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Exploring the characteristics of microbial community and enzyme activity in the aged refuse landfill environment of Taiyuan, China

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Pedosphere 2024年第5期34卷 879-891页

作者： fen hou Junjie DU Yuzhou MENG Xihui WU Department of Land Resource Management School of Public Administration Shanxi University of Finance and Economics College of Life Science Shanxi Engineering Research Center of Microbial Application Technologies Shanxi Normal University

Municipal solid waste landfill is the main disposal option for domestic garbage, in which microbial activities play an important role. However, despite the widespread practice of landfilling, the metagenomic microbial profiles of landfill sites remain poorly characterized. In this study, we used a combination of physicochemical analysis, ultraviolet-visible spectrophotometry, and high-throughput Illumina shotgun sequencing to systematically investigate the changes in soil enzyme activities, microbial community structure, and functional attributes in aged refuse collected from the Xingou Municipal Solid Waste Landfill in Taiyuan, China, with ordinary topsoil from an area within 5 km of the landfill as control soil. Except for neutral phosphatase (P=0.065), the activities of urease, laccase, dehydrogenase, sucrase, neutral protease, and β-glucosidase were all significantly reduced (P <0.05) in the aged refuse compared with the control soil. Contrastingly, catalase activity was found to be significantly elevated in the aged refuse. Compared with the control soil, aged refuse was characterized by higher richness and diversity of microbial communities, as reflected by the higher values of community richness estimators (Chao 1 and ACE) and diversity indices (Shannon and Simpson). In total, 186 phyla, 4 354 genera, and 34 459 species were identified, with 132 phyla, 1 914 genera, and7 369 species showing significantly different abundances between the aged refuse and the control soil. Actinobacteria and Acidobacteria were identified as the dominant phyla in the control soil, whereas Proteobacteria, Euryarchaeota (archaea), and Firmicutes were found to predominate in the aged ***, Euryarchaeota and Methanoculleus were the major taxa detected in the aged refuse, but were almost completely absent in the control soil. Xenobiotic biodegradation and bacterial chemotaxis were the main functions of the microflora in the aged refuse, whereas the carbohydrate, amino acid,

关键词： functional attribute metabolism pathway municipal solid waste landfill resource utilization soil microflora

Embedded Majorana islands

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Science China(Physics,Mechanics & Astronomy) 2024年第9期67卷 154-164页

作者： Jin-Xing hou Alex Weststrom rui Wang Wen-Li Yang Jian Li Institute of Modern Physics Northwest UniversityXi’an 710127China Department of Physics School of ScienceWestlake UniversityHangzhou 310030China Shaanxi Key Laboratory for Theoretical Physics Frontiers Xi’an 710127China Institute of Natural Sciences Westlake Institute for Advanced StudyHangzhou 310024China National Laboratory of Solid State Microstructures and Department of Physics Nanjing UniversityNanjing 210093China Collaborative Innovation Center for Advanced Microstructures Nanjing 210093China Peng Huanwu Center for Fundamental Theory Xi’an 710127China

Mesoscopic superconducting islands hosting Majorana zero modes(MZMs),or Majorana islands in short,offer a prototype of topological *** this work we investigate theoretically the model of a generic Majorana island tunneling-coupled to a singlepiece metallic substrate,hence an embedded Majorana *** show the crucial consequences of an interplay between the topological ground states nonlocally addressed by the MZMs and the metallic bath with coherent electron propagation:on the one hand,the topological degeneracy on the Majorana island can be preserved,by virtue of the particle-hole symmetry,despite the apparent bath-induced coupling between MZMs;on the other hand,the electronic interference in the metallic bath may lead to profound alterations to the renormalization group behavior of the hybrid system towards low energy/temperature compared with conventional Kondo *** work serves to establish the model of embedded Majorana islands as an experimentally relevant and theoretically intriguing problem particularly in the direction of topological quantum computation.

关键词： topological quantum computation Majorana zero modes topological qubit mesoscopic superconductor topological Kondo effect

A real-time intelligent lithology identification method based on a dynamic felling strategy weighted random forest algorithm

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Petroleum Science 2024年第2期21卷 1135-1148页

作者： Tie Yan rui Xu Shi-Hui Sun Zhao-Kai hou Jin-Yu feng School of Petroleum Engineering Northeast Petroleum UniversityDaqing163318HeilongjiangChina Sanya Offshore Oil&Gas Research Institute Northeast Petroleum UniversitySanya572025HainanChina

Real-time intelligent lithology identification while drilling is vital to realizing downhole closed-loop drilling. The complex and changeable geological environment in the drilling makes lithology identification face many challenges. This paper studies the problems of difficult feature information extraction,low precision of thin-layer identification and limited applicability of the model in intelligent lithologic identification. The author tries to improve the comprehensive performance of the lithology identification model from three aspects: data feature extraction, class balance, and model design. A new real-time intelligent lithology identification model of dynamic felling strategy weighted random forest algorithm(DFW-RF) is proposed. According to the feature selection results, gamma ray and 2 MHz phase resistivity are the logging while drilling(LWD) parameters that significantly influence lithology identification. The comprehensive performance of the DFW-RF lithology identification model has been verified in the application of 3 wells in different areas. By comparing the prediction results of five typical lithology identification algorithms, the DFW-RF model has a higher lithology identification accuracy rate and F1 score. This model improves the identification accuracy of thin-layer lithology and is effective and feasible in different geological environments. The DFW-RF model plays a truly efficient role in the realtime intelligent identification of lithologic information in closed-loop drilling and has greater applicability, which is worthy of being widely used in logging interpretation.

关键词： Intelligent drilling Closed-loop drilling Lithology identification Random forest algorithm Feature extraction

Further study on the genesis of lamellar calcite veins in lacustrine black shale--A case study of Paleogene in Dongying Depression, China

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Petroleum Science 2024年第3期21卷 1508-1523页

作者： Guan-Min Wang Yun-Jiao Zhang Zi-Yuan Yin rui Zhu Zhi-Yao hou Yu Bai School of Geosciences China University of Petroleum(East China)Qingdao266580ShandongChina

Lamellar calcite veins are prevalent in carbonate-rich,lacustrine dark *** formation mechanisms of these veins have been extensively debated,focusing on factors such as timing,depth,material source,and driving *** paper examines dark lacustrine shale lamellar calcite veins in the Paleogene strata of Dongying Depression,using various analytical techniques:petrography,isotope geochemistry,cathodoluminescence,inclusion thermometry,and electron probe *** distinct types of calcite veins have been identified:granular calcite veins and sparry calcite *** two types differ significantly in color,grain structure,morphology,and *** further investigation,it was observed that vein generation occurred from the shallow burial period to the maturation of organic matter,with a transition from granular calcite veins to sparry calcite *** granular calcite veins exhibit characteristics associated with the shallow burial period,including plastically deformed laminae and veins,the development of strawberry pyrite,the absence of oil and gas,weak fractionation in oxygen isotopes,and their contact relationship with sparry calcite *** granular calcite veins were likely influenced by the reduction of sulfate *** the other hand,sparry calcite veins with fibrous grains are antitaxial and closely linked to the evolution and maturation of organic *** contain oil and gas inclusions and show a distribution range of homogenization temperature between 90℃ and 120℃ and strong fractionation in oxygen isotopes,indicating formation during the hydrocarbon expulsion *** carbon isotope analysis of the surrounding rocks and veins suggests that the material for vein formation originates from the shale itself,specifically authigenic micritic calcite modified by the action of *** opening of horizontal fractures and vein formation is likely driven by fluid overpressure resulting from undercompaction and hydrocarb

关键词： Calcite veins Shale diagenesis Material source Formation period Formation mechanism

Recent Advances in the Electrochemical Defluorinative Transformations of C-F Bonds

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Chinese Journal of Chemistry 2024年第16期42卷 1913-1928页

作者： Qinhui Wan rui-Xue Liu Zhongyi Zhang Xia-Die Wu Zhong-Wei hou Lei Wang Advanced Research Institute and Schoolof Pharmaceutical Sciences Taizhou UniversityJiaojiangZhejiang 318000China Department of Chemistry Southern University of Science and TechnologyhenzhenGuangdong 518055China College of Material Chemistry and Chemical Engineering Key Laboratory of Organosilicon Chemistry and Material Technology Ministryof EducationHangzhou Normal UniversityHangzhouZhejiang 311121China

Organic fluorine compounds are ubiquitous and pivotally important organic molecules,yet their activation and transformation have long been a formidable challenge due to the high energy and low reactivity of C-F *** electrosynthesis,an environmentally benign synthetic method in organic chemistry,enables a myriad of chemical transformations without the need for external redox *** recent years,organic electrochemistry has emerged as a powerful tool for achieving the activation and transformation of C-F bonds in fluorine-containing *** review aims to succinctly recapitulate the latest advancements in the electrochemical defluorinative transformations of C-F bonds and to delve into the reaction design,mechanistic insights,and developmental prospects ofthese methods.

关键词： Organic electrochemistry Electroreduction Defluorination C-F bond activation Organic fluorine compounds

Advanced cellulose-based materials toward stabilizing zinc anodes

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Science China Chemistry 2024年第5期67卷 1465-1484页

作者： Zhijiang Li Xiang Chen rui Zhang Taoyi Shen Jianchao Sun Zhongce Hu Lin Li Lanlan Yang hou-Yong Yu College of Textile Science and Engineering(International Institute of Silk) Zhejiang Sci-Tech UniversityHangzhou 310018China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Donghua UniversityShanghai 201620China School of Environment and Material Engineering Yantai UniversityYantai 264005China Institute for Carbon Neutralization College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China

Rechargeable aqueous zinc metal batteries(RAZMBs) have received extensive attention for large-scale energy storage systems due to the merits of Zn anodes, including moderate volumetric and gravimetric energy density, low redox potential, abundant reserve, low cost and impressive intrinsic safety. However, Zn anodes suffer from a series of adverse reactions(dendrite growth,hydrogen evolution, and surface passivation) resulting in low Coulombic efficiency, large polarization, and unsatisfied cycling performance, which inevitably hinder the wide application of RAZMBs. To address the above issues, cellulose-based materials are widely used for Zn anode protection because of their unique physical and chemical properties and other advantages such as biocompatibility, non-toxicity, degradability and easy extraction. In order to better understand the current progress in cellulosebased materials for the Zn anode protection, we have classified and summarized the relevant literatures. In this review, we summarize and elaborate the causes of poor reversibility for Zn anodes, including dendrite formation, hydrogen evolution, and surface passivation. Subsequently, the effective strategies(anode interfacial engineering, gel electrolyte optimization, and separator modification) of cellulose-based materials toward stabilizing Zn anodes are overviewed. In the end, the existing challenges and prospects of cellulose-based materials in Zn anode protection are summarized to shed light on future work.

关键词： Zn anode cellulose anode interfacial engineering gel electrolyte optimization separator modification

Influence of Component Size on the Corrosion Behavior of Ti6Al4V Alloy Fabricated by Electron Beam Powder Bed Fusion

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Acta Metallurgica Sinica(English Letters) 2024年第1期37卷 159-168页

作者： Hongyu Zheng Xin Gai Yun Bai Wentao hou Shujun Li Yulin Hao R.D.K.Misra rui Yang Institute of Metal Research Chinese Academy of SciencesShenyang110016China School of Materials Science and Engineering University of Science and Technology of ChinaShenyang110016China Nuclear Power Institute of China Chengdu610213China Department of Metallurgical Materialsand Biomedical EngineeringThe University of Texas at El Paso500WUniversity AvenueEl PasoTX79968USA

The electrochemical behavior of Ti-6Al-4V with 1 mm and 16 mm thickness prepared by electron beam powder bed fusion(EB-PBF)was investigated in phosphate buffered *** results showed that EB-PBF Ti-6Al-4V with a larger component size was more resistant to corrosion compared to the smaller component,because of less acicularαʹphase content and moreβphase *** a non-equilibrium phase in the“high-energy state”,αʹphase has a greater susceptibility to corrode and reduces the corrosion resistance of the material,whileβphase improves corrosion resistance of titanium *** results show that the phase composition has a more significant effect on the corrosion performance than the grain size.

关键词： Electron beam powder bed fusion Ti6Al4V alloy Corrosion resistance Component size Polarisation

Enhancing Li-S battery performance via functional polymer binders for polysulfide inhibition

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Journal of Energy Chemistry 2024年第10期97卷 228-236,I0005页

作者： Jinpeng Jian Qian Chen Hao Sun rui Li Yaolin hou Yulong Liu Jia Liu Haiming Xie Jiefang Zhu Nation&Local United Engineering Laboratory for Power Batteries Faculty of ChemistryNortheast Normal UniversityChangchun 130024JjilinChina Jilin Province Dongchi New Energy Technology Co. Ltd.Changchun 13000oJilinChina Department of Chemistry-Angstrom Laboratory Uppsala UniversitySE-75121Sweden

The commercialization of lithium-sulfur(Li-S)batteries faces several challenges,including poor conductivity,unexpected volume expansion,and continuous sulfur loss from the cathode due to redox *** this study,we introduce a novel polymer via a simple cross-linking between poly(ether-thioureas)(PETU)and poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate)(PEDOT:PSS)as a bifunctio nal binder for Li-S batteries(devotes as"PPTU").Compared to polyvinylidene fluoride(PVDF),as-prepared PPTU exhibits significantly higher electrical conductivity,facilitating electrochemical ***,PPTU demonstrates effective adsorption of lithium polysulfides,leading to improved cycling stability by suppressing the shuttling *** investigate this behavior by monitoring morphological changes at the cell interface using synchrotron X-ray *** with PPTU binders exhibit remarkable rate performance,desired reversibility,and excellent cycling stability even under stringent bending and twisting *** work represents promising progress in functional polymer binder development for Li-S batteries.

关键词： Li-S batteries Bifunctional binders Electrode conductivity Shuttle effect

Cystic hepatic echinococcosis with intrabiliary rupture

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Hepatobiliary Surgery and Nutrition 2024年第3期13卷 573-574页

作者： Jianming Ma Qifu Yan Zha Xi Yun Dan Yucheng hou rui Tang General Surgery Department Lhasa People’s HospitalLhasaChina Hepatopancreatobiliary Center Beijing Tsinghua Changgung HospitalSchool of Clinical MedicineTsinghua UniversityBeijingChina

A 43-year-old Tibetan female was brought to the department of general surgery with abdominal *** tomography(CT)scan revealed cystic hepatic echinococcosis in the right liver(Figure 1A).Further magnetic resonance cholangiopancreatography showed that there were cyst-biliary communications at right posterior bile duct,and several hydatid cysts inside common bile duct(Figure 1B,yellow arrow head showed rupture,white arrow heads showed bile duct hydatid cysts).Low confluence of right posterior bile duct to the common hepatic duct suggests biliary *** serum total bilirubin was normal,serum alkaline phosphatase and gamma-glutamyl transpeptidase were elevated mildly with the value of 278 and 107 U/L *** underwent right hemihepatectomy plus choledochoscopic hydatid cysts extraction through right posterior hepatic duct stump(Figure 1C,yellow arrow head showed right posterior bile duct stump,white arrow heads showed bile duct hydatid cysts).To prevent the spread of echinococcosis,we covered the surgical area with hypertonic saline gauze.A large number of hydatid cysts presented inside hepatectomy specimen that mixed with a lot of bile(Figure 1D).Hydatid cyst inside bile duct was removed completely,and postoperative recovery was *** removed all the liver cysts,and no signs of any lesion residue in post-operative image.

关键词： rupture hepatic biliary