检索结果-南通市图书馆

Quasi-Solid-State Composite Electrolytes with Multifunctional 2D Molecular Brush Fillers for Long-Cycling Lithium Metal Batteries

引用

Chinese Journal of Chemistry 2023年第21期41卷 2848-2854页

作者： Yin Cui Guofang Yu ruliang liu Dongtian Miao Dingcai Wu PCFM Lab School of ChemistrySun Yat-sen UniversityGuangzhouGuangdong510006 China School of Chemistry and Materials Science Guangdong University of EducationGuangzhouGuangdong510303 China

The ever-growing demand for next-generation high-energy-density devices drives the development of lithium metal batteries with enough safety and high performance,in which quasi-solid-state composite electrolytes(QSCEs)with high ionic conductivity and lithium ion transference number(urn:x-wiley:1001604X:media:cjoc202300232:cjoc202300232-math-0001)are highly desirable.Herein,we successfully synthesize a kind of two-dimensional(2D)molecular brush(GO-g-PFIL)via grafting poly(ionic liquid)side-chain(poly(3-(3,3,4,4,4-pentafluorobutyl)-1-vinyl-1H-imidazol-3-ium bis(trifluoromethanesulfonyl)imide),denoted as PFIL)on the surface of 2D graphene oxide(GO)sheet.GO-g-PFIL is used as multifunctional filler to prepare novel composite membranes and corresponding QSCEs(e.g.,QSCE-PH/GPFIL3/P).The as-obtained QSCE-PH/GPFIL3/P integrates features of PFIL side-chain-enhanced lithium ion conduction,poly(vinylidene fluoride-co-hexafluoropropene)backbone-induced flexibility,and GO-strengthened mechanical property.As a result,our ultrathin(21μm)self-supporting QSCE-PH/GPFIL3/P exhibits high ionic conductivity(3.24×10^(−4)S·cm^(−1))and excellent urn:x-wiley:1001604X:media:cjoc202300232:cjoc202300232-math-0002(0.82)at room temperature,and Li/LFP full cell with QSCE-PH/GPFIL3/P shows superior rate performance(high specific capacities of 79 mAh·g^(−1)at 30°C and 5 C)and excellent cycling performance(high capacity retention of 91%after 500 cycles at 80°C and 1 C).

关键词： Quasi-solid-state composite electrolyte I Filler 2D molecular brush Lithium metal battery Poly(ionic liquid)

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Centimeter-sized Cs_(3)Cu_(2)I_(5)single crystals grown by oleic acid assisted inverse temperature crystallization strategy and their films for high-quality X-ray imaging

引用

Journal of Energy Chemistry 2023年第4期79卷 382-389页

作者： Tao Chen Xin Li Yong Wang Feng Lin ruliang liu Wenhua Zhang Jie Yang Rongfei Wang Xiaoming Wen Bin Meng Xuhui Xu Chong Wang National Center for International Research on Photoelectric and Energy Materials School of Materials and EnergyYunnan UniversityKunming 650091YunnanChina College of Materials Science and Engineering Key Laboratory of Advanced Materials of Yunnan ProvinceKunming University of Science and TechnologyKunming 650093YunnanChina Centre for Translational Atomaterials Swinburne University of TechnologyHawthorn 3122Australia

Low-dimensional halide perovskites have become the most promising candidates for X-ray imaging,yet the issues of the poor chemical stability of hybrid halide perovskite,the high poisonousness of lead halides and the relatively low detectivity of the lead-free halide perovskites which seriously restrain its commercialization.Here,we developed a solution inverse temperature crystal growth(ITCG)method to bring-up high quality Cs_(3)Cu_(2)I_(5)crystals with large size of centimeter order,in which the oleic acid(OA)is introduced as an antioxidative ligand to inhibit the oxidation of cuprous ions effieiently,as well as to decelerate the crystallization rate remarkalby.Based on these fine crystals,the vapor deposition technique is empolyed to prepare high quality Cs_(3)Cu_(2)I_(5)films for efficient X-ray imaging.Smooth surface morphology,high light yields and short decay time endow the Cs_(3)Cu_(2)I_(5)films with strong radioluminescence,high resolution(12 lp/mm),low detection limits(53 nGyair/s)and desirable stability.Subsequently,the Cs_(3)Cu_(2)I_(5)films have been applied to the practical radiography which exhibit superior X-ray imaging performance.Our work provides a paradigm to fabricate nonpoisonous and chemically stable inorganic halide perovskite for X-ray imaging.

关键词： Inverse temperature crystal growth Cs_(3)Cu_(2)I_(5)single crystal Vapor deposition Cs_(3)Cu_(2)I_(5)films X-ray imaging

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

减氮对引黄灌区春玉米氮素吸收利用和淋失的影响

引用

农业资源与环境学报 2024年第3期41卷 576-584页

作者：王英刘汝亮王芳洪瑜冒辛平马建森宁夏农林科学院农业资源与环境研究所银川750002 国家农业环境银川观测实验站银川750002 宁夏大学农学院银川750002

为探究不同减氮水平下春玉米产量及氮素吸收利用和氮素淋失损失特征,为宁夏引黄灌区春玉米氮肥合理施用提供理论依据,本研究于2021—2022年在宁夏引黄灌区基于渗漏池进行了连续两年的田间定位试验,以先玉1225为供试玉米品种,设置了5个... 详细信息

为探究不同减氮水平下春玉米产量及氮素吸收利用和氮素淋失损失特征,为宁夏引黄灌区春玉米氮肥合理施用提供理论依据,本研究于2021—2022年在宁夏引黄灌区基于渗漏池进行了连续两年的田间定位试验,以先玉1225为供试玉米品种,设置了5个氮水平,施氮量分别为常规施氮420 kg·hm^(-2)(N-420)、减氮14.29%(N-360)、减氮35.71%(N-270)、减氮57.14%(N-180)、不施氮处理(CK),对春玉米产量、氮素吸收利用和氮素淋失损失量进行测定分析。两年数据均表明,农户常规施肥与减氮14.29%处理籽粒产量没有显著差异(P<0.05),减氮35.71%处理较常规施肥处理产量降低。2021年减氮35.71%、减氮14.29%处理较常规施肥处理籽粒产量分别降低了8.60%和3.59%,2022年减氮35.71%处理籽粒产量较常规施肥处理降低11.46%,而减氮14.29%处理与常规施肥处理相比籽粒产量增加1.42%。氮肥表观利用率、氮肥农学效率、地上部氮素收获指数两年数据均显示减氮35.71%处理高于减氮14.29%处理和常规施肥处理。氮肥偏生产力随着施氮量的增加逐渐降低,与减氮57.14%处理相比,减氮35.71%、减氮14.29%和常规施肥处理分别降低19.57%、33.81%、42.59%。总氮淋失量随施氮量的增加而升高,减氮35.71%、减氮14.29%处理总氮淋失损失量较常规施氮处理降低42.51%和18.09%。各处理氮素淋失中,硝态氮是主要形式,占总氮的45.50%~54.68%。相关性分析表明,施氮量与总氮淋失量呈正相关,随着施氮量的增加,总氮淋失量呈指数型增加(R2=0.9986)。研究表明,与常规施氮量相比,减少35.71%施氮量下,春玉米产量平均减少10.03%,总氮淋失量平均降低42.51%,氮肥表观利用率、农学效率和偏生产力均提高。综合考虑认为,施氮270 kg·hm^(-2)可作为协调引黄灌区春玉米产量和环境安全的合理选择。

关键词：春玉米引黄灌区减氮产量氮素淋失

来源：

维普期刊数据库

同方期刊数据库博看期刊评论

在线全文

学校读者我要写书评

暂无评论

开关寿命连续型的不同型部件冷贮备系统可靠度

引用

南昌大学学报（理科版） 2023年第1期47卷 10-15,20页

作者：杨顺令董秋仙刘君刘汝良南昌大学数学与计算机学院江西南昌330031

为了讨论开关寿命连续型的不同型多部件冷贮备不可修系统的可靠度,假设系统由1个部件和n-1个冷贮备部件组成,转换开关寿命和部件的工作寿命都服从指数分布、所有随机变量均相互独立。首先根据两部件、三部件、四部件冷贮备系统可靠度以... 详细信息

为了讨论开关寿命连续型的不同型多部件冷贮备不可修系统的可靠度,假设系统由1个部件和n-1个冷贮备部件组成,转换开关寿命和部件的工作寿命都服从指数分布、所有随机变量均相互独立。首先根据两部件、三部件、四部件冷贮备系统可靠度以及冷贮备系统可靠度的定义推导了多部件开关寿命指数型的冷贮备系统可靠度关于部件个数的递推关系式,从而得出该系统可靠度的理论表达式,最后从开关完全可靠的多部件冷贮备系统这方面来实例验证该系统可靠度函数的正确性。

关键词：多部件冷贮备可靠度指数分布

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Effectiveness and safety of acupuncture in treatment of pregnancyrelated symptoms:a systematic review and Meta-analysis

引用

Journal of Traditional Chinese Medicine 2024年第1期44卷 16-26页

作者： liu Tingting liu Tongou liu Mingfu School of Traditional Chinese Medicine Clinical Medicine Hubei University of Traditional Chinese MedicineWuhan 430000China First Clinical College of Hubei University of Traditional Chinese Medicine Wuhan 430000China Department of Acupuncture and Tuina Affiliated Hospital of Hubei University of Traditional Chinese MedicineHubei Provincial Hospital of Traditional Chinese MedicineWuhan 430000China

OBJECTIVE:To systematically evaluate the efficacy and safety of acupuncture(AM)in the treatment of pregnancyrelated symptoms such as acute vomiting during pregnancy.METHODS:We comprehensively searched the available literature up to November 2021,including Pub Med,Embase,Cochrane Library,Chinese Biomedical Literature Database,and China National Knowledge Infrastructure Database,for randomized controlled trials(RCTs)on AM for the treatment of severe vomiting,insomnia,pharyngeal and pelvic pain,mood abnormalities,and dyspepsia during pregnancy.RESULTS:Sixteen RCTs with a cumulative sample size of 1178 cases were included.Of these,964 patients were included in the Meta-analysis.The Meta-analysis results showed that AM was more efficient than Western medicine in treating discomfort during pregnancy[odds ratio(OR)=1.19,95%confidence interval(CI)(1.11,1.28),P<0.01].AM was better than the control group in improving the visual analog scale scores[standard mean difference(SMD)=0.62,95%CI(0.53,0.71),P<0.01].AM was superior to the control group in improving Numerical Rating Scale(NRS)symptom scores[OR=7.31,95%CI(3.36,15.94),P<0.01].There was no significant difference in adverse effects between the AM and sham-AM groups and the analgesic drug group[OR=0.70,95%CI(0.39,1.28),P=0.25],but the treatment and control groups had mild adverse effects with a low incidence.CONCLUSIONS:AM is more effective than other treatments or pharmacotherapy alone in the treatment of pregnancy-related symptoms,and is relatively safe.However,the quality of the included trials was rather poor,and high-quality studies are required to confirm our findings.

关键词： acupuncture pregnancy nausea vomiting sleep initiation and maintenance disorders low back pain pelvic pain mood abnormalities Meta-analysis systematic review

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Removal of Cr(Ⅵ)by glutaraldehyde-crosslinked chitosan encapsulating microscale zero-valent iron:Synthesis,mechanism,and longevity

引用

Journal of Environmental Sciences 2024年第8期142卷 115-128页

作者： Yijun Duan Fang liu Xiang liu Miao Li School of Environment Tsinghua UniversityBeijing 100084China Transportation Institute of Inner Mongolia University Hohhot 010070China

Microscale zero-valent iron(mZVI)has shown great potential for groundwater Cr(Ⅵ)remediation.However,low Cr(Ⅵ)removal capacity caused by passivation restricted the wide use of mZVI.We prepared mZVI/GCS by encapsulating mZVI in a porous glutaraldehydecrosslinked chitosan matrix,and the formation of the passivation layer was alleviated by reducing the contact between zero-valent iron particles.The average pore diameter of mZVI/GCS was 8.775 nm,which confirmed the mesoporous characteristic of this material.Results of batch experiments demonstrated that mZVI/GCS exhibited high Cr(Ⅵ)removal efficiency in a wide range of pH(2-10)and temperature(5-35℃).Common groundwater coexisting ions slightly affected m ZVI/GCS.The material showed great reusability,and the average Cr(Ⅵ)removal efficiency was 90.41%during eight cycles.In this study,we also conducted kinetics and isotherms analysis.Pseudo-second-order model was the most matched kinetics model.The Cr(Ⅵ)adsorption process was fitted by both Langmuir and Freundlich isotherms models,and the maximum Langmuir adsorption capacity of m ZVI/GCS reached243.63 mg/g,which is higher than the adsorption capacities of materials reported in most of the previous studies.Notably,the column capacity for Cr(Ⅵ)removal of a mZVI/GCS-packed column was 6.4 times higher than that of a mZVI-packed column in a 50-day experiment.Therefore,mZVI/GCS with a porous structure effectively relieved passivation problems of mZVI and showed practical application prospects as groundwater Cr(Ⅵ)remediation material with practical application prospects.

关键词： Chitosan Glutaraldehyde mZVI Cr(Ⅵ) Groundwater

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Frequency Regulation of VSC-MTDC System with Offshore Wind Farms

引用

Journal of Modern Power Systems and Clean Energy 2024年第1期12卷 275-286页

作者： Haoyu liu Chongru liu North China Electric Power University Beijing 102206China

Frequency regulation of voltage source converter-based multi-terminal high-voltage direct current(VSC-MTDC)system with offshore wind farms enhances the frequency stability by compensating the power for a disturbed AC system.However,it is difficult to reasonably allocate frequency-regulation resources due to a lack of coordination mechanisms between wind farms and the MTDC system.Moreover,it is difficult for the frequency control of the wind farms to manage changes in wind speed;and the risk of wind-turbine stalls is high.Thus,based on the kinetic energy of wind turbines and the power margin of the converters,the frequency-regulation capability of wind turbines is evaluated,and a dynamic frequency-support scheme considering the real-time frequency-support capability of the wind turbines and system frequency evolution is proposed to improve the frequency-support performance.A power adaptation technique at variable wind speeds is developed;the active power in the frequency-support stage and restoration stage is switched according to the wind speed.A hierarchical zoning frequency-regulation scheme is designed to use the frequency-regulation resources of different links in the MTDC system with wind farms.The simulation results show that the novel frequency-regulation strategy maintains frequency stability with wind-speed changes and avoids multiple frequency dips.

关键词： Wind generation voltage source converter-based multi-terminal high-voltage direct current(VSC-MTDC) frequency regulation cooperative control adaptive control variable wind speed

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Characteristics and sources of peroxyacetyl nitrate(PAN)in the rural North China Plain:Results from1-year continuous observations

引用

Journal of Environmental Sciences 2024年第4期138卷 719-731页

作者： Xin liu Xiaowei He Chenglong Zhang Yifei Song Shuyang Xie Chengtang liu Pengfei liu Yuanyuan Zhang Yujing Mu Junfeng liu Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

Peroxyacetyl nitrate(PAN)is an important photochemical pollutant in the troposphere,whereas long-term measurements are scarce in rural areas in North China Plain(NCP),resulting in unclear seasonal variations and sources of PAN in rural NCP.In this study,we conducted a 1-year observation of PAN during 2021-2022 at the rural NCP site.The average concentrations of PAN were 1.10,0.75,0.65,and 0.88 ppbv in spring,summer,autumn,and winter,respectively,with a 1-year average of 0.81±0.60 ppbv.Calculations indicate that the loss of PAN through thermal decomposition in summer accounts for 43.2% of the total formed PAN,which is an important reason for the low concentration of PAN in summer.We speculate that since the correlation between PAN and O_(3) in winter is significantly lower than that in other seasons,the observed regional transport of PAN cannot be ignored in winter.Through budget analysis,regional transport accounted for 12.8% and 55.9% of the observed PAN on the spring and winter pollution days,respectively,which showed that regional transport played key roles during the photochemical pollution of the rural NCP in winter.The potential source contribution function revealed that the transported PAN mainly comes from southern Hebei in spring.In winter,the transported PAN was mainly from Langfang,Hengshui,and southern Beijing.Our findings may aid in understanding PAN variations in different seasons in rural areas and highlight the impact of regional transport on the PAN budget.

关键词： Photochemical pollution Peroxyacetyl nitrate(PAN) Seasonal variations Regional transport Rural area

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

High-performance,stable CoNi LDH@Ni foam composite membrane with innovative peroxymonosulfate activation for 2,4-dichlorophenol destruction

引用

Journal of Environmental Sciences 2024年第7期141卷 235-248页

作者： Yu liu Weibao liu Xinrui Gan Jiangwei Shang Xiuwen Cheng College of Chemistry and Environmental Science Xinjiang Laboratory of Phase Transitions and Microstructures of Condensed Matter PhysicsYili Normal UniversityYining 835000China Key Laboratory for Environmental Pollution Prediction and Control Gansu ProvinceCollege of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China

In this study,the cobalt-nickel layered double hydroxides(CoNi LDH)were synthesized with a variety of Co/Ni mass ratio,as CoxNiyLDHs.In comparison,Co1Ni3LDH presented the best peroxymonosulfate(PMS)activation efficiency for 2,4-dichlorophenol removal.Meanwhile,CoNi LDH@Nickel foam(CoNi LDH@NF)composite membrane was constructed for enhancing the stability of catalytic performance.Herein,CoNi LDH@NF-PMS system exerted high degradation efficiency of 99.22%within 90 min for 2,4-DCP when[PMS]_(0)=0.4 g/L,Co^(1)Ni^(3)LDH@NF=2 cm×2 cm(0.2 g/L),reaction temperature=298 K.For the surface morphology and structure of the catalyst,it was demonstrated that the CoNi LDH@NF composite membrane possessed abundant cavity structure,good specific surface area and sufficient active sites.Importantly,·OH,SO_(4)·^(-)and^(1)O_(2)played the primary role in the CoNi LDH@NF-PMS system for 2,4-DCP decomposition,which revealed the PMS activation mechanism in CoNi LDH@NF-PMS system.Hence,this study eliminated the stability and adaptability of CoNi LDH@NF composite membrane,proposing a new theoretical basis of PMS heterogeneous catalysts selection.

关键词： CoNi LDH@NF composite membrane Peroxymonosulfate 2,4-dichlorophenol Reactive radicals

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

不同型多部件温贮备系统可靠度计算的算法实现

引用

南昌大学学报（理科版） 2023年第6期47卷 530-536,542页

作者：杨顺令董秋仙占志文刘君刘汝良南昌大学数学与计算机学院江西南昌330031

针对多部件温贮备系统,随着部件数的增加,可靠度难以精确求解的问题,本文采用算法研究n部件温贮备系统的可靠度的计算。假设系统由1个部件和n-1个温贮备部件组成,转换开关完全可靠,各部件的工作寿命和贮备寿命都服从指数分布、所有随机... 详细信息

针对多部件温贮备系统,随着部件数的增加,可靠度难以精确求解的问题,本文采用算法研究n部件温贮备系统的可靠度的计算。假设系统由1个部件和n-1个温贮备部件组成,转换开关完全可靠,各部件的工作寿命和贮备寿命都服从指数分布、所有随机变量均相互独立。首先求出两部件、三部件、四部件可靠度的解析式,然后研究可靠度解析式的项数和系数的规律性,运用算法得出n部件温贮备系统的可靠度,最后从少部件温贮备系统、多部件冷贮备系统和同型多部件温贮备系统三方面实例验证算法的正确性。

关键词：多部件温贮备可靠度指数分布

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：