检索结果-南通市图书馆

Transition Metal Aluminum Boride as a New Candidate for Ambient-Condition Electrochemical Ammonia Synthesis

Nano-Micro Letters 2020年第5期12卷 106-118页

作者： Yang Fu Peter Richardson Kangkang Li Hai Yu Bing Yu scott donne Erich Kisi Tianyi Ma Discipline of Chemistry School of Environmental and Life SciencesUniversity of NewcastleCallaghanNSW 2308Australia School of Engineering University of NewcastleCallaghanNSW 2308Australia CSIRO Energy 10 Murray Dwyer CircuitMayfield WestNSW 2304Australia School of Environmental Science and Engineering Fujian Normal UniversityFuzhou 350007FujianPeople’s Republic of China

Achieving more meaningful N2 conversion by reducing the energy input and carbon footprint is now being investigated through a method of N2 fixation instead of the Haber-Bosch process.Unfortunately,the electrochemical N2 reduction reaction(NRR)method as a rising approach currently still shows low selectivity(Faradaic efficiency<10%)and high-energy consumption[applied potential at least-0.2 V versus the reversible hydrogen electrode(RHE)].Here,the role of molybdenum aluminum boride single crystals,belonging to a family of ternary transition metal aluminum borides known as MAB phases,is reported for the electrochemical NRR for the first time,at a low applied potential(-0.05 V versus RHE)under ambient conditions and in alkaline media.Due to the unique nano-laminated crystal structure of the MAB phase,these inexpensive materials have been found to exhibit excellent electrocatalytic performances(NH3 yield:9.2μg h^-1cm^-2mgcat^-1.,Faradaic efficiency:30.1%)at the low overpotential,and to display a high chemical stability and sustained catalytic performance.In conjunction,further mechanism studies indicate B and Al as main-group metals show a highly selective affinity to N2 due to the strong interaction between the B 2p/Al 3p band and the N 2p orbitals,while Mo exhibits specific catalytic activity toward the subsequent reduction reaction.Overall,the MAB-phase catalyst under the synergy of the elements within ternary compound can suppress the hydrogen evolution reaction and achieve enhanced NRR performance.The significance of this work is to provide a promising candidate in the future synthesis of ammonia.

关键词： MAB phase N2 reduction reaction Electrocatalysis Nanostructure

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Effects of Enriched Biochars Containing Magnetic Iron Nanoparticles on Mycorrhizal Colonisation,Plant Growth,Nutrient Uptake and Soil Quality Improvement

引用

Pedosphere 2015年第5期25卷 749-760页

作者： Stephen JOSEPH Hossain M.ANAWAR Paul STORER Paul BLACKWELL Chee CHIA Yun LIN Paul MUNROE scott donne Josip HORVAT Jianli WANG Zakaria M.SOLAIMAN School of Materials Science and Engineering University of New South WalesSydney Discipline of Chemistry University of Newcastle Institute for Superconducting and Electronic Materials and School of Physics University of Wollongong Soil Biology and Molecular Ecology Group School of Earth and Environment (M087) and UWA Institute of AgricultureFaculty of ScienceThe University of Western Australia Australian Mineral Fertilisers Pty Ltd. Department of Agriculture and Food Western Australia Geraldton Regional Office Institute for Superconducting and Electronic Materials University of Wollongong

At present, there is little commercial sale of biochar, since farmers find they can not gain a return on their investment in this amendment in the first few years after its application, because of the high cost associated with large application rates. To overcome this constraint, development of artificially aged enriched biochar-mineral complexes(BMCs), having a higher mineral content, surface functionality, exchangeable cations, high concentration of magnetic iron(Fe) nanoparticles, and higher water-extractable organic compounds has been undertaken by a combined team of researchers and a commercial company. Two biochars produced under different pyrolysis conditions were activated with a phosphoric acid treatment. A mixture of clay, chicken litter, and minerals were added to the biochar, and then this composite was torrefied at either 180 or 220?C. In this study a pot experiment was carried out in glasshouse conditions to determine the effects of four different BMCs, with different formulations applied at rates of 100 and 200 kg ha-1, on the mycorrhizal colonisation, wheat growth and nutrient uptake, and soil quality improvement. It was found that the phosphorus(P) and nitrogen uptake in wheat shoots were significantly greater for a low application rate of BMCs(100 kg ha-1). The present formulation of BMC was effective in enhancing growth of wheat at low application rate(100 kg ha-1). The increase in growth appeared due to an increase in P uptake in the plants that could be partly attributed to an increase in mycorrhizal colonisation and partly due to the properties of the BMC.

关键词：养分吸收植物生长土壤质量生物炭磁性纳米粒子菌根矿物质含量小麦生长

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Developing More Effective Enhanced Biochar Fertilisers for Improvement of Pepper Yield and Quality

引用

Pedosphere 2015年第5期25卷 703-712页

作者： YAO Chunxue Stephen JOSEPH LI Lianqing PAN Genxing Yun LIN Paul MUNROE Ben PACE Sarasadat TAHERYMOOSAVI Lukas VAN ZWIETEN Torsten THOMAS Shaun NIELSEN Jun YE scott donne Institute of Resources Ecosystem and Environment of Agriculture Nanjing Agricultural University Discipline of Chemistry University of Newcastle School of Materials Science and Engineering University of New South Wales New South Wales Department of Primary Industries School of Biotechnology and Biomolecular Sciences & Centre for Marine Bio-Innovation University of New South Wales

Utilization of biochar at high application rates can increase soil C and crop yields, decrease greenhouse gas emissions and reduce nutrient run-off from soils. However, the high application rate of 10 t ha-1may not return a profit to the farmer due to the high cost of biochar. In this study biochar was modified through pre-treating the biomass and post-treating with phosphoric acid, minerals and different chemical fertilisers to study the effects of two new enhanced biochar fertilisers on the yield and quality of green pepper in a field experiment with 5 fertilisation treatments and 3 replications. The two new biochar fertilisers significantly(P < 0.05) increased the yield of green pepper(11.33–11.47 t ha-1), compared with the conventional chemical fertiliser(9.72 t ha-1). The biochar fertiliser treatments improved the vitamin C content of green pepper from 236.99 to 278.28 mg kg-1, and also significantly(P < 0.05) reduced the nitrate content from 132.32 to 101.92 mg kg-1, compared with chemical fertiliser. This study indicated that, compared to the use of conventional chemical fertiliser, all of the biochar fertiliser treatments could significantly improve the yield and quality of green pepper.

关键词：作物产量生物肥料辣椒质量土壤养分流失温室气体排放量开发常规化肥

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Feeding Biochar to Cows:An Innovative Solution for Improving Soil Fertility and Farm Productivity

引用

Pedosphere 2015年第5期25卷 666-679页

作者： Stephen JOSEPH Doug POW Kathy DAWSON David R.G.MITCHELL Aditya RAWAL James HOOK Sarasadat TAHERYMOOSAVI Lukas VAN ZWIETEN Joshua RUST scott donne Paul MUNROE Ben PACE Ellen GRABER Torsten THOMAS Shaun NIELSEN Jun YE Yun LIN PAN Genxing LI Lianqing Zakaria M.SOLAIMAN Discipline of Chemistry University of Newcastle School of Materials Science and Engineering University of New South Wales Electron Microscopy Center AIIMUniversity of Wollongong Institute of Resources Ecosystem and Environment of AgricultureNanjing Agricultural University Marron Brook Farm Warren Catchments Council 52 Bath StManjimup 6258 (Australia) Mark Wainwright Analytical Centre University of New South Wales Wollongbar Primary Industries Institute NSW Department of Primary Industries Institute of Soil Water and Environmental SciencesThe Volcani CenterAgricultural Research Organization Centre for Marine Bio-Innovation School of Biotechnology and Biomolecular SciencesThe University of New South Wales Soil Biology and Molecular Ecology Group School of Earth and Environment (M087)The University of Western Australia

Addition of biochar produced through thermal decomposition of biomass has been seen as a strategy to improve soils and to sequester carbon(C), but wide scale implementation of the technology requires to devise innovative profitable solutions. To develop biochar utilisation with an integrated system approach, an innovative program was implemented in 2012 on a 53-ha farm in Western Australia to determine the costs and benefits of integrating biochar with animal husbandry and improvement of pastures. Biochar was mixed with molasses and fed directly to cows. The dung-biochar mixture was incorporated into the soil profile by dung beetles.We studied the changes in soil properties over 3 years. Biochar extracted from fresh dung and from the soil to a depth of 40 cm was characterised. A preliminary financial analysis of the costs and benefits of this integrated approach was also undertaken. The preliminary investigation results suggested that this strategy was effective in improving soil properties and increasing returns to the farmer. It was also concluded that the biochar adsorbed nutrients from the cow's gut and from the dung. Dung beetles could transport this nutrient-rich biochar into the soil profile. There was little evidence that the recalcitrant component of the biochar was reduced through reactions inside the gut or on/in the soil. Further research is required to quantify the long-term impact of integrating biochar and dung beetles into the rearing of cows.

关键词：土壤肥力生物炭农业生产率创新喂牛土壤性质新鲜粪便生物利用

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Biochar and its importance on nutrient dynamics in soil and plant

引用

Biochar 2020年第4期2卷 379-420页

作者： Md Zahangir Hossain Md Mezbaul Bahar Binoy Sarkar scott Wilfred donne Young Sik Ok Kumuduni Niroshika Palansooriya Mary Beth Kirkham Saikat Chowdhury Nanthi Bolan Global Centre for Environmental Remediation Faculty of ScienceThe University of NewcastleCallaghanNSW 2308Australia Cooperative Research Centre for High Performance Soils CallaghanNSW 2308Australia Agrotechnology Discipline Khulna UniversityKhulna 9208Bangladesh Lancaster Environment Centre Lancaster UniversityLancaster LA14YQUK Discipline of Chemistry The University of NewcastleCallaghanNSW 2308Australia O‑Jeong Eco‑Resilience Institute and Division of Environmental Science and Ecological Engineering Korea UniversitySeoul 02841Republic of Korea Department of Agronomy Kansas State UniversityManhattanKS 66506‑5501USA Department of Soil Science Sher-e-Bangla Agricultural UniversityDhaka 1207Bangladesh

Biochar,an environmentally friendly soil conditioner,is produced using several thermochemical processes.It has unique characteristics like high surface area,porosity,and surface charges.This paper reviews the fertilizer value of biochar,and its effects on soil properties,and nutrient use efficiency of crops.Biochar serves as an important source of plant nutrients,especially nitrogen in biochar produced from manures and wastes at low temperature(≤400℃).The phosphorus,potassium,and other nutrient contents are higher in manure/waste biochars than those in crop residues and woody biochars.The nutrient contents and pH of biochar are positively correlated with pyrolysis temperature,except for nitrogen content.Biochar improves the nutrient retention capacity of soil,which depends on porosity and surface charge of biochar.Biochar increases nitrogen retention in soil by reducing leaching and gaseous loss,and also increases phosphorus availability by decreasing the leaching process in soil.However,for potassium and other nutrients,biochar shows inconsistent(positive and negative)impacts on soil.After addition of biochar,porosity,aggregate stability,and amount of water held in soil increase and bulk density decreases.Mostly,biochar increases soil pH and,thus,influences nutrient availability for plants.Biochar also alters soil biological properties by increasing microbial populations,enzyme activity,soil respiration,and microbial biomass.Finally,nutrient use efficiency and nutrient uptake improve with the application of biochar to soil.Thus,biochar can be a potential nutrient reservoir for plants and a good amendment to improve soil properties.

关键词： Biochar Nutrients Manure Soil properties Nutrient use efficiency

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Restimate:Recovery Estimation Tool for Resilience Planning

引用

Journal of Safety Science and Resilience 2024年第1期5卷 47-63页

作者： scott Miles Megan Ly Nick Terry Youngjun Choe Department of Human Centered Design&Engineering Campus Box 352315University of WashingtonSeattleWA 98195United States of America Department of Industrial&Systems Engineering Box 352650University of WashingtonSeattleWA 98195United States of America

The U.S.National Institute of Standards and Technology(NIST)published the Community Resilience Planning Guide in 2016.The NIST Guide advocates for a participatory process for developing a performance measurement framework for the jurisdiction’s resilience against a scenario hazard.The framework centers around tables of expected and desired recovery times for selected community assets,such as electricity,water,and natural gas infrastructures.The NIST Guide does not provide a method for estimating the expected recovery times.However,building high-fidelity computer models for such estimations requires substantial resources that even larger ju-risdictions cannot cost-justify.The most promising approach to recovery time estimation is to systematically use data elicited from people to tap into the wisdom of the(knowledgeable)crowd.This paper describes a novel research-through-design project to enable the computer-supported elicitation of recovery time series data.This work is the first in the literature to examine people’s ability to estimate recovery curves and how design in-fluences such estimations.Its main contribution to resilience planning is three-fold:development of a new elicitation tool called Restimate,understanding its potential user base,and providing insights into how it can facilitate resilience planning.Restimate is the first tool to enable evidence-based expert elicitation in any community with limited resources for resilience planning.Beyond resilience planning,those who facilitate high-stakes planning activities under large uncertainties(e.g.,mission-critical system design and planning)will benefit from a similar research-through-design process.

关键词： expert elicitation disaster natural hazard infrastructure community resilience restoration user-centered design computer-supported cooperative work

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Status of biomarker development for frontotemporal dementia and amyotrophic lateral sclerosis

引用

Neural Regeneration Research 2024年第10期19卷 2117-2118页

作者： Yue Yang Qi Cheng Jianqun Gao Woojin scott Kim Brain and Mind Centre&School of Medical Sciences The University of SydneySydneyNSWAustralia Department of Neurology and Neurophysiology Liverpool HospitalSydneyNSWAustralia Stroke and Neurology Research Group Ingham Institute for Applied Medical ResearchSydneyNSWAustralia Shanghai Key Laboratory of Anesthesiology and Brain Functional Modulation ShanghaiChina Clinical Research Center for Anesthesiology and Perioperative Medicine ShanghaiChina Translational Research Institute of Brain and Brain-Like Intelligence Shanghai Fourth People’s HospitalSchool of MedicineTongji UniversityShanghaiChina

Frontotemporal dementia(FTD) and amyotrophic lateral sclerosis(ALS) are neurodegenerative diseases that belong to the same disease spectrum,with overlapping of genetic and pathological features.Genetic mutations in TA... 详细信息

关键词： amyotrophic sclerosis diseases

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Piezoelectric resonant ice protection systems-Part 2/2:Evaluation of benefits at aircraft level

引用

Chinese Journal of Aeronautics 2024年第6期37卷 50-63页

作者： Valerian PALANQUE Thomas PLANES Pommier-Budinger VALERIE Budinger MARC Delbecq scott Institut Clement Ader(ICA) INSAISAE-SUPAEROMINES ALBIUPSCNRSUniversity of Toulouse31400 ToulouseFrance Federation ENAC ISAE-SUPAERO ONERA University of Toulouse31400 ToulouseFrance

Piezoelectric resonant de-icing systems are attracting great interest.This paper aims to assess the implementation of these systems at the aircraft level.The article begins with the model to compute the power requirement of a piezoelectric resonant de-icing system sized from the prototype detailed in Part 1/2 of this article.Then the mass,drag,and fuel consumption of this system and the subcomponents needed for its implementation are assessed.The features of a piezoelectric resonant de-icing system are finally computed for aircraft similar to Airbus A320 aircraft and aircraft of different categories(Boeing 787,ATR 72 and TBM 900)and compared with the existing thermal and mechanical ice protection systems.A sensitivity analysis of the main key sizing parameters of the piezoelectric de-icing system is also performed to identify the main axes of improvement for this technology.The study shows the potential of such ice protection systems.In particular,for the realistic input parameters chosen in this work,the electro-mechanical solution can provide a 54% reduction in terms of mass and a 92% reduction in terms of power consumption for an A320 aircraft architecture,leading to a 74% decrease in the associated fuel consumption compared to the actual air bleed system.

关键词： Ice protection system De-icing Piezoelectric Electro-mechanical system Power Fuel consumption

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Stomatal dynamics are regulated by leaf hydraulic traits and guard cell anatomy in nine true mangrove species

引用

Plant Diversity 2024年第3期46卷 395-405页

作者： Ya-Dong Qie Qi-Wei Zhang scott A.M.McAdam Kun-Fang Cao State Key Laboratory for Conservation and Utilization of Subtropical Agro-Bioresources College of ForestryGuangxi UniversityNanning 530004China Guangxi Key Laboratory of Forest Ecology and Conservation College of ForestryGuangxi UniversityNanning 530004China Key Laboratory of Ecology of Rare and Endangered Species and Environmental Protection Ministry of EducationGuangxi Normal UniversityGuilin 541001China Guangxi Key Laboratory of Landscape Resources Conservation and Sustainable Utilization in Lijiang River Basin Guangxi Normal UniversityGuilin 541001China Purdue Center for Plant Biology Department of Botany and Plant PathologyPurdue UniversityWest LafayetteIN 47907USA

Stomatal regulation is critical for mangroves to survive in the hyper-saline intertidal zone where water stress is severe and water availability is highly fluctuant.However,very little is known about the stomatal sensitivity to vapour pressure deficit(VPD)in mangroves,and its co-ordination with stomatal morphology and leaf hydraulic traits.We measured the stomatal response to a step increase in VPD in situ,stomatal anatomy,leaf hydraulic vulnerability and pressure-volume traits in nine true mangrove species of five families and collected the data of genome size.We aimed to answer two questions:(1)Does stomatal morphology influence stomatal dynamics in response to a high VPD in mangroves?with a consideration of possible influence of genome size on stomatal morphology;and(2)do leaf hydraulic traits influence stomatal sensitivity to VPD in mangroves?We found that the stomata of mangrove plants were highly sensitive to a step rise in VPD and the stomatal responses were directly affected by stomatal anatomy and hydraulic traits.Smaller,denser stomata was correlated with faster stomatal closure at high VPD across the species of Rhizophoraceae,and stomata size negatively and vein density positively correlated with genome size.Less negative leaf osmotic pressure at the full turgor(πo)was related to higher operating steady-state stomatal conductance(gs);and a higher leaf capacitance(Cleaf)and more embolism resistant leaf xylem were associated with slower stomatal responses to an increase in VPD.In addition,stomatal responsiveness to VPD was indirectly affected by leaf morphological traits,which were affected by site salinity and consequently leaf water status.Our results demonstrate that mangroves display a unique relationship between genome size,stomatal size and vein packing,and that stomatal responsiveness to VPD is regulated by leaf hydraulic traits and stomatal morphology.Our work provides a quantitative framework to better understand of stomatal regulation in mangroves in an environment with high salinity and dynami

关键词： Stomatal temporal kinetics Vapour-pressure deficit(VPD) Leaf water relations Leaf hydraulic vulnerability Leaf osmotic potential Genome size

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Nondestructive and active interrogation system for special nuclear material:proof of principle and initial results

引用

Nuclear Science and Techniques 2024年第5期35卷 216-225页

作者： Mahmoud Bakr Kai Masuda Yoshiyuki Takahashi Tsuyoshi Misawa Norio Yamakawa Tomas scott Institute of Advanced Energy Kyoto UniversityGokashoUjiKyoto 611‑0011Japan School of Physics University of BristolBs81TL Tyndall AvenueBristolUK Physics Department Faculty of ScienceAssiut UniversityAssiut 71516Egypt Research Reactor Institute Kyoto University2 Asashiro‑NishiKumatoriOsaka 590‑0494Japan Pony Industry Co.Ltd. 2‑3‑6 Kitakyuhoji‑MachiChuo‑KuOsaka 541‑0057Japan Astral Neutronics LTD Unit H5HallenBristol BS107SBUK

Herein,we employ the threshold energy neutron analysis(TENA)technique to introduce the world's first active interrogation system to detect special nuclear materials(SNMs),including U-235 and Pu-239.The system utilizes a DD neutron generator based on inertial electrostatic confinement(IEC)to interrogate suspicious objects.To detect secondary neutrons produced during fission reactions induced in SNMs,a tensioned metastable fluid detector(TMFD)is employed.The current status of the system's development is reported in this paper,accompanied by the results from experiments conducted to detect 10 g of highly enriched uranium(HEU).Notably,the experimental findings demonstrate a distinct difference in the count rates of measurements with and without HEU.This difference in count rates surpasses two times the standard deviation,indicating a confidence level of more than 96% for identifying the presence of HEU.The paper presents and extensively discusses the proof-of-principle experimental results,along with the system's planned trajectory.

关键词： Special nuclear materials Uranium detection Inertial electrostatic confinement fusion TENA HEU CTMFD

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：