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Enhancing electrolyte ion diffusion via direct ink writing pillar array structure of graphene electrodes for high-performance microsupercapacitors

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Nano Research 2024年第7期17卷 6203-6211页

作者： Yan Zhang Huandi Zhang Xiaoxiao Wang Cheng Tang Xiaowei shi Zehua Zhao Jiamei Liu Guolong Wang Jianfeng shen Lei Li State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and EngineeringXi’an Jiaotong University28 Xianning West RoadXi’an 710049China Center for Materials Chemistry Frontier Institute of Science and TechnologyXi’an Jiaotong UniversityXi’an 710049China Instrument Analysis Center of Xi'an Jiaotong University Xi’an Jiaotong University28 Xianning West RoadXi’an 710049China Institute of special materials and technology Fudan UniversityShanghai 200433China

The graphene-based microsupercapacitors(MSCs)suffer from graphene aggregation issue in *** reduces the electrolyte ions transportation in the electrodes to degrade the charge storage ability of MSCs,hampering their practical *** the electrolyte ions transportation in the electrodes can boost the charge storage ability of ***,we design and experimentally realize pillar array structure of graphene electrodes for MSCs by direct ink writing *** graphene electrodes with pillar array structure increase the contact area with electrolyte and short the electrolyte ions transport path,facilitating electrolyte ions transport in *** MSCs exhibit high areal capacitance of 25.67 mF·cm^(−2),high areal energy density of 20.54μWh·cm^(−2),and high power density of 1.45 mW·cm^(−2).One single MSCs can power timer for 10 min and pressure sensor more than 160 min,showing high practical application *** work provides a new avenue for developing high performance MSCs.

关键词： microsupercapacitors pillar array structure direct ink writing areal energy density ion transport

Polyzwitterionic cross-linked double network hydrogel electrolyte enabling high-stable Zn anode

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Nano Research 2024年第6期17卷 5278-5287页

作者： Mengyu shi Junlong Zhang Guochuan Tang Ben Wang Sen Wang Xiaoxian Ren Guojie Li Weihua Chen Chuntai Liu Changyu shen State Key Laboratory of Structural Analysis Optimization and CAE Software for Industrial EquipmentNational Engineering Research Center for Advanced Polymer Processing TechnologyZhengzhou UniversityZhengzhou 450002China College of Chemistry and Green Catalysis Center Zhengzhou UniversityZhengzhou 450001China Research Institute of Interdisciplinary Science and School of Materials Science and Engineering Dongguan University of TechnologyDongguan 523808China

Zn metal anode suffers from dendrite issues and passive byproducts,which severely plagues the practical application of aqueous Zn metal ***,a polyzwitterionic cross-linked double network hydrogel electrolyte composed of physical crosslinking(hyaluronic acid)and chemical crosslinking(synthetic zwitterionic monomer copolymerized with acrylamide)is introduced to overcome these *** the one hand,highly hydrophilic physical network provides an energy dissipation channel to buffer stress and builds a H_(2)O-poor interface to avoid side *** the other hand,the charged groups(sulfonic and imidazolyl)in chemical crosslinking structure build anion/cation transport channels to boost ions’kinetics migration and regulate the typical solvent structure[Zn(H_(2)O)_(6)]^(2+)to R-SO_(3)^(−)[Zn(H_(2)O)_(4)]^(2+),with uniform electric field distribution and significant resistance to dendrites and parasitic *** on the above functions,the symmetric zinc cell exhibits superior cycle stability for more than 420 h at a high current density of 5 mA·cm^(−2),and Zn||MnO_(2)full cell has a reversible specific capacity of 150 mAh·g^(−1)after 1000 cycles at 2 C with this hydrogel ***,the pouch cell delivers impressive flexibility and cyclability for energy-storage applications.

关键词： Zn anode dendrites parasitic reactions polyzwitterion double network hydrogel electrolyte

Cross-national Perspectives on Using Sustainable Development Goals(SDGs) Indicators for Monitoring Sustainable Development: A Database and Analysis

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Chinese Geographical Science 2021年第4期31卷 600-610页

作者： WANG Xiangyu SONG Changqing CHENG Changxiu YE Sijing shen shi Key Laboratory of Environmental Change and Natural Disaster Ministry of EducationBeijing Normal UniversityBeijing 100875China Center for Geodata and Analysis Faculty of Geographical ScienceBeijing Normal UniversityBeijing 100875China National Tibetan Plateau Data Center Beijing 100101China

Sustainable development is the theme of the 21st century. To monitor the progress of sustainable development, the United Nations launched Sustainable Development Goals(SDGs) in 2015. Subsequently, nations of the world have drawn up a list of localized indicators regarding the United Nations SDGs as a paradigm. We established a database including SDGs indicator systems of 11 economies by collecting and determining a large number of materials. Based on this database, we analyzed SDGs indicators by designing a conceptual framework of comparative analysis that included three views. We found that the SDGs indicator systems of 11 economies are different between the number of indicators, the proportion of different categories, and the connotation of indicators. Although the SDGs indicator systems among economies regarded the United Nations SDGs as a framework and included the major social problems related to sustainability, the inconsistency between SDGs indicator systems is large. It is a major reason why scholars lack the systematic method for developing indicators. There are challenges faced in data accessibility. The framework for comparative analysis could be applied to different economies.

关键词： Sustainable Development Goals(SDGs) framework indicator cross-national database

Tandem hydroalkylation and deoxygenation of lignin-derived phenolics to synthesize high-density fuels

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Chinese Journal of Chemical Engineering 2024年第2期66卷 104-109页

作者： Rui Yu Zhensheng shen Yanan Liu Chengxiang shi Juncong Qu Lun Pan Zhenfeng Huang Xiangwen Zhan g Ji-Jun Zou Key Laboratory for Green Chemical Technology of Ministry of Education School of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Collaborative Innovative Center of Chemical Science and Engineering(Tianjin) Tianjin 300072China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China

Lignin is the most abundant naturally phenolic biomass,and the synthesis of high-performance renewable fuel from lignin has attracted significant *** propose the efficient synthesis of high-density fuels using simulated lignin cracked oil in tandem with hydroalkylation and deoxygenation ***,we investigated the reaction pathway for the hydroalkylation of phenol,which competes with the hydrodeoxygenation form *** then,we investigated the effects of metal catalyst types,the loading amount of metallic,acid dosage,and reactant ratio on the reaction *** phenol hydroalkylation and hydrodeoxygenation were balanced when 180℃ and 5 MPa H_(2)with the alkanes yield of 95%.By extending the substrate to other lignin-derived phenolics and simulated lignin cracked oil,we obtained the polycyclic alkane fuel with high density of 0.918 g·ml^(-1)and calorific value of41.2 MJ·L^(-1).Besides,the fuel has good low-temperature properties(viscosity of 9.3 mm^(2)·s^(-1)at 20℃ and freezing point below-55℃),which is expected to be used as jet *** work provides a promising way for the easy and green production of high-density fuel directly from real lignin oil.

关键词： High-density fuel Biofuel Hydrogenation Alkylation Lignin Phenolics

Tilapia Head Glycolipid Alleviates Indomethacin-Induced Gastric Ulcer via Regulating Oxidative Stress and Inflammation Through COX/PGE2 Signaling Pathway in Adult Rats

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Journal of Ocean University of China 2024年第3期23卷 743-754页

作者： WANG Bohui WU Haixing SHAO Mingyang JIANG Mengqi SU Ruiheng GAO Xia XIA Guanghua shi Haohao shen Xuanri Hainan Engineering Research Center of Aquatic Resources Efficient Utilization in South China Sea College of Food Science and TechnologyHainan UniversityHaikou 570228China Collaborative Innovation Center of Marine Food Deep Processing Dalian Polytechnic UniversityDalian 116000China College of Food and Engineering Hainan Tropical Ocean UniversitySanya 572022China

The aim of this experiment was to investigate the ameliorative effect and molecular mechanism of tilapia head glycolipid(TH-GL)on indomethacin(IDM)-induced gastric ulcer in male Sprague Dawley(SD)*** gastric ulcer model was established by oral administration of 30mgkg^(-1) IDM after 7 days of TH-GL or omeprazole(OME)administration in *** the macroscopic gastric injury symptoms,gastric mucosa protective factor cyclooxygenase 1(COX-1),cyclooxygenase 2(COX-2),prostaglandin E_(2)(PGE_(2)),the levels of oxidative stress,and inflammatory cytokine expression levels in the rats were *** experimental results showed that multiple ulcers appeared on the gastric surface of the rats in the model *** to the model group,TH-GL significantly alleviated gastric ulcers and reduced the gastric damage index in *** addition,TH-GL significantly promoted the expression of constitutive enzyme COX-1 while inhibited the expression of inducible enzyme COX-2,and make PGE2 maintain at normal ***-GL also inhibited oxidative stress and inflammatory responses,increased superoxide dismutase(SOD)activity and glutathione(GSH)content,decreased the level of malondialdehyde(MDA)and the content of pro-inflammatory *** conclusion,these results suggested that TH-GL could maintain the expression levels of COX-1 and PGE2 while inhibit the expression of COX-2 in the gastric of rat and then prevent IDM-induced gastric ulcer,which may be related to the regulation of oxidative stress and inflammatory ***,TH-GL might be a new option for the prevention of gastric diseases induced by IDM.

关键词： tilapia head glycolipid indomethacin gastric ulcer oxidative stress inflammation

Crystal engineering regulation achieving inverse temperature symmetry breaking ferroelasticity in a cationic displacement type hybrid perovskite system

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Chinese Chemical Letters 2024年第5期35卷 477-481页

作者： Na Wang Wang Luo Huaiyi shen Huakai Li Zejiang Xu Zhiyuan Yue Chao shi Hengyun Ye Leping Miao Chaotic Matter Science Research Center Department of MaterialsMetallurgy and ChemistryJiangxi University of Science and TechnologyGanzhou 341000China

Ferroelastic hybrid perovskite materials have been revealed the significance in the applications of switches,sensors,actuators,***,it remains a challenge to design high-temperature ferroelastic to meet the requirements for the practical ***,we reported an one-dimensional organicinorganic hybrid perovskites(OIHP)(3-methylpyrazolium)CdCl_(3)(3-MBCC),which possesses a mmmF2/m ferroelastic phase transition at 263 ***,utilizing crystal engineering,we replace-CH_(3) with-NH_(2) and-H,which increases the intermolecular force between organic cations and inorganic *** phase transition temperature of(3-aminopyrazolium)CdCl_(3)(3-ABCC),and(pyrazolium)CdCl_(3)(BCC)increased by 73 K and 10 K,***,BCC undergoes an unconventional inverse temperature symmetry breaking(ISTB)ferroelastic phase transition around 273 ***,it transforms from a high symmetry low-temperature paraelastic phase(point group 2/m)to a low symmetry high-temperature ferroelastic phase(point group ī)originating from the rare mechanism of displacement of organic cations phase *** means that crystal BCC retains in ferroelastic phase above 273 K until melting point(446 K).Furthermore,characteristic ferroelastic domain patterns on crystal BCC are confirmed with polarized optical *** study enriches the molecular mechanism of ferroelastics in the family of organic-inorganic hybrids and opens up a new avenue for exploring high-temperature ferroic materials.

关键词： Organic-inorganic hybrid perovskite Crystal engineering Inverse temperature symmetry breaking Displacement type phase transition Ferroelasticity

Mei Symmetry of General Discrete Holonomic System

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Communications in Theoretical Physics 2008年第9期50卷 607-610页

作者： shi shen-Yang CHEN Li-Qun FU Jing-Li Department of Physics Zhejiang Sci-Tech University Hangzhou 310018 China Shanghai Institute of Applied Mathematics and Mechanics Shanghai University Shanghai 200072 China

The Mei symmetry and conserved quantity of general discrete holonomic system are investigated in *** requirement for an invariant formalism of discrete motion equations is defined to be Mei *** when a conserved quanti... 详细信息

关键词：离散力学离散保存量对称性完整系统

暗通道与交叉通道多先验联合多光谱超分辨率算法

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光学学报 2022年第10期42卷 36-44页

作者：石神尹增山王龙中国科学院上海微系统与信息技术研究所上海200050 中国科学院微小卫星创新研究院上海201203 中国科学院大学北京100049 上海科技大学信息科学与技术学院上海201210

针对多光谱遥感图像超分辨率重建易受噪声和色差影响的问题,提出了暗通道与交叉通道多先验联合的多光谱超分辨率算法。首先,在传统全变分先验的基础上,引入了暗通道先验与交叉通道先验。然后,基于最大后验概率估计理论,建立了多先验联... 详细信息

针对多光谱遥感图像超分辨率重建易受噪声和色差影响的问题,提出了暗通道与交叉通道多先验联合的多光谱超分辨率算法。首先,在传统全变分先验的基础上,引入了暗通道先验与交叉通道先验。然后,基于最大后验概率估计理论,建立了多先验联合的多光谱超分辨率重建算法。所提算法可实现图像边缘信息恢复、图像纹理信息恢复、噪声抑制、阶梯效应抑制和色差抑制,进而综合提升了重建图像的质量。最后,开展了实验验证,结果表明,在不同信噪比(10~40 dB)和色差干扰下,相比已有算法,所提算法的重建效果显著提升。

关键词：图像处理多帧超分辨率多光谱图像多先验联合

Pedestrian lane formation with following–overtaking model and measurement of system order

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Chinese Physics B 2024年第2期33卷 247-263页

作者：李碧璐李政周睿申世飞 Department of Engineering Physics Tsinghua UniversityBeijing 100084China School of Safety Science Tsinghua UniversityBeijing 100084China

Pedestrian self-organizing movement plays a significant role in evacuation studies and architectural *** formation,a typical self-organizing phenomenon,helps pedestrian system to become more orderly,the majority of following behavior model and overtaking behavior model are imprecise and unrealistic compared with pedestrian movement in the real *** this study,a pedestrian dynamic model considering detailed modelling of the following behavior and overtaking behavior is constructed,and a method of measuring the lane formation and pedestrian system order based on information entropy is *** and analysis demonstrate that the following and avoidance behaviors are important factors of lane formation.A high tendency of following results in good lane *** non-selective following behavior and aggressive overtaking behavior cause the system order to *** most orderly following strategy for a pedestrian is to overtake the former pedestrian whose speed is lower than approximately 70%of his *** influence of the obstacle layout on pedestrian lane and egress efficiency is also studied with this *** presence of a small obstacle does not obstruct the walking of pedestrians;in contrast,it may help to improve the egress efficiency by guiding the pedestrian flow and mitigating the reduction of pedestrian system orderliness.

关键词： pedestrian movement lane formation information entropy order degree