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Contamination of PAHs in Sludge Samples from the yangtze River Delta Area

Pedosphere 2007年第3期17卷 373-382页

作者： shen rong-yan LUO Yong-Ming ZHANG Gang-Ya TENG Ying LI Zhen-Gao WU Long-Hua Institute of Soil Science Chinese Academy of Sciences Nanjing 210008 （China） Graduate School of Chinese Academy of Sciences Beijing 100039 （China）

To ascertain the contaminated conditions of polycyclic aromatic hydrocarbons （PAHs） in sludge and to evaluate the risk of application of this sludge for agricultural purposes, 44 sludge samples obtained from 15 cities in the yangtze River Delta area of China were investigated using capillary gas chromatography/mass spectrometry （GC/MS） after ultrasonic extraction and silica gel cleanup. PAHs＇ contents ranged from 0.0167 to 15.4860 mg kg^-1 （dry weight, DW） and averaged 1.376 mg kg^-1, with most samples containing 〈 1.5 mg kg^-1. Pyrene （PY）, fluoranthene （FL）, benzo[b]fluoranthene （BbF）, indeno[1,2,3-cd]pyrene （IND）, benzo[a]pyrene （B[a]P）, and benzo[g,h,i]perylene （BghiP） were the most dominant compounds, ranging from 0.1582 to 0.2518 mg kg^-1. Single PAH, such as naphthalene （NAP, 2-benzene rings）, phenanthrene （PA, 3-benzene rings）, PY （4-benzene rings）, and FL （3-benzene rings）, had high detection rates （76.1%-93.5%）. The distribution patterns of PAHs were found to vary with the sludge samples; however, the patterns showed that a few compounds with 2- and 3-benzene rings were commonly found in the samples, whereas those with 4-, 5-, and 6-benzene rings were usually less commonly found. All the 44 sludge samples were within the B[a]P concentration limit for sludge applied to agricultural land in China （〈 3.0 rag kg^-1）. The probable sources of PAH contamination in the sludge samples were petroleum, petroleum products, and combustion of liquid and solid fuel. The concentrations and distributions of the 16 PAHs in sludge were related to sludge type, source, and treatment technology, together with the physicochemical properties.

关键词： municipal sludge organic pollutants polycyclic aromatic hydrocarbons yangtze River Delta

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Herbicidal activity and biochemical characteristics of the botanical drupacine against Amaranthus retroflexus L.

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Journal of Integrative Agriculture 2023年第5期22卷 1434-1444页

作者： YU Hua-long TIAN Ci shen rong-yan Zhao Han yanG Juan DONG Jin-gao ZHANG Li-hui MA Shu-jie College of Plant Protection Hebei Agricultural UniversityBaoding 071001P.R.China State Key Laboratory of North China Crop Improvement and Regulation Baoding 071001P.R.China College of Agronomy and Biotechnology Hebei Normal University of Science&TechnologyQinhuangdao 066004P.R.China

Botanical herbicide has been a hot topic in the research and development of novel pesticides. The herbicidal activity and biochemical characteristics of the botanical compound drupacine were studied by evaluating its effects on seed germination, seedling growth, morphological and physiological characteristics of Amaranthus retroflexus. Drupacine inhibited seed germination and seedling growth, and had a median inhibition concentration(IC50) value of 38.99 mg L-1against A. retroflexus root. The α-amylase activity and soluble sugar content in treated plants were significantly lower than that of the control. The expression of α-amylase gene was dosage-dependently inhibited compared to the untreated control. This suggested that inhibition of α-amylase activity was a mode of action on seed germination. The root hairs were significantly decreased and part of the root cap fell off after treatment with drupacine. The ultrastructure observation showed that cell damage of root tips increased with the treatment time. Drupacine also increased the relative conductivity and malondialdehyde(MDA) content. Peroxidase(POD), catalase(CAT), and superoxide dismutase(SOD) activities were significantly enhanced in the treatment compared to the control. These findings indicated that the physiological and biochemical reaction changes leading to morphological and membrane injuries were the main effects of drupacine on the inhibition of seedling growth. Drupacine can be developed as a botanical herbicide.

关键词： drupacine herbicidal activity physiological characteristic defense capacity Amaranthus retroflexus

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Benzo[a]pyrene and Phenanthrene in Municipal Sludge from the yangtze River Delta, China

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Pedosphere 2009年第4期19卷 523-531页

作者： shen rong-yan LUO Yong-Ming FENG sheng ZHANG Gang-Ya WU Long-Hua LI Zhen-Gao TENG Ying P. CHRISTIE Institute of Soil Science Chinese Academy of Sciences Nanjing 210008 （China） Department of Environment and Safety Engineering Jiangsu Polytechnic University Changzhou 213016 （China） Graduate University of the Chinese Academy of Sciences Beijing 100049 （China） Department of Agricultural and Environmental Science Queen＇s University Belfast Newforge Lane Belfast BT9 5PX （UK）

To evaluate the contaminated conditions of benzo[alpyrene （B[a]P） and phenanthrene （PA） in sludge and to ascertain whether B[a]P limit for land application of sludge exists, the contents of B[a]P and PA in 46 sludge samples from 15 cities in the yangtze River Delta area of China were determined using high performance liquid chromatography （HPLC） coupled with a fluorescence detector after ultrasonic extraction and silica gel cleanup. B[a]P contents ranged from non-detectable to 1.693 mg kg^-1 dry weight （DW）, averaged 0.402 mg kg^-1 DW, and were 〈 1.0 mg kg^-1 DW in most of the sludge samples. PA was found in all the sludge samples analyzed; its contents ranged between 0.028 and 1.355 mg kg^-1 DW, with an average value of 0.298 mg kg^-1 DW. Most of the sludge samples contained 〈 0.5 mg kg^-1 DW PA. All 46 municipal sludge samples analyzed in this study showed B[a]P contents 〈 3.0 mg kg^-1 DW, which is the limit value for sludge applied to agricultural lands in China. The contents and distributions of B[a]P and PA in municipal sludge were related to sludge types, sources and treatment technologies, along with the physical and chemical properties of these pollutants.

关键词： benzo[a]pyrene municipal sludge organic pollutants phenanthrene yangtze River Delta

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Remaining Life Prediction Method for Photovoltaic Modules Based on Two-Stage Wiener Process

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Energy Engineering 2025年第1期122卷 331-347页

作者： Jie Lin Hongchi shen Tingting Pei yan Wu School of Electrical Engineering and Information Engineering Lanzhou University of TechnologyLanzhou730050China

Photovoltaic (PV) modules, as essential components of solar power generation systems, significantly influence unitpower generation *** service life of these modules directly affects these costs. Over time, the performanceof PV modules gradually declines due to internal degradation and external environmental *** cumulativedegradation impacts the overall reliability of photovoltaic power generation. This study addresses the complexdegradation process of PV modules by developing a two-stage Wiener process model. This approach accountsfor the distinct phases of degradation resulting from module aging and environmental influences. A powerdegradation model based on the two-stage Wiener process is constructed to describe individual differences inmodule degradation processes. To estimate the model parameters, a combination of the Expectation-Maximization(EM) algorithm and the Bayesian method is employed. Furthermore, the Schwarz Information Criterion (SIC) isutilized to identify critical change points in PV module degradation trajectories. To validate the universality andeffectiveness of the proposed method, a comparative analysis is conducted against other established life predictiontechniques for PV modules.

关键词： Photovoltaic modules degradation stochastic processes lifetime prediction

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Pathogenesis, diagnosis, and treatment of epilepsy: electromagnetic stimulation-mediated neuromodulation therapy and new technologies

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Neural Regeneration Research 2025年第4期20卷 917-935页

作者： Dian Jiao Lai Xu Zhen Gu Hua yan Dingding shen Xiaosong Gu Academy of Medical Engineering and Translational Medicine Tianjin UniversityTianjinChina Key Laboratory of Advanced Drug Delivery Systems of Zhejiang Province College of Pharmaceutical SciencesZhejiang UniversityHangzhouZhejiang ProvinceChina Affiliated Hospital of Nantong University NantongJiangsu ProvinceChina

Epilepsy is a severe,relapsing,and multifactorial neurological *** regarding the accurate diagnosis,prognosis,and in-depth pathogenesis are crucial for the precise and effective treatment of *** pathogenesis of epilepsy is complex and involves alterations in variables such as gene expression,protein expression,ion channel activity,energy metabolites,and gut microbiota *** results are lacking for conventional treatments for *** resection of lesions,drug therapy,and non-drug interventions are mainly used in clinical practice to treat pain associated with ***-pharmacological treatments,such as a ketogenic diet,gene therapy for nerve regeneration,and neural regulation,are currently areas of research *** review provides a comprehensive overview of the pathogenesis,diagnostic methods,and treatments of *** also elaborates on the theoretical basis,treatment modes,and effects of invasive nerve stimulation in neurotherapy,including percutaneous vagus nerve stimulation,deep brain electrical stimulation,repetitive nerve electrical stimulation,in addition to non-invasive transcranial magnetic stimulation and transcranial direct current *** studies have shown that electromagnetic stimulation-mediated neuromodulation therapy can markedly improve neurological function and reduce the frequency of epileptic ***,many new technologies for the diagnosis and treatment of epilepsy are being ***,current research is mainly focused on analyzing patients’clinical manifestations and exploring relevant diagnostic and treatment methods to study the pathogenesis at a molecular level,which has led to a lack of consensus regarding the mechanisms related to the disease.

关键词： diagnosis drug treatment electroencephalography epilepsy monitoring epilepsy nerve regeneration neurostimulation non-drug interventions pathogenesis prediction

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Morphology engineering of ZnO micro/nanostructures under mild conditions for optoelectronic application

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 498-503页

作者： Liang Chu Haoyu shen Hudie Wei Hongyu Chen Guoqiang Ma Wensheng yan Institute of Carbon Neutrality and New Energy&School of Electronics and Information Hangzhou Dianzi UniversityHangzhou 310018China School of Applied Physics and Materials Wuyi UniversityJiangmen 529020China

Zinc oxide(ZnO)serves as a crucial functional semiconductor with a wide direct bandgap of approximately 3.37 *** reaction is commonly used in the synthesis of ZnO micro/nanostructures,given its low cost,simplicity,and easy ***,ZnO morphology engineering has become desirable through the alteration of minor conditions in the reaction process,particularly at room *** this work,ZnO micro/nanostructures were synthesized in a solution by varying the amounts of the ammonia added at low temperatures(including room temperature).The formation of Zn^(2+)complexes by ammonia in the precursor regulated the reaction rate of the morphology engineering of ZnO,which resulted in various structures,such as nanoparticles,nanosheets,microflowers,and single ***,the obtained ZnO was used in the optoelectronic application of ultraviolet detectors.

关键词： morphology engineering low temperature ZnO nanosheets microflowers ultraviolet detector

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Inhibiting ceramide synthase 5 expression in microglia decreases neuroinflammation after spinal cord injury

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Neural Regeneration Research 2025年第10期20卷 2955-2968页

作者： Wei Zhang Yubao Lu Ruoqi shen Yingjie Wu Chenrui Liu Xingxing Fang Liangming Zhang Bin Liu Limin rong Department of Spine Surgery The Third Affiliated HospitalSun Yat-sen UniversityGuangzhouGuangdong ProvinceChina National Medical Products Administration(NMPA)Key Laboratory for Quality Research and Evaluation of Cell Products GuangzhouGuangdong ProvinceChina Guangdong Provincial Center for Quality Control of Minimally Invasive Spine Surgery GuangzhouGuangdong ProvinceChina Guangdong Provincial Center for Engineering and Technology Research of Minimally Invasive Spine Surgery GuangzhouGuangdong ProvinceChina

Microglia,the resident monocyte of the central nervous system,play a crucial role in the response to spinal cord ***,the precise mechanism remains *** investigate the molecular mechanisms by which microglia regulate the neuroinflammatory response to spinal cord injury,we performed single-cell RNA sequencing dataset analysis,focusing on changes in microglial *** found that the MG1 subpopulation emerged in the acute/subacute phase of spinal cord injury and expressed genes related to cell pyroptosis,sphingomyelin metabolism,and neuroinflammation at high ***,we established a mouse model of contusive injury and performed intrathecal injection of siRNA and molecular inhibitors to validate the role of ceramide synthase 5 in the neuroinflammatory responses and pyroptosis after spinal cord ***,we established a PC12-BV2 cell co-culture system and found that ceramide synthase 5 and pyroptosis-associated proteins were highly expressed to induce the apoptosis of neuron *** ceramide synthase 5 expression in a mouse model of spinal cord injury effectively reduced ***,ceramide synthase 5-induced pyroptosis was dependent on activation of the NLRP3 signaling *** ceramide synthase 5 expression in microglia in vivo reduced neuronal apoptosis and promoted recovery of neurological ***2g7 formed a“bridge”between sphingolipid metabolism and ceramide synthase 5-mediated cell death by inhibiting the NLRP3 signaling ***,these findings suggest that inhibiting ceramide synthase 5 expression in microglia after spinal cord injury effectively suppressed microglial pyroptosis mediated by NLRP3,thereby exerting neuroprotective effects.

关键词： ceramide synthase 5 gasdermin D microglia neuroinflammation NLRP3 nuclear factor kappa B Pla2g7 pyroptosis sphingomyelin metabolism spinal cord injury

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非均匀加热蒸发管内两相流动不稳定性数值分析

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原子能科学技术 2015年第9期49卷 1573-1578页

作者：沈艳荣杨冬陆启亮姜勇王少飞西安交通大学动力工程多相流国家重点实验室陕西西安710049

针对蒸发管非均匀加热工况,采用包含水平、倾斜上升、垂直上升和垂直下降流动的优化内螺纹管,建立了基于均相流模型的蒸发管数学模型,采用时域法模拟了蒸发管内两相流动不稳定性。计算了不稳定发生时,进口流量在各时间点的数值,并与Siem... 详细信息

针对蒸发管非均匀加热工况,采用包含水平、倾斜上升、垂直上升和垂直下降流动的优化内螺纹管,建立了基于均相流模型的蒸发管数学模型,采用时域法模拟了蒸发管内两相流动不稳定性。计算了不稳定发生时,进口流量在各时间点的数值,并与Siemens公司的计算结果进行了对比,结果符合良好,表明本文采用的数学模型和数值方法在模拟两相流动不稳定性上具有一定的可靠性。分析了系统参数对两相流动不稳定性的影响,并与均匀加热工况进行了比较。结果表明:非均匀加热工况系统参数影响规律与均匀加热工况具有相似性,增加进口压力或进口流量系统的稳定性提高;减小进口阻力系数或增大出口阻力系数系统的稳定性降低。

关键词：非均匀加热两相流动不稳定性时域法数值分析

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Metal nanoparticles decorated CoFe-(oxy)hydroxysulfides nanosheets fabricated by a general strategy for electrocatalytic water splitting

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Journal of Energy Chemistry 2025年第1期100卷 26-38页

作者： Xiaodong yang Haochen shen Xiaoming Xiao Zhichao Li Qi Zhou Wei yang Bin Jiang Yongli Sun Luhong Zhang Zhenhua yan School of Chemical Engineering and Technology Tianjin University Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Nankai University

This study presents a novel method to fabricate metal-decorated,sulfur-doped layered double hydroxides （M/SLDH） through spontaneous redox and sulfurization *** developed Ag/SLDH and Pt/SLDH catalysts with abundant heterogeneous interfaces and hierarchical nanostructures demonstrated outstanding oxygen evolution reaction （OER） and hydrogen evolution reaction （HER） performance,achieving low overpotentials of 212 and 35 mV at 10 mA cm-2in 1 M KOH,*** both anode and cathode in water splitting,they required only 1.47 V to reach 10 mA cm-2and exhibited high structural robustness,maintaining stability at 1000 mA cm-2for 300 ***-situ Raman analysis revealed that the synergistic effects of metal nanoparticles and S doping significantly promote the transformation into the S-Co1-xFexOOH layer,which serves as the active phase for water ***,ultraviolet photoelectron spectroscopy （UPS） and density functional theory （DFT） analyses indicated that incorporating metal nanoparticles and S doping increase electron density near the Fermi level and reduce reaction energy barriers,thus enhancing intrinsic OER and HER *** study provides a scalable strategy for synthesizing high-performance electrocatalysts for water splitting,with promising potential for broader applications.

关键词： Ultraviolet photoelectron spectroscopy

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城市污泥的污染现状及其土地利用评价

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土壤 2006年第5期38卷 517-524页

作者：申荣艳骆永明滕应李振高中国科学院南京土壤研究所土壤与环境生物修复研究中心

随着城市污泥产生量的迅速增加,污泥的科学处置及土地利用是当前城市固体废弃物资源化的主要研究内容。本文较系统地阐述了污泥的基本性质、污泥污染和处置现状及土地利用的风险评价等相关研究,并指出了目前城市污泥研究中存在的问题。

关键词：城市污泥处置方式资源化土地利用

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