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Probing CO on a rutile TiO_(2)(110)surface using atomic force microscopy and Kelvin probe force microscopy

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Nano Research 2022年第3期15卷 1909-1915页

作者： Yuuki Adachi yasuhiro sugawara Yan Jun Li Department of Applied Physics Osaka University2-1 YamadaokaSuitaOsaka 565-0871Japan

Probing CO at a specific site on a metal oxide surface is essential for characterizing various applications such as CO oxidation,hydrogenation,and water–gas shift ***,we use atomic force microscopy and Kelvin probe force microscopy to probe the CO on a rutile TiO_(2)(110)*** results indicate that CO can be manipulated along the Ti row by the repulsive lateral force of“pushing”***,the joint combination of precise manipulation and the distance dependence of local contact potential difference allow us to resolve the interatomic dipole moment and charge state of CO at atomic ***,we found that the negatively charged CO with the dipole moment of negative pole down on the rutile TiO_(2)(110)*** results suppose that both the charge state as well as the on-surface dipole interaction are very effective for CO reaction on rutile TiO_(2)(110)surface.

关键词： CO rutile TiO_(2) dipole moment charge state atomic force microscopy Kelvin probe force microscopy

Distance dependence of atomic-resolution near-field imaging on α-Al2O3 （0001） surface with respect to surface photovoltage of silicon probe tip

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Nano Research 2016年第2期9卷 530-536页

作者： Junsuke Yamanishi Takashi Tokuyama Yoshitaka Naitoh Yan Jun Li yasuhiro sugawara Department of Applied Physics Graduate School of Engineering Osaka University 2-1 Yamada-oka Suita Osaka 565-0871 Japan

Recently, we achieved atomic-resolution optical imaging with near-field scanning optical microscopy using photon-induced force detection. In this technique, the surface photovoltage of the silicon-tip apex induced by the optical near field on the surface is measured as the electrostatic force. We demonstrated atomicresolution imaging of the near field on the α-Al2O3 （0001） surface of a prism. We investigated the spatial distribution of the near field by scanning at different tip-sample distances and found that the atomic corrugation of the near-field signal was observed at greater distances than that of the atomic force microscopy signal. As the tip-sample distance increased, the normalized signal-to-noise ratio of the near field is in a gradual decline almost twice that of the frequency shift （Δf）.

关键词： near-field scanning optical microscopy near field surface photovoltage ci-Al2O3 (0001) force detection

High harmonic exploring on different materials in dynamic atomic force microscopy

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Science China(Technological Sciences) 2018年第3期61卷 446-452页

作者： ZHENG ZhiYue XU Rui YE ShiLi HUSSAIN Sabir JI Wei CHENG Peng LI YanJun sugawara yasuhiro CHENG ZhiHai CAS Center for Excellence in Nanoscience and Key Laboratory of Standardization and Measurement for Nanotechnology National Center for Nanoscience and Technology Beijing 100190 China Department of Physics Renmin University of China Beijing 100872 China The State Key Laboratory of Digital Manufacturing Equipment and Technology Department of Instrument Science and Technology School of Mechanical Science and Engineering Huazhong University of Science and Technology Wuhan 430074 China University of Chinese Academy of Sciences Belting 100049 China Asylum Research Santa Barbara 93117 USA Department of Applied Physics Graduate School of Engineering Osaka University Osaka 565-0871 Japan

In atomic force microscopy(AFM), high-frequency components consisted in dynamic tip-sample interaction have been recently demonstrated as a promising technique for exploring more extensive material properties. Here we present an exploratory study of high harmonic atomic force microscopy by force-spectroscopy and high harmonic imaging. Since these components are very weak compared to the fundamental response, we firstly designed a high harmonic cantilever by tuning the second order flexural resonance frequency to an integer 6 times of its fundamental mode(i.e. ω_2=6ω_1). Moreover, it is verified that high harmonic can discern extra features than topographies on different samples with amplitude/frequency modulation(AM/FM) dynamic AFM mode. In AM mode, the first resonance amplitude and 6 th harmonic amplitude were discussed. The 6 th harmonic is more sensitive than the first order response. In FM mode, it is noted that the decaying rate of the 6 th harmonic frequency is approximately 6 multiples to the slope of the fundamental frequency shift when the tip approaches to the surface of sample. This non-destructive method was also adopted to investigate the local interlayer coupling and intercalation in the two-dimensional graphene films tentatively.

关键词： high harmonic AFM high harmonic cantilever dynamic AFM

Atom Manipulation and Force Spectroscopy on Cu(110)-O Surface with Low-Temperature AFM

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Atom Manipulation and Force Spectroscopy on Cu(110)-O Surfac...

Epitaxial fabrication of AgTe monolayer on Ag(111)and the sequential growth of Te film

中国真空学会2012学术年会

作者： yasuhiro sugawara Department of Applied Physics Graduate School of EngineeringOsaka University

Manipulation of single atoms and molecules is an innovative experimental technique of *** far,a scanning tunneling microscopy(STM) has been widely used to fabricate artificial structures by laterally pushing,pulling or sliding single atoms and ***,the driving forces involved in manipulation have not been ***,an atomic force microscopy(AFM) has been also used to manipulate single atoms and *** manipulation with an AFM is particularly promising,because it allows the direct measurement of the required *** the present study,we investigated the forces in AFM lateral manipulation for a top single Cu atom(super Cu atom)on the Cu(110)-O *** AFM tip apex was coated with Cu or O atoms in situ by slightly making a tip-sample mechanical contact on the Cu(110)-O surface prior to the *** the case of Cu-adsorbed AFM tip,the super Cu atom on the surface was pulled at a lateral tip position on the adjacent binding *** contrast,in the case of O-adsorbed AFM tip,the super Cu atom was pushed over the top of the super Cu ***,we found that the forces(attractive or repulsive forces)to move an atom laterally on the surface strongly depend on the atom species of the AFM tip apex and the ***,in order to clarify the manipulation process,we investigated the full tip-sample potential landscape necessary to manipulate *** tip-sample potentials were determined by the frequency shift versus distance curves by mathematical *** found that the tip-sample potentials which move the super Cu atom laterally on the surface strongly depended on the atom species of the AFM tip apex and the *** results strongly suggest that the chemical nature of tip-sample interaction plays an important role in lateral atom ***,we discuss the pathways for moving the super Cu atom.

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Frontiers of physics 2021年第6期16卷 125-131页

作者： Haoyu Dong Le Lei Shuya Xing Jianfeng Guo Feiyue Cao Shangzhi Gu Yanyan Geng Shuo Mi Hanxiang Wu Yan Jun Li yasuhiro sugawara Fei Pang Wei Ji Rui Xu Zhihai Cheng Beijing Key Laboratory of Optoelectronic Functional Materials&Micro-nano Devices Department of PhysicsRenmin University of ChinaBeijing 100872China Department of Applied Physics Graduate School of EngineeringOsaka University2-1 YamadaokaSuitaOsaka 565-0871Japan

Transition-metal chalcogenides(TMCs)materials have attracted increasing interest both for fundamental research and industrial *** all these materials,two-dimensional(2D)compounds with honeycomb-like structure possess exotic electronic ***,we report a systematic study of TMC monolayer AgTe fabricated by direct depositing Te on the surface of Ag(111)and *** intrinsic defects are observed and studied by scanning tunneling microscopy,indicating that there are two kinds of AgTe domains and they can form gliding ***,the monolayer AgTe can serve as the template for the following growth of Te ***,some Te atoms are observed in the form of chains on the top of the bottom Te *** findings in this work might provide insightful guide for the epitaxial growth of 2D materials for study of novel physical properties and for future quantum devices.

关键词： AgTe monolayer Te film epitaxial growth scanning tunneling microscopy two-dimensional materials transition-metal chalcogenides

Toplayer-dependent crystallographic orientation imaging in the bilayer two-dimensional materials with transverse shear microscopy

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Frontiers of physics 2021年第5期16卷 165-172页

作者： Sabir Hussain Rui Xu Kunqi Xu Le Lei Shuya Xing Jianfeng Guo Haoyu Dong Adeel Liaqat Rashid Iqbal Muhammad Ahsan Iqbal Shangzhi Gu Feiyue Cao Yan Jun Li yasuhiro sugawara Fei Pang Wei Ji Liming Xie Shanshan Chen Zhihai Cheng Beijing Key Laboratory of Optoelectronic Functional Materials&Micro-nano Devices Department of PhysicsRenmin University of ChinaBeijing100872China CAS Key Laboratory of Standardization and Measurement for Nanotechnology CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing100190China Key Laboratory of Inorganic Functional Materials and Devices Shanghai Institute of CeramicsChinese Academy of SciencesShanghai200050China University of Chinese Academy of Sciences Beijing100039China Department of Applied Physics Graduate School of EngineeringOsaka University2-1 YamadaokaSuitaOsaka565-0871Japan

Nanocontact properties of two-dimensional(2D)materials are closely dependent on their unique nanomechanical systems,such as the number of atomic layers and the supporting ***,we report a direct observation of toplayer-dependent crystallographic orientation imaging of 2D materials with the transverse shear microscopy(TSM).Three typical nanomechanical systems,MoS_(2) on the amorphous SiO_(2)/Si,graphene on the amorphous SiO_(2)/Si,and MoS_(2) on the crystallized Al_(2)O_(3),have been investigated in *** experimental observation reveals that puckering behaviour mainly occurs on the top layer of 2D materials,which is attributed to its direct contact adhesion with the AFM ***,the result of crystallographic orientation imaging of MoS_(2)/SiO_(2)/Si and MoS_(2)/Al_(2)O_(3) indicated that the underlying crystalline substrates almost do not contribute to the puckering effect of 2D *** work directly revealed the top layer dependent puckering properties of 2D material,and demonstrate the general applications of TSM in the bilayer 2D systems.

关键词： 2D materials toplayer-dependent crystallographic orientation imaging nanomechanical contact properties transverse shear microscopy

二氧化钛亚表面电荷对其表面点缺陷和吸附原子分布的影响

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物理学报 2020年第21期69卷 11-16页

作者：温焕飞菅原康弘李艳君中北大学仪器科学与动态测试教育部重点实验室太原030051 日本大阪大学工学研究科物理学系専攻大阪5650871

半导体金属氧化物二氧化钛因其稳定、高效、无毒、兼容、低廉等优点受到广泛的关注,本文在低温78 K下利用原子力显微镜探索了二氧化钛亚表面电荷的特性及其对表面点缺陷和吸附原子分布的影响.在原子结构形貌图中亚表面电荷被成像为椭圆... 详细信息

半导体金属氧化物二氧化钛因其稳定、高效、无毒、兼容、低廉等优点受到广泛的关注,本文在低温78 K下利用原子力显微镜探索了二氧化钛亚表面电荷的特性及其对表面点缺陷和吸附原子分布的影响.在原子结构形貌图中亚表面电荷被成像为椭圆形亮丘,且亮丘的高度主要分布在3个不同的区间内,这意味着亚表面电荷位于3个不同的亚表面原子层.在开尔文探针力显微镜成像中,亚表面电荷的电势分布相对低,根据电势成像机理,亚表面电荷为正电荷特性.原子力显微镜的成像图表明,亚表面电荷不仅排斥具有正电荷特性的表面氧空位、吸附氢原子和表面台阶,而且排斥具有负电荷特性的吸附氧原子.实验结果有助于二氧化钛物理特性的研究及其相关产品性能的改进和设计.

关键词：二氧化钛亚表面电荷原子力显微镜开尔文探针力显微镜

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用于旋翼飞机开发研究的多分野解析框架

Transactions of Nanjing University of Aeronautics and Astronautics 2024年第1期41卷 43-52页

作者： TANABE Yasutada sugawara Hideaki KIMURA Keita 日本宇宙航空研究开发机构航空技术部日本东京181-0015

介绍了日本宇宙航空研究开发机构研发的用于旋翼飞机的多分野解析框架。Heli Design是在各种旋翼飞机初期概念设计时使用的软件;rFlight可以提供在各种飞行条件下的平衡解析和线性化飞行模型;rBET/RMT是基于叶片要素理论的低保真度空力... 详细信息

介绍了日本宇宙航空研究开发机构研发的用于旋翼飞机的多分野解析框架。Heli Design是在各种旋翼飞机初期概念设计时使用的软件;rFlight可以提供在各种飞行条件下的平衡解析和线性化飞行模型;rBET/RMT是基于叶片要素理论的低保真度空力解析软件,和rMode提供的结构模型结合,可以推测旋转翼的弹性变形和各种飞行条件下的空力负载;rFlow3D是基于CFD计算的高保真度数值模拟软件;rGrid系列自动网格构造工具为其提供简单的网格生成;基于rFlow3D的计算结果,r Noise可以预测在任何观测点的噪声。这些软件已经广泛地被应用在各种新型旋翼飞机的开发研究中,其计算精度也已被各种实验结果所应证。

关键词：旋翼飞机多分野解析高保真模拟设计工具

Current perspectives of viral

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World Journal of Gastroenterology 2024年第18期30卷 2402-2417页

作者： Daisuke Usuda Yuki Kaneoka Rikuo Ono Masashi Kato Yuto sugawara Runa Shimizu Tomotari Inami Eri Nakajima Shiho Tsuge Riki Sakurai Kenji Kawai Shun Matsubara Risa Tanaka Makoto Suzuki Shintaro Shimozawa Yuta Hotchi Ippei Osugi Risa Katou Sakurako Ito Kentaro Mishima Akihiko Kondo Keiko Mizuno Hiroki Takami Takayuki Komatsu Tomohisa Nomura Manabu Sugita Department of Emergency and Critical Care Medicine Juntendo University Nerima HospitalNerima 177-8521TokyoJapan Department of Sports Medicine Faculty of MedicineJuntendo UniversityBunkyo 113-8421TokyoJapan

Viral hepatitis represents a major danger to public health,and is a globally leading cause of *** five liver-specific viruses:Hepatitis A virus,hepatitis B virus,hepatitis C virus,hepatitis D virus,and hepatitis E virus,each have their own unique epidemiology,structural biology,transmission,endemic patterns,risk of liver complications,and response to antiviral *** remain few options for treatment,in spite of the increasing prevalence of viral-hepatitiscaused liver ***,chronic viral hepatitis is a leading worldwide cause of both liver-related morbidity and mortality,even though effective treatments are available that could reduce or prevent most patients’*** 2016,the World Health Organization released its plan to eliminate viral hepatitis as a public health threat by the year 2030,along with a discussion of current gaps and prospects for both regional and global eradication of viral ***,treatment is sufficiently able to prevent the disease from reaching advanced ***,future therapies must be extremely safe,and should ideally limit the period of treatment necessary.A better understanding of pathogenesis will prove beneficial in the development of potential treatment strategies targeting infections by viral *** review aims to summarize the current state of knowledge on each type of viral hepatitis,together with major innovations.

关键词： Hepatitis A virus Hepatitis B virus Hepatitis C virus Hepatitis D virus Hepatitis E virus Current perspectives