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Double-confined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C toward ultra-stable Li-/Na-ion batteries

Rare Metals 2024年第5期43卷 2067-2079页

作者： Dan Wang Qun Ma Huan He Zhi-Yuan Wang run-guo Zheng Hong-Yu Sun Yan-guo Liu Chun-Li Liu School of Materials Science and Engineering Northeastern UniversityShenyang110819China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province Qinhuangdao 066004China Department of Physics and Oxide Research Center Hankuk University of Foreign StudiesYongin 17035Korea

Antimony-based materials with high capacities and moderate potentials are promising anodes for lithium-/-sodium-ion ***,their tremendous volume expansion and inferior conductivity lead to poor structural stability and sluggish reaction ***,a doubleconfined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C has been fabricated through a solvothermal method followed by low-temperature heat *** dual protection of“MXene”and“carbon”can better accommodate the volume expansion of Sb/Sb_(2)S_(3).The strong covalent bond(Ti-S,Ti-O-Sb,C-O-Sb)can firmly integrate Sb-based material with Ti_(3)C_(2)T_(x)and carbon,which significantly improves the structure *** addition,the carbon layer can restrain the oxidation of MXenes,and the nano-Sb/Sb_(2)S_(3)can facilitate electron/ion transport and suppress the restacking of *** heterogeneous interface between Sb and Sb_(2)S_(3)can further promote interfacial charge *** MXene-Sb/Sb_(2)S_(3)@C-1 with the optimal Sb content shows high specific capacities,comparable rate properties and ultra-stable cycling performances(250 m Ah·g^(-1)after 2500 cycles at 1 A·g^(-1)for sodium-ion batteries).Ex situ X-ray diffractometer(XRD)test reveals the storage mechanism including the conversion and alloying process of MXene-Sb/Sb_(2)S_(3)@*** voltammetry(CV)test results demonstrate that the pseudocapacitance behavior is dominant in MXene-Sb/Sb_(2)S_(3)@C-1,especially at large *** design paves the way for exploring high-performance alloy-based/conversion-type anode for energy storage devices.

关键词： Sb/Sb_(2)S_(3) MXene Carbon Anode Lithium-ion batteries Sodium-ion batteries

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A lithium–tin fluoride anode enabled by ionic/electronic conductive paths for garnet-based solid-state lithium metal batteries

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Rare Metals 2024年第2期43卷 575-587页

作者： Lei Zhang Qian-Kun Meng Xiang-Ping Feng Ming Shen Yu-Qing Zhang Quan-Chao Zhuang run-guo Zheng Zhi-Yuan Wang Yan-Hua Cui Hong-Yu Sun Yan-guo Liu School of Materials Science and Engineering Northeastern UniversityShenyang110819China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao066004China School of Materials and Physics China University of Mining&TechnologyXuzhou221116China Institute of Electronic Engineering China Academy of Engineering PhysicsMianyang621900China

The high energy density and stability of solid-state lithium metal batteries(SSLMBs)have garnered great ***-type oxides,especially Li_(6.4)La_(3)Zr_(1.4)Ta_(0.6)O_(12)(LLZTO),with high ionic conductivity,wide electrochemical window,and stability to Li metal anode,are promising solid-state electrolyte(SSEs)materials for ***,Li/LLZTO interface issues including high interface resistance,inhomogeneous Li deposition,and Li dendrite growth have hindered the practical application of ***,a multi-functional Li–SnF_(2) composite anode with Li,LiF,and Li-Sn alloy was specifically designed and *** composite anode improves the wettability to LLZTO,constructing an intimate contact interface between it and ***,ionic/electronic conductive paths in situ formed at the interface can effectively uniform Li deposition and suppress Li *** solid-state symmetric cell exhibits low interface resistance(11Ω·cm^(2)) and high critical current density(1.3 mA·cm^(−2))at 25℃.The full SSLMB based on LiFePO_(4) or LiNi_(0.5)Co_(0.2)Mn_(0.3)O_(2) cathode also shows stable cycling performance and high rate *** work provides a new composite anode strategy for achieving high-energy density and high-safety SSLMBs.

关键词： Solid-state lithium metal batteries(SSLMBs) Lithium-tin fluoride anode Ionic/electronic conductive Interface resistance Lithium dendrite

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Evaluation of microRNA expression profiles in human sperm frozen using permeable cryoprotectant-free droplet vitrification and conventional methods

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Asian Journal of Andrology 2024年第4期26卷 366-376页

作者： Li-Xin Zhang Jing Mao Yan-Dong Zhou Guang-Yao Mao run-Fa guo Hong-Shan Ge Xia Chen Department of Histology and Embryology Medical SchoolNantong UniversityNantong 226001China Department of Reproductive Medicine The Affiliated Taizhou People’s Hospital of Nanjing Medical UniversityTaizhou School of Clinical MedicineNanjing Medical UniversityTaizhou 225300China.

For sperm cryopreservation,the conventional method,which requires glycerol,has been used for a long *** addition,the permeable cryoprotectant-free vitrification method has been continuously *** the differences of cryopreservation effects between the two methods have being studied,differences in microRNA(miRNA)profiles between them remain *** this study,we investigated the differences in miRNA expression profiles among conventional freezing sperm,droplet vitrification freezing sperm and fresh human *** also analyzed the differences between these methods in terms of differentially expressed miRNAs(DEmiRs)related to early embryonic development and paternal *** results showed no significant differences between the cryopreservation methods in terms of sperm motility ratio,plasma membrane integrity,DNA integrity,mitochondrial membrane potential,acrosome integrity,and ultrastructural ***,sperm miRNA-sequencing showed differences between the two methods in terms of the numbers of DEmiRs(28 and 19 with vitrification using a nonpermeable cryoprotectant and the conventional method,respectively)in postthaw and fresh sperm *** related to early embryonic development and paternal epigenetics mainly included common DEmiRs between the *** results showed that the differences between conventional freezing and droplet vitrification were minimal in terms of miRNA expression related to embryonic development and *** in sperm miRNA expression due to freezing are not always detrimental to embryonic *** study compared differences in miRNA expression profiles before and after cryopreservation between cryopreservation by conventional and vitrification *** offers a new perspective to evaluate various methods of sperm cryopreservation.

关键词： cryopreservation cryoprotectant-free vitrification early embryonic development paternal epigenetic inheritance sperm miRNAs sucrose

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Simultaneously Improved Curing,Mechanical,Antioxidative Properties and Reduced ZnO Loading of Silica Filled NR Composites by Incorporation of Low-cost Crude Carbon Dots via Conventional Melt-milling Method

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Chinese Journal of Polymer Science 2024年第6期42卷 815-825页

作者： Chao-Ying Sun Hai-Jun Ji Li-Wei Li Hui Yang Xiao-Peng An Yi-Ping Chen Ming-Jian Han Can Jiang Li-Qun Zhang Peng Yu run-guo Wang State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical TechnologyBeijing100029China School of Materials Science and Engineering Wuhan Institute of TechnologyWuhan430205China

Rubbers or elastomers play an important role in hi-tech technology and civilian daily life because of their unique and strategical ***,the rubber additives are essential components for rubbers’practical ***,developing novel multifunctional additives has attracted increasing research *** this work,low-cost crude carbon dots(CCDs)were used as multifunctional additives for natural rubber/silica system(without any additional modification)through industrial compatible melt-mixing *** results revealed that the CCDs could disperse well in the NR/silica system,and they could not only endow the rubber compound with excellent anti-aging capability due to CCDs’radical scavenging activity because of their plenty of nitrogen-containing species,but also improve the curing rate and mechanical performance of the rubber ***,the CCDs could reduce the rolling resistance of the rubber composites(tanδvalue at 7%strain of the rubber composite could be decreased by 34%),which is promising for the application of energy-saving tire ***,the addition of CCDs could effectively reduce the ZnO dosage by at least 40%in the rubber composite without deteriorating its ***,this work provides valuable guidance to develop novel cheap yet effective additives for the elastomer.

关键词： Natural rubber Crude carbon dots Antioxidant ZnO reduction Vulcanization

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Clinical intervention effect of Xuefu Zhuyu decoction on chronic heart failure complicated with depression

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World Journal of Psychiatry 2024年第6期14卷 857-865页

作者： Ying Wang Jun Wang Wang Lv Hu Chen Qian Yang Yang Zhang run guo Xiao-Li Ma Qian-Yu Zhang Department of Traditional Chinese Medicine Cangzhou Central HospitalCangzhou 061000Hebei ProvinceChina Department of Cardiology Cangzhou Central HospitalCangzhou 061000Hebei ProvinceChina

BACKGROUND The diagnosis and treatment of depression in patients with chronic heart failure(CHF)is challenging,with no ideal treatment at *** To analyze the clinical intervention effect of Xuefu Zhuyu decoction(XFZYD)on CHF complicated with *** The study cohort comprised 116 patients with CHF complicated with depression who received treatment from July 2020 to July 2023,of which 55 received Western medicine(control group)and 61 received XFZYD(research group).Data on clinical effectiveness,traditional Chinese medicine(TCM)syndrome score,cardiac function,negative emotions,and serum inflammatory factors,were collected for comparative *** Compared with the control group,the research group had an evidently higher total effective ***,there were marked reductions in TCM symptom score,left ventricular end-diastolic diameter,left ventricular end-systolic diameter,Self-Rating Depression Scale,Hamilton Depression Scale,high-sensitivity C-reactive protein,monocyte chemoattractant protein-1,and matrix metalloproteinase-9 in the research group after treatment,and these were lower than the corresponding values in the control *** ventricular ejection fraction was increased and higher in the research group compared with the control group after *** Our findings conclusively proved that XFZYD was considerably superior to Western medicine for treating CHF complicated with depression because it significantly alleviated patients’symptoms,improved cardiac function,relieved negative emotions,and reduced the levels of serum inflammatory factors.

关键词： Xuefu Zhuyu decoction Chronic heart failure Depression Cardiac function Negative emotions

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CAS-ESM2.0 Dataset for the Carbon Dioxide Removal Model Intercomparison Project(CDRMIP)

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Advances in Atmospheric Sciences 2024年第5期41卷 989-1000页

作者： Jiangbo JIN Duoying JI Xiao DONG Kece FEI run guo Juanxiong HE Yi YU Zhaoyang CHAI He ZHANG Dongling ZHANG Kangjun CHEN Qingcun ZENG International Center for Climate and Environment Sciences Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China State Key Laboratory of Satellite Ocean Environment Dynamics Second Institute of OceanographyMinistry of Natural ResourcesHangzhou 310012China State Key Laboratory of Earth Surface Processes and Resource Ecology College of Global Change and Earth System ScienceBeijing Normal UniversityBeijing 100875China State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China

Understanding the response of the Earth system to varying concentrations of carbon dioxide(CO_(2))is critical for projecting possible future climate change and for providing insight into mitigation and adaptation strategies in the near *** this study,we generate a dataset by conducting an experiment involving carbon dioxide removal(CDR)—a potential way to suppress global warming—using the Chinese Academy of Sciences Earth System Model version 2.0(CASESM2.0).A preliminary evaluation is *** model is integrated from 200–340 years as a 1%yr^(−1) CO_(2) concentration increase experiment,and then to~478 years as a carbon dioxide removal experiment until CO_(2) returns to its original ***,another 80 years is integrated in which CO_(2) is kept *** in the 2-m temperature,precipitation,sea surface temperature,ocean temperature,Atlantic meridional overturning circulation(AMOC),and sea surface height are all *** the ramp-up period,the global mean 2-m temperature and precipitation both increase while the AMOC *** of all the above variables change in the opposite direction in the ramp-down period,with a delayed peak relative to the CO_(2) *** CO_(2) returns to its original value,the global mean 2-m temperature is still~1 K higher than in the original state,and precipitation is~0.07 mm d^(–1) *** the end of the simulation,there is a~0.5°C increase in ocean temperature and a 1 Sv weakening of the *** model simulation produces similar results to those of comparable experiments previously reported in the literature.

关键词： CAS-ESM2.0 CDRMIP carbon dioxide removal AMOC temperature precipitation sea surface height

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引江济淮钢渡槽316L+Q345qD不锈钢复合板焊接接头过渡层厚度对焊接接头性能影响的研究

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价值工程 2024年第8期43卷 128-130页

作者：王润国中铁四局集团钢结构建筑有限公司合肥230031

本文所涉及不锈钢复合板均采用桥梁钢板上复不锈钢板的形式,板间设置不同过渡层,复合板最大厚度24mm。为研究过渡层厚度对复合钢板性能的影响,对复合板的焊接接头进行试验分析,试验结果表明,采用不同厚度过渡层的复合板焊接接头,力学性... 详细信息

本文所涉及不锈钢复合板均采用桥梁钢板上复不锈钢板的形式,板间设置不同过渡层,复合板最大厚度24mm。为研究过渡层厚度对复合钢板性能的影响,对复合板的焊接接头进行试验分析,试验结果表明,采用不同厚度过渡层的复合板焊接接头,力学性能满足标准要求,并且选用较小的过渡层厚度可以降低成分稀释现象,保证焊接质量。

关键词：不锈钢复合板过渡层力学性能

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企业—用户互动、敏捷开发与数字产品创新绩效

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研究与发展管理 2024年第1期36卷 108-120页

作者：郭润萍冯子晴龚蓉王远吉林大学商学与管理学院长春130012

数字技术的可重新编程性、开放性等特征增强了市场需求的不确定性,企业通过与用户互动进行敏捷开发以提升数字产品创新绩效,成为获取竞争优势的关键。基于精益创业理论和利益相关者理论,深入分析企业—用户互动、敏捷开发与数字产品创... 详细信息

数字技术的可重新编程性、开放性等特征增强了市场需求的不确定性,企业通过与用户互动进行敏捷开发以提升数字产品创新绩效,成为获取竞争优势的关键。基于精益创业理论和利益相关者理论,深入分析企业—用户互动、敏捷开发与数字产品创新绩效间的作用机理。结果表明:企业—用户互动通过敏捷开发积极影响数字产品创新绩效,且组织创新氛围将增强三者间的作用关系。研究有助于丰富对于数字情境下企业—用户互动创新的理解,推动敏捷开发研究的发展,为解释数字产品创新绩效差异化提供有价值的研究思路,也为数字产品创新绩效的提升提供重要的管理启示。

关键词：企业—用户互动敏捷开发数字产品创新绩效组织创新氛围利益相关者精益创业

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支气管镜介入治疗感染后闭塞性支气管炎1例

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中华儿科杂志 2024年第4期62卷 374-376页

作者：郭润翟嘉邹映雪王雪琳毕莹天津市儿童医院(天津大学儿童医院)马场院区呼吸科天津市儿童出生缺陷防治重点实验室天津300074

患儿女,9岁,主因“咳嗽伴间断发热37 d,乏力、气促10 d”于2023年4月在天津市儿童医院马场院区呼吸科住院治疗。患儿在入院前37 d患重症肺炎,病原学检查仅提示有乙型流感病毒感染。肺炎治疗好转后,在病程1个月时出现气促及呼吸困难,听... 详细信息

患儿女,9岁,主因“咳嗽伴间断发热37 d,乏力、气促10 d”于2023年4月在天津市儿童医院马场院区呼吸科住院治疗。患儿在入院前37 d患重症肺炎,病原学检查仅提示有乙型流感病毒感染。肺炎治疗好转后,在病程1个月时出现气促及呼吸困难,听诊右肺呼吸音降低,可闻及管状呼吸音。肺CT提示右肺完全不张,支气管镜检查可见右肺各段支气管闭塞,诊断右肺闭塞性支气管炎。经过多次支气管镜介入治疗后右肺复张,随访5个月预后良好。

关键词：支气管镜检查乙型流感病毒天津市儿童医院管状呼吸音肺呼吸音肺炎治疗右肺重症肺炎

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基于双自由度转台的全向空间单目视觉室内定位测量方法

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中国光学（中英文） 2024年第3期17卷 605-616页

作者：吴军王豪爽单腾飞郭润夏张晓瑜陈玖圣中国民航大学航空工程学院天津300300 中国民航大学电子信息与自动化学院天津300300

针对传统单目视觉测量系统测量视场有限的问题,本文提出一种基于双自由度旋转平台的全向空间单目视觉测量方法。首先,对双自由度旋转平台的转轴参数进行标定,用副相机拍摄固定在双自由度转台上的棋盘格标定板,提取棋盘格角点的位置坐标... 详细信息

针对传统单目视觉测量系统测量视场有限的问题,本文提出一种基于双自由度旋转平台的全向空间单目视觉测量方法。首先,对双自由度旋转平台的转轴参数进行标定,用副相机拍摄固定在双自由度转台上的棋盘格标定板,提取棋盘格角点的位置坐标,并将其转化到同一相机坐标系下。利用PCA(主成分分析)平面拟合得到初始位置转轴参数中的方向向量,使用空间最小二乘圆拟合方法得到初始位置下转轴参数中的位置参数。然后,通过转台转动的角度以及罗德里格斯公式将不同位置下相机获取的数据进行坐标系统一,实现水平和竖直方向全向空间下的目标测量。最后,通过高精度激光测距仪验证了本方法的测量精度,并通过与双目视觉测量系统、wMPS测量系统进行比对实验,验证了本方法的全向空间测量能力。实验结果表明,本方法测量精度基本达到双目视觉测量系统水平,但测量范围远大于双目视觉测量,可以满足全向空间测量要求。

关键词：双自由度转台单目视觉全向空间测量室内定位

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