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Tailoring electron vortex beams with customizable intensity patterns by electron diffraction holography

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Opto-Electronic Advances 2024年第2期7卷 14-21页

作者： Pengcheng Huo ruixuan Yu Mingze Liu Hui Zhang Yan-qing Lu Ting Xu National Laboratory of Solid-State Microstructures and Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China College of Engineering and Applied Sciences Key Laboratory of Intelligent Optical Sensing and Manipulation and Jiangsu Key Laboratory of Artificial Functional MaterialsNanjing UniversityNanjing 210093China

An electron vortex beam(EVB) carrying orbital angular momentum(OAM) plays a key role in a series of fundamental scientific researches, such as chiral energy-loss spectroscopy and magnetic dichroism spectroscopy. So far, almost all the experimentally created EVBs manifest isotropic doughnut intensity patterns. Here, based on the correlation between local divergence angle of electron beam and phase gradient along azimuthal direction, we show that free electrons can be tailored to EVBs with customizable intensity patterns independent of the carried OAM. As proof-of-concept, by using computer generated hologram and designing phase masks to shape the incident free electrons in the transmission electron microscope, three structured EVBs carrying identical OAM are tailored to exhibit completely different intensity patterns. Furthermore, through the modal decomposition, we quantitatively investigate their OAM spectral distributions and reveal that structured EVBs present a superposition of a series of different eigenstates induced by the locally varied geometries. These results not only generalize the concept of EVB, but also demonstrate an extra highly controllable degree of freedom for electron beam manipulation in addition to OAM.

关键词： electron vortex beam orbital angular momentum diffraction holography

A Low-carbon Operation Optimization Method of ETG-RIES Based on Adaptive Optimization Spiking Neural P Systems

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Protection and Control of Modern Power Systems 2024年第5期9卷 162-177页

作者： Tao Wang Zhu Huang ruixuan Ying Luis Valencia-Cabrera School of Electrical Engineering and Electronic Information Xihua UniversityChengdu 610039China the Xiluodu Hydropower Plant China Yangtze Power Co.Ltd.Zhaotong 657300China the Institute of Multidisciplnary Research for Ad-vanced Materials Tohoku UniversitySendai 980-8577Japan Department of Computer Science and Artificial Intelligence University of SevilleAvda.Reina Mercedes s/n 41012Spain

To enhance multi-energy complementarity and foster a low carbon economy of energy resources,this paper proposes an innovative low-carbon operation opti-mization method for electric-thermal-gas regional inte-grated energy *** bolster the low-carbon operation capabilities of such systems,a coordinated operation framework is presented that integrates carbon capture devices,power to gas equipment,combined heat and power units,and a multi-energy storage *** address the challenge of high-dimensional constraint imbalance in the optimization process,a novel low-carbon operation opti-mization method is then *** new method is based on an adaptive single-objective continuous optimiza-tion spiking neural P system,specifically designed for this ***,simulation models of four typical schemes are established and employed to test and analyze the economy and carbon environmental pollution degree of the proposed system model,as well as the performance of the operation optimization ***,simulation results show that the proposed method not only considers the economic viability of the target integrated energy sys-tem,but also significantly improves the wind power utili-zation and carbon reduction *** Terms—Spiking neural P system,power-to-gas,membrane computing,regional integrated energy system,low-carbon operation optimization.

关键词： Spiking neural P system power-to-gas membrane computing regional integrated energy system low-carbon operation optimization

Supported Atomically Dispersed Pd Catalyzed Direct Alkoxylation and Allylic Alkylation

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Chinese Journal of Chemistry 2024年第7期42卷 719-724页

作者： ruixuan Qin Ziwen Chen Qingyuan Wu Nanfeng Zheng Pengxin Liu New Cornerstone Science Laboratory State Key Laboratory for Physical Chemistry of Solid SurfacesCollaborative Innovation Center of Chemistry for Energy Materialsand National&Local Joint Engineering Research Center of Preparation Technology of NanomaterialsCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamenFujian 361005China Innovation Laboratry for Scences and Technoogies of Energy Materials of Fujan Province(IKKM) Xiamen Fujian 361102China School of Physical Science and Technology Shanghai Tech UniversityShanghai 201210China Fujian Key Laboratory of Rare-earth Functional Materials Fujian Shanhai Collaborative Innovation Center of Rare-earth Functional MaterialsLongyanFujian 366300China

A new approach to allylic alkylation is realized using an atomically dispersed palladium catalyst(Pd1.TiO2-EG).Unlike conventional methods that require derivation of substrates and utilization of additives,this method allows for direct allylic alkylation from allylic alcohols,producing H2O as the sole *** catalyst's high efficiency is attributed to the local hydrogen bonding at the or-ganic-inorganic interface(Pd-EG interface),facilitating hydroxyl group activation forη3π-allyl complex *** system demonstrates successful direct C—O and C—C coupling reactions with high selectivity,requiring no *** study highlights the potential of supported atomically dispersed catalysts for greener and more efficient catalysis,meanwhile,offers unique insights into the distinct behavior of atomically dispersed catalysts in comparison to homogeneous or nanoparticle-based catalysts.

关键词： Atomically dispersed catalyst Alkylation C—C coupling Organic-inorganic Interface Hydrogen bond Tsuji-Trost reaction Green catalysis

Entangled photon pair generation in an integrated SiC platform

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Light(Science & Applications) 2024年第6期13卷 1041-1046页

作者： Anouar Rahmouni ruixuan Wang Jingwei Li Xiao Tang Thomas Gerrits Oliver Slattery Qing Li Lijun Ma National Institute of Standards and Technology 100 Bureau DrGaithersburgMD20899USA Department of Electrical and Computer Engineering Carnegie Mellon UniversityPittsburghPA15213USA

Entanglement plays a vital role in quantum information *** to its unique material properties,silicon carbide recently emerged as a promising candidate for the scalable implementation of advanced quantum information processing *** date,however,only entanglement of nuclear spins has been reported in silicon carbide,while an entangled photon source,whether it is based on bulk or chip-scale technologies,has remained ***,we report the demonstration of an entangled photon source in an integrated silicon carbide platform for the first ***,strongly correlated photon pairs are efficiently generated at the telecom C-band wavelength through implementing spontaneous four-wave mixing in a compact microring resonator in the 4H-silicon-carbide-on-insulator *** maximum coincidence-to-accidental ratio exceeds 600 at a pump power of 0.1. mW,corresponding to a pair generation rate of(9±1.×1.^(3) pairs/***-time entanglement is created and verified for such signal-idler photon pairs,with the two-photon interference fringes exhibiting a visibility larger than 99%.The heralded single-photon properties are also measured,with the heralded g^((2))(0)on the order of 1.^(−3),demonstrating the SiC platform as a prospective fully integrated,complementary metal-oxide-semiconductor compatible single-photon source for quantum applications.

关键词： quantum coincidence mixing

Relationship between the unique microstructures and behaviors of high-entropy alloys

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International Journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1350-1363页

作者： Yaqi Wu Peter KLiaw ruixuan Li Weiran Zhang Guihong Geng Xuehui Yan Guiqun Liu Yong Zhang State Key Laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing 100083China Department of Materials Science and Engineering The University of TennesseeKnoxvilleTN 37996USA Xi’an Rare Metal Materials Institute Co.Ltd. Xi’an 710016China School of Materials Science and Engineering North Minzu UniversityYinchuan 750030China GRIMAT Engineering Institute Co. Ltd.Beijing 101407China

High-entropy alloys(HEAs),which were introduced as a pioneering concept in 2004,have captured the keen interest of nu-merous ***,in this context,can be perceived as representing disorder and *** contrast,elemental composi-tions within alloy systems occupy specific structural sites in space,a concept referred to as *** accordance with Shannon entropy,structure is analogous to ***,the arrangement of atoms within a material,termed its structure,plays a pivotal role in dictating its *** addition to expanding the array of options for alloy composites,HEAs afford ample opportunities for diverse structural *** profound influence of distinct structural features on the exceptional behaviors of alloys is underscored by numer-ous *** features include remarkably high fracture strength with excellent ductility,antiballistic capability,exceptional radi-ation resistance,and corrosion *** this paper,we delve into various unique material structures and properties while elucidating the intricate relationship between structure and performance.

关键词： high-entropy alloys unique microstructure special properties alloy design

Interfacial oxidized Pd species dominate catalytic hydrogenation of polar unsaturated bonds

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Nano Research 2024年第1期17卷 228-234页

作者： Pengyao You Shaoqi Zhan Pengpeng Ruan ruixuan Qin Shiguang Mo Yazhou Zhang Kunlong Liu Lansun Zheng Nanfeng Zheng State Key Laboratory for Physical Chemistry of Solid Surfaces Collaborative Innovation Center of Chemistry for Energy Materialsand Department of ChemistryCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Department of Chemistry BMCUppsala UniversityBMC Box 576Uppsala S-75123Sweden Department of Chemistry University of OxfordOxford OX13QZUK

The determination of catalytically active sites is crucial for the design of efficient and stable catalysts toward desired ***,the complexity of supported noble metal catalysts has led to controversy over the locations of catalytically active sites(e.g.,metal,support,and metal/support interface).Here we develop a structurally controllable catalyst system(Pd/SBA-1.)to reveal the catalytic active sites for the selective hydrogenation of ketones to alcohol using acetophenone hydrogenation as model *** investigations demonstrated that unsupported Pd nanocrystals have no catalytic activity for acetophenone ***,oxidized Pd species were catalytically highly active for acetophenone *** catalytic activity decreased with the decreased oxidation state of *** work provides insights into the hydrogenation mechanism of ketones but also other unsaturated compounds containing polar bonds,e.g.,nitrobenzene,N-benzylidene-benzylamine,and carbon dioxide.

关键词： oxidized Pd metal/oxide interface constant particle size Pd/SBA-1. acetophenone hydrogenation

Dietary L-proline supplementation ameliorates autism-like behaviors and modulates gut microbiota in the valproic acid-induced mouse model of autism spectrum disorder

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Food Science and Human Wellness 2024年第5期13卷 2889-2905页

作者： Jingjing Fang ruixuan Geng Seong-Gook Kang Kunlun Huang Tao Tong Key Laboratory of Precision Nutrition and Food Quality Key Laboratory of Functional DairyMinistry of EducationCollege of Food Science and Nutritional EngineeringChina Agricultural UniversityBeijing 100083China Department of Food Engineering and Solar Salt Research Center Mokpo National UniversityMuangun 58554Korea Key Laboratory of Safety Assessment of Genetically Modified Organism(Food Safety) Ministry of AgricultureBeijing 100083China Beijing Laboratory for Food Quality and Safety Beijing 100083China

The effective intervention strategy for autism spectrum disorder(ASD)are currently ***,we attempted to evaluate the potential of L-proline(Pro),a multifunctional amino acid,in ameliorating autismlike behaviors and clarify the molecular mechanisms involved by using the typical valproic acid(VPA)-induced mouse model of *** significantly attenuates repetitive behaviors and social dysfunction in ASD *** correlation analysis revealed that the beneficial effects of Pro on autism-like behaviors are related to the modulation of gut microbiota structure and *** histological analysis revealed that Pro could reverse the decrease of Nissl-positive cells in the prefrontal cortex(PFC)induced by VPA *** sequencing demonstrated that Pro can also alter the PFC transcriptomic profile distinguished by the regulation of genes involved in Parkinson disease,neuroactive ligand-receptor interaction,oxidative phosphorylation,and mitogen activated protein kinase signaling ***,dietary Pro supplementation may be a promising intervention strategy for ASD.

关键词： L-Proline Autism spectrum disorder Gut microbiota Prefrontal cortex Behavior

Light field depth estimation:A comprehensive survey from principles to future

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High-Confidence Computing 2024年第1期4卷 92-107页

作者： Tun Wang Hao Sheng Rongshan Chen Da Yang Zhenglong Cui Sizhe Wang ruixuan Cong Mingyuan Zhao State Key Laboratory of Virtual Reality Technology and Systems School of Computer Science and EngineeringBeihang UniversityBeijing 100191China Zhongfa Aviation Institute Beihang UniversityHangzhou 311115China Faculty of Applied Sciences Macao Polytechnic UniversityMacao 999078China State Key Laboratory of Software Development Environment School of Computer Science and EngineeringBeihang UniversityBeijing 100191China

Light Field(LF)depth estimation is an important research direction in the area of computer vision and computational photography,which aims to infer the depth information of different objects in threedimensional scenes by capturing LF *** this new era of significance,this article introduces a survey of the key concepts,methods,novel applications,and future trends in this *** summarize the LF depth estimation methods,which are usually based on the interaction of radiance from rays in all directions of the LF data,such as epipolar-plane,multi-view geometry,focal stack,and deep *** analyze the many challenges facing each of these approaches,including complex algorithms,large amounts of computation,and speed *** addition,this survey summarizes most of the currently available methods,conducts some comparative experiments,discusses the results,and investigates the novel directions in LF depth estimation.

关键词： Light field Depth estimation Deep learning Sub-aperture image Epipolar-plane image

SARS-CoV-2 infection in animals: Patterns, transmission routes, and drivers

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Eco-Environment & Health 2024年第1期3卷 45-54页

作者： Ruying Fang Xin Yang Yiyang Guo Bingjie Peng ruixuan Dong Sen Li Shunqing Xu School of Environmental Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China School of Life Sciences Hainan UniversityHaikou 570228China

The severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)is more widespread in animals than previously thought,and it may be able to infect a wider range of domestic and wild *** effectively control the spread of the virus and protect animal health,it is crucial to understand the cross-species transmission mechanisms and risk factors of *** article collects published literature on SARS-CoV-2 in animals and examines the distribution,transmission routes,biophysical,and anthropogenic drivers of infected *** reported cases of infection in animals are mainly concentrated in South America,North America,and Europe,and species affected include lions,white-tailed deer,pangolins,minks,and *** factors influencing infection of animals with SARS-CoV-2 include environmental determinants,high-risk landscapes,air quality,and susceptibility of different animal species,while anthropogenic factors comprise human behavior,intensive livestock farming,animal markets,and land *** to current research gaps and surveillance capacity shortcomings,future mitigation strategies need to be designed from a One Health perspective,with research focused on key regions with significant data gaps in Asia and Africa to understand the drivers,pathways,and spatiotemporal dynamics of interspecies transmission.

关键词： SARS-CoV-2 Biophysical factors Anthropogenic factors Transmission Cross-species