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Sustainable Furfural Biomass Feedstocks Electrooxidation toward Value-Added Furoic Acid with Energy-Saving H_(2) Fuel Production Using Pt-Decorated Co_(3)O_(4) Nanospheres

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Energy & Environmental Materials 2024年第2期7卷 350-358页

作者： Talshyn Begildayeνa Jayaraman Theerthagiri seung Jun Lee Ahreum Min Gyeong-Ah Kim Siνakumar Manickam myong Yong Choi Department of Chemistry(BK21 FOUR) Core-Facility Center for Photochemistry&NanomaterialsResearch Institute of Natural SciencesGyeongsang National UniversityJinju 52828South Korea Petroleum and Chemical Engineering Faculty of EngineeringUniversiti Teknologi BruneiJalan Tungku Link GadongBandar Seri Begawan BE1410Brunei Darussalam

Here,furfural oxidation was performed to replace the kinetically sluggish O_(2)evolution reaction(OER).Pt-Co_(3)O_(4)nanospheres were developed via pulsed laser ablation in liquid(PLAL)in a single step for the paired electrocatalysis of an H_(2)evolution reaction(HER)and furfural oxidation reaction(FOR).The FOR afforded a high furfural conversion(44.2%)with a major product of 2-furoic acid after a 2-h electrolysis at 1.55 V versus reversible hydrogen electrode in a 1.0-M KOH/50-mM furfural *** Pt-Co_(3)O_(4)electrode exhibited a small overpotential of 290 mV at 10 mA cm^(-2).As an anode and cathode in an electrolyzer system,the Pt-Co_(3)O_(4)electrocatalyst required only a small applied cell voltage of~1.83 V to deliver 10 mA cm^(-2),compared with that of the pure water electrolyzer(OER||HER,~1.99 V).This study simultaneously realized the integrated production of energy-saving H_(2)fuel at the cathode and 2-furoic acid at the anode.

关键词： biomass conversion electrochemical furfural oxidation overall water splitting Pt-Co_(3)O_(4)electrocatalyst pulsed laser ablation in liquid

A Remark on Leray's Problem on Stationary Navier–Stokes Flows with Large Fluxes in Infinite Cylindrical Domains

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Acta Mathematica Sinica,English Series 2015年第10期31卷 1571-1581页

作者： myong-Hwan RI Institute of Mathematics State Academy of SciencesPyongyang DPR Korea

We consider Leray＇s problem on stationary Navier Stokes flows with arbitrary large fluxes in an unbounded cylinder with several exits to infinity. For a stationary Navier Stokes flow with large fluxes in the unbounded cylinder, we prove that, if the difference between the pressure of the main flow and the pressure of the Poiseuille flow with the same flux in a branch of the cylinder remains bounded at ｜x｜→∞, then the flow behaves at infinity of the branch like the Poiseuille flow.

关键词： Leray's problem Navier-Stokes equations large flux unbounded cylindrical domains

Manifolding active sites and in situ/operando electrochemical-Raman spectroscopic studies of single-metal nanoparticle-decorated CuO nanorods in furfural biomass valorization to H_(2) and 2-furoic acid

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Journal of Energy Chemistry 2023年第9期84卷 50-61页

作者： Jiwon Kim Talshyn Begildayeva Jayaraman Theerthagiri Cheol Joo Moon Ahreum Min seung Jun Lee Gyeong-Ah Kim myong Yong Choi Department of Chemistry(BK21 FOUR) Research Institute of Natural SciencesGyeongsang National UniversityJinju 52828Republic of Korea Core-Facility Center for Photochemistry&Nanomaterials Gyeongsang National UniversityJinju 52828Republic of Korea Department of IT-Energy Convergence(BK21 FOUR) Korea National University of TransportationChungju 27469Republic of Korea

Here,CuO nanorods fabricated via pulsed laser ablation in liquids were decorated with Ir,Pd,and Ru NPs(loading~7 wt%) through pulsed laser irradiation in the liquids *** resulting NPs-decorated CuO nanorods were characterized spectroscopically and employed as multifunctional electrocatalysts in OER,HER,and the furfural oxidation reactions(FOR).Ir-CuO nanorods afford the lowest overpotential of~345 mV(HER) and 414 mV(OER) at 10 mA cm^(-2),provide the highest 2-furoic acid yield(~10.85 mM) with 64.9% selectivity,and the best Faradaic efficiency~72.7% in 2 h of FOR at 1.58 V(***).In situ electrochemical-Raman analysis of the Ir-CuO detects the formation of the crucial intermediates,such as Cu(Ⅲ)-oxide,Cu(OH)_(2),and Ir_x(OH)_y,on the electrode-electrolyte surface,which act as a promoter for HER and *** Ir-CuO ‖ Ir-CuO in a coupled HER and FOR-electrolyzer operates at~200 mV lower voltage,compared with the conventional electrolyzer and embodies the dual advantage of energy-saving H_(2) and 2-furoic acid production.

关键词： Single-metal nanoparticle-decorated CuO nanorods Pulsed laser ablation and irradiation in liquids Furfural oxidation reaction Hydrogen evolution reaction Energy-saving H_(2)production 2-Furoic acid

Regularity for 3D Navier–Stokes Equations Based on Energy Distribution at Wavenumber Bands

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Acta Mathematica Sinica,English Series 2019年第8期35卷 1377-1392页

作者： myong-Hwan RI Institute of Mathematics State Academy of SciencesDPR Korea

We present some regularity criteria for the Leray–Hopf weak solutions to the Cauchy problem for 3D Navier–Stokes equations based on energy distribution at wavenumber bands. We show sufficient conditions for regularity based on the ratios of energy dissipation rates at sufficiently high wavenumber bands and neighboring medium wavenumber bands. Moreover, we give a regularity criterion based on relations between energy at high and low wavenumber bands.

关键词： Navier-Stokes equations global regularity energy transfer

Ligand-free monophasic CuPd alloys endow boosted reaction kinetics toward energy-efficient hydrogen fuel production paired with hydrazine oxidation

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Journal of Materials Science & Technology 2023年第12期143卷 20-29页

作者： Yujeong Jeong Shreyanka Shankar Naik Yiseul Yu Jayaraman Theerthagiri seung Jun Lee Pau Loke Show Hyun Chul Choi myong Yong Choi Department of Chemistry(BK21 FOUR) Research Institute of Natural SciencesGyeongsang National UniversityJinju 52828Republic of Korea Core-Facility Center for Photochemistry&Nanomaterials Gyeongsang National UniversityJinju 52828Republic of Korea Zhejiang Provincial Key Laboratory for Subtropical Water Environment and Marine Biological Resources Protection Wenzhou UniversityWenzhou 325035China Department of Chemical and Environmental Engineering Faculty of Science and EngineeringUniversity of Nottingham MalaysiaJalan Broga43500 SemenyihSelangor Darul EhsanMalaysia Department of Chemistry Chonnam National UniversityGwangju 61186Republic of Korea

Optimizing the structure and components is a prevalent strategy for increasing electrocatalytic energy-saving H 2 fuel *** of the sustainable and efficient techniques is electrocatalytic water split-ting for H 2 generation,but it is still restricted by the kinetically sluggish *** to the lower standard oxidation potential of−0.33 V,replacing the OER with anodic hydrazine oxidation reaction(HzOR)is an effective way to extensively reduce the use of electricity in water *** alloying,the semiconductor and adsorption characteristics of Cu,interlaced by Pd 2+solution on the Pd surface by pulsed laser ablation(PLA)in methanol,are selectively altered to maximize cathodic HER and anodic HzOR *** optimal Cu1Pd3/C ratio demonstrates outstanding HER performance with a low overpotential of 0.315 V at 10 mA cm^(−2),as well as an ultralow overpotential of 0.560 V for HzOR in 0.5 M N_(2) H_(4)/1.0 M ***,the constructed HzOR-assisted electrolyzer cell with Cu1Pd3/C||Cu1Pd3/C as anode and cathode exhibits a cell voltage of 0.505 V at 10 mA cm^(−2) with exceptional en-durance over 5 *** current study advances competent CuPd alloys as multifunctional electrocatalysts for H 2 fuel production using a HzOR-assisted energy-efficient electrolyzer.

关键词： PLA CuPd alloy Sonochemical process HzOR Hydrazine evolution reaction Hydrazine splitting Water splitting

Increased liver markers are associated with higher risk of type 2 diabetes

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World Journal of Gastroenterology 2015年第24期21卷 7478-7487页

作者： Sun-Hye Ko myong Ki Baeg Kyung-Do Han seung-Hyun Ko Yu-Bae Ahn Division of Endocrinology and Metabolism Department of Internal Medicine College of Medicine The Catholic University of Korea Division of Gastroenterology Department of Internal Medicine College of Medicine The Catholic University of Korea Department of Biostatistics College of Medicine The Catholic University of Korea

AIM: To investigate the association between liver markers and the risk of type 2 diabetes(T2DM) and impaired fasting glucose(IFG).METHODS: A total of 8863 participants(3408 men and 5455 women) over 30 years of age were analyzed from the fifth Korean National Health and Nutrition Examination Survey(2010-2011). The associations of serum liver markers such as aspartate aminotransferase(AST), alanine aminotransferase(ALT), AST/ALT, and gamma-glutamyltransferase(GGT) with T2 DM and IFG were analyzed using logistic regression models. Participants were divided into sex-specific quartiles on the basis of liver ***: The prevalence of T2 DM and IFG were 11.3% and 18.3%. Increasing quartiles of ALT and GGT were positively and AST/ALT were negatively correlated with T2 DM and IFG. Analysis of the liver marker combinations showed that if any two or more markers were in the highest risk quartile, the risks of both T2 DM and IFG increased significantly. The risk was greatest when the highest ALT and GGT and lowest AST/ALT quartile were combined, with the riskof T2 DM at 3.21(95%CI: 1.829-5.622, P ile had a 1.99 and 2.40 times increased risk of ***: Higher levels of GGT and ALT and lower AST/ALT within the physiological range are independent, additive risk factors of T2 DM and IFG.

关键词： Type 2 diabetes mellitus Liver markers Impaired fasting glucose Gamma-glutamyl transferase Aspartate aminotransferase Alanine aminotransferase

MAXIMAL L^(1)-REGULARITY OF GENERATORS FOR BOUNDED ANALYTIC SEMIGROUPS IN BANACH SPACES

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Acta Mathematica Scientia 2022年第4期42卷 1261-1272页

作者： myong-Hwan RI Reinhard FARWIG Institute of Mathematics State Academy of SciencesPyongyangDPR Korea Department of Mathematics Darmstadt University of TechnologyGermany

In this paper,we prove that the generator of any bounded analytic semigroup in(θ,1)-type real interpolation of its domain and underlying Banach space has maximal L^(1)-regularity,using a duality argument combined with the result of maximal continuous *** an application,we consider maximal L^(1)-regularity of the Dirichlet-Laplacian and the Stokes operator in inhomogeneous B_(q),^(s),1-type Besov spaces on domains of R^(n),n≥2.

关键词： Maximal L^(1)-regularity sectorial operator Stokes operator

Application of powdered activated carbon coating to fabrics in a hybrid filter to enhance mercury removal

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Journal of Environmental Sciences 2019年第6期31卷 58-65页

作者： Jin-Ho Sung seung-Ki Back Eun-Song Lee Ha-Na Jang Yong-Chil Seo Youn-Suk Kang myong-Hwa Lee Department of Environmental Engineering Yonsei University J-E Tech Co. Ltd Department of Environmental Engineering Kangwon National University

Elemental mercury(Hg0) is predominant constituent of flue gas emitted from coal-fired power plants. Adsorption has been considered the best available technology for removal of Hg0 from flue gas. However, adsorbent injection increases the amount of ash generated. In the present study, powdered activated carbon(PAC) was coated on polytetrafluoroethylene/glass fiber filters to increase Hg0 removal while concurrently reducing the amount of ash generated. The optimal PAC coating rate was determined in laboratory experiments to ensure better Hg0 removal with low pressure drop. When PAC of particle size less than 45 μm was used, and the areal density was 50 g/m2, the pressure drop remained under 30 Pa while the Hg0 removal efficiency increased to 15.8% from4.3%. The Hg0 removal efficiency also increased with decrease in filtration velocity. The optimal PAC coating rate was applied on a hybrid filter(HF), which was combined with a bag filter and an electrostatic precipitator in a single chamber. Originally designed to remove fine particulates matter, it was retrofitted to the flue gas control device for simultaneous Hg0 removal. By employing the PAC coating, the Hg removal efficiency of the HF increased to 79.79% from 66.35%. Also, a temporary reduction in Hg removal was seen but this was resolved following a cleaning cycle in which the dust layer was removed.

关键词： Mercury Hybrid filter Activated carbon Coating filter Coal-fired power plant

Fundamentals and comprehensive insights on pulsed laser synthesis of advanced materials for diverse photo-and electrocatalytic applications

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Light(Science & Applications) 2022年第9期11卷 2018-2064页

作者： Jayaraman Theerthagiri K Karuppasamy seung Jun Lee R.Shwetharani Hyun-Seok Kim S.K Khadheer Pasha Muthupandian Ashokkumar myong Yong Choi Core-Facility Center for Photochemistry&Nanomaterials Department of ChemistryResearch Institute of Natural SciencesGyeongsang National UniversityJinju 52828Republic of Korea Division of Electronics and Electrical Engineering Dongguk University-SeoulSeoul 04620Republic of Korea Centre for Nano and Material Sciences Jain UniversityJain Global CampusKanakapuraBangalore 562112 KarnatakaIndia Department of Physics Vellore Institute of Technology(Amaravati Campus)Amaravati522501 GunturAndhra PradeshIndia School of Chemistry University of MelbourneParkville CampusMelbourneVIC 3010Australia

The global energy crisis is increasing the demand for innovative materials with high purity and functionality for the development of clean energy production and *** development of novel photo-and electrocatalysts significantly depends on synthetic techniques that facilitate the production of tailored advanced *** emerging use of pulsed laser in liquid synthesis has attracted immense interest as an effective synthetic technology with several advantages over conventional chemical and physical synthetic routes,including the fine-tuning of size,composition,surface,and crystalline structures,and defect densities and is associated with the catalytic,electronic,thermal,optical,and mechanical properties of the produced ***,we present an overview of the fundamental understanding and importance of the pulsed laser process,namely various roles and mechanisms involved in the production of various types of nanomaterials,such as metal nanoparticles,oxides,non-oxides,and carbon-based *** mainly cover the advancement of photo-and electrocatalytic nanomaterials via pulsed laser-assisted technologies with detailed mechanistic insights and structural optimization along with effective catalytic performances in various energy and environmental remediation ***,the future directions and challenges of pulsed laser techniques are briefly *** review can exert practical guidance for the future design and fabrication of innovative pulsed laser-induced nanomaterials with fascinating properties for advanced catalysis applications.

关键词： insight synthesis comprehensive