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Soot combustion; Ceria; Ternary mixed oxide; Cordierite coating; Diesel particulate filter

Journal of Environmental Sciences 2018年第11期30卷 58-68页

作者： Leandro Fontanetti Nascimento Juliana Fonseca Lima Paulo Cesar de Sousa filho Osvaldo Antonio Serra Department of Chemistry FFCLRP University of Sao Paulo 14040-901 Ribeirao Preto Sao Paulo Brazil Institute of Chemistry Rio de Janeiro State University 20550-900 Rio de Janeiro Rio de Janeiro Brazil Institute of Chemistry Uniuersity of Campinas 13083-970 Campinas Silo Paulo Brazil Center of-Natural and Human Sciences Federal Uniuerty of ABC 09210-580 Santo Andre Sao Paulo Brazil

We report the application of a solid lanthanum-ceria-zinc catalyst in the catalytic regeneration of diesel particulate filters （DPF） in diesel engines. We synthesized a CeO2- ZnO-La2O3 （Ce-Zn-La） mixed oxide by a lactic acid-mediated sol-gel method, which efficiently coated cordierite substrates for soot capture and combustion. We studied the effects of La loading on the physicochemical and catalytic properties of Ce-Zn mixed oxide during lowtemperature soot combustion processes. We characterized the synthesized catalysts by X-ray diffraction （XRD）, Fourier-transform infrared spectroscopy （FTIR）, N2 adsorption, Raman spectroscopy, oxygen storage capacity （OSG）, and scanning and transmission electron microscopy （SEM and TEM）. Thermogravimetric and differential thermal analysis （TGA/DTA） confirmed that the catalysts effectively reduced the soot oxidation temperature. The ternary Ce-Zn-La mixed oxide catalyst with Ce/Zn/La atomic ratio of 2：1：0.5 had the highest catalytic activity and promoted soot oxidation at temperatures below 390℃. This indicated that the large number of oxygen vacancies in the catalyst structure generated oxygen species at low temperatures. Raman spectroscopy measurements revealed the presence of oxygen vacancies and lattice defects in Ce-Zn-La samples, which were key parameters concerning the stability and redox properties of the prepared catalysts.

关键词： Soot combustion Ceria Ternary mixed oxide Cordierite coating Diesel particulate filter

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New insights into the hardening and pitting corrosion mechanisms of thermally aged duplex stainless steel at 475℃:A comparative study between 2205 and 2101 steels

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Journal of Materials Science & Technology 2022年第3期98卷 123-135页

作者： R.Silva G.S.Vacchi C.L.Kugelmeier I.G.R.Santos A.A.Mendes filho D.C.C.Magalhães C.R.M.Afonso V.L.Sordi C.A.D.Rovere Munir Rachid Corrosion Laboratory Department of Materials EngineeringFederal University of São CarlosRodovia Washington Luis Km 23513565-905 São CarlosSPBrazil Engineering Modeling and Applied Social Sciences Center(CECS)Federal University of ABCAvenida dos Estados 500109210580 Santo AndréSPBrazil Federal University of São Carlos Graduate Program in Materials Science and EngineeringBrazil

In this study,the relationship between spinodal decomposition and the formation of Ni-rich clusters and G-phase in the ferrite on hardening and pitting corrosion of two thermally aged duplex stainless steels(DSSs)at 475℃was *** indicate that,for 2205 DSS,pitting corrosion behavior is influenced by the presence and size of G-phase precipitates for longer aging times,but this contribution is masked by the advanced stage of spinodal decomposition in the ferritic *** the other hand,for 2101 DSS,the formation of Cr-richer nitrides impairs pitting corrosion resistance more than spinodal decomposition.

关键词： Duplex stainless steel Spinodal decomposition G-phase precipitation Pitting corrosion Hardening

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Diurnal Cycle of Heating and Water Vapor in the Metropolitan Area of Porto in Portugal

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Journal of Geographic Information System 2022年第1期14卷 61-77页

作者： Hugo Abi Karam Jorge Fernando Soares Gonçalves Augusto José Pereira filho Departamento de Meteorologia Instituto de Geociências Universidade Federal do Rio de Janeiro (IGEO-UFRJ) Rio de Janeiro Brazil IBERMETEO Coimbra Portugal Departamento de Ciências Atmosféricas Instituto de Astronomia Geofísica e Ciências Atmosféricas Universidade de S&#227 o Paulo (IAG-USP) S&#227 o Paulo Brazil

In this work, it is investigated the Urban Heat Island (UHI) using conservative thermodynamic variables observed by surface weather stations on the Metropolitan Area of Porto (Oporto) in Portugal, under adiabatic conditions at the surface. These conditions are usually present and associated with the development of a mixture layer into the diurnal Convective Boundary Layer (CBL), which residual layer in the late afternoon defines the initial state for the development of the nocturnal UHI. Both the spatial structure and temporal variation of potential temperature and specific humidity were considered, along the hours and days of the year, from a statistical point of view, resulting in hourly climatology. Details of the hourly evolution of the meteorological variables on the Oporto surface are presented and discussed. Results show a seasonal variation of the potential temperature up to 17°C throughout the year, which is associated with horizontal thermal gradients that can control and trigger mesoscale circulations such as sea-land, urban and valley-mountain breezes.

关键词： Metropolitan Area of Porto (Oporto) Climatology Urban Heat Island Development Urban Boundary Layer Mesoscale Atmospheric Circulations

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Hydrometeorological Modeling of Limpopo River Basin in Mozambique with TOPMODEL and Remote Sensing

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Open Journal of Modern Hydrology 2022年第2期12卷 55-73页

作者： Tomásio Eduardo Januário Augusto José Pereira filho Marcos Figueiredo Salviano Department of Atmospheric Sciences Institute of Astronomy Geophysics and Atmospheric Sciences University of S&#227 o Paulo S&#227 o Paulo Brazil Geological Survey of Brazil S&#227 o Paulo Brazil

The Limpopo River basin (LRB) is known for its vulnerability to floods, high rates of evapotranspiration, and droughts that cause significant losses to the local community. The present study aimed to perform simulations of flood events occurring in two Mozambican sub-basins of LRB, namely Chókwè and Xai-Xai from 2000 to 2015 with TOPography-based hydrological MODEL (TOPMODEL) and satellite remote sensing data. As input in TOPMODEL, data from two high-resolution global satellite-based precipitation products: Climate Prediction Center MORPHing technique (CMORPH) and Integrated Multi-Satellite Retrievals for the Global Precipitation Mission (GPM) algorithm (IMERG), 8-day MOD16 evapotranspiration product and surface runoff data estimated by Global Land Data Assimilation System (GLDAS) were used. The sensitivity tests of TOPMODEL parameters were applied using the Monte Carlo simulation. Calibration and validation of the model were performed by the Shuffled Complex Evolution (SCE-UA) method and were evaluated with the Kling-Gupta Efficiency (KGE) index. The results indicated that simulations with the GPM-IMERG (KGE: 0.59 and 0.65) tended to underestimate the stream flows, while with the CMORPH product the performance was much better (KGE: 0.66 and 0.77) in both sub-basins. Thus, TOPMODEL can help to develop flood monitoring systems from satellite remotely sensed data in similar regions of Mozambique.

关键词： Floods Simulations Limpopo River TOPMODEL CMORPH IMERG

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Loss of the BRCA1-PALB2 interaction accelerates p53-associated tumor development in mice

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Genes & Diseases 2022年第3期9卷 807-813页

作者： Amar H.Mahdi Yanying Huo Ying Chen Pier Selenica Anchal Sharma Elise Merritt Nicola Barnard Chang Chan Shridar Ganesan Jorge S.Reis-filho Britta Weigelt Subhajyoti De Bing Xia Rutgers Cancer Institute of New Jersey New BrunswickNJ 08903USA Department of Radiation Oncology Rutgers Robert Wood Johnson Medical SchoolNew BrunswickNJ 08903USA Department of Pathology Memorial Sloan Kettering Cancer CenterNew YorkNY 10065USA Department of Pathology and Laboratory Medicine Rutgers Robert Wood Johnson Medical SchoolNew BrunswickNJ 08901USA

The BRCA1-PALB2-BRCA2 axis,or the BRCA pathway,plays key roles in genome stability maintenance and suppression of breast and several other *** to frequent p53 mutations in human BRCA1 breast cancers and mouse mammary tumors from Brcal,Brca2 and Palb2 conditional knockout models,it is often thought that p53 inactivation accelerates BRCA1/2 and PALB2-associated ***,we studied tumor development in mice with a mutation in Palb2 that disengages the PALB2-BRCA1 interaction in different Trp53 *** than mammary tumors,Palb2 and Trp53 compound mutant mice developed,with greatly reduced latencies,lymphomas and sarcomas that are typically associated with germline Trp53 *** exome sequencing failed to identify any significant differences in genomic features between the same tumor types of Trp53 single mutant and Palb2;Trp53 compound mutant *** results suggest that loss of the BRCA pathway accelerates p53-associated tumor development,possibly without altering the fundamental tumorigenic processes.

关键词： BRCA1 BRCA2 Osteosarcoma P53 PALB2 Thymic lymphoma

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Antioxidant,hypolipidemic and hypoglycemic effect of red wine in wistar rats fed with obesogenic diet

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Food Bioscience 2022年第3期47卷 756-764页

作者： Cornélio Mucaca José Henrique Tavares filho Luciana Lima Arruda André Martins Galvão Maria Bernadete de Sousa Maia Eryka Maria dos Santos Alves Eryvelton de Souza Franco Elizabeth do Nascimento Department of Nutrition Center of Health SciencesFederal University of Pernambuco (UFPE)Cidade Universitaria50670-901RecifePEBrazil Rural Technology Department Federal Rural University of Pernambuco (UFRPE)AD.Manoel de Medeiros Ave.s/nDois Irmãos52171-900RecifePEBrazil Department of Physiology and Pharmacology Center of Biological SciencesFederal University of Pernambuco (UFPE)Cidade Universitaria50670-901RecifePEBrazil

The health benefits resulting from the usual ingestion of red wines have been studied in humans and ***,the evaluation of benefits in antioxidant,hypoglycemic and hypolipemic activity concomitant with the use of an obesogenic diet in adult Wistar rats has been little *** present study investigated the use of red wine derived from Northeast Brazil in adult rats fed with an obesogenic diet on antioxidant activity,glucose tolerance,adipose,glycemic and lipemic *** 45-day old male Wistar rats formed two groups:standard diet and westernized *** changes in body mass and glycemic levels,the animals were subdivided into six subgroups (n = 10 per group) and received water,red wine or hydroalcoholic solution by *** data reveal that the moderate and chronic use of red wine improves the glycemic,lipid and oxidative stress profile,being favorable in preventing the risk of cardiovascular diseases in rats fed with an obesogenic diet.

关键词： Dyslipidemia Obesity Rats Westernized diet Red wine

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Physical Properties in Drying of Food Products with Combined Sublimation and Evaporation

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Chinese Journal of Chemical Engineering 2004年第6期12卷 814-817页

作者： Ingvald Strфmmen Odilio Alves-filho Trygve M.Eikevik Ingrid C.Claussen Department of Refrigeration and Air Conditioning The Norwegian University of Science and Technology (NTNU) Trondheim NorwaySINTEF Energy Research Department of Refrigeration and Air Conditioning Trondheim NorwaySINTEF Energy Research Department of Refrigeration and Air Conditioning Trondheim NorwayDepartment of Refrigeration and Air Conditioning The Norwegian University of Science and Technology (NTNU) Trondheim Norway

Drying is an important unit operation in processing of biological resources. The drying process may influence the product properties and quality, which may shrink, break or undergo rheological, physical and biochemical changes. The important parameters responsible for such changes are drying conditions, type of drying technology and residence drying time. Thermal conductivity, thermal-mass diffusivity, enthalpy, porosity and density are the main material property and heat-mass transfer parameters, which are essential for understanding the changes in product quality and for designing and dimensioning the drying processes. In this paper physical properties of food products undergoing a combined sublimation and evaporation were studied. Pieces of vegetables and potatoes were dried in a heat pump fluidized bed dryer at combined modes with temperatures below the freezing point in the beginning and a final drying step at temperatures above the freezing point. Samples of products were tested at different moisture contents with respect to physical properties. Physical properties of leek and potato samples were measured and mass diffusivities were determined from drying kinetic data. Based on bulk density and rehydration measurements it was clearly observed that drying temperature and modes influenced the final product physical properties. The potato cube run dried with initial atmospheric freeze-drying step had rehydration ability 430%above a run dried only above the freezing point. The average effective mass diffusivity for 5 mm slabs of leek was 0.5 x 10-11m2·s-1 for the sublimation stage and 2.2 x 10-11m2·s-1 for the evaporation stage.

关键词：升华蒸发联合法食品干燥物理性质

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Assessing the inter-annual variability of separation distances around odour sources to protect the residents from odour annoyance

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Journal of Environmental Sciences 2019年第5期31卷 11-24页

作者： Marlon Brancher Martin Piringer Davide Franco Paulo Belli filho Henrique De Melo Lisboa Gunther Schauberger Postgraduate Program in Environmental Engineering (PPGEA) Federal University of Santa Catarina (UFSC) 88040900 Florianopolis Brazil.CAPES Foundation scholarship holder (main author) Brazilian Ministry of Education Brasilia Brazil WG Environmental Health Department of Biomedical Sciences University of Veterinary Medicine ViennaVeterinarplatz1 A-1210Vienna Austria Central Institute for Meteorology and Geodynamics Hohe Warte 38 A-1190 Vienna Austria

In recent years, there has been a growing concern about potential impacts on public health and wellbeing due to exposure to environmental odour. Separation distances between odour-emitting sources and residential areas can be calculated using dispersion models, as a means of protecting the neighbourhood from odour annoyance. This study investigates the suitability of using one single year of meteorological input data to calculate reliable direction-dependent separation distances. Accordingly, we assessed and quantified the inter-annual variability of separation distances at two sites with different meteorological conditions, one in Brazil and the other in Austria. A 5-year dataset of hourly meteorological observations was used for each site. Two odour impact criteria set in current regulations were selected to explore their effect on the separation distances. The coefficient of variation was used as a statistical measure to characterise the amount of annual variation. Overall,for all scenarios, the separation distances had a low degree of inter-annual variability(mean coefficient of variation values from 8% to 21%). Reasonable agreements from year to year were therefore observed at the two sites under investigation, showing that one year of meteorological data is a good compromise to achieve reliable accuracy. This finding can provide a more cost-effective solution to calculate separation distances in the vicinity of odour sources.

关键词： Environmental odour Odour annoyance Impact assessment Dispersion modelling Regulatory criteria Separation distance

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Narrow-band imaging without magnification for detecting early esophageal squamous cell carcinoma

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World Journal of Gastroenterology 2011年第39期17卷 4408-4413页

作者： Edson Ide Fauze Maluf-filho Dalton Marques Chaves Sergio Eiji Matuguma Paulo Sakai University of So Paulo Gastrointestinal Endoscopy Unit

AIM:To compare narrow-band imaging(NBI)without image magnification,and chromoendoscopy with Lugol's solution for detecting high-grade dysplasia and intramu-cosal esophageal squamous cell carcinoma(SCC)in patients with head and neck ***:This was a prospective observational study of 129 patients with primary head and neck tumors consecutively referred to the Gastrointestinal Endoscopy Unit of Hospital das Clínicas,S?o Paulo University Medical School,Brazil,between August 2006 and Feb-ruary *** examinations with NBI and Lugol chromoendoscopy were consecutively performed,and the discovered lesions were mapped,recorded and sent for *** results of the three methods were compared regarding sensitivity,specificity,accuracy,positive predictive value,negative predictive value,positive likelihood value and negative likelihood ***:Of the 129 patients,nine(7%)were diagnosed with SCC,5 of which were in situ and 4 which were *** carcinomas were detected through NBI and Lugol *** 4 lesions were diagnosed through conventional examination,all of which were larger than 10 ***:NBI technology with optical filters has high sensitivity and high negative predictive value for detecting superficial esophageal SCC,and produces results comparable to those obtained with 2.5%Lugol chromoendoscopy.

关键词：鳞状细胞癌窄带干扰检测食管放大倍率成像早期常规检查

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Statistical Analysis of Precipitation Extremes in São Francisco River Basin, Brazil

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Atmospheric and Climate Sciences 2022年第2期12卷 383-408页

作者： Nayara Arroxelas dos Santos Siqueira Anderlan Henrique Batista Siqueira Augusto José Pereira filho Departamento de Ciências Atmosféricas Instituto de Astronomia Geofísica e Ciências Atmosféricas Universidade de S&#227 o Paulo S&#227 o Paulo Brazil Instituto de Ciências Atmosféricas Universidade Federal de Alagoas Alagoas Brazil

This study comprises a climatology of the spatial variability of precipitation over the São Francisco River Basin (SFRB), characterized by its geographic heterogeneity. The different rainfall regimes in the region were analyzed through statistical and spectral analyses. Measured precipitation data, Pacific Decennial Climate indexes, ENSO, Atlantic Multidecadal Oscillation, North Atlantic Oscillation, Atlantic dipole, and the sunspot cycle over 65 years were used. The rainfall data were filtered and filled in using the regional weighting method. The spatial and temporal variability of precipitation along the SFRB is remarkable. A pattern was observed along with the time series of precipitation over the SFRB. The cluster analysis identified four homogeneous regions in the SFRB and explained 87.4% of the total variance of the average monthly rainfall of the 199 rain gauges. The Cross-wavelet analysis identified the relationship between the precipitation data series and the climatic indexes that are analyzed in this work.

关键词： Cross-Wavelet Statistical Analysis Hydrometeorology Climatology

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