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chinese Journal of polymer science 2001年第4期19卷 399-405页

作者： Zhen-hua yuan De-yan Shen ren-yuan qian polymer physics laboratory center for molecular science, institute of chemistry chinese academy of sciences, beijing 100080 china 中科院化学所高分子物理及化学国家重点实验室北京

Viscoelastic behavior of the non-Hooke deformation of amorphous PET film before yield was investigated in the temperature region 74-80.5 degreesC around the glass transition temperature. The film specimen was drawn to yield point followed by unloading to zero stress, then the residual deformation was held constant; while the subsequent evolution of the stress was recorded. An induction period was found in the course of stress evolution followed by a stress step-increase. The induction period decreases with increasing drawing temperature with an activation energy of 1.10 MJ/mol.K, which is attributed to the time needed for the relaxation of rubbery deformation through cooperative internal rotations. At temperatures lower than 74 degreesC, there is no stress increase or the induction period becomes too long to be observed. Thus the nature of anelasticity in the non-Hooke region before yielding is attributed to stress induced rubbery deformation. The experimental results are interpreted in terms of Perez' theological model of a series connected Hooks spring and a Voigt element consisting of a parallel connected elastic spring and a dashpot.

关键词： pre-yield deformation PET uniaxial drawing non-Hooke deformation viscoelasticity stress induced rubbery deformation

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Two-dimensional materials for future information technology: status and prospects

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science china(Information sciences) 2024年第6期67卷 1-147页

作者： Hao QIU Zhihao YU Tiange ZHAO Qi ZHANG Mingsheng XU Peifeng LI Taotao LI Wenzhong BAO Yang CHAI Shula CHEN Yiqi CHEN Hui-Ming CHENG Daoxin DAI Zengfeng DI Zhuo DONG Xidong DUAN Yuhan FENG Yu FU Jingshu GUO Pengwen GUO Yue HAO Jun HE Xiao HE Jingyi HU Weida HU Zehua HU Xinyue HUANG Ziyang HUANG Ali IMRAN Ziqiang KONG Jia LI qian LI Weisheng LI Lei LIAO Bilu LIU Can LIU Chunsen LIU Guanyu LIU Kaihui LIU Liwei LIU Sheng LIU yuan LIU Donglin LU Likuan MA Feng MIAO Zhenhua NI Jing NING Anlian PAN Tian-Ling ren Haowen SHU Litao SUN Yue SUN Quanyang TAO Zi-Ao TIAN Dong WANG Hao WANG Haomin WANG Jialong WANG Junyong WANG Wenhui WANG Xingjun WANG Yeliang WANG Yuwei WANG Zhenyu WANG Yao WE... School of Electronic science and Engineering Nanjing University School of Integrated Circuits Interdisciplinary Research Center for Future Intelligent Chips (Chip-X)Nanjing University School of Integrated Circuit science and Engineering Nanjing University of Posts and Telecommunications State Key laboratory of Infrared physics Shanghai Institute of Technical Physics Chinese Academy of Sciences School of physics and Key Lab of Quantum Materials and Devices of the Ministry of Education School of Electronic Science & EngineeringSoutheast University College of Integrated Circuits State Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang University Suzhou laboratory State Key laboratory of Integrated Chips and Systems School of MicroelectronicsFudan University Shaoxin laboratory Department of Applied physics The Hong Kong Polytechnic University Key laboratory for Micro-Nano physics and Technology of Hunan Province College of Materials Science and EngineeringHunan University College of Integrated Circuits Zhejiang University Shenzhen Geim Graphene center Shenzhen Key Laboratory of Layered Materials for Value-Added ApplicationsTsinghua-Berkeley Shenzhen Institute & Institute of Materials ResearchTsinghua Shenzhen International Graduate SchoolTsinghua University State Key laboratory of Extreme Photonics and Instrumentation College of Optical Science and EngineeringInternational Research Center for Advanced PhotonicsZijingang CampusZhejiang University National Key laboratory of Materials for Integrated Circuits Shanghai Institute of Microsystem and Information TechnologyChinese Academy of Sciences CAS Key laboratory of Nanophotonic Materials and Devices & Key laboratory of Nanodevices and Applications i-LabSuzhou Institute of Nano-Tech and Nano-Bionics (SINANO)Chinese Academy of Sciences College of chemistry and Chemical Engineering Hunan University Key laboratory of Quantum State Construction and Manipulation (Ministry of Education) Department of PhysicsRenmin University of China School

Over the past 70 years, the semiconductor industry has undergone transformative changes,largely driven by the miniaturization of devices and the integration of innovative structures and materials. Two-dimensional(2D) materials like transition metal dichalcogenides(TMDs) and graphene are pivotal in overcoming the limitations of silicon-based technologies, offering innovative approaches in transistor design and functionality, enabling atomic-thin channel transistors and monolithic 3D integration. We review the important progress in the application of 2D materials in future information technology, focusing in particular on microelectronics and optoelectronics. We comprehensively summarize the key advancements across material production, characterization metrology, electronic devices, optoelectronic devices, and heterogeneous integration on silicon. A strategic roadmap and key challenges for the transition of 2D materials from basic research to industrial development are outlined. To facilitate such a transition, key technologies and tools dedicated to 2D materials must be developed to meet industrial standards, and the employment of AI in material growth, characterizations, and circuit design will be essential. It is time for academia to actively engage with industry to drive the next 10 years of 2D material research.

关键词： two-dimensional (2D) materials information technology production technology standardization of characterization microelectronicdevices optoelectronic devices multi-functional integration

降低全聚合物太阳能电池光伏效率的温度依赖性

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science china Materials 2024年第1期67卷 47-57页

作者：张伟超杨镕申乐耀昌程倩张莹玉张建齐肖林格李世麟姚果张春峰周惠琼张渊 School of chemistry Beijing Advanced Innovation Center for Biomedical EngineeringBeihang UniversityBeijing 100191China Key laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China National laboratory of Solid-State Microstructures School of Physics and Collaborative Innovation Center for Advanced MicrostructuresNanjing UniversityNanjing 210008China

全聚合物太阳能电池(All-PSCs)具有良好的机械稳定性和热稳定性,受到人们的广泛关注.目前,提高全聚合物太阳能电池性能的关键是改善活性层的形貌.本文通过逐层(LBL)工艺,优化了薄膜形貌,实现了更好的电荷产生和传输,增加了激子扩散长度... 详细信息

全聚合物太阳能电池(All-PSCs)具有良好的机械稳定性和热稳定性,受到人们的广泛关注.目前,提高全聚合物太阳能电池性能的关键是改善活性层的形貌.本文通过逐层(LBL)工艺,优化了薄膜形貌,实现了更好的电荷产生和传输,增加了激子扩散长度,提高了电荷产量,并抑制了复合损失.此外,本文进一步研究了LBL制备的全聚合物太阳能电池中的激子/电荷行为与温度的依赖性关系.详细的原位光谱测量和光电特性表征表明,独特的形态延长了激子寿命,减少了电荷陷阱,并促进了电荷传输和收集.因此,准双层PM6/PYF-T-o器件的能量转换效率(PCE)显著提高(16.70%).此外,与BHJ器件相比,通过LBL工艺制备的器件,实现了增强的分子有序性,降低了能级混乱度,使得器件填充系数和PCE温度依赖性减弱.本工作为太阳能电池在温度可变环境下的电荷传输行为和光伏性能提供了新的认识,也为其实际应用提供了理论依据.

关键词：能量转换效率太阳能电池温度依赖性电荷传输机械稳定性填充系数活性层 LBL

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CRYSTALLINE MORPHOLOGY IN A SERIES OF CH3-SUBSTITUTED THERMOTROPIC AROMATIC POLYESTERS WITH EVEN AND ODD FLEXIBLE SPACERS

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chinese Journal of polymer science 2001年第1期19卷 71-78页

作者： Shou-xi Chen Zhong-ming Hu Wen-hui Song Yong-ze Jin ren-yuan qian State Key laboratory of polymer physics and chemistry Center for Molecular Science Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China State Key Laboratory of Polymer Physics and Chemistry Center for Molecular Science Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China State Key Laboratory of Polymer Physics and Chemistry Center for Molecular Science Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China State Key Laboratory of Polymer Physics and Chemistry Center for Molecular Science Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China State Key Laboratory of Polymer Physics and Chemistry Center for Molecular Science Institute of Chemistry Chinese Academy of Sciences Beijing 100080 China

Crystalline morphology in a series of CH3-substituted main chain thermotropic aromatic polyesters with even and odd numbered methylene spacers has been studied by polarizing optical microscopy (POM), scanning electron microscopy (SEM) and transmission electron microscopy (TEM). On crystallization from solution evaporation spherulites of radial structure were observed in the polymers with even numbered spacers, but spherulites with concentric rings form in the polymer with odd numbered spacers. Both spherulites have a lamellar structure, which is about 10 nm in thickness. On crystallization from nematic glassy state spherulites can not be grown; lamellar structure was only observed around disclinations in a specimen during crystallization. Ln the case of crystallization from nematic melt two types of spherulites can be observed far the sample with even numbered spacers. For the sample with add numbered spacers spherulites can not be formed, but only irregular crystallites.

关键词： crystalline morphology spherulite even-odd flexible spacers CH3-substituted thermotropic aromatic polyester

Recent progress in perovskite solar cells:from device to commercialization

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science china chemistry 2022年第12期65卷 2369-2416页

作者： Xinhui Luo Xuesong Lin Feng Gao Yang Zhao Xiaodong Li Liqing Zhan Zexiong Qiu Jin Wang Cong Chen Lei Meng Xiaofeng Gao Yu Zhang Zijian Huang Rundong Fan Huifen Liu Yanrun Chen Xiaoxue ren Jiahong Tang Chun-Hao Chen Dong Yang Yongguang Tu Xiao Liu Dongxue Liu Qing Zhao Jingbi You Junfeng Fang Yongzhen Wu Hongwei Han Xiaodan Zhang Dewei Zhao Fuzhi Huang Huanping Zhou Yongbo yuan Qi Chen Zhaokui Wang Shengzhong(Frank)Liu Rui Zhu Jotaro Nakazaki Yongfang Li Liyuan Han State Key laboratory of Metal Matrix Composites School of Material Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China State Key Lab for Mesoscopic physics and Frontiers science center for Nano-optoelectronics School of PhysicsPeking UniversityBeijing 100871China Key laboratory of Semiconductor Materials science Institute of SemiconductorsChinese Academy of SciencesBeijing 100083China School of physics and Electronic science Engineering Research Center of Nanophotonics&Advanced InstrumentMinistry of EducationEast China Normal UniversityShanghai 200241China Key laboratory for Advanced Materials and institute of Fine Chemicals School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China Wuhan National laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China institute of Photoelectronic Thin Film Devices and Technology Renewable Energy Conversion and Storage CenterSolar Energy Research CenterNankai UniversityTianjin 300350China College of Materials science and Engineering&Engineering Research center of Alternative Energy Materials&Devices Ministry of EducationSichuan UniversityChengdu 610065China beijing National laboratory for molecular sciences CAS Key Laboratory of Organic SolidsInstitute of ChemistryChinese Academy of SciencesBeijing 100190China State Key laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China beijing Key laboratory for Theory and Technology of Advanced Battery Materials Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationSchool of Materials Science and EngineeringPeking UniversityBeijing 100871China School of physics and Electronics Hunan Key Laboratory of Nanophotonics and DevicesCentral South UniversityChangsha 410083China Experimental center for Advanced Materials School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Jia

Perovskite solar cells(PSCs) are undergoing rapid development and the power conversion efficiency reaches 25.7% which attracts increasing attention on their commercialization *** this review,we summarized the recent progress of PSCs based on device structures,perovskite-based tandem cells,large-area modules,stability,applications and ***,the challenges and perspectives are discussed,aiming at providing a thrust for the commercialization of PSCs in the near future.

关键词： perovskite solar cells device engineering stability application

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