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Understanding the catalysis of chromium trioxide added magnesium hydride for hydrogen storage and Li ion battery applications

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Journal of Magnesium and Alloys 2024年第3期12卷 1117-1130页

作者： d.Pukazhselvan IhsanÇaha Catarina de Lemos sergey M.Mikhalev Francis Leonard deepak duncan Paul Fagg department of Mechanical Engineering TEMA-Centre for Mechanical Technology and AutomationUniversity of AveiroAveiro 3810-193Portugal LASI-Intelligent Systems Associate Laboratory Guimarães 4800-058Portugal Nanostructured Materials Group International Iberian Nanotechnology Laboratory(INL)Avenida Mestre Jose VeigaBraga 4715-330Portugal

This study explores how the chemical interaction between magnesium hydride(MgH_(2))and the additive CrO_(3) influences the hydrogen/lithium storage characteristics of MgH_(2).We have observed that a 5 wt.%CrO_(3) additive reduces the dehydrogenation activation energy of MgH_(2) by 68 kJ/mol and lowers the required dehydrogenation temperature by 80℃.CrO_(3) added MgH_(2) was also tested as an anode in an Li ion battery,and it is possible to deliver over 90%of the total theoretical capacity(2038 mAh/g).Evidence for improved reversibility in the battery reaction is found only after the incorporation of additives with MgH_(2).In depth characterization study by X-ray diffraction(XRd)technique provides convincing evidence that the CrO_(3) additive interacts with MgH_(2) and produces Cr/MgO *** free energy analyses confirm the thermodynamic feasibility of conversion from MgH_(2)/CrO_(3) to MgO/Cr,which is well supported by the identification of Cr(0)in the powder by X ray photoelectron spectroscopy(XPS)*** high resolution transmission electron microscopy(HRTEM)and energy dispersive spectroscopy(EdS)we found evidence for the presence of 5 nm size Cr nanocrystals on the surface of MgO rock salt *** is also convincing ground to consider that MgO rock salt accommodates Cr in the *** observations support the argument that creation of active metal–metal dissolved rock salt oxide interface may be vital for improving the reactivity of MgH_(2),both for the improved storage of hydrogen and lithium.

关键词： Hydrogen storage Rechargeable batteries Binary hydrides Metal oxides Catalytic mechanism.

Investigation of WZ Sge-type dwarf Nova ASASSN-19oc: Optical Spectroscopy and Multicolor Light Curve Analysis

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Research in Astronomy and Astrophysics 2024年第8期24卷 22-33页

作者： Viktoriia Krushevska sergey Shugarov Paolo Ochner Yuliana Kuznyetsova Mykola Petrov Peter Kroll Astronomical Institute of the Slovak Academy of Sciences Main Astronomical Observatory of NAS of Ukraine INAF—Osservatorio Astronomico di Padova department of Physics and Astronomy University of Padova Max Planck Computing and data Facility (MPCdF) Sonneberg Observatory

In this study,we present an investigation of the newly discovered dwarf nova ASASSN-19oc during its superoutburst on 2019 June *** carried out detailed UBVRcIc-photometric observations and also obtained a spectrum on day 7 of the outburst,which shows the presence of hydrogen absorption lines commonly found in dwarf nova *** of photometric data reveals the occurrence of early superhumps in the initial days of observations,followed by ordinary and late *** have accurately calculated the period of the ordinary superhumps as Pord=0.05681（10） days and determined the periods at different stages,as well as the rate of change of the superhump period (Pdot=（5）P/P=8.1×10-5).Additionally,we have derived the mass ratio of the components （q=0.09）,and estimated the color temperature during the outburst as～11,000 K,the distance to the system （d=560 pc） and absolute magnitude of the system in outburst （MV=5.3）.We have shown that outbursts of this star are very rare:based on brightness measurements on 600 archival photographic plates,we found only one outburst that occurred in *** fact,as well as the properties listed above,convincingly shows that the variable ASASSN-19oc is a dwarf nova of WZ Sge type.

关键词： (stars:) binaries (including multiple): close (stars:) novae cataclysmic variables stars: dwarf novae

Assessment of the ecological state of haplic chernozem contaminated by oil,fuel oil and gasoline after remediation

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Petroleum Research 2024年第1期9卷 155-164页

作者： Anna Ruseva Tatiana Minnikova sergey Kolesnikov dmitry Trufanov Nikita Minin Sofya Revina Vladimir Gayvoronsky Southern Federal University Academy of Biology and Biotechnology344090Rostov-on-DonRussia

The intensive use of petroleum hydrocarbon products has made them priority environmental *** petroleum hydrocarbons enter the soil,a change in physical,chemical,and biological properties is *** natural restoration of oil-contaminated soils is a lengthy process;therefore,remediation is often *** aim of this study is to assess the change in the ecological state of haplic chernozem soil contaminated with oil,fuel oil,and gasoline after *** indicators of soil biological activity,such as phytotoxicity(germination,length of shoots and roots),the activity of oxidoreductase enzymes(catalase and dehydrogenases),and the total number of bacteria were *** effects of nitroammophoska fertilizer,sodium humate,biochar,and the biofertilizer“Baikal EM-1”on the ecological state of soils contaminated with oil,fuel oil,and gasoline were *** with oil,fuel oil,and gasoline decreased the values of all biological *** most sensitive indicator was the length of radish roots in soils polluted with oil,gasoline,and fuel oil after remediation with nitroammophoska and Baikal EM-1 *** length of roots was the most sensitive indicator when remediation was performed with biochar and sodium humate added to soil contaminated with oil and gasoline,and with contamination of haplic chernozem soil with fuel oil,the total number of bacteria was the most sensitive *** most effective ameliorant to phytotoxicity indicators for oil pollution was a 1 d dose of biochar,for fuel oil it was 1 d biochar and 2 d sodium humate,and for gasoline it was a 2 d dose of biochar and Baikal *** ameliorants at most of the studied doses increased dehydrogenase activity,but increased catalase activity only in some *** increase in the total number of bacteria in oil-contaminated soils was promoted by biochar and nitroammophoska at a dose of 2 *** was the most effective in ameliorant in soils contaminated with fuel

关键词： Pollution Petroleum hydrocarbons Haplic chernozem Ameliorant dose Biological indicators Soil properties

Polariton lasing in Mie-resonant perovskite nanocavity

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Opto-Electronic Advances 2024年第4期7卷 27-42页

作者： Mikhail A.Masharin daria Khmelevskaia Valeriy I.Kondratiev daria I.Markina Anton d.Utyushev dmitriy M.dolgintsev Alexey d.dmitriev Vanik A.Shahnazaryan Anatoly P.Pushkarev Furkan Isik Ivan V.Iorsh Ivan A.Shelykh Hilmi V.demir Anton K.Samusev sergey V.Makarov UNAM-Institute of Materials Science and Nanotechnology National Nanotechnology Research CenterDepartment of Electrical and Electronics EngineeringDepartment of PhysicsBilkent UniversityAnkara 06800Turkey ITMO University School of Physics and EngineeringSt.Petersburg 197101Russia Abrikosov Center for Theoretical Physics MIPTDolgoprudnyiMoscow Region 141701Russia LUMINOUS!Center of Excellence for Semiconductor Lighting and displays School of Electrical and Electronic EngineeringSchool of Physical and Mathematical SciencesSchool of Materials Science and EngineeringNanyang Technological UniversitySingapore 639798Singapore department of Physics Engineering Physics and AstronomyQueen’s UniversityKingstonOntario K7L 3N6Canada Science Institute University of IcelandDunhagi 3IS-107ReykjavikIceland Experimentelle Physik 2 Technische Universität DortmundDortmund 44227Germany Qingdao Innovation and development Center Harbin Engineering UniversityQingdao 266000China

deeply subwavelength lasers(or nanolasers)are highly demanded for compact on-chip bioimaging and sensing at the *** of the main obstacles for the development of single-particle nanolasers with all three dimensions shorter than the emitting wavelength in the visible range is the high lasing thresholds and the resulting *** we ex-ploit exciton-polariton condensation and mirror-image Mie modes in a cuboid CsPbBr3 nanoparticle to achieve coherent emission at the visible wavelength of around 0.53μm from its ultra-small(≈0.007μm3 or≈λ3/20)semiconductor *** polaritonic nature of the emission from the nanocavity localized in all three dimensions is proven by direct com-parison with corresponding one-dimensional and two-dimensional waveguiding systems with similar material *** a deeply subwavelength nanolaser is enabled not only by the high values for exciton binding energy(≈35 meV),re-fractive index(>2.5 at low temperature),and luminescence quantum yield of CsPbBr3,but also by the optimization of po-laritons condensation on the Mie resonances with quality factors improved by the metallic ***,the key parameters for optimal lasing conditions are intermode free spectral range and phonons spectrum in CsPbBr3,which govern polaritons condensation *** chemically synthesized colloidal CsPbBr3 nanolasers can be potentially de-posited on arbitrary surfaces,which makes them a versatile tool for integration with various on-chip systems.

关键词： nanolaser perovskite polariton Mie resonance exciton-polariton

Recent Ventures in Interdisciplinary Arctic Research:The ARCPATH Project

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Advances in Atmospheric Sciences 2024年第8期41卷 1559-1568页

作者： Astrid E.J.OGILVIE Leslie A.KING Noel KEENLYSIdE François COUNILLON Brynhildur dAVIÐSdÓTTIR Níels EINARSSON sergey GULEV Ke FAN Torben KOENIGK James R.MCGOOdWIN Marianne H.RASMUSSON Shuting YANG Institute of Arctic and Alpine Research(INSTAAR) University of ColoradoBoulder CO 80303USA Stefansson Arctic Institute AkureyriÍS-600Iceland Royal Roads University BC V9B 5Y2Canada University of Bergen Bergen N-5007Norway Nansen Environmental and Remote Sensing Centre Bergen N-5007Norway University of Iceland Reykjavík 102Iceland Shirshov Institute of Oceanology Moscow 117218Russia Moscow State University Moscow 11991Russia Chinese Academy of Sciences Beijing 100045China Swedish Meteorological and Hydrological Institute SE-60176 NorrköpingSweden danish Meteorological Institute CopenhagenØ2100Denmark Obukhov Institute of Atmospheric Physics RAS119017MoscowRussia

This paper celebrates Professor Yongqi GAO's significant achievement in the field of interdisciplinary studies within the context of his final research project Arctic Climate Predictions: Pathways to Resilient Sustainable Societies-ARCPATH(https://***/en/projects/finished-projects/arcpath). The disciplines represented in the project are related to climatology, anthropology, marine biology, economics, and the broad spectrum of social-ecological studies. Team members were drawn from the Nordic countries, Russia, China, the United States, and Canada. The project was transdisciplinary as well as interdisciplinary as it included collaboration with local knowledge holders. ARCPATH made significant contributions to Arctic research through an improved understanding of the mechanisms that drive climate variability in the Arctic. In tandem with this research, a combination of historical investigations and social, economic, and marine biological fieldwork was carried out for the project study areas of Iceland, Greenland, Norway, and the surrounding seas, with a focus on the joint use of ocean and sea-ice data as well as social-ecological drivers. ARCPATH was able to provide an improved framework for predicting the near-term variation of Arctic climate on spatial scales relevant to society, as well as evaluating possible related changes in socioeconomic realms. In summary, through the integration of information from several different disciplines and research approaches, ARCPATH served to create new and valuable knowledge on crucial issues, thus providing new pathways to action for Arctic communities.

关键词： Recent Ventures in Interdisciplinary Arctic Research:The ARCPATH Project

氧同位素3早期以来千年尺度气候事件在日本海北部的磁学记录

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海洋学报 2024年第4期46卷 106-121页

作者：邹庆超石学法葛淑兰吴永华邹建军贺湘锋 sergey A.Gorbarenko 刘建兴自然资源部第一海洋研究所海洋地质与成矿作用自然资源部重点实验室山东青岛266061 青岛海洋科技中心海洋地质过程与环境功能实验室山东青岛266237 南京大学地理与海洋科学学院江苏南京210023 俄罗斯科学院远东分院太平洋研究所俄罗斯符拉迪沃斯托克690041

日本海是西北太平洋最大的边缘海,长期以来普遍认为其沉积物处于强烈的还原环境中而导致相应的磁学信号非常微弱,以致常用的磁学方法在该区的应用一直受限。为深入探讨磁学指标在日本海古环境与古海洋学研究中是否有效,本文对位于研究... 详细信息

日本海是西北太平洋最大的边缘海,长期以来普遍认为其沉积物处于强烈的还原环境中而导致相应的磁学信号非常微弱,以致常用的磁学方法在该区的应用一直受限。为深入探讨磁学指标在日本海古环境与古海洋学研究中是否有效,本文对位于研究程度相对薄弱的北部一根626 cm长的柱状沉积物岩心(LV87-2-3孔,水深740 m)开展了系统的岩石磁学测试分析以及高分辨率的AMS14C测年和粒度分析。结果显示岩心系约48.3 ka BP以来的沉积记录,其55 cm以下层位的原生亚铁磁性矿物(主要为磁铁矿)已被大量还原而生成黄铁矿,导致磁性极弱。这与dansgaard-Oeschger(d-O)旋回间冰阶水体分层加强和表层生产力提高等因素密切相关。然而,在此背景下仍存在4个以高矫顽力矿物(如赤铁矿和针铁矿)占比较高为明显特征的强磁性层位,即“硬磁异常”层;其很好地对应了海因里希(Heinrich)事件,指示了东亚冬季风(EAWM)增强和高盐度对马暖流(TWC)注入而导致的相对减弱的还原环境。上述变化在沉积物粒度上却未见清晰体现。因此,该研究不仅表明磁学参数对于指示末次冰期日本海古海洋与古环境演化的作用不容忽视,同时也为后续相关工作提供了新视角和新思路。

关键词：日本海沉积物磁性矿物岩石磁学古环境 Heinrich事件

Exploring van der Waals materials with high anisotropy:geometrical and optical approaches

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Light(Science & Applications) 2024年第4期13卷 645-653页

作者： Aleksandr S.Slavich Georgy A.Ermolaev Mikhail K.Tatmyshevskiy Adilet N.Toksumakov Olga G.Matveeva dmitriy V.Grudinin Kirill V.Voronin Arslan Mazitov Konstantin V.Kravtsov Alexander V.Syuy dmitry M.Tsymbarenko Mikhail S.Mironov sergey M.Novikov Ivan Kruglov davit A.Ghazaryan Andrey A.Vyshnevyy Aleksey V.Arsenin Valentyn S.Volkov Kostya S.Novoselov Moscow Center for Advanced Studies Kulakova str.20Moscow 123592Russia. Emerging Technologies Research Center XPANCEOInternet CityEmmay TowerDubaiUnited Arab Emirates. donostia International Physics Center(dIPC) Donostia/San-Sebastián 20018Spain. Institute of Materials Ecole Polytechnique Federale de Lausanne1015 LausanneSwitzerland. department of Chemistry Lomonosov Moscow State UniversityMoscow 119991Russia. Laboratory of Advanced Functional Materials Yerevan State UniversityYerevan 0025Armenia. National Graphene Institute(NGI) University of ManchesterManchester M139PLUK. department of Materials Science and Engineering National University of SingaporeSingapore 03-09 EASingapore. Institute for Functional Intelligent Materials National University of Singapore117544 SingaporeSingapore

The emergence of van der Waals(vdW)materials resulted in the discovery of their high optical,mechanical,and electronic anisotropic properties,immediately enabling countless novel phenomena and *** success inspired an intensive search for the highest possible anisotropic properties among vdW ***,the identification of the most promising among the huge family of vdW materials is a challenging quest requiring innovative ***,we suggest an easy-to-use method for such a survey based on the crystallographic geometrical perspective of vdW materials followed by their optical *** our approach,we found As2S3 as a highly anisotropic vdW *** demonstrates high in-plane optical anisotropy that is~20%larger than for rutile and over two times as large as calcite,high refractive index,and transparency in the visible range,overcoming the century-long record set by *** these benefits,As2S3 opens a pathway towards nextgeneration nanophotonics as demonstrated by an ultrathin true zero-order quarter-wave plate that combines classical and the Fabry–Pérot optical phase ***,our approach provides an effective and easy-to-use method to find vdW materials with the utmost anisotropic properties.

关键词： anisotropy anisotropic high

A data-driven Rutting depth Short-Time Prediction Model With Metaheuristic Optimization for Asphalt Pavements Based on RIOHTrack

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自动化学报:英文版 2023年第10期10卷 1918-1932页

作者： Zhuoxuan Li Iakov Korovin Xinli Shi sergey Gorbachev Nadezhda Gorbacheva Wei Huang Jinde Cao School of Mathematics Southeast UniversityNanjing 210096China Scientific Research Institute of Multiprocessor Computer Systems Southern Federal UniversityTaganrog 347928Russia School of Cyber Science and Engineering Southeast UniversityNanjing 210096China Russian Academy of Engineering Moscow 125009Russia Intelligent Transportation System Research Center Southeast UniversityNanjing 210096China Nanjing Modern Multimodal Transportation Laboratory Nanjing 211100China Yonsei Frontier Laboratory Yonsei UniversitySeoulKorea(South)

Rutting of asphalt pavements is a crucial design criterion in various pavement design guides. A good road transportation base can provide security for the transportation of oil and gas in road transportation. This study attempts to develop a robust artificial intelligence model to estimate different asphalt pavements’ rutting depth clips, temperature, and load axes as primary characteristics. The experiment data were obtained from19 asphalt pavements with different crude oil sources on a 2.038km long full-scale field accelerated pavement test track(Road Track Institute, RIOHTrack) in Tongzhou, Beijing. In addition,this paper also proposes to build complex networks with different pavement rutting depths through complex network methods and the Louvain algorithm for community detection. The most critical structural elements can be selected from different asphalt pavement rutting data, and similar structural elements can be found. An extreme learning machine algorithm with residual correction(RELM) is designed and optimized using an independent adaptive particle swarm algorithm. The experimental results of the proposed method are compared with several classical machine learning algorithms, with predictions of average root mean squared error(MSE), average mean absolute error(MAE), and a verage mean absolute percentage error(MAPE) for 19 asphalt pavements reaching 1.742, 1.363, and 1.94% respectively. The experiments demonstrate that the RELM algorithm has an advantage over classical machine learning methods in dealing with non-linear problems in road engineering. Notably, the method ensures the adaptation of the simulated environment to different levels of abstraction through the cognitive analysis of the production environment parameters. It is a promising alternative method that facilitates the rapid assessment of pavement conditions and could be applied in the future to production processes in the oil and gas industry.

关键词： Extreme learning machine algorithm with residual correction(RELM) metaheuristic optimization oil-gas transportation RIOHTrack,rutting depth

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Advances in femtosecond laser direct writing of fiber Bragg gratings in multicore fibers:technology,sensor and laser applications

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Opto-Electronic Advances 2022年第4期5卷 48-68页

作者： Alexey Wolf Alexander dostovalov Kirill Bronnikov Mikhail Skvortsov Stefan Wabnitz sergey Babin Novosibirsk State University Novosibirsk 630090Russia Institute of Automation and Electrometry of the SB RAS Novosibirsk 630090Russia department of Information Electronics and Telecommunications EngineeringSapienza University of RomeRome 00184Italy

In this article,we review recent advances in the technology of writing fiber Bragg gratings(FBGs)in selected cores of multicore fibers(MCFs)by using femtosecond laser *** writing technology of such a key element as the FBG opens up wide opportunities for the creation of next generation fiber lasers and sensors based on *** advantages of the technology are shown by using the examples of 3d shape sensors,acoustic emission sensors with spatially multiplexed channels,as well as multicore fiber Raman lasers.

关键词： multicore fiber fiber Bragg grating femtosecond laser micromachining fiber laser fiber sensor