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Domain-engineered BiFeO3 thin-film photoanodes for highly enhanced ferroelectric solar water splitting

Nano Research 2018年第2期11卷 642-655页

作者： Jaesun Song Taemin Ludvic Kim Jongmin Lee sam yeon cho Jaeseong Cha Sang Yun Jeong Hyunji An Wan Sik Kim Yen-Sook Jung Jiyoon Park Gun Young Jung Dong-Yu Kim Ji Young Jo Sang Don Bu Ho Won Jang Sanghan Lee School of Materials Science and Engineering Gwangju Institute of Science and Technology (GIST) Gwangju Republic of Korea Department of Materials Science and Engineering Research Institute of Advanced Materials Seoul National University Seoul Republic of Korea Department of Physics chonbuk National University Jeonju Republic of Korea

In photoelectrochemical （PEC） water splitting, charge separation and collection by the electric field in the photoactive material are the most important factors for improved conversion efficiency. Hence, ferroelectric oxides, in which electrons are the majority carriers, are considered promising photoanode materials because their high built-in potential, provided by their spontaneous polarization, can signifi＇canfly enhance the separation and drift of photogenerated carriers. In this regard, the PEC properties of BiFeO3 thin-film photoanodes with different crystallographic orientations and consequent ferroelectric domain structures are investigated. As the crystallographic orientation changes from （001）pc via （ll0）pc to （lll）p~, the ferroelastic domains in epitaxial BiFeO3 thin films become mono-variant and the spontaneous polarization levels increase to 110 btC/cm2. Consequent136 the photocurrent density at 0 V vs. Ag/AgC1 increases approximately 5.3-fold and the onset potential decreases by 0.180 V in the downward polarization state. It is further demonstrated that ferroelectric switching in the （lll）pc BiFeO3 thin-film photoanode leads to an approximate change of 8,000% in the photocurrent density and a 0.330 V shift in the onset potential. This study strongly suggests that domain-engineered ferroelectric materials can be used as effective charge separation and collection layers for efficient solar water-splitting photoanodes.

关键词： BiFeO3 ferroelectric photoelectrochemical domain orientation pulsed laser deposition

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A dose-dependent bimodal switch by homologous Aux/IAA transcriptional repressors

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Molecular Plant 2024年第9期17卷 1407-1422页

作者： Hyung-Taeg cho Minsu Lee Hee-Seung choi Kwang-Ho Maeng Kyeonghoon Lee Ha-yeon Lee Anindya Ganguly Hoonyoung Park Chang-Hoi Ho Department of Biological Sciences Seoul National UniversitySeoulKorea School of Earth and Environmental Sciences Seoul National UniversitySeoulKorea Department of Climate and Energy Systems Engineering Ewha Womans UniversitySeoulKorea

Combinatorial interactions between different regulators diversify and enrich the chance of transcriptional regulation in eukaryotic ***,a dose-dependent functional switch of homologous transcriptional repressors has rarely been ***,we show that SHY2,an auxin/indole-3-acetic acid(Aux/IAA)repressor,exhibits a dose-dependent bimodal role in auxin-sensitive root-hair growth and gene transcrip-tion in Arabidopsis,whereas other Aux/lAA homologs consistently repress the auxin *** co-repressor(TOPLESS[TPL])-binding affinity of a bimodal Aux/IAA was lower than that of a consistently re-pressing Aux/*** switch of a single amino acid residue in the TPL-binding motif between the bimodal form and the consistently repressing form switched their TPL-binding affinity and transcriptional and bio-logical roles in auxin *** on these data,we propose a model whereby competition between homologous repressors with different co-repressor-binding affinities could generate a bimodal output at thetranscriptional anddevelopmental levels.

关键词： auxin Aux/IAA dose-dependent regulation root hair transcription TOPLESS(TPL)

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Optimal transcorneal electrical stimulation parameters for preserving photoreceptors in a mouse model of retinitis pigmentosa

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Neural Regeneration Research 2024年第11期19卷 2543-2552页

作者： sam Enayati Karen Chang Anton Lennikov Menglu Yang Cherin Lee Ajay Ashok Farris Elzaridi Christina Yen Kasim Gunes Jia Xie Kin-Sang cho Tor Paaske Utheim Dong Feng Chen Schepens Eye Research Institute of Massachusetts Eye and Ear Department of OphthalmologyHarvard Medical SchoolBostonMAUSA Institute of clinical medicine Faculty of MedicineUniversity of OsloOsloNorway Department of Medical Biochemistry Oslo University HospitalUniversity of OsloOsloNorway Department of Ophthalmology Drammen HospitalVestre Viken Hospital TrustDrammenNorway Department of Histology and Embryology School of MedicineMarmara UniversityIstanbulTurkiye

Retinitis pigmentosa is a hereditary retinal disease that affects rod and cone photoreceptors,leading to progressive photoreceptor *** research supports the beneficial effect of electrical stimulation on photoreceptor *** study aims to identify the most effective electrical stimulation parameters and functional advantages of transcorneal electrical stimulation(tcES)in mice affected by inherited retinal ***,the study seeked to analyze the electric field that reaches the retina in both eyes in mice and post-mortem *** this study,we recorded waveforms and voltages directed to the retina during transcorneal electrical stimulation in C57BL/6J mice using an intraocular needle probe with rectangular,sine,and ramp *** investigate the functional effects of electrical stimulation on photoreceptors,we used human retinal explant cultures and rhodopsin knockout(Rho^(-/-))mice,demonstrating progressive photoreceptor degeneration with *** retinal explants isolated from the donors’eyes were then subjected to electrical stimulation and cultured for 48 hours to simulate the neurodegenerative environment in *** density was evaluated by rhodopsin *** vivo Rho^(-/-)mice were subjected to two 5-day series of daily transcorneal electrical stimulation using rectangular and ramp *** function and visual perception of mice were evaluated by electroretinography and optomotor response(OMR),*** was used to assess the morphological and biochemical changes of the photoreceptor and bipolar cells in mouse *** recordings indicated effective delivery of rectangular,sine,and ramp waveforms to the retina by transcorneal electrical stimulation,of which the ramp waveform required the lowest *** of the total conductive resistance of the post-mortem human compared to the mouse eyes indicated higher cornea-to-retina resistance in human *** tem

关键词： bipolar cells electrical stimulation neuroprotection photoreceptor degeneration retina retinal explants retinitis pigmentosa transcorneal electrical stimulation waveform

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Switchable p-n-p conduction and thermoelectric properties of selenium-doped tellurium crystal

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Rare Metals 2024年第11期 5975-5984页

作者： Stanley Abbey Hanhwi Jang Brakowaa Frimpong Van Quang Nguyen Sunglae cho yeon Sik Jung Min-Wook Oh Department of Materials Science and Engineering Hanbat National University Department of Materials Science and Engineering Korea Advance Institute of Science and Technology Department of Phy sics and Energy Harvest-Storage Research Center University of Ulsan

Switchable conductivity in elementary semiconducting materials has a high potential for the design of diodes,transistors and energy conversion ***,the ability to utilize their physical properties is dependent on doping within the carrier density transition ***-crystal tellurium has a high Seebeck coefficient and intrinsic p-n-p conduction at room temperature and therefore,is not suitable for thermoelectric *** demonstrate that the addition of iso valent Se lowers the Fermi level to achieve a stable p-type conductivity with a high band degeneracy near the valence *** observed shifts in the n-p transition temperature below the intrinsic conductivity at 470 K based on changes in stoichiometry and carrier concentration above *** addition,the high thermal conductivity is significantly reduced with the increase in Se alloying due to the mass and strain *** results in a moderately high zT of 0.4 at 673 K.

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Crystal reconstruction of V2O3/carbon heterointerfaces via anodic hydration for ultrafast and reversible Mg-ion battery cathodes

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InfoMat 2024年第3期6卷 95-107页

作者： Gun Jang Yun Sang Joe Sang Joon Lee Hyun Gyu cho Sang Ha Baek Peixun Xiong Kang Ho Shin Jeong Seok yeon Min Su Kang Si Hyoung Oh Ho Seok Park School of Chemical Engineering Sungkyunkwan University(SKKU)SuwonRepublic of Korea Advanced Batteries Research Center Korea Electronics Technology InstituteSeongnamRepublic of Korea Korea Institute of Science and Technology SeoulRepublic of Korea SKKU Advanced Institute of Nano Technology(SAINT) Sungkyunkwan UniversitySuwonRepublic of Korea Department of Health Sciences and Technology Samsung Advanced Institute for Health Sciences and Technology(SAIHST)Sungkyunkwan UniversitySuwonRepublic of Korea SKKU Institute of Energy Science and Technology(SIEST) Sungkyunkwan UniversitySuwonRepublic of Korea

Magnesium-ion batteries(MIBs)have promising applications because of their high theoretical capacity and the natural abundance of magnesium ***,the kinetic performance and cyclic stability of cathode materials are limited by the strong interactions between Mg ions and the crystal ***,we demonstrate the unique Mg^(2+)-ion storage mechanism of a hierarchical accordion-like vanadium oxide/carbon heterointerface(V2O3@C),where the V2O3 crystalline structure is reconstructed into a MgV_(3)O_(7)·H_(2)O phase through an anodic hydration reaction upon first cycle,for the improved kinetic and cyclic *** verified by in situ/ex situ spectroscopic and electrochemical analyses,the fast charge transfer kinetics of the V2O3@C cathode were due to the crystal-reconstruction and chemically coupled *** V2O3@C demonstrated an ultrahigh rate capacity of 130.4 mAh g^(-1)at 50000 mA g^(-1)and 1000 cycles,achieving a Coulombic efficiency of 99.6%.The high capacity of 381.0 mA h g^(-1)can be attributed to the reversible Mg^(2+)-ion intercalation mechanism observed in the MgV_(3)O_(7)·H_(2)O phase using a 0.3 M Mg(TFSI)2/ACN(H_(2)O)***,within the voltage range of 2.25 V versus Mg/Mg^(2+),the V2O3@C exhibited a capacity of 245.1 mAh g^(-1)when evaluated with magnesium metal in a 0.3 M Mg(TFSI)^(2+)0.25 M MgCl_(2)/DME *** research findings have important implications for understanding the relationship between the Mg-ion storage mechanism and reconstructed crystal phase of vanadium oxides as well as the heterointerface reconstruction for the rational design of MIB cathode materials.

关键词： anodic hydration reaction magnesium ion battery nano crystal vanadium oxide

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Crystallographically vacancy‐induced MOF nanosheet as rational single‐atom support for accelerating CO_(2)electroreduction to CO

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Carbon Energy 2024年第8期6卷 49-62页

作者： Jin Hyuk cho Joonhee Ma Chaehyeon Lee Jin Wook Lim Youngho Kim Ho yeon Jang Jaehyun Kim Myung‐gi Seo Youngheon choi Youn Jeong Jang Sang Hyun Ahn Ho Won Jang Seoin Back Jong‐Lam Lee Soo Young Kim Department of Materials Science and Engineering Korea UniversitySeoulRepublic of Korea Department of Chemical and Biomolecular Engineering Sogang UniversitySeoulRepublic of Korea Department of Materials Science and Engineering Pohang University of Science and Technology(POSTECH)PohangRepublic of Korea Department of Materials Science and Engineering Research Institute of Advanced MaterialsSeoul National UniversitySeoulRepublic of Korea Lotte Chemical R&D Center DaejeonRepublic of Korea Department of Chemical Engineering Hanyang UniversitySeoulRepublic of Korea School of Chemical Engineering and Material Science Chung‐Ang UniversitySeoulRepublic of Korea

To attain a circular carbon economy and resolve CO_(2)electroreduction technology obstacles,single‐atom catalysts(SACs)have emerged as a logical option for electrocatalysis because of their extraordinary catalytic *** SACs,metal–organic frameworks(MOFs)have been recognized as promising support materials because of their exceptional ability to prevent metal *** study shows that atomically dispersed Ni single atoms on a precisely engineered MOF nanosheet display a high Faradaic efficiency of approximately 100%for CO formation in H‐cell and three‐compartment microfluidic flow‐cell reactors and an excellent turnover frequency of 23,699 h−1,validating their intrinsic catalytic *** results suggest that crystallographic variations affect the abundant vacancy sites on the MOF nanosheets,which are linked to the evaporation of Zn‐containing organic linkers during ***,using X‐ray absorption spectroscopy and density functional theory calculations,a comprehensive investigation of the unsaturated atomic coordination environments and the underlying mechanism involving CO^(*)preadsorbed sites as initial states was possible and provided valuable insights.

关键词： 2‐dimensional material carbon dioxide reduction metal-organic frameworks single‐atom catalysts vacancy sites

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Effects of heavy rainfall on the composition of airborne bacterial communities

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Frontiers of Environmental Science & Engineering 2018年第2期12卷 117-126页

作者： Gwang Il Jang Chung yeon Hwang Byung Cheol cho Microbial Oceanography Laboratory School of Earth and Environmental Sciences and Research Institute of Oceanography Seoul National University Seoul 08826 Republic of Korea Division of Polar Life Sciences Korea Polar Research Institute Incheon 21990 Republic of Korea

Wet deposition scavenges particles and particle-associated bacteria from the air column, but the impact of raindrops on various surfaces on Earth causes emission of surface-associated bacteria into the air column. Thus, after rainfall, these two mechanisms are expected to cause changes in airborne bacterial community composition （BCC）. In this study, aerosol samples were collected at a suburban site in Seoul, Korea before and after three heavy rainfall events in April, May, and July 2011. BCC was investigated by pyrosequencing the 16S rRNA gene in aerosol samples. Interestingly, the relative abundance of non-spore forming Actinobacteria operational taxonomic units （OTUs） was always higher in post-rain aerosol samples. In particular, the absolute and relative abundances of airborne Propionibacteriaceae always increased after rainfall, whereas those of airborne Firmicutes, including Carnobacteriaceae and Clostridiales, consistently decreased. Marine bacterial sequences, which were temporally important in aerosol samples, also decreased after rainfall events. Further, increases in pathogen-like sequences were often observed in post-rain air samples. Rainfall events seemed to affect airborne BCCs by the combined action of the two mechanisms, with potentially adverse effects on human and plant health.

关键词： Aerosol BacteriaCommunity composition PyrosequencingRain

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Septic shock due to Granulicatella adiacens after endoscopic ultrasound-guided biopsy of a splenic mass:A case report

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World Journal of Gastroenterology 2021年第8期27卷 751-759页

作者： Seo-yeon cho Eunae cho Chang-Hwan Park Hee-Joon Kim Joo-yeon Koo Division of Gastroenterology Department of Internal MedicineChonnam National University HospitalGwangju 61469South Korea Department of Surgery Chonnam National University HospitalGwangju 61469South Korea Department of Pathology Chonnam National University HospitalGwangju 61469South Korea

BACKGROUND Endoscopic ultrasound-guided fine needle aspiration or biopsy(EUS-FNA or FNB)has become a popular method for diagnosing various lesions of the gastrointestinal tract and surrounding tissue due to the accuracy and *** the best of our knowledge,no case report of severe infection after EUS-FNB of a solid lesion in the spleen has been ***,we report a rare case of septic shock after EUS-FNB of a splenic *** SUMMARY A 45-year-old male patient presented to the outpatient clinic due to an incidentally detected splenic mass.A definitive diagnosis could not be established based on the abdominal magnetic resonance *** of the spleen showed a 6 cm-sized,relatively well-demarcated,heterogeneous mass,and EUS-FNB with a 22G needle was *** days after the procedure patient developed septic shock and a splenic abscess was *** culture revealed growth of Granulicatella *** the treatment with antibiotics the patient underwent surgical resection,and the pathological examination showed diffuse large B-cell *** patient received chemotherapy and he is in complete *** Infection of a splenic mass after EUS-FNB is a rare complication and prophylactic antibiotics might be considered.

关键词： Endoscopic ultrasound Endoscopic ultrasound-guided fine needle biopsy Splenic neoplasms Lymphoma Septic shock Case report

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Global parameter estimation of the Cochlodinium polykrikoides model using bioassay data

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Acta Oceanologica Sinica 2016年第2期35卷 39-45页

作者： cho Hong-yeon PARK Kwang-Soon KIM Sung Coastal and Environmental Engineering Division Korea Institute of Ocean Science and Technology Coastal Disaster Research Center Korea Institute of Ocean Science and Technology Biological Oceanography and Marine Biology Division Korea Institute of Ocean Science and Technology

Cochlodinium polykrikoides is a notoriously harmful algal species that inflicts severe damage on the aquacultures of the coastal seas of Korea and Japan. Information on their expected movement tracks and boundaries of influence is very useful and important for the effective establishment of a reduction plan. In general, the information is supported by a red-tide（a.k.a algal bloom） model. The performance of the model is highly dependent on the accuracy of parameters, which are the coefficients of functions approximating the biological growth and loss patterns of the C. polykrikoides. These parameters have been estimated using the bioassay data composed of growth-limiting factor and net growth rate value pairs. In the case of the C. polykrikoides, the parameters are different from each other in accordance with the used data because the bioassay data are sufficient compared to the other algal species. The parameters estimated by one specific dataset can be viewed as locally-optimized because they are adjusted only by that dataset. In cases where the other one data set is used, the estimation error might be considerable. In this study, the parameters are estimated by all available data sets without the use of only one specific data set and thus can be considered globally optimized. The cost function for the optimization is defined as the integrated mean squared estimation error, i.e., the difference between the values of the experimental and estimated rates. Based on quantitative error analysis, the root-mean squared errors of the global parameters show smaller values, approximately 25%–50%, than the values of the local parameters. In addition, bias is removed completely in the case of the globally estimated parameters. The parameter sets can be used as the reference default values of a red-tide model because they are optimal and representative. However, additional tuning of the parameters using the in-situ monitoring data is highly *** opposed to the bioassay d

关键词： global and local estimation gain and loss parameters Cochlodinium polykrikoides bioassay data model performance

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Quantum logic operations on two distant atoms trapped in two optical-fibre-connected cavities

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Chinese Physics B 2011年第12期20卷 88-94页

作者：张英俏张寿 yeon Kyu-Hwang Yu Seong-cho Department of Physics College of ScienceYanbian University BK21 Physics Program and Department of Physics College of Natural SciencesChungbuk National UniversityCheongjuChungbuk361-763Republic of Korea

Based on the coupling of two distant three-level atoms in two separate optical cavities connected with two optical fibres, schemes on the generation of several two-qubit logic gates are discussed under the conditions of △ = δ- 2v cos πk/2 〉〉 g/2 and v-g. Discussion and analysis of the fidelity, gate time and experimental setups show that our schemes are feasible with current optical cavity, atomic trap and optical fibre techniques. Moreover, the atom-cavityfibre coupling can be used to generate an N-qubit nonlocal entanglement and transfer quantum information among N distant atoms by arranging N atom cavity assemblages in a line and connecting each two adjacent cavities with two optical fibres.

关键词： quantum logic gate cavity QED optical fibre

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