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Enhanced gas production and CO_(2) storage in hydrate-bearing sediments via pre-depressurization and rapid CO_(2) injection

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Chinese Journal of Chemical Engineering 2024年第3期67卷 126-134页

作者： Hongnan Chen yifei sun Bojian Cao Minglong Wang Ming Wang Jinrong Zhong Changyu sun Guangjin Chen State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing 102249China School of Chemistry and Chemical Engineering Changsha University of Science&TechnologyChangsha 410114China

Carbon emission reduction and clean energy development are urgent demands for mankind in the coming *** an efficient CO_(2) storage method can significantly reduce CO_(2) emissions in the short *** this study,we attempted to construct sediment samples with different residual CH_(4) hydrate amounts and reservoir conditions,and then investigate the potentials of both CO_(2) storage and enhanced CH_(4) recovery in depleted gas hydrate deposits in the permafrost and ocean zones,*** results demonstrate that CO_(2) hydrate formation rate can be significantly improved due to the presence of residual hydrate seeds;However,excessive residual hydrates in turn lead to the decrease in CO_(2) storage *** by the T-P conditions of the reservoir,the storage amount of liquid CO_(2) can reach 8 times that of gaseous CO_(2),and CO_(2) stored in hydrate form reaches 2-4 ***,we noticed two other advantages of this *** is that CO_(2) injection can enhance CH_(4) recovery rate and increases CH_(4) recovery by 10%-20%.The second is that hydrate saturation in the reservoir can be restored to 20%-40%,which means that the solid volume of the reservoir avoids serious ***,this is crucial for protecting the goaf *** summary,this approach is greatly promising for high-efficient CO_(2) storage and safe exploitation of gas hydrate.

关键词： Hydrate Depressurization CO_(2) storage CH_(4) production Reservoir remediation

Rate-limiting factors in hydrate decomposition through depressurization across various scales:A mini-review

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Chinese Journal of Chemical Engineering 2024年第3期67卷 206-219页

作者： Xian sun Peng Xiao Qinfeng Shi Lingban Wang Zhenbin Xu Yuhao Bu Xiaohui Wang yifei sun Changyu sun Guangjin Chen State Key Laboratory of Heavy Oil Processing China University of Petroleum(Beijing)Beijing 102249China Jining University Jining 273115China

Natural gas hydrate is an energy resource for methane that has a carbon quantity twice more than all traditional fossil fuels ***,their practical application in the field has been limited due to the challenges of long-term preparation,high costs and associated *** studies,on the other hand,offer a safe and cost-effective means of exploring the mechanisms of hydrate dissociation and optimizing exploitation *** hydrate decomposition is a complicated process along with intrinsic kinetics,mass transfer and heat transfer,which are the influencing factors for hydrate decomposition *** identification of the rate-limiting factor for hydrate dissociation during depressurization varies with the scale of the reservoir,making it challenging to extrapolate findings from laboratory experiments to the actual *** review aims to summarize current knowledge of investigations on hydrate decomposition on the subject of the research scale(core scale,middle scale,large scale and field tests)and to analyze determining factors for decomposition rate,considering the various research scales and their associated influencing factors.

关键词： Gas hydrate Rate-limiting factors Research scale Depressurization Decomposition

Transplantation of human placental chorionic plate-derived mesenchymal stem cells for repair of neurological damage in neonatal hypoxic-ischemic encephalopathy

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Neural Regeneration Research 2024年第9期19卷 2027-2035页

作者： Lulu Xue Ruolan Du Ning Bi Qiuxia Xiao yifei sun Ruize Niu Yaxin Tan Li Chen Jia Liu Tinghua Wang Liulin Xiong Transformation Research Laboratory The Affiliated Hospital of Zunyi Medical UniversityZunyiGuizhou ProvinceChina State Key Laboratory of Biotherapy Sichuan UniversityChengduSichuan ProvinceChina Institute of Neurological Disease Translational Neuroscience CenterWest China HospitalSichuan UniversityChengduSichuan ProvinceChina Department of Animal Zoology Institute of NeuroscienceKunming Medical UniversityKunmingYunnan ProvinceChina Department of Anesthesiology The Affiliated Hospital of Zunyi Medical UniversityZunyiGuizhou ProvinceChina Department of Pediatrics the People’s Liberation Army Rocket Force Characteristic Medical CenterBeijingChina

Neonatal hypoxic-ischemic encephalopathy is often associated with permanent cerebral palsy,neurosensory impairments,and cognitive deficits,and there is no effective treatment for complications related to hypoxic-ischemic *** therapeutic potential of human placental chorionic plate-derived mesenchymal stem cells for various diseases has been ***,the potential use of human placental chorionic plate-derived mesenchymal stem cells for the treatment of neonatal hypoxic-ischemic encephalopathy has not yet been *** this study,we injected human placental chorionic plate-derived mesenchymal stem cells into the lateral ventricle of a neonatal hypoxic-ischemic encephalopathy rat model and observed significant improvements in both cognitive and motor *** chip analysis showed that interleukin-3 expression was significantly elevated in neonatal hypoxic-ischemic encephalopathy model *** transplantation of human placental chorionic plate-derived mesenchymal stem cells,interleukin-3 expression was *** further investigate the role of interleukin-3 in neonatal hypoxic-ischemic encephalopathy,we established an in vitro SH-SY5Y cell model of hypoxic-ischemic injury through oxygen-glucose deprivation and silenced interleukin-3 expression using small interfering *** found that the activity and proliferation of SH-SY5Y cells subjected to oxygen-glucose deprivation were further suppressed by interleukin-3 ***,interleukin-3 knockout exacerbated neuronal damage and cognitive and motor function impairment in rat models of hypoxic-ischemic *** findings suggest that transplantation of hpcMSCs ameliorated behavioral impairments in a rat model of hypoxic-ischemic encephalopathy,and this effect was mediated by interleukin-3-dependent neurological function.

关键词： behavioral evaluations gene knockout human neuroblastoma cells(SH-SY5Y) human placental chorionic derived mesenchymal stem cells interleukin-3 neonatal hypoxic-ischemic encephalopathy nerve injury oxygen-glucose deprivation protein chip small interfering RNA

Dynamic tracking of exsolved PdPt alloy/perovskite catalyst for efficient lean methane oxidation

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Chinese Chemical Letters 2024年第4期35卷 170-175页

作者： Yanling Yang Zhenfa Ding Huimin Wang Jianhui Li Yanping Zheng Hongquan Guo Li Zhang Bing Yang Qingqing Gu Haifeng Xiong yifei sun College of Energy Xiamen UniversityXiamen 361005China School of Environment and Civil Engineering Dongguan University of TechnologyDongguan 523808China Department of Chemistry College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China CAS Key Laboratory of Science and Technology on Applied Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province(IKKEM) Xiamen 361102China

Supported Pd based catalysts are considered as the efficient candidates for low-carbon alkane oxidation for their outstanding capability to break C-H bond. Whereas, the irreversible deactivation of Pd based catalysts was still frequently observed. Herein, we reinforced the extruded Pd nanoparticles with quantitive Pt to assemble the evenly distributed Pd Pt nanoalloy onto ferrite perovskite(Pd Pt-LCF) matrix with strengthened robustness of metal/oxide support interface. We further co-achieved the enhanced performance, anti-overoxidation as well as resistance of vapor-poisoning in durability measurement. The operando X-ray photoelectron spectroscopy(O-XPS) combined with various morphology characterizations confirms that the accumulation of surface deep-oxidation species of Pd^(4+) is the culprit for fast activity loss in exsolved Pd system, especially at high temperature of 400 ℃. Conversely, it could be completely suppressed by in-situ alloying Pd with equal amount of Pt, which helps maintain the metastable Pd^(2+)/Pd shell and metallic solid-solution core structure. The density function theory(DFT) calculations further buttress that the dissociation of C–H was facilitated on alloy/perovskite interface which is, on the contrary, resistant toward O–H bond cleavage, as compared to Pd/perovskite. Our work suggests that the modification of exsolved metal/oxide catalytic interface could further enrich the toolkit of heterogeneous catalyst design.

关键词： Exsolution PdPt alloy Operando characterization Methane conversion Deep-oxidation

Gas diffusion in catalyst layer of flow cell for CO_(2) electroreduction toward C_(2+) products

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Nano Research 2024年第3期17卷 1101-1106页

作者： Xiqing Wang Qin Chen Yajiao Zhou Yao Tan Ye Wang Hongmei Li Yu Chen Mahmoud Sayed Ramadan A.Geioushy Nageh K.Allam Junwei Fu yifei sun Min Liu Hunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics and ElectronicsCentral South UniversityChangsha 410083China School of Energy and Power Engineering Beihang UniversityBeijing 100191China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450002China Central Metallurgical Research and Development Institute(CMRDI) P.O.Box 87Helwan 11421CairoEgypt Energy Materials Laboratory School of Sciences and EngineeringThe American University in CairoNew Cairo 11835Egypt Research Center for Advanced Energy and Carbon Neutrality Beihang UniversityBeijing 100191China

The use of gas diffusion electrode(GDE)based flow cell can realize industrial-scale CO_(2) reduction reactions(CO_(2)RRs).Controlling local CO_(2) and CO intermediate diffusion plays a key role in CO_(2)RR toward multi-carbon(C_(2+))*** this work,local CO_(2) and CO intermediate diffusion through the catalyst layer(CL)was investigated for improving CO_(2)RR toward C_(2+)*** gas permeability tests and finite element simulation results indicated CL can balance the CO_(2) gas diffusion and residence time of the CO intermediate,leading to a sufficient CO concentration with a suitable CO_(2)/H_(2)O supply for high C_(2+)*** a result,an excellent selectivity of C_(2+)products~79%at a high current density of 400 mA·cm^(-2) could be obtained on the optimal 500 nm Cu CL(Cu500).This work provides a new insight into the optimization of CO_(2)/H_(2)O supply and local CO concentration by controlling CL for C_(2+)products in CO_(2)RR flow cell.

关键词： gas diffusion electrode CO_(2)reduction Cu mass transfer C_(2)product

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深层坞原理对于智能体育的介入机制

西南大学学报（自然科学版） 2024年第5期46卷 186-194页

作者：吴璇孙逸飞西南大学体育学院重庆400715

随着人工智能技术的进步,“避风港原则”已难以有效应对体育领域的数据信息侵权问题.该文提出应对数据侵权或信息侵权的保障策略——深层坞原理,通过与产业链各环节主体的深度对接,实施对受侵权数据或信息的“下潜”保护,有效遏制或降... 详细信息

随着人工智能技术的进步,“避风港原则”已难以有效应对体育领域的数据信息侵权问题.该文提出应对数据侵权或信息侵权的保障策略——深层坞原理,通过与产业链各环节主体的深度对接,实施对受侵权数据或信息的“下潜”保护,有效遏制或降低侵权损害,其内在逻辑和设计思路也适应未来智能化发展的需求.深层坞原理在当前数字化发展产业链中,既能在前端激发智能化生产活力,又能在后端强化监管制度和机制建设,提高侵权成本、协调数字体育用户与数据实际控制者权力失衡问题.在未来强人工智能发展阶段,深层坞原理也将随之演进,利用未来智能对未来智能机器进行管理,展现其未来发展潜力.

关键词：人工智能深层坞原理泛智能化深度对接自适应

砂土与结构物界面的应力-位移-微结构特性及本构模型

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岩石力学与工程学报 2024年第6期43卷 1549-1560页

作者：叶至韬高玉峰黄星博孙逸飞河海大学岩土力学与堤坝工程教育部重点实验室江苏南京210024

砂土与结构物界面受剪时微结构会发生演变,并产生状态依赖的应力位移行为。采用界面直剪仪对不同常法向刚度和常法向应力条件下的砂土-钢板界面进行单调和循环剪切试验,并通过高清图像识别技术分析剪切过程中的界面微结构的演变,发现:... 详细信息

砂土与结构物界面受剪时微结构会发生演变,并产生状态依赖的应力位移行为。采用界面直剪仪对不同常法向刚度和常法向应力条件下的砂土-钢板界面进行单调和循环剪切试验,并通过高清图像识别技术分析剪切过程中的界面微结构的演变,发现:常法向刚度和常法向应力条件下单调剪切时界面均发生不同程度的剪胀,常法向应力条件下的剪切会使试样产生更明显的软化行为和较多的微结构变化,即颗粒概率熵会随着剪切位移的增大而逐渐增加;循环加载时,处于临界状态线下方的界面土会交替出现剪缩和剪胀现象,伴随着界面的微结构发生波动演变,界面总体会表现出较强的剪缩;先期循环剪切会使得界面发生强度弱化;可见微结构演化影响着界面土的剪胀。为描述此类现象,提出基于微结构演化的动态剪胀状态线,据此建立砂土-结构物界面的非关联随动硬化弹塑性本构模型。模型有12个参数,均可通过试验获得。通过模拟试验数据发现,模型可以合理描述界面的剪胀和软化等力学行为,特别是循环荷载作用下界面的强剪缩行为。

关键词：土力学界面微结构剪胀状态参数本构模型

高校技术转移机构自主权对技术转移效果的影响

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中国科技论坛 2024年第5期 54-64页

作者：张明倩冉美丽孙艺菲上海外国语大学国际金融贸易学院上海200083 中国科学技术发展战略研究院北京100036

针对中国高校技术转移机构转化动力不足、转化能力较弱、决策效率低下的现实问题,研究讨论高校技术转移机构自主权对技术转移效果的影响,发现拥有自主权的高校技术转移机构可以通过更加灵活的选人用人机制、更加充分的科技成果裁量权和... 详细信息

针对中国高校技术转移机构转化动力不足、转化能力较弱、决策效率低下的现实问题,研究讨论高校技术转移机构自主权对技术转移效果的影响,发现拥有自主权的高校技术转移机构可以通过更加灵活的选人用人机制、更加充分的科技成果裁量权和决策权对技术转移产生积极影响,区域技术市场发达程度和区域科技成果供给活跃程度会影响高校技术转移机构自主权与技术转移的关系。研究结论可为探索高校技术转移机构的制度创新,充分发挥高校技术转移机构在成果转化中的主体作用提供改革启示。

关键词：技术转移机构自主权高校

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桥梁风工程研究中的雷诺数效应研究进展

振动与冲击 2024年第2期43卷 187-200,342页

作者：刘庆宽韩原孙一飞郑云飞石家庄铁道大学省部共建交通工程结构力学行为与系统安全国家重点实验室石家庄050043 河北省风工程和风能利用工程技术创新中心石家庄050043 石家庄铁道大学土木工程学院石家庄050043 石家庄铁路职业技术学院铁道工程系石家庄050043

桥梁风工程研究中的雷诺数效应问题是伴随着风洞试验方法产生的一个基础性问题,随着桥梁尺寸的增大其雷诺数也逐渐增大,风洞试验雷诺数和实桥梁雷诺数的差别对试验结果的影响越来越受重视。该研究阐述了雷诺数效应问题的由来,回顾了雷... 详细信息

桥梁风工程研究中的雷诺数效应问题是伴随着风洞试验方法产生的一个基础性问题,随着桥梁尺寸的增大其雷诺数也逐渐增大,风洞试验雷诺数和实桥梁雷诺数的差别对试验结果的影响越来越受重视。该研究阐述了雷诺数效应问题的由来,回顾了雷诺数效应研究的发展历程,总结了针对圆形断面、矩形断面、主梁断面等不同桥梁结构断面雷诺数效应问题的研究进展,包括结构周围流场、气动力、风致振动随雷诺数的变化,指出了桥梁风工程雷诺数效应研究中尚待解决的问题,为今后该领域的研究提供参考和建议。

关键词：桥梁结构风工程雷诺数效应气动力风致振动