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Journal of Energy Chemistry 2025年第1期100卷 760-769页

作者： Lin Peng Yu Bai Hang Li Meixiu Qu Zhenhua Wang Kening sun Advanced Research Institute of Multidisciplinary Science Beijing Institute of Technology Beijing Key Laboratory of Chemical Power Source and Green Catalysis School of Chemistry and Chemical Engineering Beijing Institute of Technology

Lithium-sulfur （Li-S） batteries have gained great attention due to the high theoretical energy density and low cost,yet their further commercialization has been obstructed by the notorious shuttle effect and sluggish redox ***,we supply a strategy to optimize the electron structure of Ni2P by concurrently introducing B-doped atoms and P vacancies in Ni2P （Vp-B-Ni2P）,thereby enhancing the bidirectional sulfur *** study indicates that the simultaneous introduction of B-doped atoms and P vacancies in Ni2P causes the redistribution of electron around Ni atoms,bringing about the upward shift of d-band center of Ni atoms and effective d-p orbital hybridization between Ni atoms and sulfur species,thus strengthening the chemical anchoring for lithium polysulfides （LiPSs） as well as expediting the bidirectional conversion kinetics of sulfur ***,theoretical calculations reveal that the incorporation of B-doped atoms and P vacancies in Ni2P selectively promotes Li2S dissolution and nucleation ***,the Li-S batteries with Vp-B-Ni2P-separators present outstanding rate ability of 777 m A h g-1at 5 C and high areal capacity of 8.03 mA h cm-2under E/S of 5μL mg-1and sulfur loading of 7.20 mg *** work elucidates that introducing heteroatom and vacancy in metal phosphide collaboratively regulates the electron structure to accelerate bidirectional sulfur conversion.

关键词： Lithium sulfur batteries

Occluded Gait Emotion Recognition Based on Multi-Scale Suppression Graph Convolutional Network

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Computers, Materials & Continua 2025年第1期82卷 1255-1276页

作者： Yuxiang Zou Ning He Jiwu sun Xunrui Huang Wenhua Wang Beijing Key Laboratory of Information Service Engineering Beijing Union UniversityBeijing100101China College of Smart City Beijing Union UniversityBeijing100101China

In recent years,gait-based emotion recognition has been widely applied in the field of computer ***,existing gait emotion recognition methods typically rely on complete human skeleton data,and their accuracy significantly declines when the data is *** enhance the accuracy of gait emotion recognition under occlusion,this paper proposes a Multi-scale Suppression Graph ConvolutionalNetwork(MS-GCN).TheMS-GCN consists of three main components:Joint Interpolation Module(JI Moudle),Multi-scale Temporal Convolution Network(MS-TCN),and Suppression Graph Convolutional Network(SGCN).The JI Module completes the spatially occluded skeletal joints using the(K-Nearest Neighbors)KNN interpolation *** MS-TCN employs convolutional kernels of various sizes to comprehensively capture the emotional information embedded in the gait,compensating for the temporal occlusion of gait *** SGCN extracts more non-prominent human gait features by suppressing the extraction of key body part features,thereby reducing the negative impact of occlusion on emotion recognition *** proposed method is evaluated on two comprehensive datasets:Emotion-Gait,containing 4227 real gaits from sources like BML,ICT-Pollick,and ELMD,and 1000 synthetic gaits generated using STEP-Gen technology,and ELMB,consisting of 3924 gaits,with 1835 labeled with emotions such as“Happy,”“Sad,”“Angry,”and“Neutral.”On the standard datasets Emotion-Gait and ELMB,the proposed method achieved accuracies of 0.900 and 0.896,respectively,attaining performance comparable to other ***,on occlusion datasets,the proposedmethod significantly mitigates the performance degradation caused by occlusion compared to other methods,the accuracy is significantly higher than that of other methods.

关键词： KNN interpolation multi-scale temporal convolution suppression graph convolutional network gait emotion recognition human skeleton

Equivalent Conditions of Dominated Splitting for Volume-Preserving Diffeomorphisms

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Acta Mathematica Sinica,English Series 2007年第9期23卷 1563-1576页

作者： Chao liang Geng LIU Wen xiang sun Applied Mathematical Department The Central University of Finance and Economics ~ School of Mathematical Sciences Peking University Beijing 100871 P. R. China School of Mathematical Sciences Peking University Beijing 100871 P. R. China LMAM School of Mathematical Sciences Peking University Beijing 100871 P. R. China

We discuss the equivalent conditions of dominated splitting for conservative diffeomorphisms in C^1 topology.

关键词： Homoclinic tangency preperiodic point dominated splitting volume-preserving diffeo- morphism

Improvement in the weldability of molybdenum alloy by pre-welding solid carburising

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Journal of Materials Science & Technology 2021年第21期80卷 1-12页

作者： liang-liang Zhang Lin-Jie Zhang Jian Long xiang-Dong Ding Jun sun Yuan-Jun sun State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an710049China

Molybdenum(Mo), with its high chemical stability and resistance to neutron irradiation, has wide application prospects in the nuclear industry;however, the embrittlement of welded Mo joints limits its further application. In this study, the brittleness of the welded joints of Mo alloy was reduced and their strength was enhanced by adding carbon to the fusion zone(FZ) during laser welding. In the FZ of the Mo joints, carbon mainly existed as Mo_(2)C, and some free C atoms, and MoC and MoOxC yphases were also present. The distribution of Mo_(2)C directly influenced the bonding strength of the grain *** Mo_(2)C was dispersedly distributed as particles or discontinuous lines at the grain boundaries of Mo,it improved the resistance of the grain boundaries to the propagation of cracks and thereby increasing their strength. However, the Mo_(2)C phases distributed in a reticular pattern at the grain boundaries of Mo provided channels that enabled cracks to rapidly propagate, thereby reducing the resistance of the grain boundaries to crack propagation and weakening their strength. The emergence of the MoOxC yphase reduced the weakening effect of free oxygen atoms on the strength of grain boundaries of Mo.

关键词： Molybdenum Carbon Mo_(2)C Laser beam welding Pre-welding solid carburising

Deep eutectic solvents for separation and purification applications in critical metal metallurgy:Recent advances and perspectives

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International Journal of Minerals,Metallurgy and Materials 2025年第1期32卷 1-19页

作者： Shuo Chen Shengpeng Su Yanfang Huang Bingbing Liu Hu sun Shuzhen Yang Guihong Han School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China Zhongyuan Critical Metals Laboratory Henan ProvinceZhengzhou 450001China

Solvent extraction,a separation and purification technology,is crucial in critical metal *** solvents commonly used in solvent extraction exhibit disadvantages,such as high volatility,high toxicity,and flammability,causing a spectrum of hazards to human health and environmental *** solvents have been recognized as potential alternatives to these harmful organic *** the past two decades,several neoteric solvents have been proposed,including ionic liquids(ILs)and deep eutectic solvents(DESs).DESs have gradually become the focus of green solvents owing to several advantages,namely,low toxicity,degradability,and low *** this critical review,their classification,formation mechanisms,preparation methods,characterization technologies,and special physicochemical properties based on the most recent advancements in research have been systematically ***,the major separation and purification applications of DESs in critical metal metallurgy were comprehensively ***,future opportunities and challenges of DESs were explored in the current research *** conclusion,this review provides valuable insights for improving our overall understanding of DESs,and it holds important potential for expanding separation and purification applications in critical metal metallurgy.

关键词： deep eutectic solvents preparations properties separation and purification critical metal metallurgy

Longitudinal profiled plate straightening process based on curvature integral method

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Journal of Iron and Steel Research International 2021年第3期28卷 291-302页

作者： Jian-liang sun Kai Li Meng-qian sun xiang-hui Lu Yan Peng National Engineering Research Center for Equipment and Technology of Cold Strip Rolling Yanshan UniversityQinhuangdao066004HebeiChina Department of Mechatronics Engineering Hebei Construction Material Vocational and Technical CollegeQinhuangdao066004HebeiChina

Considering the variable cross section thickness of longitudinal profiled plate and the dynamic reductions of straightening rolls,an analytical model combining curvature integral method with linear decreasing straightening scheme was proposed to investigate the longitudinal profiled plate straightening ***,the calculation flow and solution algorithm of longitudinal profiled plate straightening process were *** verify the proposed model,calculated straightening forces were compared with the measured values,and very good agreements were ***,the reduction,contact angle,reverse bending curvature,residual curvature,straightening force and straightening moment of longitudinal profiled plate in the straightening process were calculated and analyzed,and the calculated results show that the curvature integral method can be used to reveal the mechanism of longitudinal profiled plate straightening.

关键词： Longitudinal profiled plate straightening Curvature integral method Linear decreasing straightening scheme Residual curvature

Coordinating Pricing and Inventory Control in a Fluctuating Environment

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Acta Mathematicae Applicatae Sinica 2010年第2期26卷 187-204页

作者： Ju-liang Zhang Jian Chen xiang-sun Zhang Department of Logistics Management School of Economics and Management Beijing Jiaotong UniversityBeijing 100044 China Department of Management Science and Engineering School of Economics and Management Tsinghua Uni-versity Beijing 100084 China Institute of Applied Mathematics Academy of Mathematics and Systems Science Chinese Academy of Sci-ences Beijing 100190 China

This paper addresses the simultaneous determination of pricing and inventory replenishment strate- gies under a fluctuating environment. Specifically, we analyze the single item, periodic review model. The demand consists of two parts： the deterministic component, which is influenced by the price, and the stochastic component （perturbation）. The distribution of the stochastic component is determined by the current state of an exogenous Markov chain. The price that is charged in any given period can be specified dynamically. A replenishment order may be placed at the beginning of some or all of the periods, and stockouts are fully backlogged. Ordering costs that are lower semicontinuous, and inventory/backlog （or surplus） costs that are continuous with polynomial growth. Finite-horizon and infinite-horizon problems are addressed. Existence of optimal policies is established. Furthermore, optimality of （s,S,p）-type policies is proved when the ordering cost consists of fixed and proportional cost components and the surplus cost （these costs are all state-dependent） is convex.

关键词： Stochastic inventory management Markov chains pricing finite horizon infinite horizon

Mutual regulation of microglia and astrocytes after Gas6 inhibits spinal cord injury

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Neural Regeneration Research 2025年第2期20卷 557-573页

作者： Jiewen Chen Xiaolin Zeng Le Wang Wenwu Zhang Gang Li Xing Cheng Peiqiang Su Yong Wan xiang Li Department of Spine Surgery The First Affiliated HospitalSun Yat-sen UniversityGuangzhouGuangdong ProvinceChina Guangdong Province Key Laboratory of Orthopedics and Traumatology GuangzhouGuangdong ProvinceChina

Invasive inflammation and excessive scar formation are the main reasons for the difficulty in repairing nervous tissue after spinal cord *** and astrocytes play key roles in the spinal cord injury micro-environment and share a close ***,the mechanisms involved remain *** this study,we found that after spinal cord injury,resting microglia(M0)were polarized into pro-inflammatory phenotypes(MG1 and MG3),while resting astrocytes were polarized into reactive and scar-forming *** expression of growth arrest-specific 6(Gas6)and its receptor Axl were significantly down-regulated in microglia and astrocytes after spinal cord *** vitro experiments showed that Gas6 had negative effects on the polarization of reactive astrocytes and pro-inflammatory microglia,and even inhibited the cross-regulation between *** further demonstrated that Gas6 can inhibit the polarization of reactive astrocytes by suppressing the activation of the Yes-associated protein signaling ***,in turn,inhibited the polarization of pro-inflammatory microglia by suppressing the activation of the nuclear factor-κB/p65 and Janus kinase/signal transducer and activator of transcription signaling *** vivo experiments showed that Gas6 inhibited the polarization of pro-inflammatory microglia and reactive astrocytes in the injured spinal cord,thereby promoting tissue repair and motor function ***,Gas6 may play a role in the treatment of spinal cord *** can inhibit the inflammatory pathway of microglia and polarization of astrocytes,attenuate the interaction between microglia and astrocytes in the inflammatory microenvironment,and thereby alleviate local inflammation and reduce scar formation in the spinal cord.

关键词： astrocytes Axl cell polarization Gas6 Hippo signal inflammatory micro-environment intercellular interaction microglia single-cell sequencing spinal cord injury

Microspheres trigged-stress concentration regulating piezoelectric properties of PVDF/elastomer composites

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Science China Chemistry 2025年

作者： Wenxian Zhang Jiahong Yang Qijun sun Lu Peng Tong Lin Shouke Yan Xiaoli sun State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology Beijing Institute of Nanoenergy and Nanosystems Chinese Academy of Sciences State Key Laboratory of Separation Membranes and Membrane Processes School of Textile Science and EngineeringTiangong University Key Laboratory of Rubber-Plastics of Ministry of Education Shandong Provincial Key Laboratory of Rubber-PlasticsQingdao University of Science & Technology

Wearable self-powered piezoelectric pressure sensors are attracting tremendous ***,fabricating a high-sensitive elastic piezoelectric sensor for a broad response range remains ***,we assemble polar poly（vinylidene fluoride）(PVDF) microsphere-elastomer composites,achieving high-sensitive and wide-responsive pressure *** polar PVDF microspheres are produced cost-effectively through phase separation,enabling *** piezoelectric composite （PC） film demonstrates low Young’s modulus,and excellent anti-fatigue ***,the PC-based piezoelectric sensor exhibits a rather high sensitivity of 540 mV N-1in a wide sensing range （5–40 N）,240 times greater than the PVDF film-based sensor and comparable to the inorganic piezoelectric *** excellent performance is attributed to the highest average stress concentration on the spherical PVDF coupled with the remarkable deformation of dipoles of spherical PVDF in the flexible *** on excellent performance,this piezoelectric sensor achieves precise recognition of motions and sound *** high-sensitive flexible piezoelectric sensor enabling large area production with ultralow price exerts great potential in smart monitoring and intelligent robots.

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Fluorinated poly(p-triphenylene isatin) anion exchange membranes based on hydrophilic hydroxyl side chain modulation for fuel cells

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Journal of Energy Chemistry 2025年第1期100卷 702-709页

作者： Yiman Gu Yanchao Zhang Zhanyu Li Yijia Lei Baozeng sun Xiaoyu Yu Zhe Wang College of Chemistry and Life Science Changchun University of Technology College of Chemical Engineering Changchun University of Technology School of Materials Science and Engineering Changchun University of Technology Key Laboratory of Advanced Functional Polymer Membrane Materials of Jilin Province

The development of alkaline fuel cells is moving forward at an accelerated pace,and the application of ether-free bonded polymers to anion exchange membranes （AEMs） has been widely ***,the question of the“trade-off”between AEM ionic conductivity and dimensional stability remains *** strategy of inducing microphase separation to improve the performance of AEM has attracted much attention recently,but the design of optimal molecular structures is still being ***,this work introduced different ratios of 3-bromo-1,1,1-trifluoroacetone （x=40,50,and 60） into the main chain of poly（p-terphenylene isatin）.Because fluorinated groups have excellent hydrophobicity,hydrophilic hydroxyl-containing side chains are introduced to jointly adjust the formation of phase separation *** results show that PTI-PTF50-NOH AEM with the appropriate fluorinated group ratio has the best ionic conductivity and alkali stability under the combined effect of *** has an ionic conductivity of 133.83 mS cm-1at 80°*** addition,the OH-conductivity remains at 89%of the initial value at 80°C and 3 M KOH for 1056 h of *** cell polarization curve based on PTI-PTF50-NOH shows a power density of 734.76 mW cm-2at a current density of 1807.7 mA cm-2.

关键词： Potassium hydroxide