and computationally efficient in calculating the structural vibration,acoustic radiation,and sound propagation of arbitrarily shaped radiators in practical ocean environments.

关键词： elastic structure acoustic radiation Pekeris waveguide wave superposition method Green’s function image source method spherical wave decomposition

Boosting low-temperature selective catalytic reduction of NO_(x)with NH_(3)of V_(2)O_(5)/TiO_(2)catalyst via B-doping

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Chinese Journal of Chemical Engineering 2022年第4期35卷 377-383页

作者： Hanghang Li Wei zhao Licheng Wu qian Wang Danhong shang Qin Zhong School of Energy&Power Engineering Jiangsu UniversityZhenjiang 212013China School of Environmental and Chemical Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China School of Chemical Engineering Nanjing University of Science and TechnologyNanjing 210094China

A series of B-doped V_(2)O_(5)/TiO_(2) catalysts has been prepared the by sol-gel and impregnation methods to investigate the influence of B-doping on the selective catalytic reduction(SCR)of NOxwith NH_(3).X-ray diffraction,Brunauer-Emmett-Teller specific surface area,scanning electron microscope,X-ray photoelectron spectroscopy,temperature-programmed reduction of H_(2) and temperature-programmed desorption of NH_(3)technology were used to study the effect of the B-doping on the structure and NH_(3)-SCR activity of V_(2)O_(5)/TiO_(2) *** experimental results demonstrated that the introduction of B not only improved the low-temperature SCR activity of the catalysts,but also broadened the activity temperature *** best SCR activity in the entire test temperature range is obtained for VTiB_(2.0) with 2.0%doping amount of B and the NO_(x) conversion rate is up to 94.3%at 210℃.The crystal phase,specific surface area,valence state reducibility and surface acidity of the active components for the as-prepared catalysts are significantly affected by the B-doping,resulting in an improved NH_(3)-SCR *** results suggest that the V_(2)O_(5)/TiO_(2) catalysts with an appropriate B content afford good candidates for SCR in the low temperature window.

关键词： B-doping Catalyst SCR NO_(x) Support

Molecule‑Level Multiscale Design of Nonflammable Gel Polymer Electrolyte to Build Stable SEI/CEI for Lithium Metal Battery

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Nano-Micro Letters 2025年第1期17卷 404-423页

作者： Qiqi Sun Zelong Gong Tao Zhang Jiafeng Li Xianli Zhu Ruixiao Zhu Lingxu Wang Leyuan Ma Xuehui Li Miaofa Yuan Zhiwei Zhang Luyuan Zhang zhao qian Longwei Yin Rajeev Ahuja Chengxiang Wang Key Laboratory for Liquid‑Solid Structural Evolution and Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinan 250061People’s Republic of China Condensed Matter Theory Department of Physics and AstronomyUppsala UniversityUppsala 75120Sweden

The risk of flammability is an unavoidable issue for gel polymer electrolytes(GPEs).Usually,flameretardant solvents are necessary to be used,but most of them would react with anode/cathode easily and cause serious interfacial instability,which is a big challenge for design and application of nonflammable ***,a nonflammable GPE(SGPE)is developed by in situ polymerizing trifluoroethyl methacrylate(TFMA)monomers with flame-retardant triethyl phosphate(TEP)solvents and LiTFSI–LiDFOB dual lithium *** is strongly anchored to PTFMA matrix via polarity interaction between-P=O and-CH_(2)CF_(3).It reduces free TEP molecules,which obviously mitigates interfacial reactions,and enhances flame-retardant performance of TEP *** TEP molecules are also inhibited in solvation of Li^(+),leading to anion-dominated solvation sheath,which creates inorganic-rich solid electrolyte interface/cathode electrolyte interface *** coordination structure changes Li^(+)transport from sluggish vehicular to fast structural transport,raising ionic conductivity to 1.03 mS cm^(-1) and transfer number to 0.41 at 30℃.The Li|SGPE|Li cell presents highly reversible Li stripping/plating performance for over 1000 h at 0.1 mA cm^(−2),and 4.2 V LiCoO_(2)|SGPE|Li battery delivers high average specific capacity>120 mAh g^(−1) over 200 *** study paves a new way to make nonflammable GPE that is compatible with Li metal anode.

关键词： Anchoring effect Nonflammable gel electrolyte In situ cross-linked Electrode-electrolyte interface Li metal battery

Inducible overexpression of porcine homeobox A10 in the endometrium of transgenic mice

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Journal of Integrative Agriculture 2016年第6期15卷 1338-1344页

作者： LIN Rui-yi WU Di zhao Chang-zhi CHEN shang-shang XIAO qian LI Xin-yun zhao Shu-hong Key Lab of Agricultural Animal Genetics Breeding and Reproduction Ministry of Education/The Cooperative Innovation Center for Sustainable Pig Production Huazhong Agricultural University Wuhan 430070 P.R China College of Animal Science and Technology Northeast Agricultural University Harbin 150030 P.R.China

Homeobox A10 （HOXA 10） is a well-known transcription factor that plays an important role in directing endometrial differ- entiation and establishing the conditions required for implantation. Interestingly, the expression level of HOXAIO may be associated with litter size. To study the effects of the porcine HOXAIO promoter fragment on the expression of HOXAIO gene in vivo, we generated a transgenic mouse model using pronuclear microinjection, and measured the expression of HOXAIO in the endometrium. There was no difference in the expression level of HOXAIO between transgenic and wild- type mice in the absence of hormone stimulation. However, following treatment with progesterone and estradiol benzoate, the expression level of HOXAIO was significantly increased in transgenic mice compared with that of wild-type mice. Fur- thermore, the litter size of transgenic females was larger than that of wild-type females （7.02±1.73 vs. 6.48＋1.85; P=0.14）. Moreover, the difference of litter size was greater in the later parities （7.33±1.62 vs. 6.37±2.02; P=0.08） compared with the first parity （6.76±1.81 vs. 6.61v1.67; P=0.77） between transgenic and wild-type mice. Therefore, our transgenic mouse model provides exciting insights regarding the actions of HOXAIO and its hormone-inducible promoter in vivo. The present study offers valuable proof of principle to develop transgenic pigs with a hormone-inducible promoter regulating HOXAIO to alter litter size.

关键词： porcine HOXA 10 transgenic mice endometrium

Some Interesting Features for External Region of Spherical Symmetric Mass in New Theory of Gravitation VGM

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Communications in Theoretical Physics 2006年第5X期46卷 879-880页

作者： qian shang-Wu Physics Department Peking University Beijing 100871 China

This paper briefly discusses some interesting features for the external region of the spherical symmetric mass in the new theory of gravitation VGM, i.e. the theory of gravitation by considering the vector graviton field and the metric field, such as pseudo-singularity, curvature tensor, static limit, event horizon, and the radial motion of a particle. All these features are different from the corresponding features obtained from general relativity.

关键词： pseudo-singularity curvature tensor static limit event horizon radial motion of the particle

Biofilm effects on size gradation,drag coefficient and settling velocity of sediment particles

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International Journal of Sediment Research 2014年第4期29卷 471-480页

作者： qian-qian shang Hong-wei FANG Hui-ming zhao Guo-jian HE Zheng-hui CUI Department of Hydraulic Engineering State Key Laboratory of Hydroscience and EngineeringTsinghua University Nanjing Hydraulic Research Institute China Institute of Water Resources and Hydropower Research

Sediment particles are often colonized by biofilm in a natural aquatic ecological system,especially in eutrophic water body.A series of laboratory experiments on particle size gradation,drag coefficient and settling velocity were conducted after natural sediment was colonized by biofilm for 5,10,15 and 20 *** image acquisition,particle tracking techniques of Particle Image Velocimetry and Particle Tracking Velocimetry were utilized to analyze the changes of these *** experimental results indicate that the size gradation,the drag force exerted on bio-particles,and the settling velocity of bio-particles underwent significant change due to the growth of biofilm onto the sediment *** study proposes a characteristic particle size formula and a bio-particle settling velocity formula based on the regression of experiment results,that the settling velocity is only 50%to 60%as the single particle which has the same diameter and ***,biofilm growth causes large particle which the settling velocities are approximately 10 times larger than that of primary *** results may be specifically used in the low energy reservoir or lake environment.

关键词： Sediment particle Biofilm Size gradation Drag coefficient Settling velocity